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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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All sourcesNASA NTRSDOE OSTI
NASA NTRS2017

Mars Atmospheric Conversion to Methane and Water: An Engineering Model of the Sabatier Reactor with Characterization of Ru/Al2O3 for Long Duration Use on Mars

The Atmospheric Processing Module (APM) is a Mars In-Situ Resource Utilization (ISRU) technology designed to demonstrate conversion of the Martian atmosphere into methane and water. The Martian atmosphere consists of approximately 95 carbon dioxide (CO2) and residual argon and nitrogen. APM utilizes cryocoolers for CO2 acquisition from a simulated Martian atmosphere and pressure. The captured CO2 is sublimated and pressurized as a feedstock into the Sabatier reactor, which converts CO2 and hydrogen to methane and water. The Sabatier reaction occurs over a packed bed reactor filled with Ru/Al2O3 pellets. The long duration use of the APM system and catalyst was investigated for future scaling and failure limits. Failure of the catalyst was detected by gas chromatography and temperature sensors on the system. Following this, characterization and experimentation with the catalyst was carried out with analysis including x-ray photoelectron spectroscopy and scanning electron microscopy with elemental dispersive spectroscopy. This paper will discuss results of the catalyst performance, the overall APM Sabatier approach, as well as intrinsic catalyst considerations of the Sabatier reactor performance incorporated into a chemical model.

Ru/Al2O3 Catlayst↗
NASA NTRS2017

Mars Atmospheric Conversion to Methane and Water: An Engineering Model of the Sabatier Reactor with Characterization of Ru/Al2O3 for Long Duration Use on Mars

The Atmospheric Processing Module (APM) is a Mars In-Situ Resource Utilization (ISRU) technology designed to demonstrate conversion of the Martian atmosphere into methane and water. The Martian atmosphere consists of approximately 95 carbon dioxide (CO2) and residual argon and nitrogen. APM utilizes cryocoolers for CO2 acquisition from a simulated Martian atmosphere and pressure. The captured CO2 is sublimated and pressurized as a feedstock into the Sabatier reactor, which converts CO2 and hydrogen to methane and water. The Sabatier reaction occurs over a packed bed reactor filled with Ru/Al2O3 pellets. The long duration use of the APM system and catalyst was investigated for future scaling and failure limits. Failure of the catalyst was detected by gas chromatography and temperature sensors on the system. Following this, characterization and experimentation with the catalyst was carried out with analysis including x-ray photoelectron spectroscopy and scanning electron microscopy with elemental dispersive spectroscopy. This paper will discuss results of the catalyst performance, the overall APM Sabatier approach, as well as intrinsic catalyst considerations of the Sabatier reactor performance incorporated into a chemical model.

Catlayst↗
NASA NTRS2017

Atmospheric Form Drag Coefficients Over Arctic Sea Ice Using Remotely Sensed Ice Topography Data, Spring 2009-2015

Sea ice topography significantly impacts turbulent energy/momentum exchange, e.g., atmospheric (wind) drag, over Arctic sea ice. Unfortunately, observational estimates of this contribution to atmospheric drag variability are spatially and temporally limited. Here we present new estimates of the neutral atmospheric form drag coefficient over Arctic sea ice in early spring, using high-resolution Airborne Topographic Mapper elevation data from NASA's Operation IceBridge mission. We utilize a new three-dimensional ice topography data set and combine this with an existing parameterization scheme linking surface feature height and spacing to form drag. To be consistent with previous studies investigating form drag, we compare these results with those produced using a new linear profiling topography data set. The form drag coefficient from surface feature variability shows lower values [less than 0.5-1 × 10(exp. −3)] in the Beaufort/Chukchi Seas, compared with higher values [greater than 0.5-1 ×10(exp. −3)] in the more deformed ice regimes of the Central Arctic (north of Greenland and the Canadian Archipelago), which increase with coastline proximity. The results show moderate interannual variability, including a strong increase in the form drag coefficient from 2013 to 2014/2015 north of the Canadian Archipelago. The form drag coefficient estimates are extrapolated across the Arctic with Advanced Scatterometer satellite radar backscatter data, further highlighting the regional/interannual drag coefficient variability. Finally, we combine the results with existing parameterizations of form drag from floe edges (a function of ice concentration) and skin drag to produce, to our knowledge, the first pan-Arctic estimates of the total neutral atmospheric drag coefficient (in early spring) from 2009 to 2015.

sea ice↗
NASA NTRS2017

Results from a Set of Three-Dimensional Numerical Experiments of a Hot Jupiter Atmosphere

We present highlights from a large set of simulations of a hot Jupiter atmosphere, nominally based on HD 209458b, aimed at exploring both the evolution of the deep atmosphere, and the acceleration of the zonal flow or jet. We find the occurrence of a super-rotating equatorial jet is robust to changes in various parameters, and over long timescales, even in the absence of strong inner or bottom boundary drag. This jet is diminished in one simulation only, where we strongly force the deep atmosphere equator-to-pole temperature gradient over long timescales. Finally, although the eddy momentum fluxes in our atmosphere show similarities with the proposed mechanism for accelerating jets on tidally-locked planets, the picture appears more complex. We present tentative evidence for a jet driven by a combination of eddy momentum transport and mean flow.

hydrodynamics↗
NASA NTRS2017

The Net Decay Time of Anomalies in Concentrations of Atmospheric Pollutants

This paper introduces a new parameter to characterize the random component in temporal variability of atmospheric pollutants and proposes a simple statistical technique for its evaluation. That parameter is the net decay time (or the time scale) of the local anomalies in concentrations of atmospheric pollutants, rather than the traditionally used chemical lifetimes of total amounts of the species. Using widely available data of hourly multi-year surface trace gas pollutant concentrations we demonstrate a simplified way to estimate the net decay time with an exponential approximation of lag-correlation functions. We assessed the decay times of fluctuations in observations of eight atmospheric pollutants (SO2, NO, NO2, NOy, O3, CO, NH3, and HNO3) at two urban sites and one cleaner rural site in the Eastern US. The time scales of temporal fluctuations (net decay times) vary from about one hour to slightly more than one day. These scales are generally much shorter in urban environments than in remote regions. We also compared day- and night-time observations in warm and cold seasons. At night in the cold season, time scales of fluctuations in atmospheric pollutants are usually the longest. Such estimates should be useful to air quality prediction, public health, and satellite remote sensing research communities.

air quality prediction↗
NASA NTRS2018

Does Orbital Angular Momentum Have Effect on Laser’s Scattering by Molecular Atmosphere?

Lasers with orbital angular momentum (OAM) have potential applications in communication technology, manipulation of particles, and remote sensing. Because of its unusual light-scattering properties, the OAM laser’s interaction with a molecular atmosphere must be studied to ensure that it is not lossy for communication or remote-sensing applications that involve its transmission through an atmospheric environment. In this study, the finite-difference time-domain (FDTD) method [21] is applied to calculate the light scattering of the purely azimuthal (the radial mode number is assumed to be zero) Laguerre-Gaussian (LG) beams with OAM by very small dielectric particles. Not like Lorentz-Mie solutions, the FDTD method can calculate for particles off the central axis of the LG beam. It is found that when the particles are very small, and the topological charge number of the OAM of a laser is not extremely large, the laser’s OAM has little effect on the scattering phase function. This suggests that Rayleigh theory can be applied directly to calculate the light scattering by atmospheric molecules. The transmission of a laser beam with OAM in a molecular atmosphere is not different from that of a regular Gaussian beam.

Molecular atmosphere↗
NASA NTRS2021

Atmospheric Correction Over Ocean for Hyperspectral Radiometers Using Multi-Angle Polarimetric Retrievals

We developed a fast and accurate POLYnomial based Atmospheric Correction (POLYAC) algorithm for hyperspectral radiometric measurements, which parameterizes the atmospheric path radiances using aerosol properties retrieved from co-located multi-wavelength Multi-Angle Polarimeter (MAP) measurements. This algorithm has been applied to co-located Spectrometer for Planetary Exploration (SPEX) airborne and Research Scanning Polarimeter (RSP) measurements, where SPEX airborne was used as a proxy of hyperspectral radiometers, and RSP as the MAP. The hyperspectral remote sensing reflectance obtained from POLYAC is accurate when compared to Aerosol Robotic Network (AERONET), and Visible Infrared Imaging Radiometer Suite (VIIRS) ocean color products. POLYAC provides a robust alternative atmospheric correction algorithm for hyperspectral or multi-spectral radiometric measurements for scenes involving coastal oceans and/or absorbing aerosols, where traditional atmospheric correction algorithms are less reliable.

ocean color↗
NASA NTRS2020

Decadal Changes in the Interannual Variability of Heat Waves in East Asia Caused by Atmospheric Teleconnection Changes

The heat wave in East Asia is examined by using empirical orthogonal function analysis to isolate dominant heat-wave patterns in the ground-based temperature observations over the Korean Peninsula and China and related large-scale atmospheric circulations obtained from the National Centers for Environmental Prediction–National Center for Atmospheric Research Reanalysis 1 during 1973–2012. This study focuses particularly on the interannual variability of heat waves and its decadal change. The analysis identifies two major atmospheric teleconnection patterns playing an important role in developing typical heat-wave patterns in East Asia—the Scandinavian (SCAND) and the circumglobal teleconnection (CGT) patterns, which exhibit a significant decadal change in the interannual variability in the mid-1990s. Before the mid-1990s, heat-wave occurrence was closely related to the CGT pattern, whereas the SCAND pattern is more crucial to explain heat-wave variability in the recent period. The stationary wave model experiments suggest an intensification of the SCAND pattern in the recent period driven by an increase in land–atmosphere interaction over Eurasia and decadal change in the dominant heat-wave patterns in East Asia.

heat wave patterns↗
NASA NTRS2022

Optimal Estimation Framework for Ocean Color Atmospheric Correction and Pixel-level Uncertainty Quantification

Ocean color remote sensing requires compensation for atmospheric scattering and absorption (aerosol, Rayleigh, and trace gases), referred to as atmospheric correction (AC). AC allows inference of parameters such as spectrally resolved remote sensing reflectance ( R rs )(λ) ; sr 1 ) at the ocean surface from the top-of-atmosphere reflectance. Often, the uncertainty of this process is not fully explored. Bayesian inference techniques provide a simultaneous AC and uncertainty assessment via a full posterior distribution of the relevant variables, given the prior distribution of those variables and the radiative transfer (RT) likelihood function. Given uncertainties in the algorithm inputs, the Bayesian framework enables better constraints on the AC process by using the complete spectral information compared to traditional approaches that use only a subset of bands for AC. This paper investigates a Bayesian inference research method (Optimal Estimation, OE) for ocean color AC by simultaneously retrieving atmospheric and ocean properties using all visible and near-infrared spectral bands. The OE algorithm analytically approximates the posterior distribution of parameters based on normality assumptions and provides a potentially viable operational algorithm with a reduced computational expense. We developed a Neural Network (NN) RT forward model look-up-table-based emulator to increase algorithm efficiency further and thus speed up the likelihood computations. We then applied the OE algorithm to synthetic data and observations from the MODerate resolution Imaging Spectroradiometer (MODIS) on NASA’s Aqua spacecraft. We compared the R rs )(λ) retrieval and its uncertainty estimates from the OE method with in-situ validation data from the SeaWiFS Bio-optical Archive and Storage System (SeaBASS) and Aerosol Robotic Network Ocean Color (AERONET-OC) datasets. The OE algorithm improved R rs )(λ) estimates relative to the NASA standard operational algorithm by improving all statistical metrics at 443, 555, and 667 nm. Unphysical negative R rs )(λ) , which often appear in complex water conditions, was reduced by a factor of 3. The OE-derived pixel-level R rs )(λ) uncertainty estimates were also assessed relative to in-situ data and were shown to have skill.

Atmospheric correction↗
NASA NTRS2015

Stratospheric Temperatures and Water Loss From Moist Greenhouse Atmospheres of Earth-Like Planets

A radiative-convective climate model is used to calculate stratospheric temperatures and water vapor concentrations for ozone-free atmospheres warmer than that of modern Earth. Cold, dry stratospheres are predicted at low surface temperatures, in agreement with recent 3D calculations. However, at surface temperatures above 350 K, the stratosphere warms and water vapor becomes a major upper atmospheric constituent, allowing water to be lost by photodissociation and hydrogen escape. Hence, a moist greenhouse explanation for loss of water from Venus, or some exoplanet receiving a comparable amount of stellar radiation, remains a viable hypothesis. Temperatures in the upper parts of such atmospheres are well below those estimated for a gray atmosphere, and this factor should be taken into account when performing inverse climate calculations to determine habitable zone boundaries using 1D models.

Astrobiology↗
NASA NTRS2023

Future Atmospheric Rivers and Impacts on Precipitation: Overview of the ARTMIP Tier2 High-Resolution Global Warming Experiment

Atmospheric rivers (ARs) are long, narrow synoptic scale weather features important for Earth’s hydrological cycle typically transporting water vapor poleward, delivering precipitation important for local climates. Understanding ARs in a warming climate is problematic because the AR response to climate change is tied to how the feature is defined. The Atmospheric River Tracking Method Intercomparison Project (ARTMIP) provides insights into this problem by comparing 16 atmospheric river detection tools (ARDTs) to a common dataset consisting of high resolution climate change simulations from a global atmospheric general circulation model. ARDTs mostly show increases in frequency and intensity, but the scale of the response is largely dependent on algorithmic criteria. Across ARDTs, bulk characteristics suggest intensity and spatial footprint are inversely correlated, and most focus regions experience increases in precipitation volume coming from extreme ARs. The spread of the AR precipitation response under climate change is large and dependent on ARDT selection.

Atmospheric Rivers↗
NASA NTRSDate not supplied

Warming Reduces the Efficacy of Wet Conditions to Moderate Extreme Heat and Atmospheric Aridity Across the Central Plains

In the literature, dry land surface conditions possess a well-established association with extreme heat and high atmospheric aridity, especially in regions that experience strong land-atmosphere feedbacks. However, few studies have examined whether global warming will impact the ability of wet conditions to constrain high temperatures and atmospheric aridity occurrences. Here we investigate how wet conditions, which we define using precipitation and soil moisture, constrain high temperature and high vapor pressure deficit during the warm season over the Central Plains in North America at different global warming levels (0-3 degrees K). Using a CMIP6 multi-model ensemble, we show that absolute changes in the maximum temperature distribution outweigh the historical cooling effect of high precipitation or soil moisture conditions, reducing the probability of non-extreme maximum temperatures under global warming. Strikingly, the conditional likelihood of non-extreme maximum temperatures falls from 97-98% at baseline conditions to 50-58% at 1 degree of global warming. Once 2 degrees of warming is reached, there is very little probability of constraining extreme maximum temperatures. On the other hand, high precipitation and high soil moisture are able to better retain the ability to constrain concurrent high vapor pressure deficit conditions – moving from 99% at baseline conditions to 81-91% at 1 degree of warming and 26-42% at 2 degrees of warming. With our results, we find that the extent of this retention is dependent on how individual models represent relative changes in the VPD distribution as temperatures warm. Overall, our results highlight the growing vulnerability of the Central North American region to warmer temperatures and drier atmospheric conditions, even during periods of high precipitation and soil moisture.

Extreme heat↗
NASA NTRSDate not supplied

PACE UV-VIS Polarimetric Remote Sensing of Atmosphere-Ocean Systems: Sensitivity to Variations in Brown Carbon

The NASA Plankton, Aerosol, Cloud, and ocean Ecosystem (PACE) mission, scheduled for launch in 2024, will carry two instruments that measure ultraviolet (UV) radiance emerging from the top of the atmosphere: the Ocean Color Instrument (OCI) and the Spectro-Polarimeter for Planetary Exploration (SPEXone) instrument. OCI will provide single-view, hyperspectral radiometric data, whereas SPEXone will provide multi-angle, multispectral polarimetric data. Together, these instruments will be the most advanced in NASA’s history for the combined observation of ocean color and atmospheric aerosols in the UV, and they will therefore provide unprecedented research opportunities for the ocean color and atmospheric aerosol communities. In particular, UV observations are best suited to retrieve properties of Colored Dissolved Organic Matter (CDOM) in the ocean, and of Brown Carbon (BrC) aerosols in the atmosphere. However, both CDOM and BrC exhibit very similar absorption spectra in the UV and the visible (VIS) spectrum; hence, care must be taken in accurately modeling these spectra for analyses of OCI and SPEXone measurements. In this presentation, we summarize a simple but highly accurate three-parameter model for complex refractive index spectra of BrC in the UV and VIS. We apply this model to simulations of PACE-like total and polarized multiangle radiance in the UV, and demonstrate that the impact of BrC and CDOM variations can be similar in total radiance, but is easy to distinguish in polarized radiance.

PACE↗
NASA NTRSDate not supplied

Moon to Mars (M2M): Exploration Atmosphere

As humans leave the bounds of Earth to explore the lunar surface and beyond, crew will don extravehicular activity (EVA) suits to learn more about these extraterrestrial environments, establish sustained presence, and perform needed upgrades and maintenance to their space vehicle and habitation systems. Spacefaring vehicle and habitation design will need to support these EVA excursions while ensuring crew health and safety. A crucial technological design advancement towards this goal is the use of a lower pressure exploration atmosphere (EA) that enables high efficiency EVA, rather than the sea level atmosphere of 14.7 psia, 21% oxygen (O 2 ) found on the International Space Station, Shuttle, and most other Russian and Chinese space vehicles and stations. Early space vehicles (Mercury through Apollo Programs) used a 5 psia, 100% O 2 environment, which eliminated the need for pre-EVA denitrogenation protocols, simplified the life support system to a single gas, and saved structural mass. For longer duration missions (Skylab), a diluent gas was added, changing the atmosphere to 5 psia, 70-74% O 2 to prevent atelectasis while remaining normoxic. As in-flight science became a top priority, Shuttle and ISS atmospheres were chosen to operate at sea level allowing for simpler ground-based study control conditions. Consequently this led to long pre-EVA denitrogenation protocols involving up to 4 hours of O 2 prebreathe because the EVA suit still operated at a low pressure of 4.3 psid. To increase operational efficiency, the Shuttle was retroactively certified to operate using 10.2 psia, 26.5% O 2 , reducing O 2 prebreathe time to 40-75 min. Current plans for M2M habitats on the Lunar surface require EVA, thus EA recommendation became 8 psia and 32% O 2 but was revised to 8.2 psia and 34% O 2 to decrease hypoxia exposure. Unfortunately, the benefits of EA in support of safe and efficient EVAs comes with the challenge of fire management in a higher-than-normal O 2 % environment. Although known for decades, the recommended forward work to address fire management has only recently begun. Current flammability tests include examining material propagation and ignition sources as well as fire mitigation processes to better understand these properties for proposed new EA environments. Fire safety, DCS risk, and mission design all contribute to the multifaceted parameters of EA. Thus while it is clear that EA is required to achieve the goals of future exploratory space missions, final specifications are still being evaluated for optimizing crew health and safety.

space atmosphere↗
DOE OSTI2014

ntermediate frequency atmospheric disturbances: A dynamical bridge connecting western U.S. extreme precipitation with East Asian cold surges

In this study, an atmospheric river (AR) detection algorithm is developed to investigate the downstream modulation of the eastern North Pacific ARs by another weather extreme, known as the East Asian cold surge (EACS), in both reanalysis data and high-resolution global model simulations. It is shown that following the peak of an EACS, atmospheric disturbances of intermediate frequency (IF; 10 30 day period) are excited downstream. This leads to the formation of a persistent cyclonic circulation anomaly over the eastern North Pacific that dramatically enhances the AR occurrence probability and the surface precipitation over the western U.S. between 30 N and 50 N. A diagnosis of the local geopotential height tendency further confirms the essential role of IF disturbances in establishing the observed persistent anomaly. This downstream modulation effect is then examined in the two simulations of the National Center for Atmospheric Research Community Climate System Model version 4 with different horizontal resolutions (T85 and T341) for the same period (1979 2005). The connection between EACS and AR is much better captured by the T341 version of the model, mainly due to a better representation of the scale interaction and the characteristics of IF atmospheric disturbances in the higher-resolution model. The findings here suggest that faithful representations of scale interaction in a global model are critical for modeling and predicting the occurrences of hydrological extremes in the western U.S. and for understanding their potential future changes.

atmospheric river↗
DOE OSTI2017

Evaluation of Routine Atmospheric Sounding Measurements Using Unmanned Systems (ERASMUS) Field Campaign Report

The Evaluation of Routine Atmospheric Sounding Measurements using Unmanned Systems (ERASMUS) campaign was proposed with two central goals; to obtain scientifically relevant measurements of quantities related to clouds, aerosols, and radiation, including profiles of temperature, humidity, and aerosol particles, the structure of the arctic atmosphere during transitions between clear and cloudy states, measurements that would allow us to evaluate the performance of retrievals from U.S. Department of Energy (DOE) Atmospheric Radiation Measurement (ARM) Climate Research Facility remote sensors in the Arctic atmosphere, and information on the spatial variability of heat and moisture fluxes from the arctic surface; and to demonstrate unmanned aerial system (UAS) capabilities in obtaining measurements relevant to the ARM and ASR programs, particularly for improving our understanding of Arctic clouds and aerosols.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2018

Atmosphere to Electrons: Enabling the Wind Plant of Tomorrow

The U.S. Department of Energy’s (DOE’s) Atmosphere to Electrons (A2e) research initiative is focused on improving the performance and reliability of wind plants by establishing an unprecedented understanding of how the Earth’s atmosphere interacts with the wind plants and developing innovative technologies to maximize energy extraction from the wind. The A2e initiative pursues an integrated research portfolio to coordinate and optimize advancements in four main research areas: 1) plant performance and financial risk assessment, 2) atmospheric science, 3) wind plant aerodynamics, and 4) next-generation wind plant technology. It offers an integrated systems approach to developing the next generation of System Management of the Atmospheric Resource by Turbines (SMART) wind plant technologies necessary to increase wind deployment.

a2e↗
DOE OSTI2024

West African Monsoon System’s Responses to Global Ocean–Regional Atmosphere Coupling

This study explores the added value (AV) of a regional Earth system model (ESM) compared to an atmosphere-only regional climate model (RCM) in simulating West African monsoon (WAM) rainfall. The primary goals are to foster discussions on the suitability of coupled RCMs for WAM projections and deepen our understanding of ocean–atmosphere coupling’s influence on the WAM system. The study employs results from dynamical downscaling of the ERA-Interim reanalysis and Max Plank Institute ESM, low resolution (MPI-ESM-LR), by two RCMs, atmosphere only (REMO) and REMO coupled with Max Planck Institute Ocean Model (MPIOM) (ROM), at ~25-km horizontal resolution. Results show that in regions distant from coupling domain boundaries such as West Africa (WA), constraint conditions from ERA-Interim are more beneficial than coupling effects. REMO, reliant on oceanic sea surface temperatures (SSTs) from observations and influenced by ERA-Interim, is biased under coupling conditions, although coupling offers potential advantages in representing heat and mass fluxes. Contrastingly, as intended, coupling improves SSTs and monsoon fluxes’ relationships under ESM-forced conditions. In this latter case, the coupling features a dipole-like spatial structure of AV, improving precipitation over the Guinea Coast but degrading precipitation over half of the Sahel. Our extensive examination of physical processes and mechanisms underpinning the WAM system supports the plausibility of AV. Additionally, we found that the monsoonal dynamics over the ocean respond to convective activity, with the Sahara–Sahel surface temperature gradient serving as the maintenance mechanism. While further efforts are needed to enhance the coupled RCM, we advocate for its use in the context of WAM rainfall forecasts and projections.

54 ENVIRONMENTAL SCIENCES↗

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