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At least 181 records · Page 10

Evaluation of cosmogenic production of 39 Ar and 42 Ar for rare-event physics using underground argon

Underground argon (UAr) with lower cosmogenic activities of 39 Ar and 42 Ar has been planned as a detector in detecting scintillation light and charge collection using time projection chambers for dark matter searches and as a veto detector in suppressing backgrounds for neutrinoless double beta decay (0$vββ$ ) experiments. Long-lived radioactive isotopes, 39 Ar and 42 Ar, can also be produced on the surface when UAr is pumped out from a deep well. Understanding the production of long-lived isotopes in Ar is important for utilizing UAr for dark matter and 0$vββ$ experiments in terms of its production, transportation, and storage. Ar exposure to cosmic rays at sea-level is simulated using Geant4 for a given cosmic ray muon, neutron, and proton energy spectrum. Here we report the simulated cosmogenic production rates of 39 Ar, 42 Ar, and other long-lived isotopes at sea-level from fast neutrons, high energy muons, and high energy protons. Total production rates of 938.53/kg Ar day and 5.81 × 10 -3 /kg Ar day for 39 Ar and 42 Ar are found from our simulation. Utilizing these production rates, we set a time limit of 954 days constrained by the production of 39 Ar for UAr to be on the surface before it compromises the sensitivity for a dark matter experiment. Similarly, a time limit of 1702 days constrained by the production of 42 Ar is found for a 0$vββ$ experiment.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

A preliminary investigation into the electrodeposition and synthesis of radiopure Copper–Chromium alloys for rare-event physics detector systems

Current investigations into neutrinoless double beta decay and the direct detection of dark matter require increasingly sensitive detector systems that demand ultra-low background materials. These requirements have previously been attained using ultra-radiopure electroformed (EF) copper. However, pure copper possesses high ductility and relatively low strength, which necessitates the need for large amounts of material and extra care during fabrication to help minimize galling and mechanical failure. Furthermore, we investigate an alloying alternative to pure EF copper by examining low wt% copper chrome (Cu–Cr) solid solution alloys, with inquiries into alloy hardness, strength, and radiopurity. Alloyed Cu–Cr layered samples are shown to exhibit significantly increased hardness compared to EF copper, for example showing a 50% increase in exhibited hardness using less than 1% Cr by weight, with limited negative impact to the material’s radiopurity.

Background↗

Design and production of the high voltage electrode grids and electron extraction region for the LZ dual-phase xenon time projection chamber

The dual-phase xenon time projection chamber (TPC) is a powerful tool for direct-detection experiments searching for WIMP dark matter, other dark matter models, and neutrinoless double-beta decay. Successful operation of such a TPC is critically dependent on the ability to hold high electric fields in the bulk liquid, across the liquid surface, and in the gas. Careful design and construction of the electrodes used to establish these fields is therefore required. We present the design and production of the LUX-ZEPLIN (LZ) experiment's high-voltage electrodes, a set of four woven mesh wire grids. Grid design drivers are discussed, with emphasis placed on design of the electron extraction region. Here, we follow this with a description of the grid production process and a discussion of steps taken to validate the LZ grids prior to integration into the TPC.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Temperature-dependent charge barrier height of amorphous germanium contact detector

The exploration of germanium (Ge) detectors with amorphous Ge (a-Ge) contacts has drawn attention to the searches for rare-event physics such as dark matter and neutrinoless double-beta decay. The charge barrier height (CBH) of the a-Ge contacts deposited on the detector surface is crucial to suppress the leakage current of the detector in order to achieve a low-energy detection threshold and high-energy resolution. The temperature-dependent CBH of a-Ge contacts for three Ge detectors is analyzed to study the bulk leakage current (BLC) characteristics. The detectors were fabricated at the University of South Dakota using homegrown crystals. The CBH is determined from the BLC when the detectors are operated in the reverse bias mode with a guard-ring structure, which separates the BLC from the surface leakage current (SLC). Here the results show that CBH is temperature dependent. The direct relation of the CBH variation to temperature is related to the barrier inhomogeneities created on the interface of a-Ge and crystalline Ge. The inhomogeneities that occur at the interface were analyzed using the Gaussian distribution model for three detectors.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Ultra-sensitive radon assay using an electrostatic chamber in a recirculating system

Rare event searches such as neutrinoless double beta decay and Weakly Interacting Massive Particle detection require ultra-low background detectors. Radon contamination is a significant challenge for these experiments, which employ highly sensitive radon assay techniques to identify and select low-emission materials. This work presents the development of ultra-sensitive electrostatic chamber (ESC) instruments designed to measure radon emanation in a recirculating gas loop, for future lower background experiments. Unlike traditional methods that separate emanation and detection steps, this system allows continuous radon transport and detection. This is made possible with a custom-built recirculation pump. A Python-based analysis framework, PyDAn, was developed to process and fit time-dependent radon decay data. Radon emanation rates are given for various materials measured with this instrument. A radon source of known activity provides an absolute calibration, enabling statistically-limited minimal detectable activities of 20 µBq. These devices are powerful tools for screening materials in the development of low-background particle physics experiments.

47 OTHER INSTRUMENTATION↗

Demonstration of Selective Single-Barium Ion Detection with Dry Diazacrown Ether Naphthalimide Turn-on Chemosensors

Single-molecule fluorescence imaging (SMFI) of gas-phase ions has been proposed for “barium tagging,” a burgeoning area of research in particle physics to detect individual barium daughter ions. This has potential to significantly enhance the sensitivity of searches for neutrinoless double-beta decay (0νββ) that is obscured by background radiation events. The chemistry required to make such sensitive detection of Ba 2+ by SMFI in dry Xe gas at solid interfaces has implications for solid-phase detection methods but has not been demonstrated. Here, we synthesized simple, robust, and effective Ba 2+ -selective chemosensors capable of function within ultrapure high-pressure 136 Xe gas. Turn-on fluorescent naphthalimide-(di)azacrown ether chemosensors were Ba 2+ -selective and achieved SMFI in a polyacrylamide matrix. Here, fluorescence and NMR experiments supported a photoinduced electron transfer mechanism for turn-on sensing. Ba 2+ selectivity was achieved with computational calculations correctly predicting the fluorescence responses of sensors to barium, mercury, and potassium ions. With these molecules, dry-phase single-Ba 2+ ion imaging with turn-on fluorescence was realized using an oil-free microscopy technique for the first time—a significant advance toward single-Ba 2+ ion detection within large volumes of 136 Xe, plausibly enabling a background-independent technique to search for the hypothetical process of 0νββ.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Ba +2 ion trapping using organic submonolayer for ultra-low background neutrinoless double beta detector

If neutrinos are their own antiparticles the otherwise-forbidden nuclear reaction known as neutrinoless double beta decay can occur. The very long lifetime expected for these exceptional events makes its detection a daunting task. In order to conduct an almost background-free experiment, the NEXT collaboration is investigating novel synthetic molecular sensors that may capture the Ba dication produced in the decay of certain Xe isotopes in a high-pressure gas experiment. The use of such molecular detectors immobilized on surfaces must be explored in the ultra-dry environment of a xenon gas chamber. Here, using a combination of highly sensitive surface science techniques in ultra-high vacuum, we demonstrate the possibility of employing the so-called Fluorescent Bicolor Indicator as the molecular component of the sensor. We unravel the ion capture process for these molecular indicators immobilized on a surface and explain the origin of the emission fluorescence shift associated to the ion trapping.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

First-Principles insights into group-V impurities and their impact on germanium detector performance

The outstanding properties of high-purity germanium (HPGe) detectors, such as excellent energy resolution, high energy sensitivity, and a low background-to-signal ratio, make them essential and ideal candidates for detecting particle signatures in nuclear processes such as neutrino-less double beta decay (0νββ). However, the presence of defects and impurities in HPGe crystals can lead to charge trapping, which affects carrier mobility and results in significant energy resolution degradation. In this work, we employ density functional theory with a hybrid functional to study the energetics of possible point defects in Ge. Our findings indicate that group-V impurities form more readily in Ge compared to vacancy and interstitial of Ge. Unlike N dopants, which yield deep trap states, P, As, and Sb create shallow traps close to the conduction band edge of Ge. Furthermore, we predict that group-V defects can condense into defect complexes with Ge vacancies. These vacancy-impurity complexes form deep traps in Ge, similar to Ge vacancies, suggesting that both vacancies and vacancy-impurity complexes contribute to charge trapping in these detectors, thereby diminishing their performance.

36 MATERIALS SCIENCE↗

Controlling T c of iridium films using the proximity effect

A superconducting Transition-Edge Sensor (TES) with low-$T_c$ is essential in a high resolution calorimetric detection. With a motivation of developing sensitive calorimeters for applications in cryogenic neutrinoless double beta decay searches, we have been investigating methods to reduce the $T_c$ of an Ir film down to 20 mK. Utilizing the proximity effect between a superconductor and a normal metal, we found two room temperature fabrication recipes of making Ir-based low-$T_c$ films. In the first approach, an Ir film sandwiched between two Au films, a Au/Ir/Au trilayer, has a tunable $T_c$ in the range of 20-100 mK depending on the relative thicknesses. In the second approach, a paramagnetic Pt thin film is used to create Ir/Pt bilayer with a tunable $T_c$ in the same range. We present detailed study of fabrication and characterization of Ir-based low-$T_c$ films, and compare the experimental results to theoretical models. We show that Ir-based films with predictable and reproducible critical temperature can be consistently fabricated for use in large scale detector applications.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Performance of a large area photon detector for rare event search applications

We present the design and characterization of a large-area Cryogenic PhotoDetector designed for active particle identification in rare event searches, such as neutrinoless double beta decay and dark matter experiments. The detector consists of a 45.6 cm 2 surface area by a 1-mm-thick 10.6 g Si wafer. It is instrumented with a distributed network of Quasiparticle-trap-assisted Electrothermal feedback Transition-edge sensors with superconducting critical temperature T c = 41.5 mK to measure a thermal phonons released from interactions with photons.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Large low background kTon-scale liquid argon time projection chambers

Here we find that it is possible to increase sensitivity to low energy physics in a third or fourth Deep Underground Neutrino Experiment (DUNE)-like module with careful controls over radiopurity and targeted modifications to a detector similar to the DUNE Far Detector design. In particular, sensitivity to supernova and solar neutrinos can be enhanced with improved MeV-scale reach. A neutrinoless double beta decay search with 136 Xe loading appears feasible. Furthermore, sensitivity to Weakly-Interacting Massive Particle (WIMP) Dark Matter becomes competitive with the planned world program in such a detector, offering a unique seasonal variation detection that is characteristic of the nature of WIMPs.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Neutrino mass and mass ordering: no conclusive evidence for normal ordering

The extraction of the neutrino mass ordering is one of the major challenges in particle physics and cosmology, not only for its implications for a fundamental theory of mass generation in nature, but also for its decisive role in the scale of future neutrinoless double beta decay experimental searches. It has been recently claimed that current oscillation, beta decay and cosmological limits on the different observables describing the neutrino mass parameter space provide robust decisive Bayesian evidence in favor of the normal ordering of the neutrino mass spectrum. We further investigate these strong claims using a rich and wide phenomenology, with different sampling techniques of the neutrino parameter space. Contrary to the findings of Jimenez et al., no decisive evidence for the normal mass ordering is found. Neutrino mass ordering analyses must rely on priors and parameterizations that are ordering-agnostic: robust results should be regarded as those in which the preference for the normal neutrino mass ordering is driven exclusively by the data, while we find a difference of up to a factor of 33 in the Bayes factors among the different priors and parameterizations exploited here. An ordering-agnostic prior would be represented by the case of parameterizations sampling over the two mass splittings and a mass scale, or those sampling over the individual neutrino masses via normal prior distributions only. In this regard, we show that the current significance in favor of the normal mass ordering should be taken as 2.7σ (i.e. moderate evidence), mostly driven by neutrino oscillation data. Let us stress that, while current data favor NO only mildly, we do not exclude the possibility that this may change in the future. Eventually, upcoming oscillation and cosmological data may (or may not) lead to a more significant exclusion of IO.

79 ASTRONOMY AND ASTROPHYSICS↗

Search for charged excitations of dark matter by KamLAND-Zen experiment

There are many scenarios in which dark matter is a part of a multiplet with an electrically charged state. If WIMP dark matter is accompanied by a charged state separated by a small mass difference, it can form stable bound states with nuclei. The region of observable energy deposition via this process of bound state formation is O(1˜10 MeV). KamLAND-Zen is a large scintillator detector designed for neutrino-less double-beta decay search. This detector is also useful to detect dark matter bound state formations with nuclei. The result from the KamLAND-Zen 400 dataset is reported.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Perspectives of lowering CUORE thresholds with Optimum Trigger

CUORE is a cryogenic experiment that focuses on the search of neutrinoless double beta decay in 130Te and it is located at the Gran Sasso National Laboratories. Its detector consists of 988 TeO 2 crystals operating at a base temperature of ~10 mK. It is the first ton-scale bolometric experiment ever realized for this purpose. Thanks to its large target mass and ultra-low background, the CUORE detector is also suitable for the search of other rare phenomena. In particular the low energy part of the spectra is interesting for the detection of WIMP-nuclei scattering reactions. One of the most important requirements to perform these studies is represented by the achievement of a stable energy threshold lower than 10 keV. Here, the CUORE capability to accomplish this purpose using a low energy software trigger will be presented and described.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Radio frequency and DC high voltage breakdown of high pressure helium, argon, and xenon

Motivated by the possibility of guiding daughter ions from double beta decay events to single-ion sensors for barium tagging, the NEXT collaboration is developing a program of R&D to test radio frequency (RF) carpets for ion transport in high pressure xenon gas. This would require carpet functionality in regimes at higher pressures than have been previously reported, implying correspondingly larger electrode voltages than in existing systems. This mode of operation appears plausible for contemporary RF-carpet geometries due to the higher predicted breakdown strength of high pressure xenon relative to low pressure helium, the working medium in most existing RF carpet devices. In this paper we present the first measurements of the high voltage dielectric strength of xenon gas at high pressure and at the relevant RF frequencies for ion transport (in the 10 MHz range), as well as new DC and RF measurements of the dielectric strengths of high pressure argon and helium gases at small gap sizes. We find breakdown voltages that are compatible with stable RF carpet operation given the gas, pressure, voltage, materials and geometry of interest.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

DIREXENO—an apparatus for measuring correlated scintillation signatures in liquid xenon

We present a detector apparatus, DIREXENO (DIREctional XENOn), designed to measure the spatial and temporal properties of scintillation in liquid xenon to very high accuracy. The properties of scintillation are of primary importance for dark matter and neutrinoless double beta decay experiments; however the complicated microphysics involved limits theoretical predictions. We will explore the possibility that scintillation emission exhibits spatial correlations such as super-radiance which manifests in temporal and spatial structure, depending on the interaction type. Such properties of scintillation light may open a new window for background rejection as well as directionality measurements. We present the apparatus' technical design and the concepts driving it. We demonstrate that for an energy deposition of ~2.5 keV (~7.5 keV) electron (nuclear) recoil the detector is sensitive to an anisotropy fraction of as little as ~ 20% of the total photons emitted over a solid angle of ~0.85 steradian or less. We show results from commissioning runs in which the detector operated with 17 PMTs for over 44 days in stable conditions. The time resolution for individual photons in different PMTs was measured to be ≲1.4 ns full-width at half-maximum

47 OTHER INSTRUMENTATION↗

Pulse shape discrimination in CUPID-Mo using principal component analysis

CUPID-Mo is a cryogenic detector array designed to search for neutrinoless double-beta decay ($0\nu\beta\beta$) of $^{100}$Mo. It uses 20 scintillating $^{100}$Mo-enriched Li$_2$MoO$_4$ bolometers instrumented with Ge light detectors to perform active suppression of $\alpha$ backgrounds, drastically reducing the expected background in the $0\nu\beta\beta$ signal region. As a result, pileup events and small detector instabilities that mimic normal signals become non-negligible potential backgrounds. These types of events can in principle be eliminated based on their signal shapes, which are different from those of regular bolometric pulses. We show that a purely data-driven principal component analysis based approach is able to filter out these anomalous events, without the aid of detector response simulations.

47 OTHER INSTRUMENTATION↗

Optical calibration of the SNO+ detector in the water phase with deployed sources

SNO+ is a large-scale liquid scintillator experiment with the primary goal of searching for neutrinoless double beta decay, and is located approximately 2 km underground in SNOLAB, Sudbury, Canada. The detector acquired data for two years as a pure water Cherenkov detector, starting in May 2017. During this period, the optical properties of the detector were measured in situ using a deployed light diffusing sphere, with the goal of improving the detector model and the energy response systematic uncertainties. The measured parameters included the water attenuation coefficients, effective attenuation coefficients for the acrylic vessel, and the angular response of the photomultiplier tubes and their surrounding light concentrators, all across different wavelengths. Finally, the calibrated detector model was validated using a deployed tagged gamma source, which showed a 0.6% variation in energy scale across the primary target volume.

47 OTHER INSTRUMENTATION↗