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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 181 records · Page 10
All sourcesNASA NTRSDOE OSTI
NASA NTRS1994

Theoretical studies of spectroscopic problems of importance for atmospheric radiation measurements

Many of the instruments used to deduce the physical parameters of the Earth's atmosphere necessary for climate studies or for pollution monitoring (for instance, temperature versus pressure or number densities of trace molecules) rely on the existence of accurate spectroscopic data and an understanding of the physical processes responsible for the absorption or emission of radiation. During the summer, research was either continued or begun on three distinct problems: (1) an improved theoretical framework for the calculation of the far-wing absorption of allowed spectral lines; (2) a refinement of the calculation of the collision-induced fundamental spectrum of N2; and (3) an investigation of possible line-mixing effects in the fundamental spectrum of CH4. Progress in these three areas is summarized below. During the past few years, we have developed a theoretical framework for the calculation of the absorption of radiation by the far wings of spectral lines. Such absorption due to water vapor plays a crucial role in the greenhouse effect as well as limiting the retrieval of temperature profiles from satellite data. Several improvements in the theory have been made and the results are being prepared for publication. Last year we published results for the theoretical calculation of the absorption of radiation due to the dipoles induced during binary collisions of N2 molecules using independently measured molecular parameters; the results were in reasonable agreement with experimental data. However, recent measurements have revealed new fine structure that has been attributed to line-mixing effects. We do not think that this is correct, rather that the structure results from short-range anisotropic dipoles. We are in the process of including this refinement in our theoretical calculation in order to compare with the new experimental data. Subtle changes in the spectra of CH4 measured by researchers at Langley have also been attributed to line-mixing effects. By analyzing the same spectral lines we have attempted to verify or rule out possible line-mixing mechanisms. Due to the complexity and richness of the spectrum of this highly symmetric molecule, as well as the small magnitude of the effects, a detailed first-principle calculation of the mixing is a difficult problem. Before such a program is undertaken it is important to glean as much information as possible concerning the possible mechanisms by a systematic analysis of the existing data.

Tipping, Richard H.↗
NASA NTRS2011

Photocatalytic Active Radiation Measurements and Use

Photocatalytic materials are being used to purify air, to kill microbes, and to keep surfaces clean. A wide variety of materials are being developed, many of which have different abilities to absorb various wavelengths of light. Material variability, combined with both spectral illumination intensity and spectral distribution variability, will produce a wide range of performance results. The proposed technology estimates photocatalytic active radiation (PcAR), a unit of radiation that normalizes the amount of light based on its spectral distribution and on the ability of the material to absorb that radiation. Photocatalytic reactions depend upon the number of electron-hole pairs generated at the photocatalytic surface. The number of electron-hole pairs produced depends on the number of photons per unit area per second striking the surface that can be absorbed and whose energy exceeds the bandgap of the photocatalytic material. A convenient parameter to describe the number of useful photons is the number of moles of photons striking the surface per unit area per second. The unit of micro-einsteins (or micromoles) of photons per m2 per sec is commonly used for photochemical and photoelectric-like phenomena. This type of parameter is used in photochemistry, such as in the conversion of light energy for photosynthesis. Photosynthetic response correlates with the number of photons rather than by energy because, in this photochemical process, each molecule is activated by the absorption of one photon. In photosynthesis, the number of photons absorbed in the 400 700 nm spectral range is estimated and is referred to as photosynthetic active radiation (PAR). PAR is defined in terms of the photosynthetic photon flux density measured in micro-einsteins of photons per m2 per sec. PcAR is an equivalent, similarly modeled parameter that has been defined for the photocatalytic processes. Two methods to measure the PcAR level are being proposed. In the first method, a calibrated spectrometer with a cosine receptor is used to measure the spectral irradiance. This measurement, in conjunction with the photocatalytic response as a function of wavelength, is used to estimate the PcAR. The photocatalytic response function is determined by measuring photocatalytic reactivity as a function of wavelength. In the second method, simple shaped photocatalytic response functions can be simulated with a broad-band detector with a cosine receptor appropriately filtered to represent the spectral response of the photocatalytic material. This second method can be less expensive than using a calibrated spectrometer.

Davis, Bruce A.↗
NASA NTRS2011

Numerical Prediction of Radiation Measurements Taken in the X2 Facility for Mars and Titan Gas Mixtures

Thermochemical relaxation behind a normal shock in Mars and Titan gas mixtures is simulated using a CFD solver, DPLR, for a hemisphere of 1 m radius; the thermochemical relaxation along the stagnation streamline is considered equivalent to the flow behind a normal shock. Flow simulations are performed for a Titan gas mixture (98% N2, 2% CH4 by volume) for shock speeds of 5.7 and 7.6 km/s and pressures ranging from 20 to 1000 Pa, and a Mars gas mixture (96% CO2, and 4% N2 by volume) for a shock speed of 8.6 km/s and freestream pressure of 13 Pa. For each case, the temperatures and number densities of chemical species obtained from the CFD flow predictions are used as an input to a line-by-line radiation code, NEQAIR. The NEQAIR code is then used to compute the spatial distribution of volumetric radiance starting from the shock front to the point where thermochemical equilibrium is nominally established. Computations of volumetric spectral radiance assume Boltzmann distributions over radiatively linked electronic states of atoms and molecules. The results of these simulations are compared against experimental data acquired in the X2 facility at the University of Queensland, Australia. The experimental measurements were taken over a spectral range of 310-450 nm where the dominant contributor to radiation is the CN violet band system. In almost all cases, the present approach of computing the spatial variation of post-shock volumetric radiance by applying NEQAIR along a stagnation line computed using a high-fidelity flow solver with good spatial resolution of the relaxation zone is shown to replicate trends in measured relaxation of radiance for both Mars and Titan gas mixtures.

Palmer, Grant↗
NASA NTRS1978

Microwave radiation measurements near the electron plasma frequency of the NASA Lewis bumpy torus plasma

Microwave emission near the electron plasma frequency was observed, and its relation to the average electron density and the dc toroidal magnetic field was examined. The emission was detected using a spectrum analyzer and a 50 omega miniature coaxial probe. The radiation appeared as a broad amplitude peak that shifted in frequency as the plasma parameters were varied. The observed radiation scanned an average plasma density ranging from 10 million/cu cm to 8 hundred million/cu cm. A linear relation was observed betweeen the density calculated from the emission frequency and the average plasma density measured with a microwave interferometer. With the aid of a relative density profile measurement of the plasma, it was determined that the emissions occurred from the outer periphery of the plasma.

Mallavarpu, R.↗
NASA NTRS1978

Microwave radiation measurements near the electron plasma frequency of the NASA Lewis Bumpy Torus plasma

Microwave emission near the electron plasma frequency of the NASA Lewis Bumpy Torus plasma has been observed, and its relation to the average electron density and the dc toroidal magnetic field was examined. The emission was detected using a spectrum analyzer and a 50-ohm miniature coaxial probe. The radiation appeared as a broad amplitude peak that shifted in frequency as the plasma parameters were varied. The observed radiation scanned an average plasma density ranging from 20 billion to 800 billion per cu cm. A linear relation was observed between the density calculated from the emission frequency and the average plasma density measured with a microwave interferometer. With the aid of a relative density profile measurement of the plasma, it was determined that the emissions occurred from the outer periphery of the plasma.

Mallavarpu, R.↗
NASA NTRS2005

Satellite Infrared Radiation Measurements Prior to the Major Earthquakes

This work describes our search for a relationship between tectonic stresses and increases in mid-infrared (IR) flux as part of a possible ensemble of electromagnetic (EM) phenomena that may be related to earthquake activity. We present and &scuss observed variations in thermal transients and radiation fields prior to the earthquakes of Jan 22, 2003 Colima (M6.7) Mexico, Sept. 28 .2004 near Parkfield (M6.0) in California and Northern Sumatra (M8.5) Dec. 26,2004. Previous analysis of earthquake events has indicated the presence of an IR anomaly, where temperatures increased or did not return to its usual nighttime value. Our procedures analyze nighttime satellite data that records the general condtion of the ground after sunset. We have found from the MODIS instrument data that five days before the Colima earthquake the IR land surface nighttime temperature rose up to +4 degrees C in a 100 km radius around the epicenter. The IR transient field recorded by MODIS in the vicinity of Parkfield, also with a cloud free environment, was around +1 degree C and is significantly smaller than the IR anomaly around the Colima epicenter. Ground surface temperatures near the Parkfield epicenter four days prior to the earthquake show steady increase. However, on the night preceding the quake, a significant drop in relative humidity was indicated, process similar to those register prior to the Colima event. Recent analyses of continuous ongoing long- wavelength Earth radiation (OLR) indicate significant and anomalous variability prior to some earthquakes. The cause of these anomalies is not well understood but could be the result of a triggering by an interaction between the lithosphere-hydrosphere and atmospheric related to changes in the near surface electrical field and/or gas composition prior to the earthquake. The OLR anomaly usually covers large areas surrounding the main epicenter. We have found strong anomalies signal (two sigma) along the epicentral area signals on Dec 21, five days prior to the Northern Sumatra quake compared to the reference field for December 2001-2004 periods. Our recent results support the hypothesis of a possible relationship between a thermodynamic processes produced by increasing tectonic stress in the Earth's crust and a subsequent electro-chemical interaction between this crust and the atmosphere/ionosphere.

Ouzounov, Dimitar↗
NASA NTRS1980

Simulation study of a geometric shape factor technique for estimating earth-emitted radiant flux densities from wide-field-of-view radiation measurements

Geometric shape factors were computed and applied to satellite simulated irradiance measurements to estimate Earth emitted flux densities for global and zonal scales and for areas smaller than the detector field of view (FOV). Wide field of view flat plate detectors were emphasized, but spherical detectors were also studied. The radiation field was modeled after data from the Nimbus 2 and 3 satellites. At a satellite altitude of 600 km, zonal estimates were in error 1.0 to 1.2 percent and global estimates were in error less than 0.2 percent. Estimates with unrestricted field of view (UFOV) detectors were about the same for Lambertian and limb darkening radiation models. The opposite was found for restricted field of view detectors. The UFOV detectors are found to be poor estimators of flux density from the total FOV and are shown to be much better as estimators of flux density from a circle centered at the FOV with an area significantly smaller than that for the total FOV.

Weaver, W. L.↗
NASA NTRS1982

Reassessment of net radiation measurements in the atmosphere of Venus

An analysis was performed of the possible error mechanisms which degraded the IR net flux measurements made by the three small atmospheric probes dispatched from the Pioneer Venus spacecraft. The larger errors began below 30 km, and caused the data to be inconsistent with previous estimates of the atmospheric opacity. Evaluations were made of the possible radiation field perturbations behind each probe, cloud particle deposition on the sensor windows, and thermal disturbances within the sensors because of gas flow through the window retainers. The gas flow through the retainers was identified as the most likely error source, and was demonstrated in laboratory tests. A strong Reynolds number dependence was also found. Radiative transfer calculations were performed to account for the errors, using the constraints defined by the tests. Upper and lower bounds were calculated for the true net flux for both day and night conditions.

Revercomb, H. E.↗
NASA NTRS2018

Shock Tube Radiation Measurements in Nitrogen

Spectrally and spatially resolved radiance has been measured in the Electric Arc Shock Tube (EAST) facility, with the aim of improving fundamental understanding of high enthalpy flows in pure nitrogen. These tests provide data to inform models used for simulations of high speed flight in nitrogen rich atmospheres, such as Earth or Titan. The experiments presented in this paper cover conditions from approximately 6 km/s to 11 km/s at an initial pressure of 0.2 Torr. A wide range of physics, with different degrees of non-equilibrium and nitrogen dissociation, are covered. The EAST data are presented in different formats for analysis and comparisons. These formats include the spectral radiance at equilibrium (where appropriate), the spatial dependence of radiance over defined wavelength ranges and the mean non-equilibrium spectral radiance (the so-called "spectral non-equilibrium metric"). All the information needed to simulate each experimental trace, including free-stream conditions, shock time of arrival (i.e. x-t) relation, and the spectral and spatial resolution functions, are provided. Equilibrium radiation calculations are shown as a reference. It is the intention of this paper to motivate code comparisons benchmarked against this data set.

shock tube↗
DOE OSTI2026

Surface Observations From Atmospheric Radiation Measurement Sites Constrain the Anthropogenic Contribution to Cloud Droplet Number

Uncertainty in anthropogenic forcing driven by aerosol-cloud interactions (aci) limits our ability to infer the sensitivity of the Earth system to forcing from historical records. The driver of aci is the change in cloud droplet number concentration (N d ) due to changes in aerosol serving as cloud condensation nuclei (CCN). Here, we combine a perturbed parameter ensemble run in a global Earth system model with observations of CCN and single-layer-cloud N d at surface sites in the Azores, the Southern Great Plains, and Ascension Island to provide a constraint on the anthropogenic contribution to present-day N d . These observational lines of evidence constrain the preindustrial to present-day change in N d to be between 11 and 43 cm −3 . This is consistent with the upper end of some previous estimates but has a higher minimum perturbation, pointing to a stronger historical aerosol cooling.

ARM↗