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All sourcesNASA NTRSDOE OSTI
DOE OSTI2026

Fingerprinting Uranium Oxides with Electron Energy Loss Spectroscopy Supported by Theoretical Computations

Uranium oxides occur in a variety of phases that differ in crystal structure and uranium oxidation states. Electron energy loss spectroscopy (EELS) is one of the few techniques that has sufficient spatial resolution and sensitivity to electronic structure to distinguish amongst phases at the nanoscale. However, beam-sensitive materials such as uranium oxides are subject to spectral modification due to interactions with the electron beam. Therefore, theory support is essential to reliably exclude the impact of beam damage and generate true reference datasets. Here we use a comparison of theoretical and experimental spectra to probe the impact of beam damage on O K-edge and U N-edge (N6,7 and N4,5) EELS spectra of various single-valent and mixed-valence uranium oxide bulk phases. Using a low-dose experimental set-up, we show that the O K-edge theoretical spectra are in excellent agreement with experiment for both peak positions and relative intensities of respective peaks. In contrast, U N-edge features are less distinguishing due to the partially localized nature of the U 5f orbitals and overlapping multiplet and spin–orbit coupling effects. This work demonstrates that O K-edge EELS is sufficiently diagnostic to distinguish a wide range of uranium oxides and that the experimental approach used here minimizes beam damage and allows valence state discrimination across the U(IV), U(V) and U(VI) series. When combined with imaging modes available in electron mi-croscopy, the work enables detailed investigation and characterization of uranium redox transformations at the nanoscale.

Carbone, Jacopo↗
DOE OSTI2021

3D simulations of vertical displacement events in tokamaks: A benchmark of M3D-C 1 , NIMROD, and JOREK

In recent years, the nonlinear 3D magnetohydrodynamic codes JOREK, M3D-C1, and NIMROD developed the capability of modeling realistic 3D vertical displacement events (VDEs) including resistive walls. In this paper, a comprehensive 3D VDE benchmark is presented between these state-of-the-art codes. The simulated case is based on an experimental NSTX plasma but with a simplified rectangular wall. There are differences between the physics models and numerical methods, and the VDE evolution leads to sensitivities on the initial conditions that cannot be avoided as can be done in edge localized modes (ELM) and sawtooth simulations (due to the non-cyclical nature of VDEs). Nonetheless, the comparison serves to quantify the level of agreement in the relevant quantities used to characterize disruptions, such as the 3D wall forces and energy decay. The results bring confidence regarding the use of the mentioned codes for disruption studies, and they distinguish aspects that are specific to the models used (e.g., reduced vs full MHD models). Here, the simulations show important 3D fea- tures for a NSTX plasma, such as the self-consistent evolution of the halo current and the origin of the wall forces. In contrast to other reduced MHD models based on an ordering in the aspect ratio, the ansatz-based JOREK reduced MHD model allows capturing many aspects of the 3D dynamics even in the spherical tokamak limit considered here.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2024

Wetting and drying trends in the land–atmosphere reservoir of large basins around the world

Abstract. Global change is altering hydrologic regimes worldwide, including large basins that play a central role in the sustainability of human societies and ecosystems. The basin water budget is a fundamental framework for understanding these basins' sensitivity and future dynamics under changing forcings. In this budget, studies often treat atmospheric processes as external to the basin and assume that atmosphere-related water storage changes are negligible in the long term. These assumptions are potentially misleading in large basins with strong land–atmosphere feedbacks, including terrestrial moisture recycling, which is critical for global water distribution. Here, we introduce the land–atmosphere reservoir (LAR) concept, which includes atmospheric processes as a critical component of the basin water budget and use it to study long-term changes in the water storage of some of the world's largest basins. Our results show significant LAR water storage trends over the last 4 decades, with a marked latitudinal contrast: while low-latitude basins have accumulated water, high-latitude basins have been drying. If they continue, these trends will disrupt the discharge regime and compromise the sustainability of these basins, resulting in widespread impacts.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2017

Nonlinear response of hail precipitation rate to environmental moisture content: A real case modeling study of an episodic midlatitude severe convective event: Hail and Environmental Moisture

The dependence of hail production on initial moisture content in a simulated midlatitude episodic convective event occurred in northeast China on 10–11 June 2005 was investigated using the Weather Research and Forecasting (WRF) model with a double-moment microphysics scheme where both graupel and hail are considered. Three sensitivity experiments were performed by modifying the initial water vapor mixing ratio profile to 90% (“Q-10%”), 105% (“Q+5%”), and 110% (“Q+10%”) of the initial conditions used for the control simulation. It was found that increasing the initial water vapor content caused the hail and total precipitation rates to increase during the first 5 h. The precipitation response to increasing water vapor content was monotonic for this first episode; however, for the event's second episode, the hail precipitation rate responds to the initial water vapor profile nonlinearly, while the total precipitation rate responds mostly monotonically. In particular, simulation Q+5% achieves the largest hail production rate while simulation Q+10% has the largest total precipitation rate. In contrast, during the second episode simulation Q-10% has the strongest vertical motion, produces the most cloud ice and snow, but has the lowest hail production. Analysis shows that increasing the initial moisture content directly increases the precipitation during the first episode, which subsequently induces a stronger, longer-asting cold pool that limits the development of deep convection during the second episode.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2014

A Holocene East Asian winter monsoon record at the southern edge of the Gobi Desert and its comparison with a transient simulation

The East Asian winter monsoon (EAWM) exhibits significant variability on intraseasonal, interannual, and interdecadal time scales and the variability can be extended to Holocene centennial and millennial scales. Previous Holocene EAWM proxy data records, which were mostly located in Central, Eastern and Southern China, did not show a consistent Holocene EAWM history. Therefore, it is difficult to provide insights into mechanisms of the long-term winter monsoon variability on the basis of the records. Eolian sediments at the southern edge of the Gobi Desert, Western China, are sensitive to the EAWM changes and less affected by the East Asian summer monsoon due to an obstruction of the Qinghai–Tibet Plateau. Here, this paper presents a comparison between a well-dated Holocene EAWM record and coupled climate model simulations, so as to explore physical processes and influencing factors of the Holocene EAWM. Sediment samples from two Holocene eolian sedimentary sections [Huangyanghe (a) and Huangyanghe (b)] were acquired at the southern edge of the Gobi Desert. Chronologies were established based on twenty bulk organic matter AMS 14 C ages and five pollen concentrates AMS 14 C ages. Proxy data, including grain-size, total organic carbon, magnetic susceptibility and carbonate content were obtained from the two eolian sections. The grain-size standard deviation model was applied to determine components sensitive to variability of the Holocene EAWM. After a comparison of environmentally-sensitive grain-size components and proxy data, the 20–200 μm component at the Huangyanghe (a) and the 20–159 μm component at the Huangyanghe (b) section were selected as indicators of the Holocene EAWM, which show a strong early Holocene winter monsoon and a decline of the winter monsoon since the mid-Holocene. We also present equilibrium and transient simulations of the climate evolution for the Holocene using a state-of-art coupled climate model: the Community Climate System Model version 3 (CCSM3). Indices for the Holocene EAWM were calculated and are consistent with the reconstructed Holocene EAWM intensity. The simulations indicate that orbital forcing effects on the land-sea temperature and sea level pressure contrast can account for the observed EAWM trends. Other forcings that were present in the early Holocene, including the remnant Laurentide ice sheet and meltwater forcing in the North Atlantic, were not responsible for the Holocene trends.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2015

Exploring the decision-space for renewable energy generation to enhance spatial efficiency

Decentralized power generation can play a significant role in contributing to renewable energy (RE) supply. Accordingly, regions can be important players in the transformation of the energy system. However, only scarce spatial capacities are available for a sustainable RE generation. Knowledge gaps exist concerning data and methods for integrating RE assessment and environmental planning methods. This paper presents a methodology for the integrated assessment of different RE potentials and their land requirements. The potential is contrasted with the actual availability of land for RE-generation considering environmental restrictions. An application in the Hanover region demonstrates that using energy capacity maps supports using the most efficient mixture in RE generation. Generally, a combination of wind and solar energies produces the highest energy yield per ha. Furthermore, relying primarily on generalized environmental restrictions for defining exclusion areas can be only a first step: On the one hand the assessment is probably underrating the potential for environmentally sound RE generation due to the undifferentiated exclusion of large areas of a certain protective status. On the other hand, some energy sources, in particular energy crops for bioenergy generation, are malpositioned due to missing spatially explicit information about ecosystem sensitivities and a lack of regulative possibilities. Further research is needed to explore synergistic combinations of energy potentials and their environmentally sound spatial allocation in more detail. - Highlights: • We combine models of RE potentials with technical and environmental restrictions. • We explore the resulting “decision-spaces” for regional RE development. • “Decision-spaces” are small and need to be developed carefully to avoid trade-offs. • Planning needs more differentiated analyses to test RE allocation-scenarios. • We recommend detailed analyses on (cumulative) impacts of (multifunctional) RE use.

14 SOLAR ENERGY↗
DOE OSTI2021

High-resolution multicontrast tomography with an X-ray microarray anode–structured target source

Multicontrast X-ray imaging with high resolution and sensitivity using Talbot–Lau interferometry (TLI) offers unique imaging capabilities that are important to a wide range of applications, including the study of morphological features with different physical properties in biological specimens. The conventional X-ray TLI approach relies on an absorption grating to create an array of micrometer-sized X-ray sources, posing numerous limitations, including technical challenges associated with grating fabrication for high-energy operations. We overcome these limitations by developing a TLI system with a microarray anode–structured target (MAAST) source. The MAAST features an array of precisely controlled microstructured metal inserts embedded in a diamond substrate. Using this TLI system, tomography of a Drum fish tooth with high resolution and tri-contrast (absorption, phase, and scattering) reveals useful complementary structural information that is inaccessible otherwise. The results highlight the exceptional capability of high-resolution multicontrast X-ray tomography empowered by the MAAST-based TLI method in biomedical applications.

47 OTHER INSTRUMENTATION↗
DOE OSTI2023

Vegetation Representation Influences Projected Streamflow Changes in the Colorado River Basin

Vegetation parameters for the Variable Infiltration Capacity (VIC) hydrologic model were recently updated using observations from the Moderate Resolution Imaging Spectroradiometer (MODIS). Previous work showed that these MODIS-based parameters improved VIC evapotranspiration simulations when compared to eddy covariance observations. Due to the importance of evapotranspiration within the Colorado River basin, this study provided a basin-by-basin calibration of VIC soil parameters with updated MODIS-based vegetation parameters to improve streamflow simulations. Interestingly, while both configurations had similar historic streamflow performance, end-of-century hydrologic projections, driven by 29 downscaled global climate models under the RCP8.5 emissions scenario, differed between the two configurations. The calibrated MODIS-based configuration had an ensemble mean that simulated little change in end-of-century annual streamflow volume (+0.4%) at Lees Ferry, Arizona, relative to the historical period (1960–2005). In contrast, the previous VIC configuration, which is used to inform decisions about future water resources in the Colorado River basin, projected an 11.7% decrease in annual streamflow. Both VIC configurations simulated similar amounts of evapotranspiration in the historical period. However, the MODIS-based VIC configuration did not show as much of an increase in evapotranspiration by the end of the century, primarily within the upper basin’s forested areas. Differences in evapotranspiration projections were the result of the MODIS-based vegetation parameters having lower leaf area index values and less forested area compared to previous vegetation estimates used in recent Colorado River basin hydrologic projections. These results highlight the need to accurately characterize vegetation and better constrain climate sensitivities in hydrologic models.

54 ENVIRONMENTAL SCIENCES↗
NASA NTRS1994

Monitoring Mars with the Hubble Space Telescope: 1990-1991 observations

Images of Mars obtained using the Planetary Camera on the Hubble Space Telescope during 1990 and 1991 are described and analyzed. Multispectral images of Mars record the martian season between L(sub s) = 348 deg and 60 deg corresponding to late winter and spring in the northern hemisphere. The wavelengths of these observations varied between 230 nm in the ultraviolet and 890 nm in the near infrared. We use these images to discuss atmospheric and polar phenomena, to constrain the aerosols and ozone in the martian atmosphere, and to compare surface albedo features within this data set as well as with previous observations. Two methods are used to constrain the opacity of the martian atmosphere: comparisons of ultraviolet images with atmospheric scattering models and examination of contrast changes of surface features observed at visible wavelengths. Our observations are consistent with a Mars which was quite different from the planet when it was viewed by Viking; we estimate an upper limit of 0.1 for equatorial dust opacity near vernal equinox, compared to values of 0.4 to 0.5 measured in Chryse by Viking Lander 1. Later, at L(sub s) = 60 deg, and upper limit of 0.2 was found for dust in the southern hemisphere. Except for suggestions of local dust activity near the north polar cap in late spring, there was no visual evidence of dust storms on the planet. The Hartley band of ozone is within the F230W filter bandpass, and the 230W/336W ratio is therefore sensitive to ozone. High latitude ozone is observed at a concentration similar to that observed by Mariner 9; a seasonal dependence in ozone concentration was observed with concentration decreasing at northern arctic latitudes and increasing at southern midlatitudes as L(sub s) increases from 350 deg to 60 deg. Despite the difference in dust loading, the behavior of condensate clouds and the recession of the north polar cap are consistent with those observed during Viking years. Late winter images of the north polar region reveal an active north polar hood with a maximum (UV) opacity of about 0.25 near 50 deg latitude; the hood seems to have an annular form, with the central, polar regions having smaller opacity. Clouds observed in the northern hemisphere to the south of the hood boundary are suggestive of fronts similar to those observed during the Mariner 9 mission. A diurnal variation in the hood clouds which is (anti) correlated with the amount of water vapor in the atmosphere is noted. Images were deconvolved using the Richardson-Lucy iterative algorithm to remove the defocussing effects of the spherical aberration of the HST primary. Even when Mars subtended less than 5 arcsec, in May 1991, the images were scientifically useful and comparable to photographic images obtained at opposition. Although the data are subject to the solar pointing constraint for HST, the relatively slow movement of the allowed observation window, which is more than one half martian year, with respect to the martian seasons will permit us to address the question of major variations in the martian atmosphere.

James, Philip B.↗
NASA NTRS2004

Diffraction and imaging study of imperfections of crystallized lysozyme with coherent X-rays

Phase-contrast X-ray diffraction imaging and high-angular-resolution diffraction combined with phase-contrast radiographic imaging were employed to characterize defects and perfection of a uniformly grown tetragonal lysozyme crystal in the symmetric Laue case. The full-width at half-maximum (FWHM) of a 4 4 0 rocking curve measured from the original crystal was approximately 16.7 arcsec and imperfections including line defects, inclusions and other microdefects were observed in the diffraction images of the crystal. The observed line defects carry distinct dislocation features running approximately along the <1 1 0> growth front and have been found to originate mostly in a central growth area and occasionally in outer growth regions. Inclusions of impurities or formations of foreign particles in the central growth region are resolved in the images with high sensitivity to defects. Slow dehydration led to the broadening of a fairly symmetric 4 4 0 rocking curve by a factor of approximately 2.6, which was primarily attributed to the dehydration-induced microscopic effects that are clearly shown in X-ray diffraction images. The details of the observed defects and the significant change in the revealed microstructures with drying provide insight into the nature of imperfections, nucleation and growth, and the properties of protein crystals.

Muramidase/chemistry↗
DOE OSTI2019

Frequency-based detection of chemical expansion dynamics in thin films

Current techniques for measuring chemical expansion in thin film structures are too slow, too imprecise, or require synchrotrons. In contrast, nanoscale electrochemomechanical spectroscopy (NECS) can be used to make nanoscale measurements at time scales of seconds with simple contact or non-contact sensors. In a NECS measurement, a sample, such as thin-film oxide structure, is subjected to a temporally modulated stimulus, such as a sinusoidally alternating voltage. The stimulus causes the sample to expand, contract, deflect, or otherwise deform. A sensor, such as a contact probe or optical sensor, produces an electrical signal in response to this deformation that is correlated with the temporal modulation of the stimulus. Because the stimulus and deformation are correlated, the temporal modulation of the stimulus can be used to filter the deformation signal produced by the sensor, producing a precise, sensitive measurement of the deformation.

36 MATERIALS SCIENCE↗
DOE OSTI2025

Temperature sensitivity of the equilibrium neutronics and accident analysis of the HTR-10

Pebble-Bed High-Temperature Gas-cooled Reactors (PB-HTGR) are moderated by the graphite in the fuel pebbles and the graphite reflector surrounding the pebble-bed. Because graphite is by far the most abundant material in PB-HTGRs and the primary moderator, accurate modeling of the graphite material, including density, impurities, and temperatures, is crucial for accurate computational modeling and simulation of these reactors. While main characteristics of the graphite components are often known, the local temperature is less well known and often averaged over all components. Here, this work studies the impact of considering accurate temperature profiles in the graphite material on the generation of a small PB-HTGR model at the state of equilibrium operation and on short-term accident progression. The fuel compositions for the PB-HTGR were determined using a jump-in equilibrium modeling method, the Axial Radial Zone Equilibrium Modeling (AR-ZEM) method. In contrast to previous work, the AR-ZEM method was used considering thermal-hydraulic feedback from the MELCOR code to determine temperatures of the fuel pebbles and the surrounding graphite reflector. The consideration of an axial and radial temperature profile in the core and reflector, as opposed to uniform material temperatures, had an impact of almost 1,300 pcm on the equilibrium core eigenvalue and caused significant differences in the discharged plutonium fuel inventory with up to 4.9% and 11.0% for Pu-239 and Pu-242, respectively. To assess the impact on short-term accident progression, two Anticipated Transient Without SCRAM (ATWS) events, a Pressurized Loss of Forced Coolant (PLOFC) and a Control Rod Withdrawal (CRW) with loss of flow, were simulated with MELCOR. The use of temperature profiles in the equilibrium core models did not reveal a significant impact on the temperature, power, or reactivity responses during the transients. In conclusion, a need for consideration of accurate temperature profiles, in particular for the graphite reflector, was found for the generation of equilibrium PB-HTGRs core models using jump-in methods, but detailed temperature profiles may not be necessary when performing conservative transient analysis.

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗
DOE OSTI2025

Unraveling the Structural Sensitivity of Metal Catalysts in Ethylene Hydroformylation: Insights from Theory and Experiments

Here, in this study, we combined experimental and theoretical methods to investigate the structural sensitivity of metal catalysts in the ethylene hydroformylation reaction. Among Rh, Pt, Ir, Ni, Au, Ag, Pd, and Cu catalysts studied using experimental and theoretical methods, Rh showed the highest selectivity toward the C-C coupling product from CO and C 2 H 5 (i.e., C 2 H 5 CHO). The results from DFT and microkinetic simulations revealed that the activation energy barrier for C-C coupling is lowest on the Rh nanocluster, which explains the experimentally observed highest C 2 H 5 CHO selectivity on the Rh catalyst. Furthermore, DFT results demonstrated that the sites located on the flat surfaces of nanoparticles primarily promote the hydrogenation reaction, leading to the formation of undesired C 2 H 6 . In contrast, undercoordinated edge and corner sites of the nanocluster promote the C-C coupling reaction. Thus, our results illustrate that the selectivity toward C 3 oxygenates in ethylene hydroformylation reaction can be steered by tuning the size of Rh nanoparticles (the best-performing catalyst) to optimize the active (edge and corner) sites that preferentially promote the C-C coupling reaction.

58 GEOSCIENCES↗
DOE OSTI2015

Systematic theoretical investigation of the zero-field splitting in Gd(III) complexes: Wave function and density functional approaches

The zero-field splitting (ZFS) of the electronic ground state in paramagnetic ions is a sensitive probe of the variations in the electronic and molecular structure with an impact on fields ranging from fundamental physical chemistry to medical applications. A detailed analysis of the ZFS in a series of symmetric Gd(III) complexes is presented in order to establish the applicability and accuracy of computational methods using multiconfigurational complete-active-space self-consistent field wave functions and of density functional theory calculations. The various computational schemes are then applied to larger complexes Gd(III)DOTA(H{sub 2}O){sup −}, Gd(III)DTPA(H{sub 2}O){sup 2−}, and Gd(III)(H{sub 2}O){sub 8}{sup 3+} in order to analyze how the theoretical results compare to experimentally derived parameters. In contrast to approximations based on density functional theory, the multiconfigurational methods produce results for the ZFS of Gd(III) complexes on the correct order of magnitude.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2018

Impact ignition and combustion of micron-scale aluminum particles pre-stressed with different quenching rates

Pre-stressing aluminum (Al) particles by annealing and quenching alters dilatational strain and is linked to increased particle reactivity. The quenching rate associated with pre-stressing is a key parameter affecting the final stress state within the Al particle, with faster quenching rates theoretically favoring a higher, more desirable stress state. Micron scale Al particles are annealed to 573 K, then quenched at different rates (i.e., 200 and 900 K/min), mixed with bismuth oxide (Bi2O 3 ), and the Al + Bi2O 3 mixtures are examined under low-velocity, drop-weight impact conditions. Both quenching rates showed increased impact ignition sensitivity (i.e., between 83% and 89% decrease in ignition energy). However, the slower quenching rate showed a 100% increase in pressurization rate compared to untreated particles, while the faster quenching rate showed a 97% increase in peak pressure, indicating that these two quenching rates affect Al particles differently. Surprisingly, synchrotron X-ray diffraction data show that the 200 K/min quenched particles have a higher dilatational strain than the untreated particles or the 900 K/min quenched particles. Results are rationalized with the help of a simple mechanical model that takes into account elastic stresses, creep in the alumina shell, and delamination of shell from the core. The model predicts that Al powder quenched at 200 K/min did not experience delamination. In contrast, Al quenched at 900 K/min did not have creep but does have delamination, and under impact, delamination led to major fracture, greater oxygen access to the core, and significant promotion of reaction. Thus, the increase in quenching rate and shell-core delamination are more important for the increase in Al reactivity than pre-stressing alone.

42 ENGINEERING↗
DOE OSTI2014

Constraints on the progenitor system and the environs of SN 2014J from deep radio observations

We report deep EVN and eMERLIN observations of the Type Ia SN 2014J in the nearby galaxy M82. Our observations represent, together with JVLA observations of SNe 2011fe and 2014J, the most sensitive radio studies of Type Ia SNe ever. By combining data and a proper modeling of the radio emission, we constrain the mass-loss rate from the progenitor system of SN 2014J to M-dot ≲7.0×10{sup −10} M{sub ⊙} yr{sup −1} (for a wind speed of 100 km s{sup –1}). If the medium around the supernova is uniform, then n {sub ISM} ≲ 1.3 cm{sup –3}, which is the most stringent limit for the (uniform) density around a Type Ia SN. Our deep upper limits favor a double-degenerate (DD) scenario—involving two WD stars—for the progenitor system of SN 2014J, as such systems have less circumstellar gas than our upper limits. By contrast, most single-degenerate (SD) scenarios, i.e., the wide family of progenitor systems where a red giant, main-sequence, or sub-giant star donates mass to an exploding WD, are ruled out by our observations. (While completing our work, we noticed that a paper by Margutti et al. was submitted to The Astrophysical Journal. From a non-detection of X-ray emission from SN 2014J, the authors obtain limits of M-dot ≲1.2×10{sup −9} M {sub ☉} yr{sup –1} (for a wind speed of 100 km s{sup –1}) and n {sub ISM} ≲ 3.5 cm{sup –3}, for the ρ∝r {sup –2} wind and constant density cases, respectively. As these limits are less constraining than ours, the findings by Margutti et al. do not alter our conclusions. The X-ray results are, however, important to rule out free-free and synchrotron self-absorption as a reason for the radio non-detections.) Our estimates on the limits on the gas density surrounding SN2011fe, using the flux density limits from Chomiuk et al., agree well with their results. Although we discuss the possibilities of an SD scenario passing observational tests, as well as uncertainties in the modeling of the radio emission, the evidence from SNe 2011fe and 2014J points in the direction of a DD scenario for both.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2015

WEATHER ON OTHER WORLDS. II. SURVEY RESULTS: SPOTS ARE UBIQUITOUS ON L AND T DWARFS

We present results from the Weather on Other Worlds Spitzer Exploration Science program to investigate photometric variability in L and T dwarfs, usually attributed to patchy clouds. We surveyed 44 L3-T8 dwarfs, spanning a range of J – K{sub s} colors and surface gravities. We find that 14/23 (61%{sub −20%}{sup +17%}, 95% confidence) of our single L3-L9.5 dwarfs are variable with peak-to-peak amplitudes between 0.2% and 1.5%, and 5/16 (31%{sub −17%}{sup +25%}) of our single T0-T8 dwarfs are variable with amplitudes between 0.8% and 4.6%. After correcting for sensitivity, we find that 80%{sub −27%}{sup +20%} of L dwarfs vary by ≥0.2%, and 36%{sub −17%}{sup +26%} of T dwarfs vary by ≥0.4%. Given viewing geometry considerations, we conclude that photospheric heterogeneities causing >0.2% 3-5 μm flux variations are present on virtually all L dwarfs, and probably on most T dwarfs. A third of L dwarf variables show irregular light curves, indicating that L dwarfs may have multiple spots that evolve over a single rotation. Also, approximately a third of the periodicities are on timescales >10 hr, suggesting that slowly rotating brown dwarfs may be common. We observe an increase in the maximum amplitudes over the entire spectral type range, revealing a potential for greater temperature contrasts in T dwarfs than in L dwarfs. We find a tentative association (92% confidence) between low surface gravity and high-amplitude variability among L3-L5.5 dwarfs. Although we can not confirm whether lower gravity is also correlated with a higher incidence of variables, the result is promising for the characterization of directly imaged young extrasolar planets through variability.

79 ASTRONOMY AND ASTROPHYSICS↗
NASA NTRS1989

On the Nature of Navier-stokes Turbulence

Several turbulent and nonturbulent solutions of the Navier-Stokes equations are obtained. The unaveraged equations are used numerically in conjunction with tools and concepts from nonlinear dynamics, including time series, phase portraits, Poincare sections, largest Liapunov exponents, power spectra, and strange attractors. Initially neighboring solutions for a low-Reynolds-number fully developed turbulence are compared. The solutions, separate exponentially with time, having a positive Liapunov exponent. Thus the turbulence is characterized as chaotic. In a search for solutions which contrast with the turbulent ones, the Reynolds number is reduced. Several qualitatively different flows are noted. These are, fully chaotic, complex period, weakly chaotic, simple periodic, and fixed-point. Of these, only the fully chaotic flows are classified as turbulent. Those flows have both a positive Liapunov exponent and Poincare sections without pattern. By contrast, the weakly chaotic flows have some pattern in their Poincare sections. The fixed-point and periodic flows are nonturbulent, since turbulence, is both time-dependent and aperiodic. Turbulent solutions are obtained in which energy cascades from large to small-scale motions. In general, the spectral energy transfer takes place between wavenumber bands that are considerably separated. The special transfer can occur either as a result of nonlinear turbulence self-interaction or by interaction of turbulence with mean gradients. Turbulent systems are compared with those studied in kinetic theory. The two types of systems are fundamentally different (continuous and dissipative as opposed to discrete and conservative), but there are similarities. For instance, both are nonlinear and show sensitive dependence on initial conditions. Also, the turbulent and molecular stress tensors are identical if the macroscopic velocities for the turbulent stress are replaced by molecular velocities.

Deissler, Robert G.↗

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