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DOE OSTI2025

Search for a diffuse flux of photons with energies above tens of PeV at the Pierre Auger Observatory

Diffuse photons of energy above 0.1 PeV, produced through the interactions between cosmic rays and either interstellar matter or background radiation fields, are powerful tracers of the distribution of cosmic rays in the Galaxy. Furthermore, the measurement of a diffuse photon flux would be an important probe to test models of super-heavy dark matter decaying into gamma-rays. In this work, we search for a diffuse photon flux in the energy range between 50 PeV and 200 PeV using data from the Pierre Auger Observatory. For the first time, we combine the air-shower measurements from a 2 km 2 surface array consisting of 19 water-Cherenkov surface detectors, spaced at 433 m, with the muon measurements from an array of buried scintillators placed in the same area. Using 15 months of data, collected while the array was still under construction, we derive upper limits to the integral photon flux ranging from 13.3 to 13.8 km -2 sr -1 yr -1 above tens of PeV. We extend the Pierre Auger Observatory photon search program towards lower energies, covering more than three decades of cosmic-ray energy. This work lays the foundation for future diffuse photon searches: with the data from the next 10 years of operation of the Observatory, this limit is expected to improve by a factor of ∼20.

cosmic rays detectors↗

DOE OSTI2023

Intensified Tpx3Cam, a fast data-driven optical camera with nanosecond timing resolution for single photon detection in quantum applications

Here we describe a fast data-driven optical camera, Tpx3Cam, with nanosecond scale timing resolution and 80 Mpixel/sec throughput. After the addition of intensifier, the camera is single photon sensitive with quantum efficiency determined primarily by the intensifier photocathode. The single photon performance of the camera was characterized with results on the gain, timing resolution and afterpulsing reported here. The intensified camera was successfully used for measurements in a variety of applications including quantum applications. As an example of such application, which requires simultaneous detection of multiple photons, we describe registration of photon pairs from the spontaneous parametric down-conversion source in a spectrometer. We measured the photon wavelength and timing with respective precisions of 0.15 nm and 3 ns, and also demonstrated that the two photons are anti-correlated in energy.

79 ASTRONOMY AND ASTROPHYSICS↗

DOE OSTI2021

Light by design: emerging frontiers in ultrafast photon sciences and light–matter interactions

Photon sciences and technologies establish the building blocks for myriad scientific and engineering frontiers in life and energy sciences. Because of their overarching functionality, the developmental roadmap and opportunities underpinned by photonics are often semiotically mediated by the delineation of subject areas of application. In this perspective article, we map current and emerging linkages between three intersecting areas of research stewarded by advanced photonics technologies, namely light by design, outlined as (a) quantum and structured photonics, (b) light–matter interactions in accelerators and accelerator-based light sources, and (c) ultrafast sciences and quantum molecular dynamics. In each section, we will concentrate on state-of-the-art achievements and present prospective applications in life sciences, biochemistry, quantum optics and information sciences, and environmental and chemical engineering, all founded on a broad range of photon sources and methodologies. We hope that this interconnected mapping of challenges and opportunities seeds new concepts, theory, and experiments in the advancement of ultrafast photon sciences and light–matter interactions. Additionally, through this mapping, we hope to inspire a critically interdisciplinary approach to the science and applications of light by design.

42 ENGINEERING↗

DOE OSTI2026

Photon temporal-mode readout for inference of neutron star merger remnant gravitational waves

Gravitational waves emitted after neutron star binary coalescences and the information they carry about dense matter are a high-priority target for next-generation detectors. Even though such detectors are expected to observe millions of signals, detectable postmerger emission will remain rare. Here, in this work, we explore postmerger detectability and inference through an alternative detector readout scheme for data dominated by quantum-noise, which is the case above 1 kHz; photon-counting. In such a readout, signals and noise become quantized into discrete distributions corresponding to the detection of single photons measured in a chosen basis of modes. Through simulated data, we demonstrate that photon counting can be efficient even for weak signals. We find ∼1 in 100 signals with a postmerger signal-to-noise ratio of 0.2 can result in a single photon and thus be detected. Furthermore, after 2 ×10 4 signals—equivalent to 10 −2 to 1.5 years of observation—photon counting results in a twofold improvement in the measurement of the radius of a 1.6⁢𝑀 ⊙ neutron star. Constraints can be further tightened if the detector classical noise is reduced. Photon counting offers a promising alternative to traditional homodyne readout techniques for extracting information from low signal-to-noise ratio postmerger signals.

gravitational wave detection↗

DOE OSTI2023

Interplay of effects of neutron skins in coordinate space and proton skins in momentum space on emission of hard photons in heavy-ion collisions near the Fermi energy

Within an isospin- and momentum-dependent Boltzmann-Uehling-Uhlenbeck transport model, we investigate the hard photons emission from neutron-proton bremsstrahlung in the reaction system of 208 Pb + 208 Pb around Fermi energy. Effects of neutron skins in coordinate (r) space and proton skins in momentum (k) space on the time evolution, the angular distribution, and the transverse momentum spectra of hard photons with different energies are studied. It is shown that the emission of direct hard photons is sensitive to the neutron skin, which has larger effects for more energetic hard photons. Meanwhile, we find that the proton skins have an important influence on the emission of direct hard photons, and its effect is actually even larger than that of neutron skins. Furthermore, it needs to take the effect of proton skins into account when we determine the size of neutron skins by comparing transport mode predictions of hard photons with the corresponding experimental measurements.

190 ≤ A ≤ 219↗

DOE OSTI2025

Thermodynamics of continuous spin photons

Special relativity allows massless particles to have states of different integer (or half-integer) helicities that mix under boosts, much like the spin states of a massive particle. Such massless particles are known as “continuous spin” particles (CSPs), a term coined by Wigner, and they are notable for their infinite tower of spin polarizations. The mixing under boosts is controlled by a spin scale 𝜌 with units of momentum. Normally, we assume 𝜌 = 0. The interactions of CSPs are known to satisfy certain simple properties, one of which is that the 𝜌 → 0 limit generically recovers familiar interactions of massless scalars, photons, or gravitons, with all other polarizations decoupling in this limit. Thus, one can ask if the photon of the Standard Model is a CSP at small but nonzero 𝜌. One concern about this possibility—originally raised by Wigner—is that the infinite tower of polarizations could pose problems for thermodynamics. To address this question, we study the thermal evolution of a CSP photon gas coupled to isothermal matter, across CSP helicity modes and phase space. We find that the structure of the interactions dictated by Lorentz symmetry implies well-behaved thermodynamics. When the CSP photon’s interactions with charged matter are turned on, the primary ℎ =±1 helicity modes thermalize quickly, while the other modes require increasingly long time scales to thermalize, set by powers of 𝑇/𝜌. In familiar thermal systems, the CSP photon behaves like the QED photon with small 𝜌- and time-dependent corrections to its effective relativistic degrees of freedom. Sizable departures from familiar thermal behavior arise at energy scales comparable to 𝜌 and could have testable experimental consequences.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

DOE OSTI2021

Inelastic Scattering of a Photon by a Quantum Phase Slip

Spontaneous decay of a single photon is a notoriously inefficient process in nature irrespective of the frequency range. We report that a quantum phase-slip fluctuation in high-impedance superconducting waveguides can split a single incident microwave photon into a large number of lower-energy photons with a near unit probability. The underlying inelastic photon-photon interaction has no analogs in non-linear optics. Instead, the measured decay rates are explained without adjustable parameters in the framework of a new model of a quantum impurity in a Luttinger liquid. Our result connects circuit quantum electrodynamics to critical phenomena in two-dimensional boundary quantum field theories, important in the physics of strongly-correlated systems. Here, the photon lifetime data represents a rare example of verified and useful quantum many-body simulation.

1-dimensional systems↗

DOE OSTI2023

Time-Resolved Line Shapes of Single Quantum Emitters via Machine Learned Photon Correlations

Solid-state single-photon emitters (SPEs) are quantum light sources that combine atomlike optical properties with solid-state integration and fabrication capabilities. SPEs are hindered by spectral diffusion, where the emitter’s surrounding environment induces random energy fluctuations. Timescales of spectral diffusion span nanoseconds to minutes and require probing single emitters to remove ensemble averaging. Photon correlation Fourier spectroscopy (PCFS) can be used to measure time-resolved single emitter line shapes, but is hindered by poor signal-to-noise ratio in the measured correlation functions at early times due to low photon counts. Here, we develop a framework to simulate PCFS correlation functions directly from diffusing spectra that match well with experimental data for single colloidal quantum dots. We use these simulated datasets to train a deep ensemble autoencoder machine learning model that outputs accurate, noiseless, and probabilistic reconstructions of the noisy correlations. Using this model, we obtain reconstructed time-resolved single dot emission line shapes at timescales as low as 10 ns, which are otherwise completely obscured by noise. This enables PCFS to extract optical coherence times on the same timescales as Hong-Ou-Mandel two-photon interference, but with the advantage of providing spectral information in addition to estimates of photon indistinguishability. Further, our machine learning approach is broadly applicable to different photon correlation spectroscopy techniques and SPE systems, offering an enhanced tool for probing single emitter line shapes on previously inaccessible timescales.

74 ATOMIC AND MOLECULAR PHYSICS↗

DOE OSTI2026

Optimal filtering and generation of entangled photons for quantum applications in the presence of noise

Filtering is commonly used in quantum optics to reject noise photons, and also to enable interference between independent photons. However, filtering the joint spectrum of photon pairs can reduce the inherent coincidence probability or loss-independent heralding efficiency. Here we investigate filtering for multiphoton applications based on entanglement and interference (e.g., quantum teleportation). We multiplex C-band entangled photons and C-band classical communications into the same long-distance fibers, which enables scalable low-loss quantum networking but requires filtering of spontaneous Raman scattering noise from classical light. Using tunable-bandwidth filters, low-jitter detectors, and polarization filters, we distribute wavelength-degenerate time-bin entangled photons in the C band (1536.5 nm) over 25 km/25 km standard fibers (50 km) each carrying 10 Gbit/s C-band classical data signals. Narrow filtering enables milliwatt-level C-band power, which exceeds the power achieved by comparable studies by roughly an order of magnitude and could feasibly support terabit per second classical rates. We evaluate how performance depends on pump and filter bandwidths, multipair emission, filter shapes, loss, phase matching, and how quantum information is measured. We find a trade-off between reducing noise impact and increasing single-mode purity, and discuss mitigation methods toward optimal multiphoton applications. Importantly, these results apply to noise in free space and in quantum devices (sources, frequency converters, switches, detectors, etc.) and provide insight into filter-induced degradation of single-photon purity and rates even in noise-free environments.

Thomas, Jordan M. [Fermilab; Northwestern U.]↗

DOE OSTI2021

Passive Inter-Photon Imaging

Digital camera pixels measure image intensities by converting incident light energy into an analog electrical current, and then digitizing it into a fixed-width binary representation. This direct measurement method, while conceptually simple, suffers from limited dynamic range and poor performance under extreme illumination --- electronic noise dominates under low illumination, and pixel full-well capacity results in saturation under bright illumination. We propose a novel intensity cue based on measuring inter-photon timing, defined as the time delay between detection of successive photons. Based on the statistics of inter-photon times measured by a time-resolved single-photon sensor, we develop theory and algorithms for a scene brightness estimator which works over extreme dynamic range; we experimentally demonstrate imaging scenes with a dynamic range of over ten million to one. The proposed techniques, aided by the emergence of single-photon sensors such as single-photon avalanche diodes (SPADs) with picosecond timing resolution, will have implications for a wide range of imaging applications: robotics, consumer photography, astronomy, microscopy and biomedical imaging.

97 MATHEMATICS AND COMPUTING↗

DOE OSTI2025

Fast data-driven spectrometer with direct measurement of time and frequency for multiple single photons

We present a single-photon-sensitive spectrometer based on a linear array of 512 single-photon avalanche diode detectors with 0.04 nm spectral and 40 ps temporal resolutions. We employ a fast data-driven operation that allows direct measurement of time and frequency for simultaneous single photons, time- and frequency-stamping each single-photon detection. Our results combine excellent temporal and spectral resolution. This work opens numerous applications in quantum photonics, especially when both spectral and temporal properties of single photons can be exploited.

79 ASTRONOMY AND ASTROPHYSICS↗

DOE OSTI2021

Hybrid integrated photonic platforms: opinion

While photonic integration has made remarkable progress in recent years, there is no one integrated photonic platform that offers all desired functionalities and manufacturability on the same platform. GaAs and InP-based optoelectronic integrated circuits (OEICs) were very popular in the past decades; however, silicon photonics has recently emerged as a preferred platform due to its high-density and high-yield manufacturability leveraging the CMOS ecosystem, although it lacks optical gain, the Pockels effect, and other characteristics. On the other hand, hybrid photonic integration adds new and diverse functionalities to the host materials like silicon. This opinion paper investigates hybrid integrated photonic platforms, and discusses the new functionalities added to the silicon CMOS photonic platform.

42 ENGINEERING↗

DOE OSTI2020

Toward 1% single-photon anharmonicity with periodically poled lithium niobate microring resonators

The absence of the single-photon nonlinearity has been a major roadblock in developing quantum photonic circuits at optical frequencies. In this paper, we demonstrate a periodically poled thin film lithium niobate microring resonator (PPLNMR) that reaches 5,000,000%/W second-harmonic conversion efficiency—almost 20-fold enhancement over the state-of-the-art—by accessing its largest χ <#comment/> ( 2 ) tensor component d 33 via quasi-phase matching. The corresponding single-photon coupling rate g / 2 π <#comment/> is estimated to be 1.2 MHz, which is an important milestone as it approaches the dissipation rate κ <#comment/> / 2 π <#comment/> of best-available lithium niobate microresonators developed in the community. Using a figure of merit defined as g / κ <#comment/> , our device reaches a single-photon nonlinear anharmonicity approaching 1%. We show that, by further scaling of the device, it is possible to improve the single-photon anharmonicity to a regime where photon blockade effect can be manifested.

Lu, Juanjuan (ORCID:0000000319389119)↗

DOE OSTI2022

The photon content of the proton in the CT18 global analysis

Recently, two photon PDF sets based on implementations of the LUX ansatz into the CT18 global analysis were released. In CT18lux, the photon PDF is calculated directly using the LUX master formula for all scales, \mu μ . In an alternative realization, CT18qed, the photon PDF is initialized at the starting scale, \mu_0 μ 0 , using the LUX formulation and evolved to higher scales \mu(>\mu_0) μ ( > μ 0 ) with a combined QED+QCD kernel at \mathcal{O}(\alpha),~\mathcal{O}(\alpha\alpha_s) 𝒪 ( α ) , 𝒪 ( α α s ) and \mathcal{O}(\alpha^2) 𝒪 ( α 2 ) . In the small- x x region, the photon PDF uncertainty is mainly induced by the quark and gluon PDFs, through the perturbative DIS structure functions. In comparison, the large- x x photon uncertainty comes from various low-energy, nonperturbative contributions, including variations of the inelastic structure functions in the resonance and continuum regions, higher-twist and target-mass corrections, and elastic electromagnetic form factors of the proton. We take the production of doubly-charged Higgs pairs, (H^{++}H^{--}) ( H + + H − − ) , as an example of scenarios beyond the Standard Model to illustrate the phenomenological implications of these photon PDFs at the LHC.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

DOE OSTI2021

Photon Entanglement Spectroscopy and Imaging in Actinide Research

Quantumly entangled particles are capable of affecting the quantum state of their entangled counterpart instantaneously once one particle has changed. Herein, quantumly entangled photons are generated by spontaneous parametric down conversion through a temperature controlled non-linear crystals. This process generates two pairs of photons of lower energy of which the sum of energy equals the energy of the pump photons. These entangled photons can be separated and provide imaging capabilities by using one set of photons for imaging and the other set of photons for detection.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

DOE OSTI2024

Dark SRF, a cavity-based search for the Dark Photon: new exclusion limit and path forward

The dark photon is a hypothesized particle in extension to the Standard Model (SM) that would weakly interact with ordinary SM photons. An effective way to search for hidden sector photons in a laboratory set up is through light-shining-through-wall (LSW) schemes.We present here the first results of Dark SRF, a LSW experiment that leverages ultra-high quality factor superconducting radio frequency (SRF) cavities to search for dark photons. The use of Nb SRF cavities combined with a strict calibration and measurement protocol increased sensitivity to dark photons by several orders of magnitude compared to other LSW experiments, as demonstrated by our new exclusion limit on the dark photon mixing angle.In addition to the results of the search conducted in liquid helium using 1.3GHz SRF cavities, we also present the first steps of the second phase of the experiment, which will take place in a dilution refrigerator using 2.6GHz SRF cavities.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

DOE OSTI2024

The International Conference on Surface Plasmon Photonics 10

The International Conference on Surface Plasmon Photonics (SPP Conference) is widely regarded as the premier global conference in nanoscale photonics. The SPP10 meeting was held in the United States for the first time, at Rice University in Houston, Texas, on May 21-26, 2023. This conference was an outstanding venue for communicating research breakthroughs and accomplishments in the represented fields, as well as for visibility, networking, and recruiting, for students, postdoctoral fellows, and faculty throughout the US and the world as they attended this conference. The SPP10 conference hosted sessions on fundamental science, innovations, and applications in modern photonics with high potential for commercialization. Plenary sessions, invited talks from leading scientists in the field, and contributed talks from the larger photonics community on highly multidisciplinary topics of Quantum Plasmonics and Photonics; Energy Harvesting and Plasmonic Chemistry; Active Photonics and Devices; Ultrafast and Nonlinear Phenomena; and Machine Learning/Artificial Intelligence. The meeting schedule includes 3 plenary speakers, 31 Invited talks and 58 contributed talks. There were three well attended poster sessions which included lively discussions. Lunch time in the University Colleges allowed unstructured time for additional networking and discussions. The attendees represented the spectrum of endeavor in this field coming from academia, industry, and government laboratories, both U.S. and foreign scientists, senior researchers, young investigators, and students. The co-chairs of the conference were Prof. Naomi Halas and Prof. Peter Nordlander. The grant from DoE supported student’s and early career scientist’s registration and housing on campus.

77 NANOSCIENCE AND NANOTECHNOLOGY↗

DOE OSTI2024

MicroBooNE investigations on the photon interpretation of the MiniBooNE low energy excess

The MicroBooNE experiment is a liquid argon time projection chamber with 85-ton active volume at Fermilab, operated from 2015 to 2020 to collect neutrino data from Fermilab's Booster Neutrino Beam. One of MicroBooNE's physics goals is to investigate possible explanations of the low-energy excess observed by the MiniBooNE experiment in $\nu_{\mu}\rightarrow \nu_{e}$ neutrino oscillation measurements. MicroBooNE has performed searches to test hypothetical interpretations of the MiniBooNE low-energy excess, including the underestimation of the photon background or instrinic $\nu_{e}$ background. This thesis presents MicroBooNE's searches for two neutral current (NC) single-photon production processes that contribute to the photon background of the MiniBooNE measurement: NC $\Delta$ resonance production followed by $\Delta$ radiative decay: $\Delta \rightarrow N\gamma$, and NC coherent single-photon production. Both searches take advantage of boosted decision trees to yield efficient background rejection, and a high-statistic NC $\pi^0$ measurement to constrain dominant background, and make use of MicroBooNE's first three years of data. The NC $\Delta \rightarrow N\gamma$ measurement yielded a bound on the $\Delta$ radiative decay process at 2.3 times the predicted nominal rate at 90\% confidence level(C.L.), disfavoring a candidate photon interpretation of the MiniBooNE low-energy excess as a factor of 3.18 times the nominal NC Δ radiative decay rate at the 94.8\% C.L. The NC coherent single photon measurement leads to the world's first experimental limit on the cross-section of this process below 1 GeV, of $1.49 \times 10^{-41} \text{cm}^2$ at 90\% C.L., corresponding to 24.0 times the nominal prediction.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗