The CHIMAERA system for retrievals of cloud top, optical and microphysical properties from imaging sensors
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Galina (Gala) Wind↗
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Results for “cloud microphysical properties”
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Impact of a New Cloud Microphysics Parameterization on the Simulations of Mesoscale Convective Systems in E3SM
Abstract Mesoscale convective systems (MCSs) are one of the most climatically significant forms of convection because of their large role in water and energy cycles. The mesoscale features associated with MCS are difficult to represent in climate models because the relevant dynamics and physics are absent or poorly represented with coarse model resolution (∼100 km). Using a regionally refined model (RRM) with 0.25° grid spacing embedded in the Energy Exascale Earth System Model (E3SM), we explore the impact of cloud microphysics parameterizations on the simulation of precipitation, particularly MCS precipitation over the contiguous United States. The Predicted Particle Properties (P3) cloud microphysics scheme has been modified and implemented into E3SM to overcome the limitations of the default Morrison and Gettelman (MG2) scheme in which rimed precipitating ice particles (graupel/hail) are absent and frozen particles are artificially partitioned into cloud ice and snow. We show that P3 improves the simulation of precipitation statistics including frequency distribution compared with MG2 with a limited effect on the diurnal cycle. P3 predicts higher hourly rain rates, resulting in 20% more MCSs and a higher total MCS precipitation (4.4%) compared to MG2, agreeing better with observations. The improvements with P3 mainly result from improved representations of ice microphysics, which not only produces higher rain rates through melting but also leads to a stronger large‐scale ascending motion by releasing more latent heating. This study suggests that improving microphysics parameterization is important for simulating MCS precipitation as future climate model resolutions continue to increase.
54 ENVIRONMENTAL SCIENCES↗
Global Multispectral Cloud Retrievals from MODIS
The Moderate Resolution Imaging Spectroradiometer (MODIS) was developed by NASA and launched onboard the Terra spacecraft on December 18,1999 and Aqua spacecraft on May 4,2002. It achieved its final orbit and began Earth observations on February 24, 2000 for Terra and June 24, 2002 for Aqua. A comprehensive set of remote sensing algorithms for cloud masking and the retrieval of cloud physical and optical properties has been developed by members of the MODIS atmosphere science team. The archived products from these algorithms have applications in climate change studies, climate modeling, numerical weather prediction, as well as fundamental atmospheric research. In addition to an extensive cloud mask, products include cloud-top properties (temperature, pressure, effective emissivity), cloud thermodynamic phase, cloud optical and microphysical parameters (optical thickness, effective particle radius, water path), as well as derived statistics. We will describe the various cloud properties being analyzed on a global basis from both Terra and Aqua, and will show characteristics of cloud optical and microphysical properties as a function of latitude for land and ocean separately, and contrast the statistical properties of similar cloud types in various parts of the world.
King, Michael D.↗
Global Multispectral Cloud Retrievals from MODIS
The Moderate Resolution Imaging Spectroradiometer (MODIS) was developed by NASA and launched onboard the Terra spacecraft on December 18,1999 and Aqua spacecraft on May 4,2002. It achieved its final orbit and began Earth observations on February 24, 2000 for Terra and June 24, 2002 for Aqua. A comprehensive set of remote sensing algorithms for cloud masking and the retrieval of cloud physical and optical properties has been developed by members of the MODIS atmosphere science team. The archived products from these algorithms have applications in climate change studies, climate modeling, numerical weather prediction, as well as fundamental atmospheric research. In addition to an extensive cloud mask, products include cloud-top properties (temperature, pressure, effective emissivity), cloud thermodynamic phase, cloud optical and microphysical parameters (optical thickness, effective particle radius, water path), as well as derived statistics. We will describe the various cloud properties being analyzed on a global basis from both Terra and Aqua, and will show characteristics of cloud optical and microphysical properties as a function of latitude for land and ocean separately, and contrast the statistical properties of similar cloud types in various parts of the world.
King, Michael D.↗
Summertime Coincident Observations of Ice Water Path in the Visible/Near-IR, Radar, and Microwave Frequencies
Accurate representation of the physical and radiative properties of clouds in climate models continues to be a challenge. At present, both remote sensing observations and modeling of microphysical properties of clouds rely heavily on parameterizations or assumptions on particle size distribution (PSD) and cloud phase. In this study, we compare Ice Water Path (IWP), an important physical and radiative property that provides the amount of ice present in a cloud column, using measurements obtained via three different retrieval strategies. The datasets we use in this study include Visible/Near-IR IWP from the Moderate Resolution Imaging Spectroradiometer (MODIS) instrument flying aboard the Aqua satellite, Radar-only IWP from the CloudSat instrument operating at 94 GHz, and NOAA/NESDIS operational IWP from the 89 and 157 GHz channels of the Microwave Humidity Sounder (MHS) instrument flying aboard the NOAA-18 satellite. In the Visible/Near-IR, IWP is derived from observations of optical thickness and effective radius. CloudSat IWP is determined from measurements of cloud backscatter and assumed PSD. MHS IWP retrievals depend on scattering measurements at two different, non-water absorbing channels, 89 and 157 GHz. In order to compare IWP obtained from these different techniques and collected at different vertical and horizontal resolutions, we examine summertime cases in the tropics (30S - 30N) when all 3 satellites are within 4 minutes of each other (approximately 1500 km). All measurements are then gridded to a common 15 km x 15 km box determined by MHS. In a grid box comparison, we find CloudSat to report the highest IWP followed by MODIS, followed by MHS. In a statistical comparison, probability density distributions show MHS with the highest frequencies at IWP of 100-1000 g/m(exp 2) and CloudSat with the longest tail reporting IWP of several thousands g/m(exp 2). For IWP greater than 30 g/m(exp 2), MODIS is consistently higher than CloudSat, and it is higher at the lower IWPs but lower at the higher IWPs that overlap with MHS. Some of these differences can be attributed to the limitations of the measuring techniques themselves, but some can result from the assumptions made in the algorithms that generate the IWP product. We investigate this issue by creating categories based on various conditions such as cloud type, precipitation presence, underlying liquid water content, and surface type (land vs. ocean) and by comparing the performance of the IWP products under each condition.
Pittman, Jasna V.↗
Survey of microphysical properties of marine boundary-layer clouds in the Western North Atlantic
Oceanic low level clouds strongly affect the atmospheric radiation budget. Uncertainties in their microphysical properties and cover currently limit the accuracy of climate predictions. Further, studies quantifying the relative importance of aerosol and dynamics on cloud properties in specific meteorological regimes are poorly constrained by observations in the Western North Atlantic boundary layer. Low level clouds were measured during the Aerosol Cloud meTereology Interactions oVer the western ATlantic Experiment (ACTIVATE) campaign in winter and summer 2020. The two NASA LaRC research aircraft HU-25 Falcon and UC-12 B-200 King Air conducted 35 simultaneous flights to investigate aerosol-cloud interactions of maritime clouds and their impact on radiation. Number concentration, liquid water content, ice water content, and particle size distribution in the size range of 3 µm to 1460 µm in diameter were measured with the fast forward scattering cloud probe (FCDP) and 2-dimensional optical array imaging probe (2D-S) onboard the Falcon. Here, we present an overview of late winter (February-March) and late summer (August-September) oceanic cloud properties in the region 65°W to 80°W and 30°N to 40°N. We compare cloud properties in these two seasons and investigate their dependence on meteorological parameters and aerosol abundance. In a case study, we present cloud observations in a cold air outbreak event on 1 March 2020 with a specific focus on mixed-phase clouds.
microphysical properties↗
Partition between supercooled liquid droplets and ice crystals in mixed-phase clouds based on airborne in situ observations
Abstract. The onset of ice nucleation in mixed-phase clouds determines the lifetime and microphysical properties of ice clouds. In this work, we develop a novel method that differentiates between various phases of mixed-phase clouds, such as clouds dominated by pure liquid or pure ice segments, compared with those having ice crystals surrounded by supercooled liquid water droplets or vice versa. Using this method, we examine the relationship between the macrophysical and microphysical properties of Southern Ocean mixed-phase clouds at −40 to 0 °C (e.g. stratiform and cumuliform clouds) based on the in situ aircraft-based observations during the US National Science Foundation Southern Ocean Clouds, Radiation, Aerosol Transport Experimental Study (SOCRATES) flight campaign. The results show that the exchange between supercooled liquid water and ice crystals from a macrophysical perspective, represented by the increasing spatial ratio of regions containing ice crystals relative to the total in-cloud region (defined as ice spatial ratio), is positively correlated with the phase exchange from a microphysical perspective, represented by the increasing ice water content (IWC), decreasing liquid water content (LWC), increasing ice mass fraction, and increasing ice particle number fraction (IPNF). The mass exchange between liquid and ice becomes more significant during phase 3 when pure ice cloud regions (ICRs) start to appear. Occurrence frequencies of cloud thermodynamic phases show a significant phase change from liquid to ice at a similar temperature (i.e. −17.5 °C) among three types of definitions of mixed-phase clouds based on ice spatial ratio, ice mass fraction, or IPNF. Aerosol indirect effects are quantified for different phases using number concentrations of aerosols greater than 100 or 500 nm (N>100 and N>500, respectively). N>500 shows stronger positive correlations with ice spatial ratios compared with N>100. This result indicates that larger aerosols potentially contain ice-nucleating particles (INPs), which facilitate the formation of ice crystals in mixed-phase clouds. The impact of N>500 is also more significant in phase 2 when ice crystals just start to appear in the mixed phase compared with phase 3 when pure ICRs have formed, possibly due to the competing aerosol indirect effects on primary and secondary ice production in phase 3. The thermodynamic and dynamic conditions are quantified for each phase. The results show stronger in-cloud turbulence and higher updraughts in phases 2 and 3 when liquid and ice coexist compared with pure liquid or ice (phases 1 and 4, respectively). The highest updraughts and turbulence are seen in phase 3 when supercooled liquid droplets are surrounded by ice crystals. These results indicate both updraughts and turbulence support the maintenance of supercooled liquid water amongst ice crystals. Overall, these results illustrate the varying effects of aerosols, thermodynamics, and dynamics through various stages of mixed-phase cloud evolution based on this new method that categorizes cloud phases.
54 ENVIRONMENTAL SCIENCES↗
Look-up Table for Lidar and Polarimeter Liquid Water Cloud Studies
- Combined lidar and polarimeter retrievals of aerosol, cloud and ocean microphysical properties involve single scattering cloud calculations that are time consuming. - We create a look-up table to speed up calculations for water droplets in the atmosphere. The gained increase in computational efficiency is up to 10^(4). - In our new Lorenz-Mie look-up table we tabulate the light scattering by an ensemble of homogeneous isotropic spheres at wavelengths starting from 0.35 µm. - The look-up table covers liquid water cloud particles with radii in the range of 0.001—500 µm. - The covered complex refractive indices range from 1.25 to 1.36 for the real part and from 0 to 0.001 for the imaginary part. - Using look-up table, we can precisely compute inherent optical properties for the particle size distributions ranging up to 100 µm for the effective radius and up to 0.6 for the effective variance. - We test wavelengths from 0.35 to 2.3 µm and find that the P12 element of the normalized scattering matrix is precise to within 1% for 96.7% of cases; the absorption and backscatter coefficients, and lidar ratio are precise to within 1% for 99% of cases; the P11 , P33 and P34 elements of the normalized scattering matrix, the asymmetry parameter, the extinction and scattering coefficients are precise to within 1% for all cases. - We provide an example of using the look-up table with in situ measurements to determine agreement with remote sensing. - The look-up table along with examples of its use soon will be freely available at https://science.larc.nasa.gov/polarimetry
Eduard Chemyakin↗
Correlations among the Optical Properties of Cirrus-Cloud Particles: Microphysical Interpretation
Cirrus measurements obtained with a ground-based polarization Raman lidar at 67.9 deg N in January 1997 reveal a strong positive correlation between the particle optical properties, specifically depolarization ratio delta(sub par) and extinction- to-backscatter (lidar) ratio S, for delta(sub par) less than approximately 40%, and an anti-correlation for delta(sub par) greater than approximately 40%. Over the length of the measurements the particle properties vary systematically. Initially, delta (sub par) approximately equals 60% and S approximately equals 10sr are observed. Then, with decreasing delta(sub par), S first increases to approximately 27sr (delta(sub par) approximately equals 40%) before decreasing to values around 10sr again (delta(sub par) approximately equals 20%). The analysis of lidar humidity and radiosonde temperature data shows that the measured optical properties stem from scattering by dry solid ice particles, while scattering by supercooled droplets, or by wetted or subliming ice particles can be excluded. For the microphysical interpretation of the lidar measurements, ray-tracing computations of particle scattering properties have been used. The comparison with the theoretical data suggests that the observed cirrus data can be interpreted in terms of size, shape, and, under the assumption that the lidar measurements of consecutive cloud segments can be mapped on the temporal development of a single cloud parcel moving along its trajectory, growth of the cirrus particles: Near the cloud top in the early stage of cirrus development, light scattering by nearly isometric particles that have the optical characteristics of hexagonal columns (short, column-like particles) is dominant. Over time the ice particles grow, and as the cloud base height extends to lower altitudes characterized by warmer temperatures they become morphologically diverse. For large S and depolarization values of approximately 40%, the scattering contributions of column- and plate-like particles are roughly the same. In the lower ranges of the cirrus clouds, light scattering is predominantly by plate-like ice particles. This interpretation assumes random orientation of the cirrus particles. Simulations with a simple model suggest, however, that the positive correlation between S and delta(sub par) which is observed for depolarization ratios less than 40% mainly at low cloud altitudes, can be alternatively explained by horizontal alignment of a fraction of the cirrus particle population.
Reichardt, J.↗
Reducing Aerosol Forcing Uncertainty by Combining Models With Satellite and Within-The-Atmosphere Observations: A Three-Way Street
Aerosol forcing uncertainty represents the largest climate forcing uncertainty overall. Its magnitude has remained virtually undiminished over the past 20 years despite considerable advances in understanding most of the key contributing elements. Recent work has produced modest increases only in the confidence of the uncertainty estimate itself. This review summarizes the contributions toward reducing the uncertainty in the aerosol forcing of climate made by satellite observations, measurements taken within the atmosphere, as well as modeling and data assimilation. We adopt a more measurement-oriented perspective than most reviews of the subject in assessing the strengths and limitations of each; gaps and possible ways to fill them are considered. Currently planned programs supporting advanced, global-scale satellite and surface-based aerosol, cloud, and precursor gas observations, climate modeling, and intensive field campaigns aimed at characterizing the underlying physical and chemical processes involved, are all essential. But in addition, new efforts are needed: (a) to obtain systematic aircraft in situ measurements capturing the multi-variate probability distribution functions of particle optical, microphysical, and chemical properties (and associated uncertainty estimates), as well as co-variability with meteorology, for the major aerosol airmass types; (b) to conceive, develop, and implement a suborbital (aircraft plus surface-based) program aimed at systematically quantifying the cloud-scale microphysics, cloud optical properties, and cloud-related vertical velocities associated with aerosol-cloud interactions; and (c) to focus much more research on integrating the unique contributions of satellite observations, suborbital measurements, and modeling, to reduce the persistent uncertainty in aerosol climate forcing.
aerosol climate forcing↗
Understanding Differences Between Co-Incident CloudSat, Aqua/MODIS and NOAA18 MHS Ice water Path Retrievals Over the Tropical Oceans
Accurate measurement of the physical and radiative properties of clouds and their representation in climate models continues to be a challe nge. Model parameterizations are still subject to a large number of t unable parameters; furthermore, accurate and representative in situ o bservations are very sparse, and satellite observations historically have significant quantitative uncertainties, particularly with respect to particle size distribution (PSD) and cloud phase. Ice Water Path (IWP), or amount of ice present in a cloud column, is an important cl oud property to accurately quantify, because it is an integral measur e of the microphysical properties of clouds and the cloud feedback pr ocesses in the climate system. This paper investigates near co-incident retrievals of IWP over tropical oceans using three diverse measurem ent systems: radar from CloudSat, Vis/IR from Aqua/MODIS, and microwa ve from NOAA-18IMHS. CloudSat 94 GHz radar measurements provide high resolution vertical and along-orbit structure of cloud reflectivity a nd enable IWP (and IWC) retrievals. Overlapping MODIS measurements of cloud optical thickness and phase allow estimates of IWP when cloud tops are identified as being ice. Periodically, NOAA18 becomes co-inci dent in space I time to enable comparison of A-Train measurements to IWP inferred from the 157 and 89 GHz channel radiances. This latter m easurement is effective only for thick convective anvil systems. We s tratify these co-incident data (less than 4 minutes separation) into cirrus only, cirrus overlying liquid water clouds, and precipitating d eep convective clouds. Substantial biases in IWP and ice effective ra dius are found. Systematic differences in these retrievals are consid ered in light of the uncertainties in a priori assumptions ofPSDs, sp ectral sensitivity and algorithm strategies, which have a direct impact on the IWP product.
Pittman, Jasna↗
Observations of multi-layered clouds using K-band radar
Rudimentary ground-based K-band radars were once used by the U.S. Air Force to monitor clouds over air bases. The NOAA wave Propagation Laboratory has developed a significantly advanced dual-polarization Doppler K-band system that provides remarkably detailed visualizations of the structure and kinematics of nonprecipitating and weakly precipitating clouds. Unlike lidar and infrared radiometer systems, K-band radar can penetrate liquid water cloud layers and obtain measurements through moderate rainfall and heavy snowfall to reveal intricate cloud features including multiple layers of cloud. This is accomplished at less cost than would be possible with traditional longer wavelength weather radars. The radar's capabilities have been demonstrated in several recent cloud research field projects. In combination with measurements by other remote sensors, the radar can help detect aircraft icing hazards and infer microphysical properties of clouds. An automated, unattended version of the radar could provide a continuous, detailed depiction of the cloud environment in the vicinity of airports.
Martner, Brooks E.↗
Derivation of Cumulus Cloud Dimensions and Shape from the Airborne Measurements by the Research Scanning Polarimeter
The Research Scanning Polarimeter (RSP) is an airborne instrument, whose measurements have been extensively used for retrievals of microphysical properties of clouds. In this study we show that for cumulus clouds the information content of the RSP data can be extended by adding the macroscopic parameters of the cloud, such as its geometric shape, dimensions, and height above the ground. This extension is possible by virtue of the high angular resolution and high frequency of the RSP measurements, which allow for geometric constraint of the cloud's 2D cross section between a number of tangent lines of view. The retrieval method is tested on realistic 3D radiative transfer simulations and applied to actual RSP data.
Remote sensing↗
Progress on the National Solar Radiation Data Base (NSRDB): A New DNI Computation
This study introduces a new technique to compute direct normal irradiance (DNI) for improving the National Solar Radiation Data Base (NSRDB). A finite-surface integration algorithm is developed to compute solar radiation in differential solid angles and efficiently infer its contribution to a surface perpendicular to the solar direction. A lookup table of cloud bi-directional transmittance distribution function (BTDF) is developed by use of the discrete ordinates radiative transfer (DISORT) model for possible solar and observing directions and various cloud optical and microphysical properties. In each solar incident direction, DNI is given by the cloud BTDFs from approximately 200 differential solid angles. The simulated DNI is calibrated and evaluated using surface observations at the National Renewable Energy Laboratory's (NREL's) Solar Energy Research Laboratory (SRRL) and the Atmospheric Radiation Measurement (ARM) Southern Great Plains (SGP) facility.
41 EE - Solar Energy Technologies Office (EE-4S)↗
The Estimation of Hydrometeor Profiles from Wideband Microwave Observations
Profiles of the microphysical properties of clouds and raincells are essential in many areas of atmospheric research and operational meteorology. In order to enhance the understanding of the nonlinear and underconstrained relationships between cloud and hydrometeor microphysical profiles and passive microwave brightness temperatures, estimations of cloud profiles for an anvil, a convective, and an updraft region of an oceanic squall were performed. The estimations relied on comparisons between radiative transfer calculations of incrementally estimated microphysical profiles and concurrent dual-altitude wideband brightness temperatures from the 22 February 1993 flight during TOGA-COARE. The wideband observations (10--220 GHz) are necessary for estimating cloud profiles reaching up to 20 km. The low frequencies enhance the rain and cloud water profiles, while the high frequencies are required to detail the higher altitude ice microphysics. A microphysical profile was estimated for each of the three regions of the storm. Each of the three estimated profiles produced calculated brightness temperatures within approximately 10 K of the observations. A majority, of the total iterative adjustment were to the estimated profile's frozen hydrometeor characteristics and were necessary to match the high frequency calculations with the observations. This indicates a need to validate cloud resolving models using high frequencies. Some difficulties matching the 37 GHz observation channels on the DC-8 and ER-2 aircrafts with the calculations simulated at the two aircraft heights (approximately 11 km and 20 km, respectively) were noted and potential causes presented.
Gail M Skofronick-Jackson↗
Optical and microphysical properties of a cold cirrus cloud - Evidence for regions of small ice particles
An airborne lidar and a scanning radiometer aboard an ER-2 aircraft were used to observe a cold cirrus cloud, and a Forward Scattering Spectrometer Probe (FSSP) was used to obtain simultaneous in situ microphysical observations at two altitudes within the cloud. Lidar depolarization ratio data show that the clouds were composed predominantly of ice crystals. At an altitude where the temperature was -62.7 C, the lidar and radiometer analysis gave a visible extinction to infrared absorption ratio (alpha) of 2.3, while the cloud microphysics data provided an alpha value of 3.77. The discrepancy is attributed to undersizing of particles by the FSSP. Direct and remote measurements showed better agreement for a lower layer where the temperature was -47.3 C.
Platt, C. M. R.↗
Ice and Supercooled Liquid Water Distributions over the Southern Ocean based on In Situ Observations and Climate Model Simulations
Three climate models are evaluated using in situ airborne observations from the Southern Ocean Clouds, Radiation, Aerosol Transport Experimental Study (SOCRATES) campaign. The evaluation targets cloud phases, microphysical properties, thermodynamic conditions, and aerosol indirect effects from –40°C to 0°C. Compared with 580-s averaged observations (i.e., 100 km horizontal scale), the Community Atmosphere Model version 6 (CAM6) shows the most similar result for cloud phase frequency distribution and allows more liquid-containing clouds below –10°C compared with its predecessor—CAM5. The Energy Exascale Earth System Model (E3SM) underestimates (overestimates) ice phase frequencies below (above) –20°C. CAM6 and E3SM show liquid and ice water contents (i.e., LWC and IWC) similar to observations from –25°C to 0°C, but higher LWC and lower IWC than observations at lower temperatures. Simulated in-cloud RH shows higher minimum values than observations, possibly restricting ice growth during sedimentation. As number concentrations of aerosols larger than 500 nm (Na 500 ) increase, observations show increases of LWC, IWC, liquid, and ice number concentrations (N liq , N ice ). Number concentrations of aerosols larger than 100 nm (Na 100 ) only show positive correlations with LWC and N liq . From –20°C to 0°C, higher aerosol number concentrations are correlated with lower glaciation ratio and higher cloud fraction. From –40°C to –20°C, large aerosols show positive correlations with glaciation ratio. CAM6 shows small increases of LWC and N liq with Na 500 and Na 100 . E3SM shows small increases of N ice with Na 500 . Altogether, CAM6 and E3SM underestimate aerosol indirect effects on ice crystals and supercooled liquid droplets over the Southern Ocean.
54 ENVIRONMENTAL SCIENCES↗
A Multi-Instrument Cloud Condensation Nuclei Spectrum Product (Final Technical Report)
A wealth of observational data exists on the characteristics of atmospheric particulate matter, over multiple years, at the DOE ARM Southern Great Plains (SGP) Central Facility site. This site is located in a region of the country that frequently experiences weather extremes, and that is removed from many local sources of pollution but is affected by transported smoke, dust, and urban emissions. The relationships between particulate matter, cloud formation and evolution, and precipitation are therefore of strong interest, and are being explored via modeling on a variety of scales. These models require as input detailed information on the characteristics of particles capable of serving as the nuclei for cloud formation. Sufficient data exist to be able to put together a picture of the nature of the total aerosol and the cloud condensation nuclei (CCN) subset, and their variability, through merged data products. This study was aimed at exploiting the multiple measurement types at SGP to develop the first such multi-year estimates. Further, the resulting data were analyzed to understand temporal patterns ranging from hourly to seasonal, thereby gaining insights into the particle sources affecting the atmosphere in this region. DOE-funded datasets that were analyzed in this study include total particle number concentrations, submicron aerosol scattering coefficients, dry aerosol size distributions, and more recently, time-resolved submicron aerosol chemical composition. Data are also available for the number concentrations of particles that are activated in a cloud condensation nucleus instrument at a series of setpoint supersaturations, providing direct observations of the number concentrations of “CCN”. This variable is the quantity that is generally desired for inclusion in numerical models that seek to represent and predict the impacts of varying aerosol characteristics on the formation and microphysical properties of clouds. One limitation of the use of direct CCN observations is that they are not available for supersaturations larger than about 1%, which is insufficient for deep convection and may be insufficient even for shallow convection, depending on the nature of the available CCN and the dynamics of the cloud. We developed a data-based approach to representing the full aerosol size spectrum with size-dependent hygroscopicity, and used this to extrapolate CCN spectra beyond the limited measurements. Five years of SGP aerosol data (2009 -2013) were analyzed. As a side product of our work, we identified and communicated several previously-unflagged data quality issues. The resulting merged aerosol distributions, along with fits for seasonal averages, were published and submitted to the ARM archive as a special value-added product (VAP; submitted as a PI product). CCN spectra were computed for the same data period and will similarly be published and submitted to the archive for use by the community. We also note that our methodologies and findings have been discussed at several Joint ARM User Facility/Atmospheric System Research (ASR) Principal Investigators Meetings and that recent ARM/ASR aerosol data reporting strategies have included similar ideas for data merging, indicating that this work has had a lasting impact on ARM aerosol data acquisition and reporting. The proposed work advances the science of the interactions of aerosols, clouds and precipitation, with direct application to improve representation of such interactions for clouds in regional and global climate models. The archived data will continue to serve research studies in the future.
54 ENVIRONMENTAL SCIENCES↗