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At least 181 records · Page 10
All sourcesNASA NTRSDOE OSTI
NASA NTRS1995

Stratospheric Aerosol and Gas Experiments 1 and 2: Comparisons with ozonesondes

Ozone profiles measured by the Stratospheric Aerosol and Gas Experiments (SAGE) 1 and 2 are compared with ozonesonde profiles at 24 stations over the period extending from 1979 through 1991. Ozonesonde/satellite differences at 21 stations with SAGE 2 overpasses were computed down to 11.5 km in midlatitudes, to 15.5 km in the lower latitudes, and for nine stations with SAGE 1 overpasses down to 15.5 km. The set of individual satellite and ozonesonde profile comparisons most closely colocated in time and space shows mean absolute differences relative to the satellite measurement of 6 +/- 2% for SAGE 2 and 8 +/- 3% for SAGE 1. The ensemble of ozonesonde/satellite differences, when averaged over all altitudes, shows that for SAGE 2, 70% were less than 5%, whereas for SAGE 1, 50% were less than 5%. The best agreement occurred in the altitude region near the ozone density maximum where almost all the relative differences were less than 5%. Most of the statistically significant differences occurred below the ozone maximum down to the tropopause in the region of steepest ozone gradients and typically ranged between 0 and -20%. Correlations between ozone and aerosol extinction in the northern midlatitudes indicate that aerosols had no discernible impact on the ozonesonde/satellite differences and on the SAGE 2 ozone retrieval for the levels of extinction encountered in the lower stratosphere during 1984 to mid-1991.

Veiga, Robert E.↗
NASA NTRS2019

Detecting Layer Height of Smoke Aerosols over Vegetated Land and Water Surfaces via Oxygen Absorption Bands: Hourly Results from EPIC/DSCOVR in Deep Space

We present an algorithm for retrieving aerosol layer height (ALH) and aerosol optical depth (AOD) for smoke over vegetated land and water surfaces from measurements of the Earth Polychromatic Imaging Camera (EPIC) onboard the Deep Space Climate Observatory (DSCOVR). The algorithm uses Earth-reflected radiances in six EPIC bands in the visible and near-infrared and incorporates flexible spectral fitting that accounts for specifics of land and water surface reflectivity. The fitting procedure first determines AOD using EPIC atmospheric window bands (443 nm, 551 nm, 680nm, and 780 nm), then uses oxygen (O2) A and B bands (688 nm and 764 nm) to derive ALH, which represents an optical centroid altitude. ALH retrieval over vegetated surface primarily takes advantage of measurements in the O2B band. We applied the algorithm to EPIC observations of several biomass burning events over the United States and Canada in August 2017. We found that the algorithm can be used to obtain AOD and ALH multiple times daily over water and vegetated land surface. Validation is performed against aerosol extinction profiles detected by the Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP) and against AOD observed at nine Aerosol Robotic Network (AERONET) sites, showing, on average, an error of 0.58 km and a bias of -0.13 km in retrieved ALH and an error of 0.05 and a bias of 0.03 in retrieved AOD. Additionally, we show that the aerosol height information retrieved by the present algorithm can potentially benefit the retrieval of aerosol properties from EPIC’s ultraviolet (UV) bands.

Cloud–Aerosol Lidar with Orthogonal Polarization (↗
DOE OSTI2020

Simultaneous transmission/absorption photometry of particle-laden filters from wildland fires during the Biomass Burning Observation Project (BBOP) field campaign

Transmissivity and absorptivity measurements were carried out simultaneously in the visible (wavelength of 532 nm) at laboratory conditions using particle-laden filters obtained from a three-wavelength particle/soot absorption photometer (PSAP). Here, the particles were collected on filters from wildland fires over the Pacific Northwest during the Department of Energy Biomass Burning Observation Project (BBOP) field campaign in 2013. The objective of this investigation was to apply this measurement approach, referred to as simultaneous transmission/absorption photometry (STAP), to estimate the aerosol extinction coefficient from actual field-campaign filter aerosol, and compare results with the PSAP. The STAP approach offers several advantages over the PSAP, including estimation of the extinction coefficient from temperature measurements (avoiding the complexities associated with filter reflectivity/scattering measurements), as well as determination of the filter optical properties and filter effects on particle absorption (resulting in particle absorption enhancement). The experimental arrangement included a laser probe beam impinging normal to the particle-coated surface of a vertically mounted filter, and a thermocouple placed flush in the middle of (and in thermal contact with) the filter uncoated back surface. With this simple arrangement, the transmissivity and absorptivity were determined simultaneously at a given laser beam wavelength. The measurement repeatability was better than 0.3 K (95% confidence level) for temperature and 0.4 mW for laser power. The limit of detection for the extinction coefficient was estimated to be (8–12) Mm -1 (95% confidence level) at about 1.9 mW laser power. The extinction coefficient was determined through measurement of both PSAP blank and exposed filters. Filters were obtained from nine different aircraft flights conducted during the BBOP campaign, representing different flight patterns, days, stages of burning, landscapes, and wildland fires. The STAP extinction coefficient matched the darkness of the filter coating, however the PSAP-filter results did not follow the same order. Although there were differences in transmissivity between the two techniques, the estimated values for absorption coefficient were in good agreement.

54 ENVIRONMENTAL SCIENCES↗
NASA NTRS1980

Remote sensing of the middle atmospheric aerosol

It is shown that current or planned spacecraft measurements could contribute toward the input data required for studies of natural anthropogenic influences on the middle atmosphere and their effects on weather and climate. Emphasis is placed on the solar occultation sounding technique used in the SAGE I experiment on board the Atmospheric Explorer Mission B spacecraft. It is shown that the aerosol and ozone number densities cannot be recovered simultaneously without introducing some formula for the aerosol extinction, or assumptions on the form of the aerosol size distribution.

Fymat, A. L.↗
NASA NTRS1985

Variations in stratospheric aerosol optical depth during northern warmings

In this paper, the properties of the stratospheric aerosol optical depth (above 50 mbar) have been studied by using aerosol extinction profiles (at 1 micron) derived from the Stratospheric Aerosol Measurement and Stratospheric Aerosol and Gas Experiment (SAGE) during warming periods in the Northern Hemisphere. It is shown that, during the disturbed periods in winter, low values of aerosol optical depth (less than 0.0002) are found within the low-pressure system(s) (at the 30-mbar pressure surface), while high values are found outside. Similar characteristics are found to exist for the simultaneously observed SAGE O3 and NO2 columnar density distributions. Strong longitudinal gradients are shown with the low values within and wherever the vortex exists. This characteristic is maintained during and after the circumpolar vortex is disturbed, even after breakdown, indicating an isolation of the material within the vortex.

Wang, P.-H.↗
NASA NTRS1991

Separation of cloud and aerosol in two-wavelength satellite occultation data

The separation of cloud and aerosol extinction in satellite solar occultation data is discussed in the context of a simple model for the wavelength dependence of extinction. The model is shown graphically in terms of a scatter plot of 0.525-micron extinction versus 1.02-micron extinction. This plot contains two regions: one arising from aerosol and the other from an aerosol/cloud mixture. Examples of two-wavelength data obtained by the SAGE II instrument are presented and found to agree well with the model. The single wavelength criteria used previously to separate cloud and aerosol are examined in the context of the two-wavelength model.

Kent, G. S.↗
NASA NTRS2015

Nature, Origin, Potential Composition, and Climate Impact of the Asian Tropopause Aerosol Layer (ATAL)

Satellite observations from SAGE II and CALIPSO indicate that summertime aerosol extinction has more than doubled in the Asian Tropopause Aerosol Layer (ATAL) since the late 1990s. Here we show remote and in-situ observations, together with results from a chemical transport model (CTM), to explore the likely composition, origin, and radiative forcing of the ATAL. We show in-situ balloon measurements of aerosol backscatter, which support the high levels observed by CALIPSO since 2006. We also show in situ measurements from aircraft, which indicate a predominant carbonaceous contribution to the ATAL (Carbon/Sulfur ratios of ~2- 10), which is supported by the CTM results. We show that the peak in ATAL aerosol lags by ~1 month the peak in CO from MLS, associated with deep convection over Asia during the summer monsoon. This suggests that secondary formation and growth of aerosols in the upper troposphere on monthly timescales make a significant contribution to ATAL. Back trajectory calculations initialized from CALIPSO observations provide evidence that deep convection over India is a significant source for ATAL through the vertical transport of pollution to the upper troposphere.

Fairlie, T. D.↗
NASA NTRS1992

Stratospheric Backscatter, Extinction, and Lidar Ratio Profiling After the Mt. Pinatubo Eruptions

Since August 1991 the stratospheric aerosol layer is continuously monitored with a combination Raman elastic-backscatter lidar, groundbased systems. XeCl excimer laser is used as the radiation source. Signals elastically backscattered from air molecules and particles and inelastically Raman backscattered from nitrogen molecules are detected. The measurements of these two signal profiles up to 35 km height allows the separate and independent determination of aerosol extinction and backscatter properties in the perturbed lower stratosphere. The extinction coefficient is derived from the nitrogen Raman signal profile, while the backscatter coefficient is obtained from the elastic-to-inelastic backscatter signal ratio. In this way, also the extinction-to-backscatter, or lidar, ratio profile is determined. For the first time, lidar ratios are determined in the perturbed stratospheric layer by the use of remote sensing only. The lidar ratio contains information about the size range of the stratospheric particles which are assumed to be sulfuric acid droplets, and it is needed in the calculation of aerosol optical properties from data taken with a typical backscatter lidar.

Ansmann, Albert↗
NASA NTRS2024

Opinion: Aerosol Remote Sensing Over the Next Twenty Years

More than two decades ago, aerosol remote sensing underwent a revolution with the launch of the Terra and Aqua satellites. Advancement continued via additional launches carrying new passive and active sensors. Capable of retrieving parameters characterizing aerosol loading, rudimentary particle properties and in some cases aerosol layer height, the satellite view of Earth’s aerosol system came into focus.The modeling communities have made similar advances. Now the efforts have continued long enough that we can see developing trends in both remote sensing and modeling communities, allowing us to speculate about the future and how the community will approach aerosol remote sensing twenty years from now. We anticipate technology that will replace today’s standard multi-wavelength radiometers with hyperspectral and/or polarimetry all viewing in multiple angles.These will be supported by advanced active sensors with the ability to measure profiles of aerosol extinction in addition to backscatter. The result will be greater insight into aerosol particle properties. Algorithms will move from being primarily physically-based to include an increasing degree of Machine Learning methods, but physically-based techniques will not go extinct. However, the practice of applying algorithms to a single sensor will be in decline. Retrieval algorithms will encompass multiple sensors and all available ground measurements into a unifying framework, and these inverted products will be ingested directly into assimilation systems, becoming “cyborgs”: half observations, half model. In twenty years we will see a true democratization in space with nations large and small, private organizations and commercial entities of all sizes launching space sensors. With this increasing amount of data and aerosol products available, there will be a lot of bad data. User communities will organize to set standards and the large national space agencies will lead the effort to maintain quality by deploying and maintaining validation ground networks and focused field experiments. Through it all, interest will remain high in the global aerosol system and how that system affects climate, clouds, precipitation and dynamics, air quality, the environment and public health, transport of pathogens and fertilization of ecosystems, and how these processes are adapting to a changing climate.

aerosol remote sensing↗
NASA NTRS2000

LIDAR Measurements During Aerosols99

The Aerosols99 cruise took place during the period from January 14, to February 8 1999 on the R/V Ron Brown. The cruise track was almost a straight line from Norfolk, Va. to Cape Town, South Africa and afforded the opportunity to sample several different aerosol regimes over the North and South Atlantic. A Micro Pulse LIDAR system was used continually during this cruise to profile the aerosol vertical structure. Inversions of this data illustrated a varying vertical structure depending on the dominant air mass. In clean maritime aerosols in the Northern and Southern Hemispheres the aerosols were capped at 1 km. When a Dust event from Africa was encountered the aerosol extinction increased its maximum height to above 2 km. During a period in which the air mass was dominated by biomass burning from Southern Africa, the aerosol layer extended to 4 km. Comparisons of the aerosol optical depth derived from LIDAR inversion and surface sunphotometers showed an agreement within +/- 0.05 RMS Similar comparisons between the extinction measured with a nephelometer and particle soot absorption photometer (at 19 m altitude) and the lowest LIDAR measurement (75 m) showed good agreement (+/- 0.014/km . The LIDAR underestimated surface extinction during periods when an elevated aerosol layer was present over a relatively clean surface layer, but otherwise gave accurate results.

Voss, Kenneth J.↗
DOE OSTI2020

Reducing uncertainties in satellite estimates of aerosol–cloud interactions over the subtropical ocean by integrating vertically resolved aerosol observations

Satellite quantification of aerosol effects on clouds relies on aerosol optical depth (AOD) as a proxy for aerosol concentration or cloud condensation nuclei (CCN). However, the lack of error characterization of satellite-based results hampers their use for the evaluation and improvement of global climate models. We show that the use of AOD for assessing aerosol–cloud interactions (ACIs) is inadequate over vast oceanic areas in the subtropics. Instead, we postulate that a more physical approach that consists of matching vertically resolved aerosol data from the Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observations (CALIPSO) satellite at the cloud-layer height with Moderate Resolution Imaging Spectroradiometer (MODIS) Aqua cloud retrievals reduces uncertainties in satellite-based ACI estimates. Combined aerosol extinction coefficients (σ) below cloud top (σBC) from the Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP) and cloud droplet number concentrations (N d ) from MODIS Aqua yield high correlations across a broad range of σBC values, with σBC quartile correlations ≥0.78. In contrast, CALIOP-based AOD yields correlations with MODIS Nd of 0.54–0.62 for the two lower AOD quartiles. Moreover, σBC explains 41% of the spatial variance in MODIS N d , whereas AOD only explains 17%, primarily caused by the lack of spatial covariability in the eastern Pacific. Compared with σBC, near-surface σ weakly correlates in space with MODIS N d , accounting for a 16% variance. It is concluded that the linear regression calculated from ln(N d )–ln(σBC) (the standard method for quantifying ACIs) is more physically meaningful than that derived from the Nd–AOD pair.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
NASA NTRS1993

The impact of the eruptions of Mount Pinatubo and Cerro Hudson on antarctic aerosol levels during the 1991 austral spring

At the beginning of the 1991 Austral spring, volcanic aerosols from Mt. Pinatubo and Cerro Hudson were present in the polar stratosphere of the Southern Hemisphere. Satellite observations of aerosol extinction were used to identify and track the movement of these aerosols in the vicinity of the Antarctic vortex during August through November 1991. A layer of mature Mt. Pinatubo aerosols was identified near 21 km and a layer of fresh Cerro Hudson aerosols was identified near 12 km. This altitude separation of the Mt. Pinatubo and Cerro Hudson aerosols was observed throughout the period. Below 15 km, the polar stratosphere was subject to episodes of strong wave activity which transported the Cerro Hudson aerosols poleward and, after the middle of September, they became a persistent feature beneath the vortex. Above 15 km, signatures of Mt. Pinatubo aerosols were observed near the vortex boundary, but significant portions of the vortex interior remained free of any detectable intrusions of Mt. Pinatubo aerosols until the final warming in mid-November.

Pitts, M. C.↗
NASA NTRS2024

Vertical Structure of a Springtime Smoky and Humid Troposphere Over the Southeast Atlantic From Aircraft and Reanalysis

The springtime atmosphere over the southeast Atlantic Ocean (SEA) is subjected to a consistent layer of biomass burning (BB) smoke from widespread fires on the African continent. An elevated humidity signal is coincident with this layer, consistently proportional to the amount of smoke present. The combined humidity and BB aerosol has potentially significant radiative and dynamic impacts. Here, we use aircraft-based observations from the NASA ORACLES (ObseRvations of Aerosols above CLouds and their intEractionS) deployments in conjunction with reanalyses to characterize covariations in humidity and BB smoke across the SEA. The observed plume–vapor relationship, and its agreement with the European Centre for Medium-Range Weather Forecasts (ECMWF) Reanalysis version 5 (ERA5) and Copernicus Atmosphere Monitoring Service (CAMS) reanalysis, persists across all observations, although the magnitude of the relationship varies as the season progresses. Water vapor is well represented by the reanalyses, while CAMS tends to underestimate carbon monoxide especially under high BB. While CAMS aerosol optical depth (AOD) is generally overestimated relative to ORACLES AOD, the observations show a consistent relationship between carbon monoxide (CO) and aerosol extinction, demonstrating the utility of the CO tracer to understanding vertical aerosol distribution. We next use k-means clustering of the reanalyses to examine multi-year seasonal patterns and distributions. We identify canonical profile types of humidity and of CO, allowing us to characterize changes in vapor and BB atmospheric structures, and their impacts as they covary. While the humidity profiles show a range in both total water vapor concentration and in vertical structure, the CO profiles primarily vary in terms of maximum concentration, with similar vertical structures in each. The distribution of profile types varies spatiotemporally across the SEA region and through the season, ranging from largely one type in the northeast and southwest to more evenly distributed between multiple types where air masses meet in the middle of the SEA. These distributions follow patterns of transport from the humid, smoky source region (greatest influence in the northeast of the SEA) and the seasonal changes in both humidity and smoke (increasing and decreasing through the season, respectively). With this work, we establish a framework for a more complete analysis of the broader radiative and dynamical effects of humid aerosols over the SEA.

Kristina Pistone↗
NASA NTRS2019

CALIPSO Level 3 Stratospheric Aerosol Product: Version 1.00 Algorithm Description and Initial Assessment

In August 2018,the Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observation (CALIPSO) project released a new level 3 stratospheric aerosol profile data product derived from nearly 12 years of measurements acquired by the space-borne Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP).This monthly averaged, gridded level 3 product is based on version 4.2 of the CALIOP level 1 and level 2 data products, which feature significantly improved calibration that now makes it possible to reliably retrieve profiles of stratospheric aerosol extinction and backscatter coefficients. This paper describes the science algorithm and data handling techniques that were developed to generate the CALIPSO version 1.00 level 3 stratospheric aerosol profile product. Further, we show that the retrieved extinction profiles capture the major stratospheric perturbations over the last decade resulting from volcanic eruptions, extreme smoke events, and signatures of stratospheric dynamics. Initial assessment of the product by inter-comparison with the stratospheric aerosol retrievals from the Stratospheric Aerosol and Gas Experiment III (SAGE III) on the International Space Station (ISS) indicates good agreement in the tropical stratospheric aerosol layer (30oN-30oS),where the average difference between zonal mean extinction profiles is typically less than 25% between 20km and 30km. However, differences can exceed 100% in the very low aerosol loading regimes found above 25 km at higher latitudes.

Jayanta Kar↗
NASA NTRS1986

SAM II measurements of Antarctic PSC's and aerosols

Measurements by the SAM II satellite instrument show that polar stratospheric clouds (PSC's) are a regular feature of the austral winter season in either nonvolcanically or volcanically disturbed periods. The tops of these clouds are observed above 20 km in early winter and descend in altitude over the course of the season to heights near 15 km in mid September. Typically, PSC's persist in the lowest stratospheric altitudes throughout September. Subsequently, October always represents a relative annual minimum in aerosol extinction above 15 km and in stratospheric column amount. In addition, volcanically produced aerosols in Antarctica peaked in early 1983 and, if linearly related to ozone losses, are probably not a contributing factor to the continued loss of total ozone in the Antarctic spring in 1984 and 1985.

Mccormick, M. P.↗
NASA NTRS2002

Airborne Lidar Measurements of Aerosol Optical Properties During SAFARI-2000

The Cloud Physics Lidar (CPL) operated onboard the NASA ER-2 high altitude aircraft during the SAFARI-2000 field campaign. The CPL provided high spatial resolution measurements of aerosol optical properties at both 1064 nm and 532 nm. We present here results of planetary boundary layer (PBL) aerosol optical depth analysis and profiles of aerosol extinction. Variation of optical depth and extinction are examined as a function of regional location. The wide-scale aerosol mapping obtained by the CPL is a unique data set that will aid in future studies of aerosol transport. Comparisons between the airborne CPL and ground-based MicroPulse Lidar Network (MPL-Net) sites are shown to have good agreement.

McGill, M. J.↗