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At least 181 records · Page 10
All sourcesNASA NTRSDOE OSTI
DOE OSTI2024

Generalized rate theory for void and bubble swelling and its application to δ -plutonium

A rate theory for void and bubble swelling is derived that allows both vacancies and self-interstitial atoms to be generated by thermal activation at all sinks. In addition, they can also be produced by displacement damage from external and internal radiation. This generalized rate theory (GRT) is applied to swelling of gallium-stabilized δ-plutonium in which α-decay causes the displacement damage. Since the helium atoms produced also become trapped in vacancies, a distinction is made between empty and occupied vacancies. The growth of helium bubbles observed by transmission electron microscopy in weapons-grade and in material enriched with Pu238 is analyzed, using different values for the formation energy of self-interstitial atoms (SIA) and two different sets of relaxation volumes for the vacancy and for the SIA. One set allows preferential capture of SIA at dislocations, while the other set gives equal preference to both vacancy and SIA. It is found that the helium bubble diameters observed are in better agreement with GRT predictions if no preferential capture occurs at dislocations. Therefore, helium bubbles in δ-plutonium will not evolve into voids. Furthermore, the helium density within the bubbles remains sufficiently high to cause thermal emission of SIA. Based on a helium density between two to three helium atoms per vacant site, the sum of formation and migration energies must be around 2.0 eV for SIA in δ-plutonium.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗
DOE OSTI2026

Nuclear activation analysis of zirconium-90 isomeric and ground-state reactions at the OMEGA Laser Facility

Nuclear activation is a well-established technique for inferring neutron yields in laser direct-drive deuterium–tritium (DT) and deuterium–deuterium (D 2 ) implosions at the OMEGA Laser Facility. Zirconium has long been considered an excellent candidate for measuring DT neutron fusion yields by observing decays of the 90 Zr(n,2n) 89 Zr ground-state reaction. As it has a higher energy threshold than present activation detectors utilizing copper, zirconium provides a means to infer primary neutron yields that are less susceptible to being skewed due to neutron scattering within the experimental environment. However, with a 78.41-h half-life, it is not operationally practical to utilize this reaction for OMEGA experiments, which have a 1-h shot cycle. Zirconium’s 90 Zr(n,2n) 89 mZr reaction presents itself as a viable candidate to infer neutron yields within a shot cycle, given its half-life of 4.16 min. Here, we present an overview of the approach and methodology, utilizing first principles techniques, to infer the primary neutron yields from OMEGA DT fusion experiments by using both the isomeric and the ground-state reaction. Yields inferred from both reactions are compared, which are in good agreement between the two.

Activation analysis↗
DOE OSTI2021

Investigation of the ground-state spin inversion in the neutron-rich Cl 47 , 49 isotopes

A first γ -ray study of Cl 47 , 49 spectroscopy was performed at the Radioactive Isotope Beam Factory with Ar 50 projectiles at 217 MeV/nucleon, impinging on the liquid hydrogen target of the MINOS device. Prompt deexcitation γ rays were measured with the NaI(Tl) array DALI2 + . Through the one-proton knockout reaction Ar 50 ( p , 2 p ) , a spin assignment could be determined for the low-lying states of Cl 49 from the momentum distribution obtained with the SAMURAI spectrometer. A spin-parity J π = 3 / 2 + is deduced for the ground state of Cl 49 , similar to the recently studied N = 32 isotope K 51 . The evolution of the energy difference E ( 1 / 2 1 + ) - E ( 3 / 2 1 + ) is compared to state-of-the-art theoretical predictions.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2021

Total fusion yield measurements using deuterium–tritium gamma rays

The deuterium–tritium (DT) fusion reaction, D ( T , γ ) 5 He , has a rare (4.2 × 10 – 5 ) branching ratio that releases a ~16 MeV gamma ray instead of the more common 14.1 MeV fusion neutron. These fusion gamma rays can be used as a complementary source of measuring the net fusion yield of experiments. Fusion gamma rays have the advantage of having negligible Doppler broadening, being isotropic and less down-scattered compared to fusion neutrons. At the National Ignition Facility, we measured the DT fusion gamma rays by the Gamma Reaction History diagnostic that thresholds to only measure >10 MeV gamma rays. After removing a ~12% contribution from neutron capture interactions in deuterium, D ( n , γ ) T , and carbon, 12 C ( n , γ ) 13 C , the deviation between GRH measurements and neutron-based yield measurements has been reduced to 10%. Further improvements are needed for detailed physics comparison.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2023

Understanding the fusion yield dependencies in OMEGA DT-layered implosion experiments using a physics-based statistical mapping model

Improving the performance of inertial confinement fusion implosions requires physics models that can accurately predict the response to changes in the experimental inputs. Good predictive capability has been demonstrated for the fusion yield using a statistical mapping of simulated outcomes to experimental data [Gopalaswamy et al., Nature 565(771), 581–586 (2019)]. In this paper, a physics-based statistical mapping approach is used to extract and quantify all the major sources of degradation of fusion yield for direct-drive implosions on the OMEGA laser. Here, the yield is found to be dependent on the age of the deuterium tritium fill, the ℓ = 1 asymmetry in the implosion core, the laser beam-to-target size ratio, and parameters related to the hydrodynamic stability. A controlled set of experiments were carried out where only the target fill age was varied while keeping all other parameters constant. The measurements were found to be in excellent agreement with the fill age dependency inferred using the mapping model. In addition, a new implosion design was created, guided by the statistical mapping model by optimizing the trade-offs between increased laser energy coupling at larger target size and the degradations caused by the laser beam-to-target size ratio and hydrodynamic instabilities. When experimentally performed, an increased fusion yield was demonstrated in targets with larger diameters.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2023

Development of a bright MeV photon source with compound parabolic concentrator targets on the National Ignition Facility Advanced Radiographic Capability (NIF-ARC) laser

Compound parabolic concentrator (CPC) targets are utilized at the National Ignition Facility Advanced Radiographic Capability (NIF-ARC) laser to enhance the acceleration of electrons and production of high energy photons, for laser durations of 10 ps and energies up to 2.4 kJ. A large enhancement of mean electron energy (>2 ×) and photon brightness (>10×) is found with CPC targets compared to flat targets. Using multiple diagnostic techniques at different spatial locations and scaling by gold activation spatial data, photon spectra are characterized for E photon = 0.5-30 MeV. Beam width and pointing variations are given. The efficient production of MeV photons at I laser ≈ 2 x 10 18 W/cm 2 with CPCs is observed, with doses of >10 rad in air at 1 m for E photon > 0.5 MeV; these exceed those previously reported with laser-driven sources. Using this source, sub-mm resolution radiographs are generated through large areal density radiograph objects. Hence these results are promising for the development of bright MeV x-ray and particle sources on Petawatt class laser systems.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2024

Radioisotope production using lasers: From basic science to applications

The discovery of chirped pulse amplification has led to great improvements in laser technology, enabling energetic laser beams to be compressed to pulse durations of tens of femtoseconds and focused to a few micrometers. Protons with energies of tens of MeV can be accelerated using, for instance, target normal sheath acceleration and focused on secondary targets. Under such conditions, nuclear reactions can occur, with the production of radioisotopes suitable for medical application. The use of high-repetition lasers to produce such isotopes is competitive with conventional methods mostly based on accelerators. In this paper, we study the production of 67Cu, 63Zn, 18F, and 11C, which are currently used in positron emission tomography and other applications. At the same time, we study the reactions 10B(p,α)7Be and 70Zn(p,4n)67Ga to put further constraints on the proton distributions at different angles, as well as the reaction 11B(p,α)8Be relevant for energy production. The experiment was performed at the 1 PW laser facility at Vega III in Salamanca, Spain. Angular distributions of radioisotopes in the forward (with respect to the laser direction) and backward directions were measured using a high purity germanium detector. Our results are in reasonable agreement with numerical estimates obtained following the approach of Kimura and Bonasera [Nucl. Instrum. Methods Phys. Res., Sect. A 637, 164–170 (2011)].

11C↗
DOE OSTI2024

Neutron-producing gas puff Z-pinch experiments on a fast, low-impedance, 0.5 MA linear transformer driver

A study on the neutron production from single and double gas puff Z-pinches on the CESZAR linear transformer driver with ~0.45 MA current and 170 ns rise time is presented. Total neutron yield measurements made with a LaBr activation detector are compared for three configurations, using a double nozzle setup. When a single, hollow, deuterium gas shell was used, reliable implosions could only be attained at higher load mass than the optimal value to match implosion time with the driver rise time, with neutron yields of ~10 6 per pulse. The use of a double gas puff configuration with a deuterium center jet allowed a reduction in the shell density and operation closer to machine-matched conditions, recording up to (4.1 ± 0.3) × 10 7 neutrons/pulse when either Kr or D 2 was used in the shell. For a comparable mass and implosion time, using a higher atomic-number gas in the outer shell results in more unstable plasma surface and smaller plasma radius at the location of instability bubbles, which, however, do not seem to consistently correlate with a higher neutron yield. Comparing implosion dynamics with models and neutron yields with literature scaling suggests that the machine current is not well coupled to the plasma during the final stages of compression. Optimizing current and energy coupling to the pinched plasma is critical to improving performance, particularly in low-impedance drivers.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2025

Progress toward hydro-equivalent ignition in OMEGA direct-drive DT-layered implosions

Considerable progress has been made in deuterium-tritium-layered implosion experiments on the OMEGA Laser System, bringing the prospects for thermonuclear ignition in direct-drive configurations with megajoule-class lasers closer to reality. Doing so has required navigating the balance between improved 1D performance and multidimensional stability. Using statistical modeling based on over 350 cryogenic implosions to identify various degradation mechanisms, and combined with multidimensional simulations and experimental techniques such as target offsets to combat residual flows, core conditions have repeatably been achieved that extrapolate to the burning-plasma state when scaled to 2.15 MJ of symmetric laser illumination. Using high implosion velocities (⁠> 450 km/s) and moderately high adiabats (⁠~5⁠), these experiments produced record-high scaled Lawson parameters in direct drive equal to 89 ± 2% of that required for ignition with expected yields of up to 1.5 ± 0.2 MJ. To improve these results still further, focused physics studies are performed to improve physics understanding and identify routes to even greater performance. Recent studies include investigations into the impact of mounting features, laser imprint, reduced fuel temperatures, and greater on-target intensities through subscale experiments. This manuscript gives a summary of the cryogenic direct-drive program on the OMEGA laser, including routes taken to achieve the current best performance, the status of recent focused physics investigations, and future designs—such as target solutions to laser imprint and reducing vapor density to increase convergence—that are expected lead to the demonstration of hydro-equivalent ignition on OMEGA.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2026

Design and simulation of a muon detector to characterize geological overburden

This study presents the design, construction, and simulation of a mobile muon detector tailored for geological overburden characterization. The detector employs plastic scintillator paddles with silicon photomultipliers (SiPMs) and a QuarkNet data acquisition system, offering a portable solution suitable for remote field deployment. The simulator’s modular aluminum frame allows for adjustable geometry and directional sensitivity, while its battery system supports over a week of autonomous operation. Preliminary experimental tests confirmed that its muon flux measurements were consistent with theoretical expectations. A comprehensive simulation framework using Geant4 and CORSIKA was developed to model detector response and overburden effects. Analytical and Monte Carlo methods were used to assess quadrant resolution and infer muon directionality. This work lays the foundation for future overburden mapping and supports the development of reconstruction algorithms for geological applications.

72 - PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2025

The lessons learned from ephemeral nuclei

Recent experimental analyses of fleeting clusters of protons and neutrons put the very notion of the atomic nucleus in a new light.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2022

A puzzle solved after two decades: SN 2002gh among the brightest of superluminous supernovae

ABSTRACT We present optical photometry and spectroscopy of the superluminous SN 2002gh from maximum light to +204 d, obtained as part of the Carnegie Type II Supernova (CATS) project. SN 2002gh is among the most luminous discovered supernovae ever, yet it remained unnoticed for nearly two decades. Using Dark Energy Camera archival images we identify the potential supernova (SN) host galaxy as a faint dwarf galaxy, presumably having low metallicity, and in an apparent merging process with other nearby dwarf galaxies. We show that SN 2002gh is among the brightest hydrogen-poor SLSNe with MV = −22.40 ± 0.02, with an estimated peak bolometric luminosity of 2.6 ± 0.1 × 1044 erg s−1. We discount the decay of radioactive nickel as the main SN power mechanism, and assuming that the SN is powered by the spin-down of a magnetar we obtain two alternative solutions. The first case, is characterized by significant magnetar power leakage, and Mej between 0.6 and 3.2 M⊙, Pspin = 3.2 ms, and B = 5 × 1013 G. The second case does not require power leakage, resulting in a huge ejecta mass of about 30 M⊙, a fast spin period of Pspin ∼ 1 ms, and B ∼ 1.6 × 1014 G. We estimate a zero-age main-sequence mass between 14 and 25 M⊙ for the first case and of about 135 M⊙ for the second case. The latter case would place the SN progenitor among the most massive stars observed to explode as an SN.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2026

𝑙-forbidden 𝑀⁢1 strengths near 100 Sn from knockout reactions in Cd and Sn

Neutron knockout reactions on beams of 104,102 Cd and 104 Sn are presented. States in the residual 103,101 Cd and 103 Sn nuclei are populated, including low-lying 7/2 + states of 𝜈⁢𝑔 7/2 character. These states have half-lives ≈ 400 ps due to their low energy and hindered 𝐵⁡(𝑀⁢1;7/2 + →5/2 + ) strengths. The excited-state half-lives were measured using their Doppler-shifted line shapes, and the resulting 𝐵⁡(𝑀⁢1) strengths are compared to valence space in medium similarity renormalization group (VS-IMSRG) calculations. Lastly, the VS-IMSRG calculations underpredict the 𝑙-forbidden 𝑀⁢1 strengths in the 100 Sn region, as well as in other regions of the nuclear chart near 40 Ca and 208 Pb.

90 ≤ A ≤ 149↗
DOE OSTI2020

Spin-trap isomers in deformed, odd-odd nuclei in the light rare-earth region near $N=98$

Masses of neutron-rich, odd-odd Pm, Eu, and Tb nuclei near N = 98 were measured using the Canadian Penning Trap mass spectrometer at the Californium Rare Isotope Breeder Upgrade (CARIBU) facility. High-resolution mass measurements yielded the discovery of spin-trap isomers at N = 97 in Tb 162 , and in the N = 99 isotones of Pm 160 and Tb 164 . Furthermore, no evidence of long-lived isomers were observed at N = 95 in Eu 158 , at N = 97 in Pm 158 , nor at N = 101 in Eu 164 and Tb 166 . Here, these experimental observations are compared to results from multiquasiparticle blocking calculations.

150 ≤ A ≤ 189↗
DOE OSTI2020

Influence of 73 Rb on the ashes of accreting neutron stars

We find that the proton separation energy, S(p), of 73 Rb is –640(40) keV, deduced from the observation of β-delayed ground-state protons following the decay of 73 Sr. This lower-limit determination of the proton separation energy of 73 Rb coupled with previous upper limits from nonobservation, provides a full constraint on the mass excess with ΔM ( 73 Rb) = –46.01 ± 0.04 MeV. With this new mass excess and the excitation energy of the J π = 5/2 – isobaric-analog state (T = 3/2) in 73 Rb, an improved constraint can be put on the mass excess of 73Sr using the isobaric-multiplet mass equation (IMME), and we find ΔM( 73 Sr) = –31.98 ± 0.37 MeV. Furthermore, these new data were then used to study the composition of ashes on accreting neutron stars following Type I x-ray bursts. Counterintuitively, we find that there should be an enhanced fraction of A > 102 nuclei with more negative proton separation energies at the 72 Kr rp-process waiting point. Larger impurities of heavier nuclei in the ashes of accreting neutron stars will impact the cooling models for such astrophysical scenarios.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2020

Structure of 30 Mg explored via in-beam γ-ray spectroscopy

In the island of inversion, ground states of neutron-rich sd-shell nuclei exhibit strong admixtures of intruder configurations from the fp shell. The nucleus 30 Mg, located at the boundary of the island of inversion, serves as a cornerstone to track the structural evolution as one approaches this region. Spin-parity assignments for excited states in 30 Mg, especially negative-parity levels, have yet to be established. In the present work, the nuclear structure of 30Mg was investigated by in-beam gamma-ray spectroscopy mainly focusing on firm spin-parity determinations. High-intensity rare-isotope beams of 31 Mg, 32 Mg, 34 Si, and 35 P bombarded a Be target to induce nucleon removal reactions populating states in 30 Mg. Gamma rays were detected by the state-of-the-art gamma-ray tracking array GRETINA. For the direct one-neutron removal reaction, final-state exclusive cross sections and parallel momentum distributions were deduced. Multi-nucleon removal reactions from different projectiles were exploited to gain complementary information. With the aid of the parallel momentum distributions, an updated level scheme with revised spin-parity assignments was constructed. Spectroscopic factors associated with each state were also deduced. Results were confronted with large-scale shell-model calculations using two different effective interactions, showing excellent agreement with the present level scheme. Furthermore, a marked difference in the spectroscopic factors indicates that the full delineation of the transition into the island of inversion remains a challenge for theoretical models.

20 ≤ A ≤ 38↗
DOE OSTI2021

Quadrupole collectivity in the neutron-rich sulfur isotopes 38,40,42,44 S

Electromagnetic transition strengths in the even-even neutron-rich sulfur isotopes 38,40,42,44 S were measured using intermediate-energy Coulomb excitation at the National Superconducting Cyclotron Laboratory. By utilizing the sensitivity of the experimental technique to E2 excitations from the ground state, the evolution of the pattern of B(E2) strengths to several low-lying 2 + states was investigated at Z = 16 from near stability to the N = 28 island of inversion. The experimental results allowed a detailed comparison with predictions from shell-model calculations using the SDPF-MU Hamiltonian, which was designed to describe collectivity in this region of the nuclear chart. While the shell-model calculations succeeded in modeling transition strengths at N = 22, 24, 26, the experimental B(E2; $0$ $^{+}_{1}$ → $2$ $^{+}_{1}$) at N = 28 was smaller than the predicted value by about a factor of 2, similar to previous observations for chlorine and argon isotopes around N = 28. The dependence of this overprediction by theory on the choice of effective charges was explored.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2022

In-beam γ-ray spectroscopy of 32 Mg via direct reactions

Background: The nucleus 32 Mg (N=20 and Z=12) plays a central role in the so-called “island of inversion,” where in the ground states sd-shell neutrons are promoted to the fp-shell orbitals across the shell gap, resulting in the disappearance of the canonical neutron magic number N=20. Purpose: The primary goals of this work are to extend the level scheme of 32Mg, provide spin-parity assignments to excited states, and discuss the microscopic structure of each state through comparisons with theoretical calculations. Method: In-beam γ-ray spectroscopy of 32 Mg was performed using two direct-reaction probes: one-neutron (two-proton) knockout reactions on 33 Mg ( 34 Si). Final-state exclusive cross sections and parallel momentum distributions were extracted from the experimental data and compared with eikonal-based reaction model calculations combined with shell-model overlap functions. Results: Owing to the remarkable selectivity of the one-neutron and two-proton knockout reactions, a significantly updated level scheme for 32 Mg, which exhibits negative-parity intruder and positive-parity normal states, was constructed. The experimental results were confronted with four different nuclear structure models. Conclusions: In some of these models, different aspects of 32 Mg and the transition into the island of inversion are well described. However, unexplained discrepancies remain, and, even with the help of these state-of-the-art theoretical approaches, the structure of this key nucleus is not yet fully captured.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗