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Evidence That Nitric Acid Increases Relative Humidity in Low-Temperature Cirrus Clouds

In situ measurements of the relative humidity with respect to ice (RH(sub(i)) and of nitric acid (HNO3) were made in both natural and contrail cirrus clouds in the upper troposphere. At temperatures lower than 202 kelvin, RH(sub i) values show a sharp increase to average values of over 130% in both cloud types. These enhanced RH(sub i) values are attributed to the presence of a new class of NHO3- containing ice particles (Delta-ice). We propose that surface HNO3 molecules prevent the ice/vapor system from reaching equilibrium by a mechanism similar to that of freezing point depression by antifreeze proteins. Delta-ice represents a new link between global climate and natural and anthropogenic nitrogen oxide emissions. Including Delta-ice in climate models will alter simulated cirrus properties and the distribution of upper tropospheric water vapor.

Gao, R. S.↗

Cirrus cloud development in a mobile upper tropospheric trough: The November 26th FIRE cirrus case study

The period from 18 UTC 26 Nov. 1991 to roughly 23 UTC 26 Nov. 1991 is one of the study periods of the FIRE (First International Satellite Cloud Climatology Regional Experiment) 2 field campaign. The middle and upper tropospheric cloud data that was collected during this time allowed FIRE scientists to learn a great deal about the detailed structure, microphysics, and radiative characteristics of the mid latitude cirrus that occurred during that time. Modeling studies that range from the microphysical to the mesoscale are now underway attempting to piece the detailed knowledge of this cloud system into a coherent picture of the atmospheric processes important to cirrus cloud development and maintenance. An important component of the modeling work, either as an input parameter in the case of cloud-scale models, or as output in the case of meso and larger scale models, is the large scale forcing of the cloud system. By forcing we mean the synoptic scale vertical motions and moisture budget that initially send air parcels ascending and supply the water vapor to allow condensation during ascent. Defining this forcing from the synoptic scale to the cloud scale is one of the stated scientific objectives of the FIRE program. From the standpoint of model validation, it is also necessary that the vertical motions and large scale moisture budget of the case studies be derived from observations. It is considered important that the models used to simulate the observed cloud fields begin with the correct dynamics and that the dynamics be in the right place for the right reasons.

Mace, Gerald G.↗

Optical and microphysical properties of a cold cirrus cloud - Evidence for regions of small ice particles

An airborne lidar and a scanning radiometer aboard an ER-2 aircraft were used to observe a cold cirrus cloud, and a Forward Scattering Spectrometer Probe (FSSP) was used to obtain simultaneous in situ microphysical observations at two altitudes within the cloud. Lidar depolarization ratio data show that the clouds were composed predominantly of ice crystals. At an altitude where the temperature was -62.7 C, the lidar and radiometer analysis gave a visible extinction to infrared absorption ratio (alpha) of 2.3, while the cloud microphysics data provided an alpha value of 3.77. The discrepancy is attributed to undersizing of particles by the FSSP. Direct and remote measurements showed better agreement for a lower layer where the temperature was -47.3 C.

Platt, C. M. R.↗

Polarimetric Retrievals of Surface and Cirrus Clouds Properties in the Region Affected by the Deepwater Horizon Oil Spill

In 2010, the Goddard Institute for Space Studies (GISS) Research Scanning Polarimeter (RSP) performed several aerial surveys over the region affected by the oil spill caused by the explosion of the Deepwater Horizon offshore platform. The instrument was deployed on the NASA Langley B200 aircraft together with the High Spectral Resolution Lidar (HSRL), which provides information on the distribution of the aerosol layers beneath the aircraft, including an accurate estimate of aerosol optical depth. This work illustrates the merits of polarization measurements in detecting variations of ocean surface properties linked to the presence of an oil slick. In particular, we make use of the degree of linear polarization in the glint region, which is severely affected by variations in the refractive index but insensitive to the waviness of the water surface. Alterations in the surface optical properties are therefore expected to directly affect the polarization response of the RSP channel at 2264 nm, where both molecular and aerosol scattering are negligible and virtually all of the observed signal is generated via Fresnel reflection at the surface. The glint profile at this wavelength is fitted with a model which can optimally estimate refractive index, wind speed and direction, together with aircraft attitude variations affecting the viewing geometry. The retrieved refractive index markedly increases over oil-contaminated waters, while the apparent wind speed is significantly lower than in adjacent uncontaminated areas, suggesting that the slick dampens high-frequency components of the ocean wave spectrum. The constraint on surface reflectance provided by the short-wave infrared channels is a cornerstone of established procedures to retrieve atmospheric aerosol microphysical parameters based on the inversion of the RSP multispectral measurements. This retrieval, which benefits from the ancillary information provided by the HSRL, was in this specific case hampered by prohibitive variability in atmospheric conditions (very inhomogeneous aerosol distribution and cloud cover). Although the results presented for the surface are essentially unaffected, we discuss the results obtained by typing algorithms in sorting the complex mix of aerosol types, and show evidence of oriented ice in cirrus clouds present in the area. In this context, polarization measurements at 1880 nm were used to infer ice habit and cirrus optical depth, which was found in the subvisual/threshold-visible regime, confirming the utility of the aforementioned RSP channel for the remote sensing of even thin cold clouds.

Polarization↗

Polarization Calibration Using Solar Radiation Background Signal Scattered from Dense Cirrus Clouds in the Visible and Ultraviolet Wavelength Regimes

In this presentation we describe the application of a previously developed technique that is now being used to correct the daytime polarization calibration of the CALIPSO lidar. The technique leverages the fact that the solar radiation background signals from dense cirrus clouds are largely unpolarized due to the internal multiple reflections within the non-spherical ice particles and the multiple scattering that occurs among these particles. Therefore, the ratio of polarization components of the cirrus background signals provides a good estimate for the polarization gain ratio (PGR) of the lidar. Using airborne backscatter lidar measurements, this technique was demonstrated to work well in the infrared regime. However, in the visible and ultraviolet regime, the molecular contribution is too large to be ignored, and thus corrections must be applied to account for the highly polarizing characteristics of the molecular scattering. Ignoring molecular scattering contributions can cause PGR errors of 2-3% at 532 nm, where the CALIPSO lidar makes its depolarization measurement. Because of the wavelength dependence of -4 of the molecular scattering, the PGR error can be even larger at the 355 nm wavelength that will be used by ESA’s EarthCARE lidar. To correct the molecular scattering contributions to the lidar received solar background signal, a look-up table has been created using a polarization-sensitive radiative transfer model. This presentation describes the theory and implementation of the molecular scattering correction.

Zhaoyan Liu↗

Above-Aircraft Cirrus Cloud and Aerosol Optical Depth From Hyperspectral Irradiances Measured By a Total-Diffuse Radiometer

This study develops the use of spectral total and diffuse irradiance measurements, made from a prototype hyperspectral total-diffuse sunshine pyranometer (SPN-S), to retrieve layer fine-mode aerosol (τ aer ) and total optical depths from airborne platforms. Additionally, we use spectral analysis in an attempt to partition the total optical depth into its τ aer and cirrus cloud optical depth (τ cld ) components in the absence of coarse-mode aerosols. Two retrieval methods are developed: one leveraging information in the diffuse irradiance and the other using spectral characteristics of the transmitted direct beam, with each approach best suited for specific cloud and aerosol conditions. The SPN-S has advantages over traditional sun photometer systems, including no moving parts and a low cost. However, a significant drawback of the instrument is that it is unable to measure the direct-beam irradiance as accurately as sun photometers. To compensate for the greater measurement uncertainty in the radiometric irradiances, these retrieval techniques employ ratioed inputs or spectral information to reduce output uncertainty. This analysis uses irradiance measurements from the SPN-S and the solar spectral flux radiometer (SSFR) aboard the National Aeronautics and Space Administration’s (NASA) P-3 aircraft during the 2018 deployment of the ObseRvations of Aerosols above CLouds and their intEractionS (ORACLES) campaign and the 2019 Cloud, Aerosol and Monsoon Processes Philippines Experiment (CAMP 2 Ex) mission to quantify above-aircraft cirrus τ cld and derive vertical profiles of layer τ aer . Validation of the τ aer retrieval is accomplished by comparison with co-located measurements of direct solar irradiance made by the Sky-Scanning Sun-Tracking Atmospheric Research (4STAR) and in situ measurements of aerosol optical depth. For the aggregated 2018 ORACLES results, regression between the SPN-S-based method and sun photometer τ aer values yields a slope of 0.96 with an R 2 of 0.96, while the root mean square error (RMSE) is 3.0 x 10 -2 . When comparing the retrieved τ aer to profiles of integrated in situ measurements of optical extinction, the slope, R 2 , and RMSE values for ORACLES are 0.90, 0.96, and 3.4 x 10 -2 , and for CAMP 2 Ex they are 0.94, 0.97, and 3.4 x 10 -2 , respectively. This paper is a demonstration of methods for deriving cloud and aerosol optical properties in environments where both atmospheric constituents may be present. With improvements to the low-cost SPN-S radiometer instrument, it may be possible to extend these methods to a broader set of sampling applications, such as ground-based settings.

spectral instrument (SPN-S)↗

The use of an airborne lidar for mapping cirrus clouds in FIRE, phase 2

The Univ. of Washington (UW) and Georgia Tech have recently built a dual wavelength airborne lidar for operation on the UW's Convair C-131A research aircraft. This lidar was used in studying aerosols and clouds. These studies demonstrated the utility of airborne lidar in a variety of atmospheric research and prompt the suggestion that this facility be included in the next FIRE cirrus experiment. The vertically pointing airborne lidar would be used as a complement to ground based lidars. The airborne lidar would ensure extended coverage of IFO cases that develop upwind of the surface lidars or which miss the ground based lidars while still being the focus of satellite and aircraft in situ studies. The airborne lidar would help assure that cirrus clouds were simultaneously viewed by satellite, sampled by aircraft, and structurally characterized by lidar. System specifications are listed and a schematic is shown of the lidar system aboard the C-131A.

Radke, Lawrence F.↗

The Relationship of Subvisible Cirrus Clouds Observed During NASA's Tropical Ozone

Thin, subvisible cirrus (SVC) clouds at the tropical tropopause have been observed by a number of methods in a variety of observational programs, including in situ sampling and aircraft and space-based lidar. Modeling studies suggest that these clouds play an important role in dehydrating tropospheric air as it enters the stratosphere. This is because particles large enough to have significant fall speeds can form under the conditions of slow cooling that are implied by the large horizontal extent of the SVC sheets. The IRA radiation that these clouds absorb, and the upward vertical motion this implies, also make them candidates for a tropical troposphere-to-stratosphere mass transfer mechanism. These sheets were observed on five flights during the Tropical Ozone Transport Experiment (TOTE) by the NASA Langley DIAL lidar aboard NASA's DC-8 research aircraft, operating during December 1995 and February 1996 south of Hawaii (12 S to 21 N). This experiment provided a unique look at these clouds since temperature profiles were available for all the SVC observations. Thus, the observed distributions of SVC's can be compared with the position of the tropopause to establish whether the SVC's are tropospheric or stratospheric. It also allows comparison of TOTE observations with in situ experiments, where water and cloud particle data is available as a function of temperature and potential temperature.

Pfister, L.↗

Polar Cirrus Cloud Properties Through Long-Term Lidar and Radiometer Observations

In comparison to mid latitude cloud cover, knowledge of polar cirrus and other cloud cover is limited. The interpretations of satellite-based cloud imaging and retrievals in polar regions have major problems due to factors such as darkness and extreme low temperatures. Beginning in 2002 a NASA orbiting lidar instrument, GLAS, (Geoscience Laser Altimeter System) will unambiguously define cloud type and fraction with good coverage of polar regions. Active laser sensing gives the spatial and temporal distribution of clouds and diamond dust. In preparation for, and supplementing the GLAS measurements are ground based MP (micro pulse) lidar experiments providing continuous profiling. MP lidar installations have been operating at the South Pole since December 1999 and at the Atmospheric Radiation Measurement (ARM) program arctic site since 1996. Both at the ARM Barrow, Alaska site and at the South Pole station, Fourier-transform interferometers also observe clouds in the wavelength intervals between approximately 5 and 18 microns. Spectral instruments can yield cloud microphysical properties with additional information from lidar about the vertical extent of clouds being modeled. We examine the simultaneous lidar and spectral data from both Barrow and South Pole, to obtain cloud properties (optical depth, particle size) by the use of both instruments. The results have applications to interpretation of current satellite data, and GLAS measurements when available.

Spinhirne, James↗

Coincident Occurrences of Tropical Individual Cirrus Clouds and Deep Convective Systems Derived from TRMM Observations

Measurements of cloud properties and atmospheric radiation taken between January and August 1998 by the Tropical Rainfall Measuring Mission (TRMM) satellite were used to investigate the effect of spatial and temporal scales on the coincident occurrences of tropical individual cirrus clouds (ICCs) and deep convective systems (DCSs). It is found that there is little or even negative correlation between instantaneous occurrences of ICC and DCS in small areas, in which both types of clouds cannot grow and expand simultaneously. When spatial and temporal domains are increased, ICCs become more dependent on DCSs due to the origination of many ICCs from DCSs and moisture supply from the DCS in the upper troposphere for the ICCs to grow, resulting in significant positive correlation between the two types of tropical high clouds in large spatial and long temporal scales. This result may suggest that the decrease of tropical high clouds with SST from model simulations is likely caused by restricted spatial domains and limited temporal periods. Finally, the radiative feedback due to the change in tropical high cloud area coverage with sea surface temperature appears small and about -0.14 W/sq m per degree Kelvin.

Lin, Bing↗

Midlatitude Cirrus Clouds Derived from Hurricane Nora: A Case Study with Implications for Ice Crystal Nucleation and Shape

Hurricane Nora traveled up the Bala Peninsula coast in the unusually warm El Nino waters of September 1997, until rapidly decaying as it approached Southern California on 24 September. The anvil cirrus blowoff from the final surge of tropical convection became embedded in subtropical flow that advected the cirrus across the western US, where it was studied from the Facility for Atmospheric Remote Sensing (FARS) in Salt Lake City, Utah. A day later, the cirrus shield remnants were redirected southward by midlatitude circulations into the Southern Great Plains, providing a case study opportunity for the research aircraft and ground-based remote sensors assembled at the Clouds and Radiation Testbed (CART) site in northern Oklahoma. Using these comprehensive resources and new remote sensing cloud retrieval algorithms, the microphysical and radiative cloud properties of this unusual cirrus event are uniquely characterized. Importantly, at both the FARS and CART sites the cirrus generated spectacular optical displays, which acted as a tracer for the hurricane cirrus, despite the limited lifetimes of individual ice crystals. Lidar polarization data indicate widespread regions of uniform ice plate orientations, and in situ particle masticator data show a preponderance of pristine, solid hexagonal plates and columns. It is suggested that these unusual aspects are the result of the mode of cirrus particle nucleation, presumably involving the lofting of sea-salt nuclei in thunderstorm updrafts into the upper troposphere. This created a reservoir of haze particles that continued to produce halide-saltcontaminated ice crystals during the extended period of cirrus cloud maintenance. The reference that marine microliters are embedded in the replicas of ice crystals collected over the CART site points to the longevity of marine effects. Various nucleation scenarios proposed for cirrus clouds based on this and other studies, and the implications for understanding cirrus radiative properties or a global scale, are discussed.

Sassen, Kenneth↗

Cirrus Clouds Optical, Microphysical and Radiative Properties Observed During Crystal-Face Experiment: I. A Radar-Lidar Retrieval System

A method of retrieving cloud microphysical properties using combined observations from both cloud radar and lidar is introduced. This retrieval makes use of an improvement to the traditional optimal estimation retrieval method, whereby a series of corrections are applied to the state vector during the search for an iterative solution. This allows faster convergence to a solution and is less processor intensive. The method is first applied to a synthetic cloud t o demonstrate its validity, and it is shown that the retrieval reliably reproduces vertical profiles of ice water content. The retrieval method is then applied to radar and lidar observations from the CRYSTAL-FACE experiment, and vertical profiles of ice crystal diameter, number concentration, and ice water content are retrieved for a cirrus cloud layers observed one day of that experiment. The validity of the relationship between visible extinction coefficient and radar reflectivity was examined. While synthetic tests showed such a functional relationship, the measured data only partially supported such a conclusion. This is due to errors in the forward model (as explained above) as well as errors in the data sets, including possible mismatch between lidar and radar profiles or errors in the optical depth. Empirical relationships between number concentrations and mean particle diameter were also examined. The results indicate that a distinct and robust relationship exists between these retrieved quantities and it is argued that such a relationship is more than an artifact of the retrieval process offering insight into the nature of the microphysical processes taking place in cirrus.

Mitrescu, C.↗

Solar radiative transfer in cirrus clouds. I - Single-scattering and optical properties of hexagonal ice crystals. II - Theory and computations of multiple scattering in an anisotropic medium

The light scattering and absorption programs of Cai and Liou (1982) and Takano and Jaweera (1985) are extended to include hexagonal ice crystals randomly and horizontally oriented in space. The scattering and polarization results for the ice crystals are calculated. The results are compared with measurement data. The single-scattering properties for horizontally oriented columns and plates are presented and used to explain halos and arcs observed in the atmopshere. In the second section, the theory and computations for multiple scattering in cirrus clouds containing oriented ice crystals are presented. The radiative transfer in clouds composed of horizontally oriented ice crystals is formulated. Also, reflected and transmitted intensities, planetary albedo, and polarization in multiple scattering by ice crystals are discussed.

Takano, Yoshihide↗

Discovery of a candidate old, isolated neutron star in the field of a galactic cirrus cloud

New x-ray optical, and radio observations of the bright, unidentified x-ray source MS 0317.7-6647 are presented suggesting that this source is a likely compact stellar remnant. As part of the Einstein Extended Medium Sensivity Survey, this source was discovered serendipitously in the Einstein Imaging Proportional Counter pointing towards the nearby (4.5 Mpc) spiral galaxy NGC 1313. The very high x-ray to optical flux ratio, pointlike ROSAT HRI detection, and extremely soft component in the x-ray spectrum of MS 0317.7-6647 eliminate all the usual classes of optical counterparts to faint x-ray sources except for a very massive x-ray binary (and black hole candidate) in NGC 1313, a nearby, companionless pulsar similar to Geminga, or a very nearby ( approximately 100 pc) isolated, old neutron star slowly accreting interstellar matter onto its magnetic poles. The presence of an IR cirrus cloud which shadows the approximately 0.25 keV x-ray background in this direction supports the latter possibilty.

Stocke, John T.↗

Radiative Transfer and Satellite Remote Sensing of Cirrus Clouds Using FIRE-2-IFO Data

Under the support of the NASA grant, we have developed a new geometric-optics model (GOM2) for the calculation of the single-scattering and polarization properties for arbitrarily oriented hexagonal ice crystals. From comparisons with the results computed by the finite difference time domain (FDTD) method, we show that the novel geometric-optics can be applied to the computation of the extinction cross section and single-scattering albedo for ice crystals with size parameters along the minimum dimension as small as approximately 6. We demonstrate that the present model converges to the conventional ray tracing method for large size parameters and produces single-scattering results close to those computed by the FDTD method for size parameters along the minimum dimension smaller than approximately 20. We demonstrate that neither the conventional geometric optics method nor the Lorenz-Mie theory can be used to approximate the scattering, absorption, and polarization features for hexagonal ice crystals with size parameters from approximately 5 to 20. On the satellite remote sensing algorithm development and validation, we have developed a numerical scheme to identify multilayer cirrus cloud systems using AVHRR data. We have applied this scheme to the satellite data collected over the FIRE-2-IFO area during nine overpasses within seven observation dates. Determination of the threshold values used in the detection scheme are based on statistical analyses of these satellite data.

Source record↗

NASA/GSFC Scanning Raman Lidar Measurements of Water Vapor and Cirrus Clouds during WVIOP2000 and AFWEX

The NASA/GSFC Scanning Raman Lidar (SRL) was deployed to the Southern Great Plains CART site from September - December, 2000 and participated in two field campaigns devoted to comparisons of various water vapor measurement technologies and calibrations. These campaigns were the Water Vapor Intensive Operations Period 2000 (WVIOP2000) and the ARM FIRE Water Vapor Experiment (AFWEX). WVIOP2000 was devoted to validating water vapor measurements in the lower atmosphere while AFWEX had similar goals but for measurements in the upper troposphere. The SRL was significantly upgraded both optically and electronically prior to these field campaigns. These upgrades enabled the SRL to demonstrate the highest resolution lidar measurements of water vapor ever acquired during the nighttime and the highest S/N Raman lidar measurements of water vapor in the daytime; more than a factor of 2 increase in S/N versus the DOE CARL Raman Lidar. Examples of these new measurement capabilities along with comparisons of SRL and CARL, LASE, MPI-DIAL, in-situ sensors, radiosonde, and others will be presented. The profile comparisons of the SRL and CARL have revealed what appears to be an overlap correction or countrate correction problem in CARL. This may be involved in an overall dry bias in the precipitable water calibration of CARL with respect to the MWR of approx. 4%. Preliminary analysis indicates that the application of a temperature dependent correction to the narrowband Raman lidar measurements of water vapor improves the lidar/Vaisala radiosonde comparisons of upper tropospheric water vapor. Other results including the comparison of the first-ever simultaneous measurements from four water vapor lidar systems, a bore-wave event captured at high resolution by the SRL and cirrus cloud optical depth studies using the SRL and CARL will be presented at the meeting.

Whiteman, D. N.↗

Evidence for liquid-phase cirrus cloud formation from volcanic aerosols - Climatic implications

Supercooled droplets in cirrus uncinus cell heads between -40 and -50 C are identified from the First International Satellite Cloud Climatology Project Regional Experiment polarization lidar measurements. Although short-lived, complexes of these small liquid cells seem to have contributed importantly to the formation of the cirrus. Freezing-point depression effects in solution droplets, apparently resulting from relatively large cloud condensation nuclei of volcanic origin, can be used to explain this rare phenomenon. An unrecognized volcano-cirrus cloud climate feedback mechanism is implied by these findings.

Sassen, Kenneth↗

Directly Measured Heating Rates of a Tropical Subvisible Cirrus Cloud

We present the first direct measurements of the infrared and solar heating rates of a tropical subvisible cirrus (SVC) cloud sampled off the east coast of Nicaragua on 25 July 2007 by the NASA ER-2 aircraft during the Tropical Composition, Cloud and Climate Coupling Experiment (TC4). On this day a persistent thin cirrus layer, with mostly clear skies underneath, was detected in real time by the cloud lidar on the ER-2, and the aircraft was directed to profile down through the SVC. Measurements of the net broadband infrared irradiance and spectrally integrated solar irradiance above, below, and through the SVC are used to determine the infrared and solar heating rates of the cloud. The lidar measurements show that the variable SVC layer was located between approximately 13 and 15 km. Its midvisible optical depth varied from 0.01 to 0.10 with a mean of 0.034 +/- 0.033. Its depolarization ratio was approximately 0.4, indicative of ice clouds. From the divergence of the measured net irradiances the infrared heating rate of the SVC was determined to be approximately 2.50 - 3.24 K/d and the solar heating rate was found to be negligible. These values are consistent with previous indirect observations of other SVC and with model-generated heating rates of SVC with similar optical depths. This study illustrates the utility and potential of the profiling sampling strategy employed here. A more fully instrumented high-altitude aircraft that also included in situ cloud and aerosol probes would provide a comprehensive data set for characterizing both the radiative and microphysical properties of these ubiquitous tropical clouds

Bucholtz, Anthongy↗