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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 181 records · Page 10
All sourcesNASA NTRSDOE OSTI
NASA NTRS2007

Atomic Data and Spectral Line Intensities for CA XVII

Electron impact collision strengths, energy levels, oscillator strengths and spontaneous radiative decay rates are calculated for Ca XVII. The configurations used are 2s(sup 2), 2s2p, 2p(sup 2), 2l3l', 214l' and 2s5l', with l = s,p and l' = s,p, d giving rise to 92 fine-structure levels in intermediate coupling. Collision strengths are calculated at seven incident energies (15, 30, 75, 112.5, 150, 187.5 and 225 Ry) for the transitions within the three lowest configurations corresponding to the 10 lowest energy levels, and five incident energies (75, 112.5, 150, 187.5 and 225 Ry) for transitions between the lowest five levels and the n = 3,4,5 configurations. Calculations have been carried out using the distorted wave approximation. Excitation rate coefficients are calculated as a function of electron temperature by assuming a Maxwellian electron velocity distribution. Using the excitation rate coefficients and the radiative transition rates of the present work, and R-Matrix results for the 2s2, 2s2p, 2p2 configurations available in the literature, statistical equilibrium equations for level populations are solved at electron densities covering the range of 10(exp 8)-10(exp 14)/cu cm at an electron temperature of log Te(K)=6.7, corresponding to the maximum abundance of Ca XVII. Spectral line intensities are calculated, and their diagnostic relevance L; discussed. This dataset will be made available in the next version of the CHIANTI database.

Bhatia, A.K.↗
NASA NTRS2010

K-shell Photoionization of Na-like to Cl-like Ions of Mg, Si, S, Ar, and Ca

We present R-matrix calculations of photoabsorption and photoionization cross sections across the K edge of Mg, Si, S, Ar, and Ca ions with more than 10 electrons. The calculations include the effects of radiative and Auger damping by means of an optical potential. The wave functions are constructed from single-electron. orbital bases obtained using a Thomas-Fermi-Dirac statistical model potential. Configuration interaction is considered among all states up to n = 3. The damping processes affect the resonances converging to the K-thresholds causing them to display symmetric profiles of constant width that smear the otherwise sharp edge at the photoionization threshold. These data are important for the modeling of features found in photoionized plasmas.

Witthoeft, M. C.↗
NASA NTRS2013

A Comprehensive X-Ray Absorption Model for Atomic Oxygen

An analytical formula is developed to accurately represent the photoabsorption cross section of atomic Oxygen for all energies of interest in X-ray spectral modeling. In the vicinity of the K edge, a Rydberg series expression is used to fit R-matrix results, including important orbital relaxation effects, that accurately predict the absorption oscillator strengths below threshold and merge consistently and continuously to the above-threshold cross section. Further, minor adjustments are made to the threshold energies in order to reliably align the atomic Rydberg resonances after consideration of both experimental and observed line positions. At energies far below or above the K-edge region, the formulation is based on both outer- and inner-shell direct photoionization, including significant shake-up and shake-off processes that result in photoionization-excitation and double-photoionization contributions to the total cross section. The ultimate purpose for developing a definitive model for oxygen absorption is to resolve standing discrepancies between the astronomically observed and laboratory-measured line positions, and between the inferred atomic and molecular oxygen abundances in the interstellar medium from XSTAR and SPEX spectral models.

supernova remnants↗
DOE OSTI2022

Updates and Validation for the n+ 63,65 Cu Cross Sections [Abstract]

The neutron induced total, elastic, and capture cross sections of 63,65 Cu isotopes were selected for evaluation in the resolved and unresolved resonance energy ranges by the National Criticality Safety Program to resolve discrepancies related to benchmark performance. This is especially evident for the series of ZEUS benchmarks in which copper is used as a reflector. Because copper is also used as structural material in both fission and fusion reactors, the need to address benchmark discrepancies linked to nuclear data deficiencies is a task of primary importance. The aim of this work is to describe the steps of evaluation work towards a consistent improvement of the benchmark performance. The R-matrix analysis with the SAMMY code focused on the 63 Cu(n,γ) reaction channel between 100-300 keV coupled to unresolved resonance region parameters up to 650 keV to fit average cross section data from a recent experiment. Due to the high sensitivity of many benchmarks to elastic scattering angular distribution data, especially for the 65 Cu isotope, the impact of these data was tested by generating Legendre coefficients from both resonance parameters and the Hauser-Feshbach model. Guided by the findings of Shaw et al., the performance of the current evaluation for 65 Cu was compared to that of ENDF/B-VII.1 and ENDF/B-VIII.0 by testing the reactivity coefficients corresponding to the validation suite of experimental criticality benchmarks for thermal, intermediate, and fast systems taken from the International Criticality Safety Benchmark Experiments Project Handbook. The benchmark performance is especially sensitive to 63 Cu(n,γ) and 65 Cu elastic scattering for neutron energies in the 100–500 keV region, whereas 100 keV is the upper limit of the resolved resonance region in the ENDF/B-VIII.0 evaluations for 63,65 Cu. The results highlight the need to handle the transition from the resolved resonance region to the high energy region carefully.

07 ISOTOPE AND RADIATION SOURCES↗
DOE OSTI2021

Progress on the reevaluation and validation of the n+233U neutron cross sections

The set of 233 U resonance parameters of the ENDF/B-VIII.0 nuclear data library was adopted from the previous ENDF/B-VII.1 evaluation using the external levels to update the thermal values. Adoption of IAEA 2017 thermal standards ( σ f = 533.0 ± 2.2 b, σ c = 44.9 ± 0.9 b, and ν ‾ tot = 2.487 ± 0.011 ) and of the IAEA-recommended thermal-neutron induced prompt fission neutron spectrum (PFNS) with average PFNS energy of 2.030 ± 0.013 MeV requires a re-evaluation of 233 U neutron cross sections in the resolved resonance region. A newly produced evaluation is being tested on benchmarks carefully selected from the Handbook of International Criticality Safety Benchmark Experiments (ICSBEP) which are highly sensitive to 233 U data. An important goal of this work was to eliminate the strong negative gradient of the calculated effective multiplication factors with respect to the epithermal fission fraction observed in the validation of the ENDF/B-VIII.0 library for those assemblies. A significant improvement in integral performance of critical 233 U solutions is observed for the newly proposed evaluation. Further work addressing the fast neutron region is needed.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗
DOE OSTI2022

Resolved Resonance Region Evaluation of n+ 140,142 Ce [Slides]

ORNL has completed new resolved resonance region (RRR) evaluations for 140,142 Ce, which were carried out using Reich-Moore formalism instead of MLBW. Lack of integral measurements makes validation difficult, but difference from Kadonis values suggest more investigation of capture cross section are warranted. The complete file (with updated File2 & File32) was submitted to NNDC repository for inclusion in next release of ENDF. Sponsor report and journal publication are in progress.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2020

Status of the RRR evaluations for 233,235 U and 239 Pu [Slides]

The presentation discusses the R -Matrix Analysis of 233 U, 235 U, and 239 Pu and how their interplay among PFNS, TNC, RRR, and neutron multiplicities has a significant impact on the benchmarks. The presentation also discusses the 233 U improved agreement on benchmarks, an additional investigation on the thickness of beryllium reflectors, work on URR (up to 40 keV) and/or extension of RRR (600 eV to 2 keV). Also discussed is how the 235 U progresses on understanding reactivity rates related to depletion calculations, improved agreement with measured (capture) data is quite insensitive to resolve the negative slope, and how the 239 Pu negative slope as a function of the temperature is not understood yet (bias over 2σ lower than measured).

07 ISOTOPE AND RADIATION SOURCES↗
DOE OSTI2020

Status of the RRR evaluations for 233,235 U and 239 Pu [Slides]

The presentation discusses the R -Matrix Analysis of 233 U, 235 U, and 239 Pu and how their interplay among PFNS, TNC, RRR, and neutron multiplicities has a significant impact on benchmarks. The presentation also discusses the 233 U improved agreement on benchmarks, an additional investigation on the thickness of beryllium reflectors, work on URR (up to 40 keV) and/or extension of RRR (600 eV to 2 keV). Also discussed is how the 235 U progresses on understanding reactivity rates related to depletion calculations, improved agreement with measured (capture) data is quite insensitive to resolve the negative slope, and how the 239 Pu negative slope as a function of the temperature is not understood yet (bias over 2σ lower than measured).

07 ISOTOPE AND RADIATION SOURCES↗
DOE OSTI2023

New Cross Section Measurements and Evaluations of Zirconium Isotopes [Slides]

This presentation gives a look to new cross section measurements and evaluations of Zirconium (Zr) isotopes. This lecture includes highlights of accomplishments made in 2022. Additionally, it explains the motivation for investigation, new measurements, and re-evaluation of the Zr isotopes. This presentation concludes with a preliminary evaluation result from RPI 90 Zr evaluation and preliminary results from Eigenvalue sensitivity study on Zr sensitive critical benchmark experiments.

07 ISOTOPE AND RADIATION SOURCES↗
DOE OSTI2024

Evaluations for Nuclear Criticality Safety Program 12 C, 139 La, minor actinides, 235 U [Slides]

For light nuclei, preliminary work extends the evaluation from 6.5 MeV to ~ 10 MeV. For 139 La, the team delivered full evaluation in fast region to ORNL, including covariances. For sup>235 U, RPI data simulations, the team performed simulations and showed some improvement for neutrons below 5 MeV. Some of the changes needed for more improvement might not be supported by the current format. Some of the changes above 12 MeV to account for the angular distribution of preequilibrium neutrons require a change in the PFNS evaluation procedure.

235U re-evaluation↗
DOE OSTI2020

Direct and Indirect Measurements for a Better Understanding of the Primordial Nucleosynthesis

The Big Bang Nucleosynthesis (BBN) model is a great success of nuclear astrophysics due to the outstanding agreement between observational and predicted light elements abundances. One exception, however, is the so-called “lithium problem.” In this context, experimental efforts to measure the relevant reactions have been brought to an increased level of accuracy in measuring primordial abundances, and the introduction of indirect methods has allowed researchers to overcome the natural limitations of direct measurements in the energy range of interest for BBN. Here we review the results obtained from the application of the Trojan Horse Method to some of the most influential reactions of the standard network, such as 2 H(d,p) 3 H, 2 H(d,n) 3 He, 3 He(d,p) 4 He, 7 Li(p,α) 4 He, and 7 Be(n,α) 4 He. The relevant cross sections have been then used as new inputs to a classical BBN code, resulting in important constraints that make suggestions for a possible solution for the lithium problem outside of nuclear physics.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2022

Phenomenological R -Matrix parameterization of direct, doorway, and compound nuclear reactions [Abstract]

Although formal expressions for scattering matrix accounting for direct, doorway, and compound nuclear (CN) resonant reactions have been derived several decades ago in both the transition ( T -)matrix formalism and the reactance ( K -)matrix formalism, the absence of corresponding expressions in phenomenological R -matrix formalism has limited the application of the latter to CN resonant reactions only. We remove this limitation by parameterizing direct, doorway, and CN resonant reactions in a phenomenological R -matrix scattering matrix, and provide a parameterization for a corresponding Reich-Moore approximation of eliminated capture channels. Direct reactions induce (previously neglected) mixing among the incoming or outgoing R -matrix channel wave functions, parameterized by real and orthonormal channel-rotation matrix, M , whereby the original scattering matrix U is transformed into M T UM . Any real and orthonormal matrix, M , can be equivalently expressed as e η , where η is a real and skew-symmetric 2 rotation-generating matrix that subsequently yields a more intuitive parameterization of eliminated direct capture reactions in Reich-Moore approximation. A phenomenological R -matrix parameterization of doorway reactions is inferred by equating the expression for reactance ( K -)matrix, given in terms of Brune’s alternative R -matrix parameterization, to a corresponding expression derived using Feshbach’s projection operator formalism. Assuming that all doorway states, just like CN states, are confined within spheres defined by R -matrix channel radii, a new R -matrix-like term induced by doorway states is gleaned, wherein each doorway state is parameterized by its energy, width, and the strength of its coupling to each CN state. Since a Reich-Moore approximation for retained-channel scattering matrix ought to approximate the effect of eliminated capture channels taking place via direct, doorway, or CN reactions, each of the three kinds of reactions contributing to the capture entails a corresponding Reich-Moore parameterization in a first-order approximation: direct contribution is parameterized by introducing finite diagonal elements of a retained-channel rotation-generating matrix, doorway contribution is parameterized by doorway capture widths, while CN contribution is parameterized by conventional Reich-Moore capture widths. We will present evidence of direct and doorway reactions observed in recent measurements of resolved resonance cross sections at the Gaerttner LINAC Center at Rensselaer Polytechnic Institute, and will outline a path for implementing this new R -matrix parameterization into the SAMMY nuclear data evaluation code.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2024

Implementation of Windowed Multipole into MCNP6.3

This work details the implementation of the Windowed MultiPole(WMP) method of generating cross sections into the monte carlo code MCNP6.3, the verification and validation performed, and potential future improvements to be implemented. Further, this work contextualizes WMP within the broader changes to how nuclear data is stored, iterated upon, and used that have been developing over the past decade.

97 MATHEMATICS AND COMPUTING↗