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At least 1,801 records · Page 100

A new generation of uranium coincidence fast neutron collars for assay of LWR fresh fuel assemblies

The active uranium neutron coincidence collar provides a means of non-destructively assaying the fissile linear density of Light Water Reactor fresh fuel assemblies containing low enriched uranium. These neutron collars can operate in two modes: a thermal and a fast mode. In fast mode, a neutron collar has an added cadmium (Cd) liner in the sample cavity of the detector to reduce the impact of the burnable poison (thermal neutron absorber) on the detector signal (doubles). The main advantage for operating in fast mode is a detected signal that is less dependent of the burnable neutron poison content and thus less dependent on facility operator declarations. The drawback is that operating in fast mode requires a longer measurement time (~hour vs tens of minutes for thermal mode) to achieve the statistically needed precision in the measurements. The trend in the modern reactor fuel assemblies is moving to higher burnup by using higher initial enrichment and, consequently, a higher number of burnable poison rods to compensate the initial neutron reactivity. The increase of the burnable poison loading has motivated the development of a new generation of high efficiency fast neutron collars to allow practical measurements in-field by nuclear inspectors. This paper describes the development and performance evaluation of a new generation of neutron collars, for both boiling water reactor (BWR) and pressurized water reactor (PWR) fuels, jointly developed between the US Department of Energy, through Los Alamos National Laboratory, and the Euratom Safeguards Directorate of the European Commission. In this work, we present here calibrations with reference fuel assemblies at Los Alamos National Laboratory as well as the results of in-field measurement campaigns in fuel fabrication plants with modern commercial fuel assemblies. The experimental results show that a typical PWR verification can be made in a total time of 30 min with an uncertainty in the measured mass of 2% at one standard deviation (1σ). A BWR verification can be made in 47 min with an uncertainty in the measured mass of 1.9% at 1σ, or a total time of 20 min with 1σ uncertainty in the measured mass of 2.5%.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Monochromatization interaction region optics design for direct s-channel Higgs production at FCC-ee

The FCC-ee offers the potential to measure the electron Yukawa coupling via direct s-channel Higgs production, e + e − → H , at a centre-of-mass (CM) energy of ∼125 GeV. This measurement is significantly facilitated if the CM energy spread of e + e − collisions can be reduced to a level comparable to the natural width of the Higgs boson, Γ H = 4.1 MeV, without substantial loss in luminosity. Achieving this reduction in collision-energy spread is possible through the “monochromatization” concept. The basic idea is to create opposite correlations between spatial position and energy deviation within the colliding beams, which can be accomplished in beam optics by introducing a nonzero dispersion function with opposite signs for the two beams at the interaction point. Since the first proposal in 2016, the implementation of monochromatization at the FCC-ee has been continuously improved, starting from preliminary parametric studies. In this paper, we present a detailed study of the interaction region optics design for this newly proposed collision mode, exploring different potential configurations and their implementation in the FCC-ee global lattice, along with beam dynamics simulations and performance evaluations including the impact of “beamstrahlung.”

43 PARTICLE ACCELERATORS↗

AI-assisted object condensation clustering for calorimeter shower reconstruction at CLAS12

Several nuclear physics studies using the CLAS12 detector rely on the accurate reconstruction of neutrons and photons from its forward angle calorimeter system. These studies often place restrictive cuts when measuring neutral particles due to an overabundance of false clusters created by the existing calorimeter reconstruction software. In this work, we present a new AI approach to clustering CLAS12 calorimeter hits based on the object condensation framework. The model learns a latent representation of the full detector topology using GravNet layers, serving as the positional encoding for an event’s calorimeter hits which are processed by a Transformer encoder. This unique structure allows the model to contextualize local and long range information, improving its performance. Evaluated on one million simulated $e^-$ $+$ $p$ collision events, our method significantly improves cluster trustworthiness: the fraction of reliable neutron clusters, increasing from 8.88% to 30.73%, and photon clusters, increasing from 51.07% to 64.73%. In conclusion, our study also marks the first application of AI clustering techniques for hodoscopic detectors, showing potential for usage in many other experiments.

Calorimeters↗

Oscillating surge wave energy converter using a novel above-water power takeoff with belt-arc speed amplification

We investigate the performance of a novel power takeoff (PTO) featuring belt-arc speed amplification for oscillating surge wave energy converters (OSWECs), aiming to address the challenges of extremely low rotary speed and large torque under the low-frequency ocean wave excitations. The belt-arc design significantly increases the rotary speed of the generator, enabling generator downsizing and decreasing the powertrain friction losses. The design also allows for placing the generator above water, eliminating the need for high Ingress Protection ratings for the generator and powertrain, and potentially leading to substantial reductions in capital and maintenance costs. Using the linear potential wave theory, the dynamics of the integrated system are analyzed, and key parameters are identified. To validate the numerical analysis, a 1:10 scale model is designed, fabricated, and tested in a wave tank. Performance evaluations are conducted under regular and irregular wave conditions, with quantified effects of parameter tuning. The results reveal an optimal wave-to-electric efficiency of 48% under regular wave excitation and 20% under irregular excitation. Furthermore, these findings underscore the effectiveness of the proposed novel PTO design in addressing the challenges of low rotation speed and large torque inherent in OSWECs, demonstrating its ability to efficiently convert wave power into electricity.

16 TIDAL AND WAVE POWER↗

Basker: Parallel sparse LU factorization utilizing hierarchical parallelism and data layouts

Transient simulation in circuit simulation tools, such as SPICE and Xyce, depend on scalable and robust sparse LU factorizations for efficient numerical simulation of circuits and power grids. As the need for simulations of very large circuits grow, the prevalence of multicore architectures enable us to use shared memory parallel algorithms for such simulations. A parallel factorization is a critical component of such shared memory parallel simulations. We develop a parallel sparse factorization algorithm that can solve problems from circuit simulations efficiently, and map well to architectural features. This new factorization algorithm exposes hierarchical parallelism to accommodate irregular structure that arise in our target problems. It also uses a hierarchical two-dimensional data layout which reduces synchronization costs and maps to memory hierarchy found in multicore processors. We present an OpenMP based implementation of the parallel algorithm in a new multithreaded solver called Basker in the Trilinos framework. Here, we present performance evaluations of Basker on the Intel SandyBridge and Xeon Phi platforms using circuit and power grid matrices taken from the University of Florida sparse matrix collection and from Xyce circuit simulation. Basker achieves a geometric mean speedup of 5.91× on CPU (16 cores) and 7.4× on Xeon Phi (32 cores) relative to state-of-the-art solver KLU. Basker outperforms Intel MKL Pardiso solver (PMKL) by as much as 30× on CPU (16 cores) and 7.5× on Xeon Phi (32 cores) for low fill-in circuit matrices. Furthermore, Basker provides 5.4× speedup on a challenging matrix sequence taken from an actual Xyce simulation.

97 MATHEMATICS AND COMPUTING↗

A review of neutronics and thermal hydraulics–based screening methods applied to accelerated nuclear fuel qualification

This paper reviews the state-of-the-art engineering approach for using thermal hydraulic (TH) and neutronics modeling and simulation (M&S) tools to perform rapid screening studies of novel nuclear fuel concepts within the context of accelerated fuel qualification. Global research efforts have introduced nuclear fuel and material concepts that mark a significant departure from traditional reactor materials. The number of new technologies being considered for development for light water reactors and advanced reactor types has created the need for an accelerated fuel qualification procedure. A key component of this procedure is the rapid identification of the most promising fuel concepts using computational screening studies. Advanced TH and neutronic M&S tools should be leveraged to efficiently determine whether the reactor performance and safety characteristics of a given concept warrant additional studies or whether the concept requires modification or elimination. This paper reviews best practices for performing these TH and neutronics screening studies at various stages during a fuel concept's progression through the qualification procedure. The motivation behind standardizing this approach is to minimize time and resources spent on qualification activities for fuel concepts that could be quickly refined or eliminated from consideration based on their reactor physics and TH characteristics. Adoption of this screening procedure—which focuses primarily on nuclear fuels but may be applicable to other reactor materials—will also help accelerate new material qualification by generating boundary conditions crucial to fuel performance evaluations and highlighting needed areas of separate effects experimentation. This article reviews the motivation behind the introduction of novel nuclear fuel concepts, provides incentive for utilizing TH- and neutronics-based screening studies, describes the screening approach and methodology, and includes discussion on how to interpret screening results to provide recommendations for the continued development of a given concept.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Promoting regulatory acceptance of combined ion and neutron irradiation testing of nuclear reactor materials: Modeling and software considerations

As the needs for the nuclear energy industry continue to evolve in the 21st century, timely adoption of new technological solutions acceptable to regulatory agencies is critical. Quantitative prediction of radiation damage in materials and its impact on mechanical properties is a key component of licensing and regulatory decisions regarding nuclear power plants. Accelerated testing methodologies such as combined ion and neutron irradiation data sets are crucial for the development and deployment of new materials and new manufacturing methods (e.g., additive manufacturing). However, regulatory acceptance of accelerated testing methodologies is necessary for their adoption. Further, the present work discusses the fundamental basis for comparing ion- and neutron-induced material microstructures, the theory behind interpreting radiation damage across length and time scales and radiation types, and the codes, standards, and quality assurance concerns surrounding different modeling methods and software. In particular, recommendations are given as to the path forward that will enable national laboratories, academia, and industry to develop the modeling and software basis for regulatory acceptance of the combined use of ion and neutron irradiation for material performance evaluation.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Operational Performance Characteristics of an Aerated L-valve Operated Within a Closed Circulating Fluidized Bed Loop

An experimental study was conducted in a large scale circulating fluidized bed (0.3 m diameter ×15.5 m tall) equipped with nonmechanical L-valve (0.25 m diameter ×1.52 m long) varying the riser superficial gas velocity (U g ), bed inventory (m), L-valve aeration velocity (U Lvalve ) and standpipe aeration velocity (U move ). The effects of these operational parameters on pressure drop were investigated in each of the different components in the CFB and on the solid circulation rate with two different Group B particles (180 μm glass bead and 750 μm phosphorescent polyethylene beads, PPE). Tests were carried out at ambient temperature and pressure conditions using air as the fluidization gas. The operating parameters were shown to significantly affect pressure drops across various sections of the CFB due to redistribution of solids within the system. The pressure drop in the horizontal section of the L-valve was affected by aeration rates in addition to the solid flow rate reported in previous studies of smaller L-valves without aeration. A new dimensionless semi-empirical correlation was able to explain > 98% of the variance between pressure drop across the horizontal section of the L-valve and operating parameters for these Group B particles. The results of present study indicated that the nonmechanical L-valve cannot be isolated from the CFB system for performance evaluation.

Monazam, Esmail R.↗

A Review of Behind-the-Meter Solar Generation Modeling and Forecasting

Solar photovoltaic systems largely integrated within the distribution grid are operated 'behind-the-meter' and power generation cannot be directly monitored by most utilities. The increasing penetration of behind-the-meter solar photovoltaic systems can deter efficient network and market operations due to variability and uncertainty in net load, which is exacerbated by limited visibility and the difficulty in analyzing the hosting capacity. Risk introduced by behind-the-meter solar contributions may hinder reliable and secure grid operations due to biased system monitoring and forecasts. Accurate behind-the-meter estimations, together with capacity and specification forecasts, thus play a key role in balancing supply and demand and this article reviews the pertinent literature, identifying key characteristics and predictive methods for efficient behind-the-meter solar photovoltaic generation. Forecasting is central to methods herein. The fundamental characteristics of behind-the-meter solar forecasting, including which methods are applicable for scenario-driven use cases, are driven by the metrics most useful for system-wide performance evaluation. To this aim, the literature is reviewed with a focus on forecasting applications for aggregate, regional behind-the-meter generation useful to bulk system and utility operations. As distinguished from net load forecasting, subtleties in these coincident tasks are explored before concluding with recommendations for current practice and future implementations.

behind-the-meter↗

A Fast All-sky Radiation Model for Solar applications with Narrowband Irradiances on Tilted surfaces (FARMS-NIT): Part I. The clear-sky model

The solar energy industry often uses individual steps to empirically compute plane-of-array (POA) irradiance from horizontal irradiance and decompose it to narrow-wavelength bands. Conventional radiative transfer models designed for meteorological applications requires significant computing efforts in practice; however, they provide a physics-based solution of radiance and therefore are capable of computing spectral POA irradiances in a single step. In this study, we integrate the advantages of the current models and develop an innovative radiative transfer model, the Fast All-sky Radiation Model for Solar applications with Narrowband Irradiances on Tilted surfaces (FARMS-NIT), to efficiently compute irradiances on inclined photovoltaics (PV) panels for 2002 narrow-wavelength bands from 0.28 to 4.0 um. This study is reported in two parts. Part I presents the methodology and performance evaluation of the new model under clear-sky conditions. The Simple Model of the Atmospheric Radiative Transfer of Sunshine (SMARTS), which was designed to compute clear-sky irradiances, is employed to rapidly provide the optical properties of a given clear-sky atmosphere. The clear-sky radiances in the narrow-wavelength bands are computed by considering three paths of photon transmission and solving the radiative transfer equation with the single-scattering approximation. The Bi-directional Transmittance Distribution Function (BTDF) of aerosols is given by their single-scattering phase function with a correction using a two-stream approximation. The validation analysis confirms that FARMS-NIT has improved accuracy compared to TMYSPEC as evaluated by both surface observations and a state-of-the-art radiative transfer model. This model substantially improves computational efficiency compared to other radiative transfer models though it uses slightly more computing time than TMYSPEC. Part II of this study addresses the model in cloud-sky conditions and will be published as a companion paper.

14 SOLAR ENERGY↗

Nanoindentation study of electrodeposited Ag thin coating: An inverse calculation of anisotropic elastic-plastic properties

A new inverse method was proposed to calculate the anisotropic elastic-plastic properties (flow stress) of thin electrodeposited Ag coating utilizing nanoindentation tests, previously reported inverse method for isotropic materials and three-dimensional (3-D) finite element analyses (FEA). Indentation depth was ~4% of coating thickness (~10 μm) to avoid substrate effect and different indentation responses were observed in the longitudinal (L) and the transverse (T) directions. The estimated elastic-plastic properties were obtained in the newly developed inverse method by matching the predicted indentation responses in the L and T directions with experimental measurements considering indentation size effect (ISE). The results were validated with tensile flow curves measured from free-standing (FS) Ag film. The current method can be utilized to characterize the anisotropic elastic-plastic properties of coatings and to provide the constitutive properties for coating performance evaluations.

Cheng, Guang (ORCID:0000000268604420)↗

Ultralow-temperature cryogenic transmission electron microscopy using a new helium flow cryostat stage

Advances in cryogenic electron microscopy have opened new avenues for probing quantum phenomena in correlated materials. This study reports the installation and performance of a new side-entry condenZero cryogenic cooling system for JEOL (Scanning) Transmission Electron Microscopes (S/TEM), utilizing compressed liquid helium (LHe) and designed for imaging and spectroscopy at ultra-low temperatures. The system includes an external dewar mounted on a vibration-damping stage and a pressurized, low-noise helium transfer line with a remotely controllable needle valve, ensuring stable and efficient LHe flow with minimal thermal and mechanical noise. Performance evaluation demonstrates a stable base temperature of 4.37 K measured using a Cernox bare chip sensor on the holder with temperature fluctuations within ±0.004 K. Complementary in-situ electron energy-loss spectroscopy (EELS) via aluminum bulk plasmon analysis was used to measure the local specimen temperature and validate cryogenic operation during experiments. The integration of cryogenic cooling with other microscopy techniques, including electron diffraction and Lorentz TEM, was demonstrated by resolving charge density wave (CDW) transitions in NbSe2 using electron diffraction, and imaging nanometric magnetic skyrmions in MnSi via Lorentz TEM. In conclusion, this platform provides reliable cryogenic operation below 7 K, establishing a low-drift route for direct visualization of electronic and magnetic phase transformations in quantum materials.

Charge density wave↗

Time Matters: A Survival Analysis of Public Electric Vehicle Charging Infrastructure Utilization

The rapid adoption of plug-in electric vehicles (PEVs) places significant demands on public charging infrastructure, making it critical to understand and optimize charger utilization. This study provides one of the most comprehensive analyses of charging behavior to date by applying a survival analysis to a dataset of nearly 16 million level 2 (L2) and direct current (DC) fast charger sessions across the United States from 2017 to 2022. Using Kaplan-Meier curves and log rank tests, our analysis reveals statistically significant and distinct duration patterns influenced by charger type, time of day, and day of the week. We find that L2 charging sessions exhibit high variability tied to venue type, whereas DC sessions are more uniform, typically lasting 30-45 min. This study introduces the operational efficiency score (OES), a metric for standardizing the performance evaluation of charging stations. Our findings offer actionable insights for optimizing charger deployment, developing dynamic pricing strategies to reduce vehicle dwell time, and improving load management for grid operators, ultimately enhancing the efficiency and availability of public charging infrastructure.

32 ENERGY CONSERVATION, CONSUMPTION, AND UTILIZATI↗

Pilot-Scale Continuous Plug-Flow Hydrothermal Liquefaction of Food Waste for Biocrude Production

Pilot-scale hydrothermal liquefaction (HTL) of biowaste is a critical step toward commercialization of the HTL technology. Despite many HTL studies conducted with wet biomass, including food waste, few were performed with a pilot-scale continuous plug-flow reactor (PFR), with the biocrude yield and quality analysis based on dewatering (ASTM D2892 Annex X1). This paper describes the development and performance evaluation of a mobile pilot-scale HTL continuous PFR, with a processing capacity of 60 L/h of wet feedstock and 6 L/h of biocrude production. The reactor system was designed for reaction conditions of up to 325 °C and 17.25 MPa. The reactor has a volume of 28.88 L with an additional counterflow heat exchanger volume of 18.07 L. Two types of food wastes, from a food processing plant and grocery store, were processed at 280 °C for 30 min, producing biocrude oil yields of 52.19 and 47.06 wt %, energy recoveries of 68.17 and 70.77%, and carbon recoveries of 66.91 and 64.78%, respectively. Furthermore, due to its high feedstock capacity and reaction volume, large amounts of biocrude oil and post-HTL wastewater (PHW) were obtained from this pilot-scale reactor to allow downstream research on upgrading biocrude oil for transportation fuel as well as PHW treatment and nutrient recovery.

09 BIOMASS FUELS↗

Catalight─An Open-Source Automated Photocatalytic Reactor Package Illustrated through Plasmonic Acetylene Hydrogenation

An open-source and modular Python package, Catalight, is developed and demonstrated to automate (photo)catalysis measurements. (Photo)catalysis experiments require studying several parameters to evaluate performance, including the temperature, gas flow rate and composition, illumination power, and spectral profile. Catalight orchestrates measurements over this complicated parameter space and systematically stores, analyzes, and visualizes the results. To showcase the capabilities of Catalight, we perform an automated apparent activation barrier measurement of acetylene hydrogenation over a plasmonic AuPd catalyst on an Al 2 O 3 support, simultaneously varying laser power, wavelength, and temperature in a multiday experiment controlled by a simple Python script. Our chemical results unexpectedly show an increased activation barrier upon light excitation, contrary to previous findings for other plasmonic reactions and catalysts. We show that the reaction rate order with respect to both acetylene and hydrogen remains unchanged upon illumination, suggesting that molecular surface coverage is not changed by light. By analyzing the inhomogeneity of the laser-induced heating, we attribute these results to a partial photothermal effect combined with a photochemical/hot electron-driven mechanism. In conclusion, our findings highlight the capabilities of a new experiment automation tool; explore the photocatalytic mechanism for an industrially relevant reaction; and identify systematic sources of error in canonical photocatalysis experimental procedures.

Catalysts↗

Poly(dimethylsiloxane- b -methyl methacrylate): A Promising Candidate for Sub-10 nm Patterning

We report herein the modular synthesis and nanolithographic potential of poly(dimethylsiloxane-block-methyl methacrylate) (PDMS-b-PMMA) with self-assembled domains approaching sub-10 nm periods. A straightforward and modular coupling strategy, optimized for low molecular weight diblocks and using copper-catalyzed azide–alkyne “click” cycloaddition, was employed to obtain a library of PDMS-b-PMMA and poly(dimethylsiloxane-block-styrene) (PDMS-b-PS) diblock copolymers. Flory–Huggins interaction parameters, determined from small-angle X-ray scattering experiments, were high for PDMS-b-PMMA (χ ~ 0.2 at 150 °C), suggesting this diblock copolymer system has promise for sub-10 nm lithographic applications when compared to the corresponding PDMS-b-PS diblock copolymers (χ ~ 0.1 at 150 °C). Furthermore, performance evaluation in thin film self-assembly experiments allowed domain periods as small as 12.1 nm to be obtained, which is among the smallest highly ordered nanoscale patterns reported hitherto for thermally annealed materials.

36 MATERIALS SCIENCE↗

Guiding Electrochemical Carbon Dioxide Reduction toward Carbonyls Using Copper Silver Thin Films with Interphase Miscibility

Steering the selectivity of Cu-based electrochemical CO2 reduction (CO2R) catalysts toward targeted products will serve to improve the technoeconomic outlook of technologies based on this process. Using physical vapor deposition as a tool to overcome thermodynamic miscibility limitations, CuAg thin films with nonequilibrium Cu/Ag alloying were prepared for CO2R performance evaluation. In comparison to pure Cu, the CuAg thin films showed significantly higher activity and selectivity toward liquid carbonyl products, including acetaldehyde and acetate. Suppressed activity and selectivity toward hydrocarbons and the competing hydrogen evolution were also demonstrated on CuAg thin films, with a greater degree of suppression observed at increasing nominal Ag compositions. Compositional-dependent CO2R trends coupled with physical characterization and density functional theory suggest that significant miscibility of Ag into the Cu-rich phase of the catalyst underpinned the observed CO2R trends through tuning of adsorbate and reaction intermediate binding energies on the surface.

10 SYNTHETIC FUELS↗

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