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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 181 records · Page 10
All sourcesNASA NTRSDOE OSTI
DOE OSTI2022

The importance of phonon spectrum measurements for accurate prediction of thermal scattering laws [Slides]

Although approximate phonon spectra (e.g. Debye model) are sufficient to reproduce integral quantities (e.g. total INS cross section) in reasonable agreement with the measured data, more accurate phonon spectra are needed to achieve agreement with the differential data. SANS component is essential for reproducing the total scattering cross section; this is the case for nanodiamonds and other materials where SANS components are present (such as porous materials like nuclear graphite). A format proposal for SANS data in ENDF or GNDS is needed. Therefore, differential (e.g. phonon spectrum) and integral (e.g. total cross section) measurements are necessary in the process of creating an ENDF evaluation. We have successfully developed a method by which ENDF evaluations can be directly compared to the relevant experimentally measured quantities. INS experiments at SNS, ILL, ISIS, and, in the future, ESS, as well as total cross section measurements at the VESUVIO instrument at ISIS, are accessible through user programs.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2016

Improvements to Thermal Neutron Scattering Law of CH{sub 2}

MCNP, as a widely accepted simulation tool, depends heavily on evaluated nuclear data found in current ENDF libraries. Modeling CH{sub 2} (polyethylene), as one of the prominent moderators, is of high importance for many applications such as spent fuel storage or shipping systems. Current thermal scattering S (α, β) evaluations are based on theoretical calculations of the phonon spectrum that are usually adjusted to match the energy dependent total scattering cross section. Double differential scattering data is not always available and thus rarely used in the evaluation. In this work double differential scattering measurements were used to obtain a phonon spectrum that can be used to generate a thermal scattering evaluation. This procedure resulted in better agreement with the experimental total cross section of CH{sub 2} and better agreement with double differential scattering experiments. (authors)

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2023

Spatiotemporal Studies of Soluble Inorganic Nanostructures with X‐rays and Neutrons

This Review addresses the use of X-ray and neutron scattering as well as X-ray absorption to describe how inorganic nanostructured materials assemble, evolve, and function in solution. We first provide an overview of techniques and instrumentation (both large user facilities and benchtop). We review recent studies of soluble inorganic nanostructure assembly, covering the disciplines of materials synthesis, processes in nature, nuclear materials, and the widely applicable fundamental processes of hydrophobic interactions and ion pairing. Reviewed studies cover size regimes and length scales ranging from sub-Ångström (coordination chemistry and ion pairing) to several nanometers (molecular clusters, i.e. polyoxometalates, polyoxocations, and metal-organic polyhedra), to the mesoscale (supramolecular assembly processes). Reviewed studies predominantly exploit 1) SAXS/WAXS/SANS (small- and wide-angle X-ray or neutron scattering), 2) PDF (pair-distribution function analysis of X-ray total scattering), and 3) XANES and EXAFS (X-ray absorption near-edge structure and extended X-ray absorption fine structure, respectively). While the scattering techniques provide structural information, X-ray absorption yields the oxidation state in addition to the local coordination. Our goal for this Review is to provide information and inspiration for the inorganic/materials science communities that may benefit from elucidating the role of solution speciation in natural and synthetic processes.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2020

Excitation of Nonradiating Anapoles in Dielectric Nanospheres

Although the study of nonradiating anapoles has long been part of fundamental physics, the dynamic anapole at optical frequencies was only recently experimentally demonstrated in a specialized silicon nanodisk structure. In this article, we report excitation of the electrodynamic anapole state in isotropic silicon nanospheres using radially polarized beam illumination. The superposition of equal and out-of-phase amplitudes of the Cartesian electric and toroidal dipoles produces a pronounced dip in the scattering spectra with the scattering intensity almost reaching zero-a signature of anapole excitation. The total scattering intensity associated with the anapole excitation is found to be more than 10 times weaker for illumination with radially vs linearly polarized beams. Our approach provides a simple, straightforward alternative path to realizing nonradiating anapole states at the optical frequencies.

36 MATERIALS SCIENCE↗
NASA NTRS1995

An Investigation of Multipath Effects on the GPS System During Auto-Rendezvous and Capture

The proposed use of a Cargo Transport Vehicle (CTV) to carry hardware to the Space Station Freedom (SSF) during the construction phase of the SSF project requires remote maneuvering of the CTV. The CTV is not a manned vehicle. Obtaining the relative positions of the CTV and SSF for remote auto-rendezvous and capture (AR&C) scenarios will rely heavily on the Global Positioning System (GPS). The GPS system is expected to guide the CTV up to a distance of 100 to 300 meters from the SSF. At some point within this range, an optical docking system will take over the remote guidance for capture. During any remote guidance by GPS it is possible that significant multipath signals may be caused by large objects in the vicinity of the module being remotely guided. This could alter the position obtained by the GPS system from the actual position. Due to the nature of the GPS signals, it has been estimated that if the difference in distance between the Line of Sight (LOS) path and the multipath is greater than 300 meters, the GPS system is capable of discriminating between the direct signal and the reflected (or multipath) signal. However, if the path difference is less than 300 meters, one must be concerned. This report details the work accomplished by the Electromagnetic Simulations Laboratory at Marquette University over the period December 1993 to May 1995. This work is an investigation of the strength and phase of a multipath signal arriving at the CTV relative to the direct or line of sight (LOS) signal. The signal originates at a GPS satellite in half geo-stationary orbit and takes two paths to the CTV: (1) the direct or LOS path from the GPS satellite to the CTV; and (2) a scattered path from the GPS satellite to the SSF module and then to the CTV. The scattering from a cylinder has been computed using the physical optics approximation for the current. No other approximations or assumptions have been made including no assumptions regarding the far field or Fresnel field approximations. The integrations required to obtain the scattered field have been computed numerically using an N dimensional Romberg integration. The total scattered electric field is then projected onto the RCP component in the direction of propagation only. The direct or line of sight signal is then used to compute the relative strength and phase of the scattered field. The trajectory of the CTV has been parameterized into 4,214 points that are calculated for each of the geometries investigated. The motion of the CTV between points is small enough for the magnitude data (dB down from direct signal) to appear very smooth; however, because of the distances and wavelengths involved, the phase of the scattered field relative to the direct signal varies very rapidly.

Richie, James E.↗
NASA NTRS1973

Interpretation of glory undulations in scattering cross sections Amplitudes

Information on the interaction potential contained in the undulations in the energy dependence of the total scattering cross section is deduced by measuring the undulation amplitude. The amplitude is interpreted with emphasis on features that are independent of any specific assumptions about the form of the interaction potential. It is shown that the previously measured spacings of the undulations describe the area of the potential well, whereas the amplitudes provide a measure of the force in the vicinity of the distance of closest approach. This information can be used to test proposed potential models and to suggest ways of improving inadequate models; if the predicted spacing is too large, then the area of the well of the model is too small, and if the predicted amplitude is too small, then the repulsive wall of the potential is too steep.

Greene, E. F.↗
DOE OSTI2017

Development of an ejecta particle size measurement diagnostic based on Mie scattering

The goal of this work is to determine the feasibility of extracting the size of particles ejected from shocked metal surfaces (ejecta) from the angular distribution of light scattered by a cloud of such particles. The basis of the technique is the Mie theory of scattering, and implicit in this approach are the assumptions that the scattering particles are spherical and that single scattering conditions prevail. The meaning of this latter assumption, as far as experimental conditions are concerned, will become clear later. The solution to Maxwell’s equations for spherical particles illuminated by a plane electromagnetic wave was derived by Gustav Mie more than 100 years ago, but several modern treatises discuss this solution in great detail. The solution is a complicated series expansion of the scattered electric field, as well as the field within the particle, from which the total scattering and absorption cross sections as well as the angular distribution of scattered intensity can be calculated numerically. The detailed nature of the scattering is determined by the complex index of refraction of the particle material as well as the particle size parameter, x, which is the product of the wavenumber of the incident light and the particle radius, i.e. x = 2rπ= λ. Figure 1 shows the angular distribution of scattered light for different particle size parameters and two orthogonal incident light polarizations as calculated using the Mie solution. It is obvious that the scattering pattern is strongly dependent on the particle size parameter, becoming more forward-directed and less polarizationdependent as the particle size parameter increases. This trend forms the basis for the diagnostic design.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
NASA NTRS1991

Calculation of far-field scattering from nonspherical particles using a geometrical optics approach

A numerical method was developed using geometrical optics to predict far-field optical scattering from particles that are symmetric about the optic axis. The diffractive component of scattering is calculated and combined with the reflective and refractive components to give the total scattering pattern. The phase terms of the scattered light are calculated as well. Verification of the method was achieved by assuming a spherical particle and comparing the results to Mie scattering theory. Agreement with the Mie theory was excellent in the forward-scattering direction. However, small-amplitude oscillations near the rainbow regions were not observed using the numerical method. Numerical data from spheroidal particles and hemispherical particles are also presented. The use of hemispherical particles as a calibration standard for intensity-type optical particle-sizing instruments is discussed.

Hovenac, Edward A.↗
DOE OSTI2026

Neutron Scattering in Sodium-Ion Battery Research: Progress and Prospects

Sodium-ion batteries have attracted renewed interest in recent years and are widely studied as a complementary power source to Li-ion batteries for large-scale stationary energy storage and small electric vehicles. Compared with Li-ion batteries, Na-ion batteries offer several advantages, including elemental abundance, lower cost, improved safety, and better low-temperature performance. An in-depth understanding of Na-ion batteries across multiple length and time scales has further accelerated the rapid development of this technology. Among the various advanced characterization techniques used to study Na-ion batteries, neutron scattering has gained significant traction in recent years. It has become a powerful and versatile tool for probing structure, morphology, and sodium-ion dynamics over a wide range of length and time scales. In this article, we will briefly review the development of neutron scattering technology and highlight recent advances in applying neutron-based techniques—including neutron diffraction, total scattering, small-angle scattering, quasi-elastic/inelastic scattering, and neutron imaging—to Na-ion battery materials. We also provide perspectives on future technique developments, particularly in the realm of in situ and operando neutron scattering characterization, and discuss how these approaches could further enhance our understanding of Na-ion battery systems.

Liu, Jue [ORNL] (ORCID:000000024453910X)↗
DOE OSTI2015

Low energy elastic electron scattering from CF{sub 3}Br molecules

CF{sub 3}Br is a potentially valuable precursor molecule for generating beams of gas phase Br radicals suitable for electron collisions studies. However, the utility of CF{sub 3}Br for this purpose depends critically on the availability of sound scattering cross sections to allow the contribution of the precursor to be isolated within the total scattering signal. To this end, here we present elastic differential cross section (DCS) measurements for CF{sub 3}Br at incident energies between 15 and 50 eV. Comparison of these DCSs to those from the only other available experimental study [Sunohara et al., J. Phys. B: At., Mol. Opt. Phys. 36, 1843 (2003)] and a Schwinger multichannel with pseudo potentials (SMCPPs) calculation [Bettega et al., J. Phys. B: At., Mol. Opt. Phys. 36, 1263 (2003)] shows generally a very good accord. Integral elastic and momentum transfer cross sections, derived from our DCSs, are also found to be in quite good agreement with the SMCPP results.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
NASA NTRS1989

Finite source depolarization factors for circumstellar scattering

A single scattering theory is used to directly derive the D(r) result of Cassinelli et al (1987) and to investigate the extent to which it can be generalized to nonuniform spherical light sources, nonspherical light sources, arbitrary spatial distributions of scattering electrons, and scattering particles other than electrons. Expressions are also obtained for the factor by which the total scattered (as well as polarized) intensity is modified by finite size light sources, which is relevant to the case where the much stronger direct unpolarized starlight is eclipsed.

Brown, John C.↗
NASA NTRS2002

Coronal Heating and the Increase of Coronal Luminosity with Magnetic Flux

We present the observed scaling of coronal luminosity with magnetic flux in a set of quiet regions. Comparison of this with the observed scaling found for active regions suggests an underlying difference between coronal heating in active regions and quiet regions. From SOHO/EIT coronal images and SOHO/MDI magnetograms of four similar large quiet regions, we measure L(sub corona) and Phi(sub total) in random subregions ranging in area from about four supergranules [(70,000 km)(exp 2)] to about 100 supergranules [(0.5 R(sub sun))(exp 2)], where L(sub corona) is the luminosity of the corona in a subregion and Phi(sub total) is the flux content of the magnetic network in the subregion. This sampling of our quiet regions yields a correlation plot of Log L(sub corona) vs Log Phi(sub total) appropriate for comparison with the corresponding plot for active regions. For our quiet regions, the mean values of L(sub corona) and Phi(sub total) both increase linearly with area (simply because each set of subregions of the same area has very nearly the same mean coronal luminosity per unit area and mean magnetic flux per unit area), and in each constant-area set the values of L(sub corona) and Phi(sub total) 'scatter' about their means for that area. This results in the linear least-squares fit to the Log ((L (sub corona)), vs Log ((Phi (sub total)) plot having a slope somewhat less than one. If active regions mimicked our quiet regions in that all large sets of same-area active regions had the same mean coronal luminosity per unit area and same mean magnetic flux per unit area, then the least-squares fit to their Log((L (sub corona)) vs Log((Phi (sub total)) plot would also have a slope of less than one. Instead, the slope for active regions is 1.2. Given the observed factor of three scatter about the least-squares linear fit, this slope is consistent with Phi(sub total) on average increasing linearly with area (A) as in quiet regions, but L(sub corona) on average increasing as the volume (A(exp 1.5)) of the active region instead of as the area. This possibility is reasonable if the heating in active regions is a burning down of previously-stored coronal magnetic energy rather than a steady dissipation of energy flux from below as expected in quiet regions.

Moore, R. L.↗
DOE OSTI2023

Ion-Selective Scattering Studied Using the Variable-Energy Electron Irradiation in the Ba 0.2 K 0.8 Fe 2 As 2 Superconductor

Low-temperature variable-energy electron irradiation was used to induce non-magnetic disorder in a single crystal of a hole-doped iron-based superconductor, Ba $1-x$ K $x$ Fe 2 As 2 , $x$ = 0.80. To avoid systematic errors, the beam energy was adjusted non-consequently for five values between 1.0 and 2.5 MeV when sample resistance was measured in situ at 22 K. For all energies, the resistivity raises linearly with the irradiation fluence suggesting the creation of uncorrelated dilute point-like disorder (confirmed by simulations). The rate of the resistivity increase peaks at energies below 1.5 MeV. Comparison with calculated partial cross-sections points to the predominant creation of defects in the iron sublattice. Simultaneously, superconducting $T_c$, measured separately between the irradiation runs, is monotonically suppressed as expected, since it depends on the total scattering rate, hence on the total cross-section, which is a monotonically increasing function of the energy. Our work experimentally confirms an often-made assumption of the dominant role of the iron sub-lattice in iron-based superconductors.

36 MATERIALS SCIENCE↗
DOE OSTI2020

One-center close-coupling approach to two-center rearrangement collisions

Calculations of ionization and electron-capture cross sections in ion-atom collisions usually require solving the Schrödinger equation governing the collision system by expanding the total scattering wave function in a basis of target- and projectile-centered pseudostates. This approach leads to the two-center close-coupling equations which in some cases may become ill-conditioned due to the non-orthogonality of the underlying combined basis. Here we develop a technique which allows to accurately extract the necessary collision information, including that for the rearrangement channels, from the computationally more convenient one-center close-coupling equations which are built from only target-centered pseudostates. The robustness of the method is demonstrated by considering the proton-hydrogen scattering problem across a wide incident energy range. The developed method is then applied to study proton scattering on multielectron target of lithium. Here, the obtained results for the 2s → 2p excitation and the total electron-capture cross sections are in good agreement with corresponding experimental data. It is concluded that the presented technique could be a simpler alternative when integrated cross sections are required.

74 ATOMIC AND MOLECULAR PHYSICS↗
DOE OSTI2015

Peripheral elastic and inelastic scattering of {sup 17,18}O on light targets at 12 MeV/nucleon

The elastic and inelastic scattering of {sup 17,18}O with light targets has been undertaken at 12 MeV/nucleon in order to determine the optical potentials needed for the transfer reaction {sup 13}C({sup 17}O,{sup 18}O){sup 12}C. Optical potentials in both incoming and outgoing channels have been determined in a single experiment. This transfer reaction was used to infer the direct capture rate to the {sup 17}F(p,γ){sup 18}Ne which is essential to estimate the production of {sup 18}F at stellar energies in ONe novae. We demonstrate the stability of the ANC method and OMP results using good quality elastic and inelastic scattering data with stable beams. The peripherality of our reaction is inferred from a semiclassical decomposition of the total scattering amplitude into barrier and internal barrier components. Comparison between elastic scattering of {sup 17}O, {sup 18}O and {sup 16}O projectiles is made.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2021

A global study of hygroscopicity-driven light-scattering enhancement in the context of other in situ aerosol optical properties

The scattering and backscattering enhancement factors (ƒ(RH) and ƒ b (RH)) describe how aerosol particle light scattering and backscattering, respectively, change with relative humidity (RH). They are important parameters in estimating direct aerosol radiative forcing (DARF). In this study we use the dataset presented in Burgos et al. (2019) that compiles ƒ(RH) and ƒ b (RH) measurements at three wavelengths (i.e., 450, 550 and 700 nm) performed with tandem nephelometer systems at multiple sites around the world. We present an overview of ƒ(RH) and ƒ b (RH) based on both long-term and campaign observations from 23 sites representing a range of aerosol types. The scattering enhancement shows a strong variability from site to site, with no clear pattern with respect to the total scattering coefficient. In general, higher ƒ(RH) is observed at Arctic and marine sites, while lower values are found at urban and desert sites, although a consistent pattern as a function of site type is not observed. The backscattering enhancement ƒ b (RH) is consistently lower than ƒ(RH) at all sites, with the difference between ƒ(RH) and ƒ b (RH) increasing for aerosol with higher ƒ(RH). This is consistent with Mie theory, which predicts higher enhancement of the light scattering in the forward than in the backward direction as the particle takes up water. Our results show that the scattering enhancement is higher for PM 1 than PM 10 at most sites, which is also supported by theory due to the change in scattering efficiency with the size parameter that relates particle size and the wavelength of incident light. At marine-influenced sites this difference is enhanced when coarse particles (likely sea salt) predominate. For most sites, ƒ(RH) is observed to increase with increasing wavelength, except at sites with a known dust influence where the spectral dependence of ƒ(RH) is found to be low or even exhibit the opposite pattern. The impact of RH on aerosol properties used to calculate radiative forcing (e.g., single-scattering albedo, ω 0 , and backscattered fraction, b) is evaluated. The single-scattering albedo generally increases with RH, while b decreases. The net effect of aerosol hygroscopicity on radiative forcing efficiency (RFE) is an increase in the absolute forcing effect (negative sign) by a factor of up to 4 at RH = 90 % compared to dry conditions (RH < 40 %). Because of the scarcity of scattering enhancement measurements, an attempt was made to use other more commonly available aerosol parameters (i.e., ω 0 and scattering Ångström exponent, α sp ) to parameterize ƒ(RH). The majority of sites (75 %) showed a consistent trend with ω 0 (higher ƒ(RH = 85 %) for higher ω 0 ), while no clear pattern was observed between ƒ(RH = 85 %) and αsp. This suggests that aerosol ω 0 is more promising than α sp as a surrogate for the scattering enhancement factor, although neither parameter is ideal. Nonetheless, the qualitative relationship observed between ω 0 and ƒ(RH) could serve as a constraint on global model simulations.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2022

Simulated effect of edge plasma density parameters on lower hybrid wave scattering in EAST

The incorporation of lower hybrid (LH) wave spectrum broadening in the poloidal wavenumber (⁠k θ ) space at the last close field surface (LCFS) is reported to lead to better agreement of the modeled LH wave current profile with the experimental results [Baek et al., Nucl. Fusion 61, 106034 (2021)]. To further understand its underlying mechanism and find the possible influence factors, effects of wave scattering caused by drift-wave type density fluctuation on the probability distribution of the LH wave polar refractive index (⁠N θ ) at the LCFS are studied under density parameters in the scrape-off-layer. According to a scattering model [P. T. Bonoli and E. Ott, Phys Fluids 25(2), 359–375 (1982)], scattering probability and scattering angle distribution are two main factors that determine the degree of spectral broadening. Studies presented here show that the total scattering probability increases first and then decreases as the wave propagates toward a smaller normalized radius of poloidal magnetic flux (⁠ρ⁠). The degree of spectral broadening is found to depend on the density and density fluctuation together by changing the intensity and a proportion of the geometrical optics approximation term and the E×B drift term in the scattering model. Additionally, the fluctuation correlation length can significantly modify the probability distribution of N θ at the LCFS, which is found to significantly change the LH wave current profile.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2014

Bulk Metallic Glass-like Scattering Signal in Small Metallic Nanoparticles

The atomic structure of Ni-Pd nanoparticles has been studied using atomic pair distribution function (PDF) analysis of X-ray total scattering data and with transmission electron microscopy (TEM). Larger nanoparticles have PDFs corresponding to the bulk face-centered cubic packing. However, the smallest nanoparticles have PDFs that strongly resemble those obtained from bulk metallic glasses (BMGs). In fact, by simply scaling the distance axis by the mean metallic radius, the curves may be collapsed onto each other and onto the PDF from a metallic glass sample. In common with a wide range of BMG materials, the intermediate range order may be fit with a damped single-frequency sine wave. When viewed in high-resolution TEM, these nanoparticles exhibit atomic fringes typical of those seen in small metallic clusters with icosahedral or decahedral order. These two seemingly contradictory results are reconciled by calculating the PDFs of models of icosahedra that would be consistent with the fringes seen in TEM. These model PDFs resemble the measured ones when significant atom-position disorder is introduced, drawing together the two diverse fields of metallic nanoparticles and BMGs and supporting the view that BMGs may contain significant icosahedral or decahedral order.

Doan-Nguyen, VVT↗