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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 181 records · Page 10
All sourcesNASA NTRSDOE OSTI
DOE OSTI2023

The microstructure and He + ion irradiation behavior of novel low-activation W-Ta-Cr-V refractory high entropy alloy for nuclear applications

Microstructure and nanohardness of a nearly equimolar W-Ta-Cr-V high entropy alloy (HEA), as well as its irradiation response under He + irradiation, were investigated. The single-phase body-centered cubic nanostructured alloy with a 1 µm thick layer was fabricated on a silicon substrate using a magnetron sputtering method. The HEA film has a complex microstructure consisting of micrometric domains that exhibit internal nanostructure controlled by their crystal orientation. The measured nanohardness of the W-Ta-Cr-V alloy is 13 ± 2 GPa, which significantly exceeds the hardness of nanocrystalline tungsten as a result of the high solid-solution strengthening effect. In order to evaluate the irradiation resistance of the HEA film, the material was irradiated with 200 keV He + ions at room temperature, with two different ion fluences: 1 × 10 16 and 5 × 10 16 ions/cm 2 . Using transmission electron microscopy, a high density of extremely fine He bubbles is observed that were uniformly distributed in the matrix. The increase of He + ion fluence increased the density of bubbles, whereas their size remained at a similar level, which indicates that the damage proceeds by the nucleation of additional He bubbles, not by their growth.

36 MATERIALS SCIENCE↗
DOE OSTI2026

Search for a boosted Higgs boson decaying to bottom quark pairs in association with a W or Z boson in proton-proton collisions at $\sqrt{s}$ = 13TeV

A search is conducted for standard model Higgs bosons with large transverse momentum ($p_\mathrm{T}$) decaying to bottom quark pairs and produced in association with a hadronically decaying W or Z boson at the LHC. The result is based on a dataset of proton-proton collisions at a center-of-mass energy of 13 TeV collected with the CMS detector in 2016$-$2018, corresponding to an integrated luminosity of 138 fb$^{-1}$. Boosted Higgs, W, and Z boson decays are reconstructed using large-radius jets with $p_\mathrm{T}$$\gt$ 450 GeV and identified with heavy-flavor classifiers based on a graph convolutional neural network. The observed signal strength relative to the standard model expectation is $μ$ = 0.72 $^{+0.75}_{-0.71}$ including statistical and systematic uncertainties.

CMS↗
DOE OSTI2021

Study of the normalized transverse momentum distribution of W bosons produced in $p\bar{p}$ collisions at $\sqrt{s}$ = 1.96 TeV

We present a study of the normalized transverse momentum distribution of W bosons produced in $p\bar{p}$ collisions, using data corresponding to an integrated luminosity of 4.35 fb -1 collected with the D0 detector at the Fermilab Tevatron collider at $\sqrt{s}$ = 1.96 TeV. The measurement focuses on the transverse momentum region below 15 GeV, which is of special interest for electroweak precision measurements; it relies on the same detector calibration methods which were used for the precision measurement of the W boson mass. The measured distribution is compared to different QCD predictions and a procedure is given to allow the comparison of any further theoretical models to the D0 data.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2025

Measurement of the Lund jet plane in hadronic decays of top quarks and W bosons with the ATLAS detector

The Lund jet plane (LJP) is measured for the first time in $t\bar{t}$ events, using 140 $\textrm{fb}^{-1}$ of $\sqrt{s} = 13$ TeV pp collision data collected with the ATLAS detector at the LHC. The LJP is a two-dimensional observable of the sub-structure of hadronic jets that acts as a proxy for the kinematics of parton showers and hadron formation. The observable is constructed from charged particles and is measured for R = 1.0 anti-$k_t$ jets with transverse momentum above 350 GeV containing the full decay products of either a top quark or a daughter W boson. The other top quark in the event is identified from its decay into a b-quark, an electron or a muon and a neutrino. The measurement is corrected for detector effects and compared with a range of Monte Carlo predictions sensitive to different aspects of the hadronic decays of the heavy particles. In the W-boson-initiated jets, all the predictions are incompatible with the measurement. In the top quark initiated jets, disagreement with all predictions is observed in smaller subregions of the plane, and with a subset of the predictions across the fiducial plane. The measurement could be used to improve the tuning of Monte Carlo generators, for better modelling of hadronic decays of heavy quarks and bosons, or to improve the performance of jet taggers.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2021

Selective Antisite Defect Formation in WS 2 Monolayers via Reactive Growth on Dilute W-Au Alloy Substrates

Defects are ubiquitous in 2D materials and can affect the structure and properties of the materials and also introduce new functionalities. Methods to adjust the structure and density of defects during bottom-up synthesis are required to control the growth of 2D materials with tailored optical and electronic properties. In this study, the authors present an Au-assisted chemical vapor deposition approach to selectively form S W and S2 W antisite defects, whereby one or two sulfur atoms substitute for a tungsten atom in WS 2 monolayers. Guided by first-principles calculations, they describe a new method that can maintain tungsten-poor growth conditions relative to sulfur via the low solubility of W atoms in a gold/W alloy, thereby significantly reducing the formation energy of the antisite defects during the growth of WS 2 . The atomic structure and composition of the antisite defects are unambiguously identified by Z-contrast scanning transmission electron microscopy and electron energy-loss spectroscopy, and their total concentration is statistically determined, with levels up to ≈5.0%. Furthermore, scanning tunneling microscopy/spectroscopy measurements and first-principles calculations also verified these antisite defects and revealed the localized defect states in the bandgap of WS 2 monolayers. This bottom-up synthesis method to form antisite defects should apply in the synthesis of other 2D materials.

2D materials↗
DOE OSTI2023

Ionothermally Synthesized Nanoporous Ti 0.95 W 0.05 Nb 2 O 7 : a Novel Anode Material for High-Performance Lithium-Ion Batteries

Although TiNb 2 O 7 is regarded as a fast-rechargeable lithium-ion battery (LIB) anode material, the intrinsic poor electrochemical kinetics of TiNb 2 O 7 still dramatically impedes its development. Herein, an ionothermal synthesis-assisted doping strategy is proposed for the preparation of a new W 6+ -doped TiNb 2 O 7 material (Ti 0.95 W 0.05 Nb 2 O 7 ) with nanoporous structure (denoted as NPTWNO). The improved Li + diffusion coefficient of NPTWNO suggests that the ionic-liquid-templated nanoporous architecture improves the Li+ diffusion kinetics. The density functional theory computational study reveals that the doped W 6+ successfully boosts the electronic conductivity due to the narrowed conduction-valance bandgap resulted from charge redistribution, which is reflected by the electrochemical impedance spectroscopy data. With the simultaneously enhanced Li+ diffusivity and electronic conductivity, NPTWNO achieves fast-rechargeability in LIBs. So this work indicates the potential of ionothermal synthesis-assisted doping strategy on energy storage materials and offers NPTWNO material with promising electrochemical performance.

25 ENERGY STORAGE↗
DOE OSTI2024

Hadronic mono- W ' probes of dark matter at colliders

Particle collisions at the energy frontier can probe the nature of invisible dark matter via production in association with recoiling visible objects. We propose a new potential production mode, in which dark matter is produced by the decay of a heavy dark Higgs boson radiated from a heavy W' boson. In such a model, motivated by left-right symmetric theories, dark matter would not be pair produced in association with other recoiling objects due to its lack of direct coupling to quarks or gluons. We study the hadronic decay mode via W' → tb and estimate the LHC exclusion sensitivity at 95% confidence level to be 10 2 - 10 5 fb for W' boson masses between 250 and 1750 GeV.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2026

Search for a Higgs boson produced in association with a charm quark and decaying to a W boson pair in proton-proton collisions at $ \sqrt{s}=13 $ TeV

This paper presents a search for a Higgs boson produced in association with a charm quark (cH) which allows to probe the Higgs-charm Yukawa coupling strength modifier κ$_{c}$. Higgs boson decays to a pair of W bosons are considered, where one W boson decays to an electron and a neutrino, and the other W boson decays to a muon and a neutrino. The data, corresponding to an integrated luminosity of 138 fb$^{−1}$, were collected between 2016 and 2018 with the CMS detector at the LHC at a center-of-mass energy of $ \sqrt{s}=13 $ TeV. Upper limits at the 95% confidence level (CL) are set on the ratio of the measured yield to the standard model expectation for cH production. The observed (expected) upper limit is 1065 (506), corresponding to an observed (expected) constraint of |κ$_{c}$| < 211 (95). When combined with the previous search for cH in the diphoton decay channel of the Higgs boson, the limits are interpreted as observed (expected) constraints at 95% CL on the value of κ$_{c}$, |κ$_{c}$| < 47 (51).[graphic not available: see fulltext]

Hayrapetyan, Aram [Yerevan Phys. Inst.]↗
DOE OSTI2021

Theoretical level energies, radiative lifetimes and transitions in W IX

The atomic states of the W IX (W{sup 8+}) tungsten ion lying below the W{sup 9+} ionisation threshold have been studied theoretically, employing the multiconfiguration Dirac–Hartree–Fock method with configuration interaction. The level electronic structures and their energies are presented. The electric dipole (E1), magnetic dipole (M1), electric quadrupole (E2), and magnetic quadrupole (M2) radiative transitions have been computed in order to calculate the radiative lifetimes of given states. Transition wavelengths, energies, and decay rates are also presented for selected high-intensity E1 transitions. The configuration interaction method was applied to estimate electron correlation effects. The aim of the present research was to fill a lack of atomic data for low-charged tungsten ions, which may be useful in low-temperature plasma diagnostics and may form the base for collisional–radiative modelling of spectra for low-charged tungsten ions.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2024

Effects of neutron irradiation on hydrogen isotope permeation on W-Re

Hydrogen and deuterium permeation behavior for neutron damaged W and W-3 %Re was evaluated using a Plasma Driven Permeation device. For neutron damaged W-3 %Re at 773 K and 1473 K, precipitation of Re and Os was observed by atom probe tomography. Neutron irradiation introduced defect damage throughout the sample and enhanced H and D diffusion toward downstream side. The existence of irradiation damage by neutron irradiation was found to increase hydrogen isotope permeation. Moreover, the existence of Re has suppressed the formation of irradiation defects for hydrogen isotope trapping sites. Further, the recovery of irradiation defects by increasing the irradiation temperature led to the structural changes due to the diffusion of Re and Os, which also affected the hydrogen isotope permeation behavior.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2025

Crystal structure and magnetic properties of CeFe 11 M (M = Mo, W)

Tetragonal CeFe 11 Mo (struct. type ThMn 12 , a = 8.529(1) Å, c = 4.766(1) Å, V = 346.68(1) Å 3 ) and novel isostructural CeFe 11 W (a = 8.539(1) Å, c = 4.754(1) Å, V = 346.62(1) Å 3 ) are obtained in bulk, as homogenized single-phase arc-melted alloys. Here, their crystal structures are evaluated by full profile Rietveld analysis of the powder X-ray diffraction patterns which confirm that Ce occupies the 2a atomic site in both cases, whereas atomic disorder is present in the Fe-sublattice, i.e., predominantly on the dumbbell 8i site and minorly on two other sites 8j and 8f. In CeFe 11 Mo the third element, M, is mixed with Fe on the 8i dumbbell site and 8f atomic position, whereas in CeFe 11 W, M is mixed on the 8i and 8j Fe sites. In these bulk CeFe 12-x M x alloys the tetragonal structure persists at lower M content, x < 1 here, in comparison to known similar alloys, with x > 1. Because of the low M content, comparably higher values of mass magnetization and Curie temperature are achieved i.e., CeFe 11 Mo: ϭ s = 104 emu/g (14.7 µ B /f.u.), T c = 420 K and CeFe 11 W: ϭ s = 99 emu/g (16.5 µ B /f.u.), T c = 450 K. Magnetocrystalline anisotropy is uniaxial with anisotropy fields H a ∼ 14.5 and 16.5 kOe, respectively. Based on Curie temperature and magnetic anisotropy enhancements, using tungsten as the stabilizing dopant is more beneficial than molybdenum.

36 MATERIALS SCIENCE↗
DOE OSTI2023

Decay spectroscopy at the two-proton drip line: Radioactivity of the new nuclides 160 Os and 156 W

The radioactivity of $^{160}_{76}$Os 84 and $^{156}_{74}$W 82 that lie at the two-proton drip line has been measured in an experiment performed at the Accelerator Laboratory of the University of Jyväskylä. The 160 Os nuclei were produced using fusion-evaporation reactions induced by a beam of 310 MeV 58 Ni ions bombarding a 106 Cd target. The 160 Os ions were separated in flight using the recoil separator MARA and implanted into a double-sided silicon strip detector, which was used to measure their decays. The α decays of the ground state of 160 Os (Ε α = 7092(15) keV, t 1/2 = 97$^{+97}_{-32}$ μs) and its isomeric state (Ε α = 8890(10) keV, t 1/2 = 41$^{+15}_{-9}$ μs) were measured, allowing the excitation energy of the isomer to be determined as 1844(18) keV. These α-decay properties and the excitation energy of the isomer are compared with systematics. The α decays were correlated with subsequent decays to investigate the β decays of the ground state of 156 W, revealing that unlike its isotones, both low-lying isomers were populated in its daughter nuclide, 156 Ta. An improved value for the half-life of the proton-decaying high-spin isomeric state in $^{156}_{73}$Ta 83 of 333$^{+25}_{-22}$ ms was obtained in a separate experiment using the same experimental systems with a 102 Pd target. This result was employed to improve the precision of the half-life determined for 156 W, which was measured as 157$^{+57}_{-34}$ ms.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2022

A boundary-based approach to the multiscale microstructural characterization of a W-Ni-Fe tungsten heavy alloy

Here, a combination electron backscattered diffraction and transmission electron microscopy based approach has been implemented to study the effects of purposefully introduced anisotropy in a tungsten heavy alloy (WHA) through hot-rolling. Particular attention has been paid to changes in number and proportion of various boundary types from a quantitative standpoint; incorporating qualitative behavioral observations from prior analyses to generate experimentally-validated bases for the examination and application of a microstructure which exhibits an optimal balance of strength and ductility. It is asserted that a combination of increased temperatures during rolling and additional isothermal hold time for the post-rolling annealing steps may lead to a reduction in unfavorable textural components due to rolling in the W-phase and a decrease in premature fracture due to W-W microcracking respectively. This is expected to further increase the proportion of interphase boundaries and improve the ductility of these rolled structures, producing a superior rolled WHA microstructure.

36 MATERIALS SCIENCE↗
DOE OSTI2023

Hadronic uncertainties versus new physics for the W boson mass and Muon g – 2 anomalies

There are now two single measurements of precision observables that have major anomalies in the Standard Model: the recent CDF measurement of the W mass shows a 7σ deviation and the Muon g – 2 experiment at FNAL confirmed a long-standing anomaly, implying a 4.2σ deviation. Doubts regarding new physics interpretations of these anomalies could stem from uncertainties in the common hadronic contributions. We demonstrate that these two anomalies pull the hadronic contributions in opposite directions by performing electroweak fits in which the hadronic contribution was allowed to float. The fits show that including the g – 2 measurement worsens the tension with the CDF measurement and conversely that adjustments that alleviate the CDF tension worsen the g – 2 tension beyond 5σ. This means that if we adopt the CDF W mass measurement, the case for new physics in either the W mass or muon g – 2 is inescapable regardless of the size of the SM hadronic contributions. Lastly, we demonstrate that a mixed scalar leptoquark extension of the Standard Model could explain both anomalies simultaneously.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2023

Synthesis, crystal and electronic structures, linear and nonlinear optical properties, and photocurrent response of oxyhalides CeHaVIO 4 (Ha = Cl, Br; VI = Mo, W)

Four heteroanionic oxyhalides, CeClMoO 4 , CeBrMoO 4 , CeClWO 4 , and CeBrWO 4 , have been studied as multifunctional materials, which show a combination of good second harmonic generation (SHG) response and photocurrent signals. Millimeter-sized CeHaVIO 4 (Ha = Cl, Br; VI = Mo, W) crystals were grown by halide salt flux. The crystal structure of CeHaVIO 4 crystals was accurately determined by single-crystal X-ray diffraction. CeClMoO 4 , CeBrMoO 4 , and CeBrWO 4 are isostructural to each other, and crystallize in the acentric LaBrMoO 4 structure type. CeClWO 4 crystallizes in a new structure type with unit cell parameters of a = 19.6059(2) Å, b = 5.89450(10) Å, c = 7.80090(10) Å, and β = 101.4746(8)°. The bandgaps of CeHaVIO 4 fall into the range of 2.8(1)–3.1(1) eV, which are much smaller than those of isotypic LaHaVIO 4 (Ha = Cl, Br; VI = Mo, W) in the range of 3.9(1)–4.3(1) eV. The narrowing of bandgaps in CeHaVIO 4 originates from the presence of partially filled 4f orbitals of cerium atoms, which was confirmed by density functional theory (DFT) calculations. The moderate bandgaps make CeHaVIO 4 suitable for infrared nonlinear optical (IR NLO) applications. CeBrMoO 4 and CeBrWO 4 exhibit moderate SHG responses of 0.58× AGS and 0.46× AGS, respectively, and are both type-I phase-matching materials. Moderate SHG response, easy growth of crystals, high ambient stability, and type-I phase-matching behavior make CeBrMoO 4 and CeBrWO 4 great materials for IR NLO applications. CeHaVIO 4 films also exhibited good photocurrent response upon light radiation. Furthermore, this work demonstrates the rich structural chemistry of the REHaVIO 4 (RE = Y, La–Lu; Ha = Cl, Br; VI = Mo, W) family and the potential presence of more multifunctional materials.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2025

Combinatorial Deposition of Ultrathick Ta-W-Au-Bi High-Entropy Alloys for Next-Generation Hohlraums by Direct-Current Magnetron Sputtering

Hohlraum temperature calculations with the model by J. H. Hammer and M. D. Rosen predict a higher X-ray drive from Ta-W-Au-Bi high-entropy alloys compared to pure Au and recently developed Ta 4 Au and Au-Bi hohlraums. Here, we study the microstructure and properties of 25-75−µm-thick Ta-W-Au-Bi alloy films deposited via combinatorial direct-current magnetron sputtering. All of the films have promising physical properties, including high electrical resistivity, that satisfy the requirements for magnetically assisted inertial confinement fusion experiments. While porosity tends to increase with increasing Bi content, we also found that films with Bi content > 44 at. % exhibited densification close to the substrate/film interface and formed a single-phase alloy. In conclusion, these findings provide a potential path forward for the development of Ta-W-Au-Bi alloys for next-generation hohlraum materials.

Magnetron sputtering↗
DOE OSTI2020

Material mixing during fuzz formation in W and Mo

Helium-induced fuzz formation in tungsten (W) and molybdenum (Mo) is investigated for a range of sample exposure temperatures from 838 K–1075 K (He fluence = 3.4 × 10 25 m -2 and ion energy <39 eV). Thin films of Mo deposited on W substrates show mixing of the film and substrate materials in the fuzz after He plasma exposure, including at 838 K (i.e. below the typical temperature range at which fuzz forms in pure W). Finally, the amount of material mixing increases with exposure temperature due to the increase in bubble size, and leads to significant accumulation of the substrate material at the fuzz surface at the highest temperature investigated, further supporting fuzz growth from the fiber tip outwards by material transport up the fibers.

36 MATERIALS SCIENCE↗
DOE OSTI2022

Identifications of RR Lyrae Stars and Quasars from the Simulated Data of Mephisto-W Survey

We have investigated the feasibilities and accuracies of the identifications of RR Lyrae stars and quasars from the simulated data of the Multi-channel Photometric Survey Telescope (Mephisto) W Survey. Based on the variable sources light curve libraries from the Sloan Digital Sky Survey (SDSS) Stripe 82 data and the observation history simulation from the Mephisto-W Survey Scheduler, we have simulated the uvgriz multi-band light curves of RR Lyrae stars, quasars and other variable sources for the first-year observation of Mephisto W Survey. We have applied the ensemble machine learning algorithm Random Forest Classifier (RFC) to identify RR Lyrae stars and quasars, respectively. We build training and test samples and extract ~150 features from the simulated light curves and train two RFCs respectively for the RR Lyrae star and quasar classification. We find that, our RFCs are able to select the RR Lyrae stars and quasars with remarkably high precision and completeness, with purity = 95.4% and completeness = 96.9% for the RR Lyrae RFC and purity = 91.4% and completeness = 90.2% for the quasar RFC. In conclusion, we have also derived relative importances of the extracted features utilized to classify RR Lyrae stars and quasars.

(galaxies:) quasars: general↗