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NASA NTRSDate not supplied

CERES Single Scanner Satellite Footprint, TOA, Surface Fluxes and Clouds (SSF) data in HDF (CER_SSF_Terra-FM1-MODIS_Edition1A)

The Single Scanner Footprint TOA/Surface Fluxes and Clouds (SSF) product contains one hour of instantaneous Clouds and the Earth's Radiant Energy System (CERES) data for a single scanner instrument. The SSF combines instantaneous CERES data with scene information from a higher-resolution imager such as Visible/Infrared Scanner (VIRS) on TRMM or Moderate-Resolution Imaging Spectroradiometer (MODIS) on Terra and Aqua. Scene identification and cloud properties are defined at the higher imager resolution and these data are averaged over the larger CERES footprint. For each CERES footprint, the SSF contains the number of cloud layers and for each layer the cloud amount, height, temperature, pressure, optical depth, emissivity, ice and liquid water path, and water particle size. The SSF also contains the CERES filtered radiances for the total, shortwave (SW), and window (WN) channels and the unfiltered SW, longwave (LW), and WN radiances. The SW, LW, and WN radiances at spacecraft altitude are converted to Top-of-the-Atmosphere (TOA) fluxes based on the imager defined scene. These TOA fluxes are used to estimate surface fluxes. Only footprints with adequate imager coverage are included on CER_SSF_TRMM-PFM-VIRS_Subset_Edition1the SSF which is much less than the full set of footprints on the CERES ES-8 product. The following CERES SSF data sets are currently available: CER_SSF_TRMM-PFM-VIRS_Edition1 CER_SSF_TRMM-PFM-VIRS_Subset_Edition1 CER_SSF_TRMM-PFM-VIRS_Edition2A CER_SSF_TRMM-SIM-VIRS_Edition2_VIRSonly CER_SSF_TRMM-PFM-VIRS_Edition2A-TransOps CER_SSF_TRMM-PFM-VIRS_Edition2B-TransOps CER_SSF_TRMM-PFM-VIRS_Edition2B CER_SSF_Terra-FM1-MODIS_Edition1A CER_SSF_Terra-FM1-MODIS_Edition1A CER_SSF_Terra-FM1-MODIS_Edition2A CER_SSF_Terra-FM2-MODIS_Edition2A CER_SSF_Terra-FM1-MODIS_Edition2B CER_SSF_Terra-FM2-MODIS_Edition2B CER_SSF_Aqua-FM4-MODIS_Beta1 CER_SSF_Aqua-FM3-MODIS_Beta2 CER_SSF_Aqua-FM4-MODIS_Beta2. [Location=GLOBAL] [Temporal_Coverage: Start_Date=1998-01-01; Stop_Date=2002-10-31] [Spatial_Coverage: Southernmost_Latitude=-90; Northernmost_Latitude=90; Westernmost_Longitude=-180; Easternmost_Longitude=180] [Data_Resolution: Temporal_Resolution=1 hour; Temporal_Resolution_Range=Hourly - < Daily].

LONGWAVE UNFILTERED RADIANCE↗
NASA NTRS1979

Detection of SO2 in the UV spectrum of Venus

The broad absorption feature below 3300 A in the Venus UV spectrum is identified as primarily due to SO2 absorption based on new higher resolution spectra of the 3000-3400 A region showing broad (10 A), unresolved absorptions in the regions at all SO2 band origins between 3000 and 3300 A. SO2 mixing ratios vary from 5 x 10 to the -7th down to an upper limit of 2 x 10 to the -8th at a phase angle of 138 deg. Previous observational determinations of the SO2 mixing ratio were biased toward large phase angles, and consequently did not detect any SO2 absorption at the 10 to the -8th level. The upper limit derived from the CS2 band head at 3206 A is not greater than 5 x 10 to the -8th. The observed range of SO2 mixing ratios is consistent with model predictions based on the sulfur photochemistry at the cloud tops. Ground-based observations of SO2 mixing ratio will provide constraints on models and check on the Venera and Pioneer Venus measurements of the mixing ratios of SO2 and other sulfur-bearing gases with altitude.

Barker, E. S.↗
NASA NTRS1980

Charge distribution in lightning flashes

Four VHF receivers about 10 km apart were used to detect three-dimensional lightning VHF sources during active thunderstorms. A computer implemented algorithm was used to determine the difference in the time of arrival (DTOA) between the VHF pulses. The three-dimensional source locations determined from the DTOA were correlated with ground electric field measurements (0.1 Hz to 1.5 MHz). Four cloud to ground (CG) and three intracloud (IC) flashes, selected randomly, were studied. A point charge model was used to determine the charge being removed during the different phases of CG and IC flashes. It was determined that return strokes lowered between 24.1 and 3.6 coulombs of negative charge to ground from heights between 10.5 and 5.8 km above MSL. The interstroke process after the first return stroke in a CG flash lowered between 3.4 and 0.9 coulombs of negative charge between the heights of 14.2 (near the cloud tops) to heights of 5.8 km (near the beginning of the leader-return stroke process).

Rustan, P. L.↗
NASA NTRS1975

Detection of water vapor on Jupiter

High-altitude (12.4 km) spectroscopic observations of Jupiter at 5 microns from the NASA 91.5 cm airborne infrared telescope have revealed 14 absorptions assigned to the rotation-vibration spectrum of water vapor. Preliminary analysis indicates a mixing ratio about 1 millionth for the vapor phase of water. Estimates of temperature (greater than about 300 K) and pressure (less than 20 atm) suggest observation of water deep in Jupiter's hot spots responsible for its 5 micron flux. Model-atmosphere calculations based on radiative-transfer theory may change these initial estimates and provide a better physical picture of Jupiter's atmosphere below the visible cloud tops.

Larson, H. P.↗
NASA NTRS2006

Model Calculations of Solar Spectral Irradiance in the 3.7 Micron Band for Earth Remote Sensing Applications

Since the launch of the first Advanced Very High Resolution Radiometer (AVHRR) instrument aboard TIROS-N, measurements in the 3.7 micron atmospheric window have been exploited for use in cloud detection and screening, cloud thermodynamic phase and surface snow/ice discrimination, and quantitative cloud particle size retrievals. The utility of the band has led to the incorporation of similar channels on a number of existing satellite imagers and future operational imagers. Daytime observations in the band include both reflected solar and thermal emission energy. Since 3.7 micron channels are calibrated to a radiance scale (via onboard blackbodies), knowledge of the top-of-atmosphere solar irradiance in the spectral region is required to infer reflectance. Despite the ubiquity of 3.7 micron channels, absolute solar spectral irradiance data comes from either a single measurement campaign (Thekaekara et al. 1969) or synthetic spectra. In this study, we compare historical 3.7 micron band spectral irradiance data sets with the recent semi-empirical solar model of the quiet-Sun by Fontenla et al. (2006). The model has expected uncertainties of about 2 % in the 3.7 pm spectral region. We find that channel-averaged spectral irradiances using the observations reported by Thekaekara et al. are 3.2-4.1% greater than those derived from the Fontenla et al. model for MODIS and AVHRR instrument bandpasses; the Kurucz spectrum (1995) as included in the MODTRAN4 distribution, gives channel-averaged irradiances 1.2-1.5 % smaller than the Fontenla model. For the MODIS instrument, these solar irradiance uncertainties result in cloud microphysical retrievals uncertainties comparable with other fundamental reflectance error sources.

Platnick, Steven↗
NASA NTRS2012

The Operational MODIS Cloud Optical and Microphysical Property Product: Overview of the Collection 6 Algorithm and Preliminary Results

Operational Moderate Resolution Imaging Spectroradiometer (MODIS) retrievals of cloud optical and microphysical properties (part of the archived products MOD06 and MYD06, for MODIS Terra and Aqua, respectively) are currently being reprocessed along with other MODIS Atmosphere Team products. The latest "Collection 6" processing stream, which is expected to begin production by summer 2012, includes updates to the previous cloud retrieval algorithm along with new capabilities. The 1 km retrievals, based on well-known solar reflectance techniques, include cloud optical thickness, effective particle radius, and water path, as well as thermodynamic phase derived from a combination of solar and infrared tests. Being both global and of high spatial resolution requires an algorithm that is computationally efficient and can perform over all surface types. Collection 6 additions and enhancements include: (i) absolute effective particle radius retrievals derived separately from the 1.6 and 3.7 !-lm bands (instead of differences relative to the standard 2.1 !-lm retrieval), (ii) comprehensive look-up tables for cloud reflectance and emissivity (no asymptotic theory) with a wind-speed interpolated Cox-Munk BRDF for ocean surfaces, (iii) retrievals for both liquid water and ice phases for each pixel, and a subsequent determination of the phase based, in part, on effective radius retrieval outcomes for the two phases, (iv) new ice cloud radiative models using roughened particles with a specified habit, (v) updated spatially-complete global spectral surface albedo maps derived from MODIS Collection 5, (vi) enhanced pixel-level uncertainty calculations incorporating additional radiative error sources including the MODIS L1 B uncertainty index for assessing band and scene-dependent radiometric uncertainties, (v) and use of a new 1 km cloud top pressure/temperature algorithm (also part of MOD06) for atmospheric corrections and low cloud non-unity emissivity temperature adjustments.

Platnick, Steven↗
NASA NTRS2001

Characterizing the Influence of the General Circulation on Marine Boundary Layer Clouds

The seasonal and intraseasonal variability of boundary layer cloud in the subtropical eastern oceans are studied using combined data from the International Satellite Cloud Climatology Project (ISCCP) and the European Centre for Medium-Range Weather Forecasts (ECMWF) reanalysis. Spectral analysis reveals that most of the time variability of cloud properties occurs on seasonal to annual time scales. The variance decreases one to two orders of magnitude for each decade of time scale decrease, indicating that daily to monthly time scales have smaller, but non-negligible variability. The length of these dominant time scales suggests that the majority of the variability is influenced by the general circulation and its interaction with boundary layer turbulence, rather than a product of boundary layer turbulence alone. Previous datasets have lacked the necessary resolution in either time or in space to properly characterize variability on synoptic scales; this is remedied by using global satellite-retrieved cloud properties. We characterize the intraseasonal subtropical cloud variability in both hemispheres and in different seasons. In addition to cloud fraction, we examine variability of cloud optical thickness - cloud top pressure frequency distributions. Despite the large concentration of research on the variability of Northern Hemisphere (NH) regions during summer, it is noted that the largest amplitude intraseasonal variability in the NH regions occurs during local winter. The effect of intraseasonal variability on the calculation and interpretation of seasonal results is investigated. Decreases in seasonally averaged cloud cover, optical thickness and cloud top pressure from the May-through-September season to the November-through-March season are most apparent in the NH regions. Further analysis indicates that these changes are due to an increase in frequency, but a decrease in the persistence of synoptic events. In addition, changes in cloud top pressure and optical thickness characteristics from the summer to winter seasons indicate that the NH subtropics undergo a change in dynamic regime with season. This change appears in the cloud fields as a shift from the more commonly seen lower-altitude, thicker optical thickness clouds to higher-altitude, thinner clouds. The latter cloud-type is associated with the lower sea level pressure, upward vertical velocity phase of the synoptic wave. Intraseasonal changes in cloud properties in the Southern Hemisphere and NH summer are much smaller in amplitude. Although they also appear to be linked to changes in the large-scale dynamics, similarly to NH winter variations, the relationships are more ambiguous due to the small amplitudes and longer time scales. We attempt to interpret some of these relationships using the results of the Betts and Ridgway (1989) box model. However, these results cannot consistently explain the patterns when results from all regions are considered, implying that this model may not adequately explain all the processes involved in the variability.

Rozendaal, Margaret A.↗
NASA NTRS2004

Diurnal, Seasonal, and Interannual Variations of Cloud Properties Derived for CERES From Imager Data

Simultaneous measurement of the radiation and cloud fields on a global basis is a key component in the effort to understand and model the interaction between clouds and radiation at the top of the atmosphere, at the surface, and within the atmosphere. The NASA Clouds and Earth s Radiant Energy System (CERES) Project, begun in 1998, is meeting this need. Broadband shortwave (SW) and longwave radiance measurements taken by the CERES scanners at resolutions between 10 and 20 km on the Tropical Rainfall Measuring Mission (TRMM), Terra, and Aqua satellites are matched to simultaneous retrievals of cloud height, phase, particle size, water path, and optical depth OD from the TRMM Visible Infrared Scanner (VIRS) and the Moderate Resolution Imaging Spectroradiometer (MODIS) on Terra and Aqua. Besides aiding the interpretation of the broadband radiances, the CERES cloud properties are valuable for understanding cloud variations at a variety of scales. In this paper, the resulting CERES cloud data taken to date are averaged at several temporal scales to examine the temporal and spatial variability of the cloud properties on a global scale at a 1 resolution.

Minnis, Patrick↗
NASA NTRS2010

A Principal Component-Based Radiative Transfer Forward Model (PCRTM) for Vertically in Homogeneous Cloud

A principal-component based radiative transfer model (PCRTM) is developed for simulating the infrared spectral radiance at the top of the atmosphere (TOA). The PCRTM approach removes the redundancy in radiative transfer calculation in high resolution infrared spectra, and saves significant amount of computational time with great accuracy. In PCRTM, both ice and water clouds are treated as effective transmissivity and reflectivity stored in a pre-calculated lookup tables. These quantities are calculated using cloud single scattering properties such as cloud optical depth, cloud particle size, cloud phase, etc. The cloud can be inserted into any pressure layer in the PCRTM model (up to 100 layers). The effective temperature of each cloud layer is treated as a function of its optical depth. To test the accuracy of this approximation, the results are compared with the more rigorous DISORT model, which treats cloud as a plane parallel layer. The root-mean-square error of PCRTM, with respect to DISORT results, is generally less than 0.5 K in brightness temperature. However, the CPU time required by PCRTM was approximately two orders of magnitude less than that required by DISORT.

Li, Hui↗
NASA NTRSDate not supplied

CERES Clouds and Radiative Swath (CRS) data in HDF (CER_CRS_TRMM-PFM-VIRS_Edition2C)

The Clouds and Radiative Swath (CRS) product contains one hour of instantaneous Clouds and the Earth's Radiant Energy System (CERES) data for a single scanner instrument. The CRS contains all of the CERES SSF product data. For each CERES footprint on the SSF the CRS also contains vertical flux profiles evaluated at four levels in the atmosphere: the surface, 500-, 70-, and 1-hPa. The CRS fluxes and cloud parameters are adjusted for consistency with a radiative transfer model and adjusted fluxes are evaluated at the four atmospheric levels for both clear-sky and total-sky. [Location=GLOBAL] [Temporal_Coverage: Start_Date=1998-01-01; Stop_Date=2000-03-31] [Spatial_Coverage: Southernmost_Latitude=-90; Northernmost_Latitude=90; Westernmost_Longitude=-180; Easternmost_Longitude=180] [Data_Resolution: Temporal_Resolution=1 hour; Temporal_Resolution_Range=Hourly - < Daily].

ICE PARTICLE DIAMETER↗
NASA NTRS2022

Assessment of Two Stochastic Cloud Subcolumn Generators Using Observed Fields of Vertically Resolved Cloud Extinction

We evaluate two stochastic subcolumn generators used in GCMs to emulate subgrid cloud variability enabling comparisons with satellite observations and simulations of certain physical processes. Our evaluation necessitated the creation of a reference observational dataset that resolves horizontal and vertical cloud variability. The dataset combines two CloudSat cloud products that resolve two-dimensional cloud optical depth variability of liquid, ice, and mixed phase clouds when blended at ~200 m vertical and ~ 2 km horizontal scales. Upon segmenting the dataset to individual “scenes”, mean profiles of the cloud fields are passed as input to generators that produce scene-level cloud subgrid variability. The assessment of generator performance at the scale of individual scenes and in a mean sense is largely based on inferred joint histograms that partition cloud fraction within predetermined combinations of cloud top pressure –cloud optical thickness ranges. Our main finding is that both generators tend to underestimate optically thin clouds, while one of them also tends to overestimate some cloud types of moderate and high optical thickness. Associated radiative flux errors are also calculated by applying a simple transformation to the cloud fraction histogram errors, and are found to approach values almost as high as 3 Wm-2 for the cloud radiative effect in the shortwave part of the spectrum.

cloud variability↗
NASA NTRSDate not supplied

CERES Monthly Gridded Single Satellite TOA and Surfaces/Clouds (SFC) data in HDF (CER_SFC_Terra-FM2-MODIS_Edition2C)

The Monthly Gridded TOA/Surface Fluxes and Clouds (SFC) product contains a month of space and time averaged Clouds and the Earth's Radiant Energy System (CERES) data for a single scanner instrument. The SFC is also produced for combinations of scanner instruments. All instantaneous shortwave, longwave, and window fluxes at the Top-of-the-Atmosphere (TOA) and surface from the CERES SSF product for a month are sorted by 1-degree spatial regions and by the local hour of observation. The mean of the instantaneous fluxes for a given region-hour bin is determined and recorded on the SFC along with other flux statistics and scene information. These average fluxes are given for both clear-sky and total-sky scenes. The regional cloud properties are column averaged and are included on the SFC. [Location=GLOBAL] [Temporal_Coverage: Start_Date=1998-01-01; Stop_Date=2005-12-31] [Spatial_Coverage: Southernmost_Latitude=-90; Northernmost_Latitude=90; Westernmost_Longitude=-180; Easternmost_Longitude=100] [Data_Resolution: Latitude_Resolution=1 degree; Longitude_Resolution=1 degree; Horizontal_Resolution_Range=100 km - < 250 km or approximately 1 degree - < 2.5 degrees; Temporal_Resolution=1 hour; Temporal_Resolution_Range=Hourly - < Daily].

CLEAR-SKY ALBEDO↗
NASA NTRS1991

Nonlinear wave scattering and electron beam relaxation

The role played by nonlinear scattering during the relaxation of a warm electron beam is investigated through a numerical code based on kinetic equations. The code encompasses the quasi-linear wave-electron interaction and wave-wave scattering off ion clouds. Ions with velocities 2 nu sub i (nu sub i being the ion thermal velocity) are found to be the most efficient for scattering the Langmuir waves off their polarization clouds. The transfer rate of the spectrum out of resonance with the beam is larger by a factor 3 compared to usual estimates. The changes produced in the dispersion relation by the presence of the beam electrons dramatically alter the characteristics of the secondary spectrum. In a late phase the classic condensate K of about 0 is depleted, with the formation of a new condensate in resonance with the flat-topped beam distribution, which follows from the fact that the mere presence of the beam electrons creates a minimum in the frequency-wave-number relation. For strong and slow beams, the predictions of the code are found to be in excellent agreement with the results of the particle simulation if a dispersion relation that includes the beam is used.

Muschietti, L.↗
NASA NTRS2024

An Airborne Multi-Frequency Microwave Analysis of Precipitation within Two Winter Cyclones

NASA’s Investigation of Microphysics and Precipitation for Atlantic Coast-Threatening Snowstorms (IMPACTS) field campaign gathered data using “satellite-simulating” (albeit with higher-resolution data than satellites currently provide) and in situ aircraft to study snowstorms, with an emphasis on banding. This study used three IMPACTS microwave instruments—two passive and one active—chosen for their sensitivity to precipitation microphysics. The 10–37-GHz passive frequencies were well suited for detecting light precipitation and differentiating rain intensities over water. The 85–183-GHz frequencies were more sensitive to cloud ice, with higher cloud tops manifesting as lower brightness temperatures, but this did not necessarily correspond well to near-surface precipitation. Over land, retrieving precipitation information from radiometer data is more difficult, requiring increased reliance on radar to assess storm structure. A dual-frequency ratio (DFR) derived from the radar’s Ku- and Ka-band frequencies provided greater insight into storm microphysics than reflectivity alone. Areas likely to contain mixed-phase precipitation (often the melting layer/bright band) generally had the highest DFR, and high-altitude regions likely to contain ice usually had the lowest DFR. The DFR of rain columns increased toward the ground, and snowbands appeared as high-DFR anomalies.

Amanda Richter↗
NASA NTRS1990

Boundary layer roll circulations during FIRE

The probable mechanism underlying the development of boundary layer roll circulations are studied using wind and temperature profiles measured by the National Center for Atmospheric Research (NCAR) Electra during the stratocumulus phase of the First ISCCP Regional Experiment (FIRE). The expected, or preferred, roll orientations, horizontal wavelengths, and propagation periods are determined by finding the minimum values of the dynamic and thermodynamic forcing parameters, which here are the eddy Reynolds number (Re) and moist Rayleigh number (Ra sub m). These minimum values depend on the height z sub T of the capping temperature inversion and on the values of the Fourier coefficients of the background height-dependent vector wind profile. As input to our nonlinear spectral model, descent and ascent runs by the Electra provide for initial estimates of the inversion height and the wind profiles. In the first phase of the investigation presented here, a mechanism is said to be a probable contributor to the development of roll circulations within the stratocumulus-topped boundary layer if the modeled roll orientation and wavelengths agree with their observed values. Preliminary results using the 14-coefficient model of Haack-Hirschberg (1988) are discussed for the 7 July 1987 Electra Mission 188-A (Flight 5). This mission was flown across a sharp cloud boundary that was within a LANDSAT/SPOT scene. The stratocumulus deck was relatively solid in the eastern part of the scene, while there was a rapid decrease in cloud cover to scattered cumulus clouds aligned in streets to the west. These cloud streets were oriented nearly parallel to the mean wind direction in the layer, which was approximately 340 degrees. The hypothesis that roll circulations occurred in both the relatively clear and the cloudy regions is investigated using as model input a descent profile obtained in the relatively clear air and an ascent profile obtained in the cloudy air. Initial results for the clear air case are that the pure inflection point mode is not possible and the pure thermal mode was oriented 35 degrees to the right of the mean wind direction. The origin of this unacceptably large discrepancy between the observed and modeled results will be investigated further and the conclusions reported at the next FIRE workshop.

Shirer, Hampton N.↗
NASA NTRSDate not supplied

CERES Monthly Gridded Single Satellite TOA and Surfaces/Clouds (SFC) data in HDF (CER_SFC_Aqua-FM4-MODIS_Edition2A)

The Monthly Gridded TOA/Surface Fluxes and Clouds (SFC) product contains a month of space and time averaged Clouds and the Earth's Radiant Energy System (CERES) data for a single scanner instrument. The SFC is also produced for combinations of scanner instruments. All instantaneous shortwave, longwave, and window fluxes at the Top-of-the-Atmosphere (TOA) and surface from the CERES SSF product for a month are sorted by 1-degree spatial regions and by the local hour of observation. The mean of the instantaneous fluxes for a given region-hour bin is determined and recorded on the SFC along with other flux statistics and scene information. These average fluxes are given for both clear-sky and total-sky scenes. The regional cloud properties are column averaged and are included on the SFC. [Location=GLOBAL] [Temporal_Coverage: Start_Date=1998-01-01; Stop_Date=2005-03-31] [Spatial_Coverage: Southernmost_Latitude=-90; Northernmost_Latitude=90; Westernmost_Longitude=-180; Easternmost_Longitude=100] [Data_Resolution: Latitude_Resolution=1 degree; Longitude_Resolution=1 degree; Horizontal_Resolution_Range=100 km - < 250 km or approximately 1 degree - < 2.5 degrees; Temporal_Resolution=1 hour; Temporal_Resolution_Range=Hourly - < Daily].

CLOUD INFRARED EMISSIVITY↗
NASA NTRSDate not supplied

CERES Clouds and Radiative Swath (CRS) data in HDF. (CER_CRS_Terra-FM2-MODIS_Edition2B)

The Clouds and Radiative Swath (CRS) product contains one hour of instantaneous Clouds and the Earth's Radiant Energy System (CERES) data for a single scanner instrument. The CRS contains all of the CERES SSF product data. For each CERES footprint on the SSF the CRS also contains vertical flux profiles evaluated at four levels in the atmosphere: the surface, 500-, 70-, and 1-hPa. The CRS fluxes and cloud parameters are adjusted for consistency with a radiative transfer model and adjusted fluxes are evaluated at the four atmospheric levels for both clear-sky and total-sky. [Location=GLOBAL] [Temporal_Coverage: Start_Date=1998-01-01; Stop_Date=2001-10-31] [Spatial_Coverage: Southernmost_Latitude=-90; Northernmost_Latitude=90; Westernmost_Longitude=-180; Easternmost_Longitude=180] [Data_Resolution: Temporal_Resolution=1 hour; Temporal_Resolution_Range=Hourly - < Daily].

SHORTWAVE UNFILTERED RADIANCE↗
NASA NTRS1982

Production and condensation of organic gases in the atmosphere of Titan

The rates and altitudes for the dissociation of atmospheric constituents on Titan are calculated for solar ultraviolet radiation, the solar wind, Saturn magnetospheric particles, the Saturn co-rotating plasma, and cosmic rays. Laboratory experiments show that a variety of simple gas phase organic molecules and more complex organic solids called tholins are produced by such irradiations of simulated Titanian atmospheres. Except for ultraviolet wavelengths longward of the methane photodissociation continuum, most dissociation events occur between about 3100 and 3600 km altitude, corresponding well to the region of EUV opacity detected by Voyager. For a wide variety of simple to moderately complex organic gases in the Titanian atmosphere, condensation occurs below the top of the main cloud deck at about 2825 km. It is proposed that such condensates, beginning with CH4 at about 2615 km, comprise the principal mass of the Titan clouds. There is a distinct tendency for the atmosphere of Titan to act as a fractional distillation device, molecules of greater complexity condensing out at higher altitudes.

Sagan, C.↗