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At least 181 records · Page 10

Cirrus Clouds Optical, Microphysical and Radiative Properties Observed During Crystal-Face Experiment: I. A Radar-Lidar Retrieval System

A method of retrieving cloud microphysical properties using combined observations from both cloud radar and lidar is introduced. This retrieval makes use of an improvement to the traditional optimal estimation retrieval method, whereby a series of corrections are applied to the state vector during the search for an iterative solution. This allows faster convergence to a solution and is less processor intensive. The method is first applied to a synthetic cloud t o demonstrate its validity, and it is shown that the retrieval reliably reproduces vertical profiles of ice water content. The retrieval method is then applied to radar and lidar observations from the CRYSTAL-FACE experiment, and vertical profiles of ice crystal diameter, number concentration, and ice water content are retrieved for a cirrus cloud layers observed one day of that experiment. The validity of the relationship between visible extinction coefficient and radar reflectivity was examined. While synthetic tests showed such a functional relationship, the measured data only partially supported such a conclusion. This is due to errors in the forward model (as explained above) as well as errors in the data sets, including possible mismatch between lidar and radar profiles or errors in the optical depth. Empirical relationships between number concentrations and mean particle diameter were also examined. The results indicate that a distinct and robust relationship exists between these retrieved quantities and it is argued that such a relationship is more than an artifact of the retrieval process offering insight into the nature of the microphysical processes taking place in cirrus.

Mitrescu, C.↗

Benefits of a 4th Ice Class in the Simulated Radar Reflectivities of Convective Systems Using a Bulk Microphysics Scheme

Numerous cloud microphysical schemes designed for cloud and mesoscale models are currently in use, ranging from simple bulk to multi-moment, multi-class to explicit bin schemes. This study details the benefits of adding a 4th ice class (hail) to an already improved 3-class ice bulk microphysics scheme developed for the Goddard Cumulus Ensemble model based on Rutledge and Hobbs (1983,1984). Besides the addition and modification of several hail processes from Lin et al. (1983), further modifications were made to the 3-ice processes, including allowing greater ice super saturation and mitigating spurious evaporationsublimation in the saturation adjustment scheme, allowing graupelhail to become snow via vapor growth and hail to become graupel via riming, and the inclusion of a rain evaporation correction and vapor diffusivity factor. The improved 3-ice snowgraupel size-mapping schemes were adjusted to be more stable at higher mixing rations and to increase the aggregation effect for snow. A snow density mapping was also added. The new scheme was applied to an intense continental squall line and a weaker, loosely-organized continental case using three different hail intercepts. Peak simulated reflectivities agree well with radar for both the intense and weaker case and were better than earlier 3-ice versions when using a moderate and large intercept for hail, respectively. Simulated reflectivity distributions versus height were also improved versus radar in both cases compared to earlier 3-ice versions. The bin-based rain evaporation correction affected the squall line case more but did not change the overall agreement in reflectivity distributions.

bulk microphysics schemes↗

Enhancing Turbulent Mixing and Microphysical Uniformity in a Tall Convection‐Cloud Chamber Through Idealized Heterogeneity of Boundaries

A large convection cloud chamber has been proposed for exploring aerosol–cloud–drizzle interactions under well‐controlled turbulent conditions. Recent theoretical and numerical studies suggest that a convection cloud chamber with two heated and two cooled sidewalls can significantly enhance the liquid water content and thus benefit drizzle initiation. However, a chamber with such a sidewall configuration develops stable stratification and extremely weak turbulence therein. In this study, we conduct large‐eddy simulations of a tall convection chamber with five different sidewall configurations consisting of alternating warm and cold patches. For each configuration, the total surface area of warm patches equals that of cold patches, resulting in the same expected cloud‐free supersaturation based on a flux budget model. Results show that changing the sidewall configuration, while keeping all other factors constant, can substantially enhance turbulent mixing and improve the uniformity of thermodynamic and cloud microphysical properties in the bulk region of the chamber. In addition, turbulence strength is positively correlated with liquid water content and negatively correlated with cloud droplet number concentration, consistent with theoretical predictions. Our results highlight the advantage of building a large cloud chamber using modular patches with individually controllable temperature and humidity to achieve well‐mixed conditions.

54 ENVIRONMENTAL SCIENCES↗

Synthesis of Aerosol Observations for Improved Understanding of Radiative Forcing

The ultimate objective of this project was to gain a better understanding of the relationship between aerosol physical and radiative properties through the integration of measurements from different approaches and platforms. Different types of information can only be gained from different approaches – for example, in situ sampling versus remote sensing – so to provide the best radiative forcing estimates they must be brought together in accurate and meaningful ways. This work involved understanding and characterizing measurement accuracy, integrating measurements from different approaches, and understanding the sensitivity of different aerosol representations from these various approaches to radiative forcing. Our progress involved the assessment of error and bias in aerosol absorption measurements made in situ and by remote sensing, assessment of new chemical composition measurements made by ARM, and determination of the sensitivity of radiative forcing to these measurement errors and the representation of absorption vertical distributions. We also examined the sensitivity of cloud condensation nuclei, cloud microphysics, and cloud radiative forcing to aerosol concentration, microphysical, chemical, and optical properties, and vertical distributions in distinct aerosol regimes.

54 ENVIRONMENTAL SCIENCES↗

Aerosol-Cloud Interactions and the Intersection of Climate Forcing and Feedback

The goal of this project has been to understand at the process level how the interaction of aerosols and cloud microphysics may alter the cloud response to climate change from the scale of turbulence to the global scale. Atmospheric aerosols (suspended particulates) have a unique role to play in the climate system. Anthropogenic aerosols may be an air pollution hazard and degrade human health. Their presence also results in the direct scattering or absorption of sunlight, with small net impacts on climate. But aerosols are also a key part of cloud formation, as the locations on which cloud droplets and ice crystals form. Understanding these Aerosol Cloud Interactions (ACI) is a critical uncertainty for climate models, including the Energy Exascale Earth System Model (E3SM), and affects how well models like E3SM can simulate the past and future. This work aims to understand cloud microphysics as well as the interaction of aerosol forcing and cloud feedback through improving our understanding of aerosol-cloud interactions (ACI) by looking at their uncertainty in critical environments at the process level. It will also contribute to the development of E3SM. Specific goals include: first, high level analysis of Perturbed Parameter Ensemble (PPE) simulations already available from the Community Earth System Model (CESM) and E3SM. Second, detailed analysis of recent changes to temperature and the role of aerosols.

54 ENVIRONMENTAL SCIENCES↗

A Climatology of Midlatitude Continental Clouds from the ARM SGP Site: Low-Level Cloud Macrophysical, Microphysical, and Radiative Properties - Part I

A record of single-layer and overcast low cloud (stratus) properties has been generated using approximately 4000 hours of data collected from January 1997 to December 2002 at the Atmospheric Radiation Measurement (ARM) Southern Great Plains Central Facility (SCF). The cloud properties include liquid-phase and liquid-dominant, mixed-phase, low cloud macrophysical, microphysical, and radiative properties including cloud-base and -top heights and temperatures, and cloud physical thickness derived from a ground-based radar and lidar pair, and rawinsonde sounding; cloud liquid water path (LWP) and content (LWC), and cloud-droplet effective radius (r(sub e)) and number concentration (N) derived from the macrophysical properties and radiometer data; and cloud optical depth (tau), effective solar transmission (gamma), and cloud/top-of-atmosphere albedos (R(sub cldy)/R(sub TOA)) derived from Eppley precision spectral pyranometer measurements. The cloud properties were analyzed in terms of their seasonal, monthly, and hourly variations. In general, more stratus clouds occur during winter and spring than in summer. Cloud-layer altitudes and physical thicknesses were higher and greater in summer than in winter with averaged physical thicknesses of 0.85 km and 0.73 km for day and night, respectively. The seasonal variations of LWP, LWC, N. tau, R(sub cldy), and R(sub TOA) basically follow the same pattern with maxima and minima during winter and summer, respectively. There is no significant variation in mean r(sub e), however, despite a summertime peak in aerosol loading, Although a considerable degree of variability exists, the 6-yr average values of LWP, LWC, r(sub e), N, tau, gamma, R(sub cldy) and R(sub TOA) are 150 gm(exp -2) (138), 0.245 gm(exp -3) (0.268), 8.7 micrometers (8.5), 213 cm(exp -3) (238), 26.8 (24.8), 0.331, 0.672, 0.563 for daytime (nighttime). A new conceptual model of midlatitude continental low clouds at the ARM SGP site has been developed from this study. The low stratus cloud amount monotonically increases from midnight to early morning (0930 LT), and remains large until around local noon, then declines until 1930 LT when it levels off for the remainder of the night. In the morning, the stratus cloud layer is low, warm, and thick with less LWC, while in the afternoon it is high, cold, and thin with more LWC. Future parts of this series will consider other cloud types and cloud radiative forcing at the ARM SCF.

Dong, Xiquan↗

Importance of ice nucleation and precipitation on climate with the Parameterization of Unified Microphysics Across Scales version 1 (PUMASv1)

Cloud microphysics is critical for weather and climate prediction. In this work, we document updates and corrections to the cloud microphysical scheme used in the Community Earth System Model (CESM) and other models. These updates include a new nomenclature for the scheme, now called Parameterization of Unified Microphysics Across Scales (PUMAS), and the ability to run the scheme on graphics processing units (GPUs). The main science changes include refactoring an ice number limiter and associated changes to ice nucleation, adding vapor deposition onto snow, and introducing an implicit numerical treatment for sedimentation. We also detail the improvements in computational performance that can be achieved with GPU acceleration. We then show the impact of these scheme changes on the (a) mean state climate, (b) cloud feedback response to warming, and (c) aerosol forcing. We find that corrections are needed to the immersion freezing parameterization and that ice nucleation has important impacts on climate. We also find that the revised scheme produces less cloud liquid and ice but that this can be adjusted by changing the loss process for cloud liquid (autoconversion). Furthermore, there are few discernible effects of the PUMAS changes on cloud feedbacks but some reductions in the magnitude of aerosol–cloud interactions (ACIs). Small cloud feedback changes appear to be related to the implicit sedimentation scheme, with a number of factors affecting ACIs.

54 ENVIRONMENTAL SCIENCES↗

Assessing the CAM5 Physics Suite in the WRF-Chem Model: Implementation, Resolution Sensitivity, and a First Evaluation for a Regional Case Study

A suite of physical parameterizations (deep and shallow convection, turbulent boundary layer, aerosols, cloud microphysics, and cloud fraction) from the global climate model Community Atmosphere Model version 5.1 (CAM5) has been implemented in the regional model Weather Research and Forecasting with chemistry (WRF-Chem). A downscaling modeling framework with consistent physics has also been established in which both global and regional simulations use the same emissions and surface fluxes. The WRF-Chem model with the CAM5 physics suite is run at multiple horizontal resolutions over a domain encompassing the northern Pacific Ocean, northeast Asia, and northwest North America for April 2008 when the ARCTAS, ARCPAC, and ISDAC field campaigns took place. These simulations are evaluated against field campaign measurements, satellite retrievals, and ground-based observations, and are compared with simulations that use a set of common WRF-Chem Parameterizations. This manuscript describes the implementation of the CAM5 physics suite in WRF-Chem provides an overview of the modeling framework and an initial evaluation of the simulated meteorology, clouds, and aerosols, and quantifies the resolution dependence of the cloud and aerosol parameterizations. We demonstrate that some of the CAM5 biases, such as high estimates of cloud susceptibility to aerosols and the underestimation of aerosol concentrations in the Arctic, can be reduced simply by increasing horizontal resolution. We also show that the CAM5 physics suite performs similarly to a set of parameterizations commonly used in WRF-Chem, but produces higher ice and liquid water condensate amounts and near-surface black carbon concentration. Further evaluations that use other mesoscale model parameterizations and perform other case studies are needed to infer whether one parameterization consistently produces results more consistent with observations.

CAM5 physics suite↗

Solar activity, the QBO, and tropospheric responses

The suggestion that galactic cosmic rays (GCR) as modulated by the solar wind are the carriers of the component of solar variability that affects weather and climate has been discussed in the literature for 30 years, and there is now a considerable body of evidence that supports it. Variations of GCR occur with the 11 year solar cycle, matching the time scale of recent results for atmospheric variations, as modulated by the quasibiennial oscillation of equatorial stratospheric winds (the QBO). Variations in GCR occur on the time scale of centuries with a well defined peak in the coldest decade of the little ice age. New evidence is presented on the meteorological responses to GCR variations on the time scale of a few days. These responses include changes in the vertical temperature profile in the troposphere and lower stratosphere in the two days following solar flare related high speed plasma streams and associated GCR decreases, and in decreases in Vorticity Area Index (VAI) following Forbush decreases of GCR. The occurrence of correlations of GCR and meteorological responses on all three time scales strengthens the hypothesis of GCR as carriers of solar variability to the lower atmosphere. Both short and long term tropospheric responses are understandable as changes in the intensity of cyclonic storms initiated by mechanisms involving cloud microphysical and cloud electrification processes, due to changes in local ion production from changes in GCR fluxes and other high energy particles in the MeV to low GeV range. The nature of these mechanisms remains undetermined. Possible stratospheric wind (particularly QBO) effects on the transport of HNO3 and other constituents incorporated in cluster ions and possible condensation and freezing nuclei are considered as relevant to the long term variations.

Tinsley, Brian A.↗

Estimated accuracy of ground-based liquid water measurements during FIRE

Since on goal of the First ISCCP Regional Experiment (FIRE) project is to improve our understanding of the relationships between cloud microphysics and cloud reflectivity, it is important that the accuracy of remote liquid measurements by microwave radiometry be thoroughly understood. The question is particularly relevant since the uncertainty in the absolute value of the radiometric liquid measurement is greatest at low liquid water contents (less than 0.1 mm). However it should be stressed that although uncertainty exists in the absolute value of liquid, it is well known that the observed radiometric signal is proportional to the amount of liquid in the antenna beam. As a result, changes in amounts of liquid are known to greater accuracy than the absolute value, which may contain a bias. Here, an assessment of the liquid measurement accuracy attained at San Nicolas Island (SNI) is presented. The vapor and liquid water data shown were computed from the radiometric brightness temperatures using statistical retrieval algorithms. The retrieval coefficients were derived from the 69 soundings made by Colorado State University during the SNI observations. Sources of error in the vapor and liquid measurements include cross-talk in the retrieval algorithms (not a factor at low liquid contents), uncertainties in the brightness temperature measurement, and uncertainties in the vapor and liquid attenuation coefficients. The relative importance of these errors is discussed. For the retrieval of path-integrated liquid water, the greatest uncertainty is caused by the temperature dependence of the absorption at microwave frequencies. As a result, the accuracy of statistical retrieval of liquid depends to large measure upon how representative the a priori radiosonde data are of the conditions prevailing during the measurements. The microwave radiometer measurements at SNI were supplemented by an infrared (IR) radiometer modified for measurement of cloud-base temperature. Thus, the IR system provides the means to incorporate continuous measurements of the liquid temperature into the retrieval process.

Snider, Jack B.↗

4-D Cloud Water Content Fields Derived from Operational Satellite Data

In order to improve operational safety and efficiency, the transportation industry, including aviation, has an urgent need for accurate diagnoses and predictions of clouds and associated weather conditions. Adverse weather accounts for 70% of all air traffic delays within the U.S. National Airspace System. The Federal Aviation Administration has determined that as much as two thirds of weather-related delays are potentially avoidable with better weather information and roughly 20% of all aviation accidents are weather related. Thus, it is recognized that an important factor in meeting the goals of the Next Generation Transportation System (NexGen) vision is the improved integration of weather information. The concept of a 4-D weather cube is being developed to address that need by integrating observed and forecasted weather information into a shared 4-D database, providing an integrated and nationally consistent weather picture for a variety of users and to support operational decision support systems. Weather analyses and forecasts derived using Numerical Weather Prediction (NWP) models are a critical tool that forecasters rely on for guidance and also an important element in current and future decision support systems. For example, the Rapid Update Cycle (RUC) and the recently implemented Rapid Refresh (RR) Weather Research and Forecast (WRF) models provide high frequency forecasts and are key elements of the FAA Aviation Weather Research Program. Because clouds play a crucial role in the dynamics and thermodynamics of the atmosphere, they must be adequately accounted for in NWP models. The RUC, for example, cycles at full resolution five cloud microphysical species (cloud water, cloud ice, rain, snow, and graupel) and has the capability of updating these fields from observations. In order to improve the models initial state and subsequent forecasts, cloud top altitude (or temperature, T(sub c)) derived from operational satellite data, surface observations of cloud base altitude, radar reflectivity, and lightning data are used to help build and remove clouds in the models assimilation system. Despite this advance and the many recent advances made in our understanding of cloud physical processes and radiative effects, many problems remain in adequately representing clouds in models. While the assimilation of cloud top information derived from operational satellite data has merit, other information is available that has not yet been exploited. For example, the vertically integrated cloud water content (CWC) or cloud water path (CWP) and cloud geometric thickness (delta Z) are standard products being derived routinely from operational satellite data. These and other cloud products have been validated under a variety of conditions. Since the uncertainties have generally been found to be less than those found in model analyses and forecasts, the satellite products should be suitable for data assimilation, provided an appropriate strategy can be developed that links the satellite-derived cloud parameters with cloud parameters specified in the model. In this paper, we briefly outline such a strategy and describe a methodology to retrieve cloud water content profiles from operational satellite data. Initial results and future plans are presented. It is expected that the direct assimilation of this new product will provide the most accurate depiction of the vertical distribution of cloud water ever produced at the high spatial and temporal resolution needed for short term weather analyses and forecasts.

Smith, William L., Jr.↗

Biogenic Aerosol - Effect on Clouds and Climate (BAECC-ERI). Extended Radiosonde Intensive Operational Period Final Campaign Summary

Large-scale properties of clouds such as lifetime, optical thickness, and precipitation are all dependent on small-scale cloud microphysical processes. Such processes determine when droplets will grow or shrink, their size, and the number of cloud droplets. Although our understanding of cloud microphysics has vastly improved over the past several decades with the development of remote sensing methods such as lidar and radar, there remain a number of processes that are not well understood, such as the effect of electrical charge on cloud microphysics. To understand the various processes and feedback mechanisms, high-vertical–resolution observations are required. Radiosondes provide an ideal platform for providing routine vertical profiles of in situ measurements at any location (with a vertical resolution of a few meters). Modified meteorological radiosondes have been extensively developed at the University of Reading for measuring cloud properties, to allow measurements beyond the traditional thermodynamic quantities (pressure, temperature and relative humidity) to be obtained cost-effectively. This project aims to investigate a number of cloud processes in which in situ cloud observations from these modified radiosondes can provide information either complementary to or not obtainable by lidar/radar systems. During two intensive operational periods (IOPs) in May and August 2014 during deployment to Hyytiälä, Finland, the Atmospheric Radiation Measurement (ARM) Climate Research Facility’s Second ARM Mobile Facility (AMF2) launched a total of 24 instrumented radiosondes through a number of different cloud types ranging from low-level stratiform cloud to cumulonimbus. Twelve balloon flights of an accelerometer turbulence sensor were made, which detected significant turbulence on eleven of these flights. Most of the turbulent episodes encountered were due to convective processes, but several were associated with the transition from troposphere to stratosphere at the tropopause. Similarities in the location of turbulent layers were generally found between the balloon turbulence sensor and the Ka-band radar, but with discrepancies between the orders of magnitude of turbulence detected. The reason for these discrepancies is the subject of future work.

54 ENVIRONMENTAL SCIENCES↗

Peering into cloud physics using ultra-fine resolution radar and lidar systems

Cloud microphysical processes, such as droplet activation, condensational growth, and collisional growth, play a central role in the evolution of clouds and precipitation. Accurate representations of these processes in numerical models are challenging partially due to incomplete understanding of them at the process-level arising from limited systematic observations. Most surface-based active remote sensors, including today’s operational cloud radars and lidars, have a resolution on the order of tens of meters. This resolution is insufficient to resolve cloud microphysical processes that manifest at finer (meter and sub-meter) scales. A new set of ultra-high-resolution ground-based radar and lidar systems have been developed to address this observational gap. The newly developed 94-GHz cloud radar has a range resolution down to 2.8 m, or a factor of 10 finer than typical radars, using a large bandwidth and quadratic phase coding techniques. The lidar has a range resolution down to 10 cm, or a factor of 100 finer than typical lidars, using a time-gated time-correlated single photon counting technique. Such high-resolution observations were previously only achievable through in situ aircraft measurements. Even then, aircraft measurements do not permit continuous long-term cloud observation as is possible with ground-based remote sensing instruments. In this study, the first-light cloud observations from the new radar and lidar systems are shown to reveal detailed cloud structures that conventional sensors could only perceive in a bulk sense, thus providing new avenues to investigate cloud microphysical processes and their impact on weather and climate.

54 ENVIRONMENTAL SCIENCES↗

Understanding ice cloud-precipitation properties of three modes of mesoscale convective systems during PECAN

This study analyzes the precipitation and ice cloud microphysical features of three common modes of linear mesoscale convective systems (MCSs) during the Plains Elevated Convection at Night (PECAN) campaign. Three cases, one for each linear MCS archetype (trailing stratiform (TS), leading stratiform (LS), and parallel stratiform (PS) precipitation), are selected. We focus primarily on analyzing ice cloud microphysical properties and precipitation rates over the classified convective core (CC) and stratiform rain (SR) regions, as well as the two stratiform regions that developed behind (SR1) and ahead (SR2) of the convective line relative to the storm motion. In the three selected cases, the ice water path (IWP) and precipitation rate (PR) have strong correlations in the CC, but not in the SR. In terms of the temporal evolution of the mean IWPs and PRs, both CC and SR IWPs, as well as CC PRs, reach peaks quickly, but take a longer time to dissipate than the increase period. For all three cases, both SR1 and SR2 IWPs are 20-70% of their corresponding CC values in both the LS and PS cases, and up to 95% for the TS case, while all of their PRs are only 7-25% of their CC values. These values suggest that the SR PRs may not only depend on IWPs, but also that the microphysical properties of ice particles such as habit and size distribution may play an important role. Utilizing cloud resolving simulations of these systems may provide better understanding of the physical meanings behind the results in the future.

Cui, Wenjun↗

Dual Microwave Radiometer Experiment Field Campaign Report

Passive microwave radiometers (MWRs) are the most commonly used and accurate instruments the U.S. Department of Energy (DOE) Atmospheric Radiation Measurement (ARM) Research Facility has to retrieve cloud liquid water path (LWP). The MWR measurements (microwave radiances or brightness temperatures) are often used to derive LWP using climatological constraints, but are frequently also combined with measurements from radar and other instruments for cloud microphysical retrievals. Nominally this latter approach improves the retrieval of LWP and other cloud microphysical quantities (such as effective radius or number concentration), but this also means that when MWR data are poor, other cloud microphysical quantities are also negatively affected. Unfortunately, current MWR data is often contaminated by water on the MWR radome. This water makes a substantial contribution to the measured radiance and typically results in retrievals of cloud liquid water and column water vapor that are biased high. While it is obvious when the contamination by standing water is large (and retrieval biases are large), much of the time it is difficult to know with confidence that there is no contamination. At present there is no attempt to estimate or correct for this source of error, and identification of problems is largely left to users. Typically users are advised to simply throw out all data when the MWR “wet-window” resistance-based sensor indicates water is present, but this sensor is adjusted by hand and is known to be temperamental. In order to address this problem, a pair of ARM microwave radiometers was deployed to the University of Washington (UW) in Seattle, Washington, USA. The radiometers were operated such that one radiometer was scanned under a cover that (nominally) prevents this radiometer radome from gathering water and permits measurements away from zenith; while the other radiometer is operated normally – open or uncovered - with the radome exposed to the sky. The idea is that (1) the covered radiometer data can provide LWP (and water vapor) along the off-zenith slant path and (2) the two sets of measurements can be compared to identify when wet-radome contamination is occurring.

47 OTHER INSTRUMENTATION↗

The influence of multiple groups of biological ice nucleating particles on microphysical properties of mixed-phase clouds observed during MC3E

Abstract. A new empirical parameterization (EP) for multiple groups of primary biological aerosol particles (PBAPs) is implemented in the aerosol–cloud model (AC) to investigate their roles as ice nucleating particles (INPs). The EP describes the heterogeneous ice nucleation by (1) fungal spores, (2) bacteria, (3) pollen, (4) detritus of plants, animals, and viruses, and (5) algae. Each group includes fragments from the originally emitted particles. A high-resolution simulation of a midlatitude mesoscale squall line by AC is validated against airborne and ground observations. Sensitivity tests are carried out by varying the initial vertical profiles of the loadings of individual PBAP groups. The resulting changes in warm and ice cloud microphysical parameters are investigated. The changes in warm microphysical parameters, including liquid water content and cloud droplet number concentration, are minimal (<10 %). Overall, PBAPs have little effect on the ice number concentration (<6 %) in the convective region. In the stratiform region, increasing the initial PBAP loadings by a factor of 1000 resulted in less than 40 % change in ice number concentrations. The total ice concentration is mostly controlled by various mechanisms of secondary ice production (SIP). However, when SIP is intentionally shut down in sensitivity tests, increasing the PBAP loading by a factor of 100 has an effect of less than 3 % on the ice phase. Further sensitivity tests revealed that PBAPs have little effect on surface precipitation and on the shortwave and longwave flux (<4 %) for a 100-fold perturbation in PBAPs.

54 ENVIRONMENTAL SCIENCES↗

An Improved Bulk Microphysical Scheme for Studying Precipitation Processes: Comparisons with Other Schemes

Cloud microphysical processes play an important role in non-hydrostatic high-resolution simulations. Over the past decade both research and operational numerical weather prediction models have started using more complex cloud microphysical schemes that were originally developed for high-resolution cloud-resolving models. An improved bulk microphysical parameterization (adopted from the Goddard microphysics schemes) has recently implemented into the Weather Research and Forecasting (WRF) model. This bulk microphysical scheme has three different options --- 2ICE (cloud ice & snow), 3ICE-graupel (cloud ice, snow & graupel) and 3ICE-hail (cloud ice, snow & hail). High-resolution model simulations are conducted to examine the impact of microphysical schemes on two different weather events (a midlatitude linear convective system and an Atlantic hurricane). In addition, this bulk microphysical parameterization is compared with WIRF's three other bulk microphysical schemes.

Tao, W. K.↗

Aircraft-Measured Indirect Cloud Effects from Biomass Burning Smoke in the Arctic and Subarctic

The incidence of wildfires in the Arctic and subarctic is increasing; in boreal North America, for example, the burned area is expected to increase by 200-300% over the next 50-100 years, which previous studies suggest could have a large effect on cloud microphysics, lifetime, albedo, and precipitation. However, the interactions between smoke particles and clouds remain poorly quantified due to confounding meteorological influences and remote sensing limitations. Here, we use data from several aircraft campaigns in the Arctic and subarctic to explore cloud microphysics in liquid-phase clouds influenced by biomass burning. Median cloud droplet radii in smoky clouds were approx. 40- 60% smaller than in background clouds. Based on the relationship between cloud droplet number (N(liq)/ and various biomass burning tracers (BBt/ across the multi-campaign data set, we calculated the magnitude of subarctic and Arctic smoke aerosol-cloud interactions (ACIs, where ACI = (1/3) x dln(N(liq))/dln(BBt)) to be approx. 0.16 out of a maximum possible value of 0.33 that would be obtained if all aerosols were to nucleate cloud droplets. Interestingly, in a separate subarctic case study with low liquid water content (0.02 gm/cu m and very high aerosol concentrations (2000- 3000/ cu cm in the most polluted clouds, the estimated ACI value was only 0.05. In this case, competition for water vapor by the high concentration of cloud condensation nuclei (CCN) strongly limited the formation of droplets and reduced the cloud albedo effect, which highlights the importance of cloud feedbacks across scales. Using our calculated ACI values, we estimate that the smoke-driven cloud albedo effect may decrease local summertime short-wave radiative flux by between 2 and 4 W/sq m or more under some low and homogeneous cloud cover conditions in the subarctic, although the changes should be smaller in high surface albedo regions of the Arctic.We lastly explore evidence suggesting that numerous northern-latitude background Aitken particles can interact with combustion particles, perhaps impacting their properties as cloud condensation and ice nuclei.

cloud microphysics↗