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DOE OSTI2022

Advanced Physics Models for Particle-Particle Interactions (UCD final report)

The LDRD "Advanced Physics Models for Particle-Particle Interactions” collaborative research with Professor Jennifer Sinclair Curtis and PhD student Chanh Nguyen at the University of California, Davis involved meso-scale, discrete element method (DEM) modeling of micron-sized particles impacting a substrate. Using DEM, physical insight into the details of particle response upon impact can be obtained. Such details provide the type of information necessary to enhance existing continuum or macro-scale simulation tools so that modeling for material strength and particle breakage models is based on particle physics versus empirical relationships. While molecular dynamics simulations of atoms can also provide physical insight into the particle response to impact, the scale of particles that are treated is on the order of angstroms, not microns. This study gives evidence to the ability of the DEM simulation technique to provide such fundamental, detailed insight for micron-sized particles as a function of particle properties and impact velocity.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

DOE OSTI2023

Agricultural Ice Nuclei at Southern Great Plains (AGINSGP) Field Campaign Report

The Agricultural Ice Nuclei at Southern Great Plains (AGINSGP) field campaign was conducted from April 4 to April 29, 2022, at the U.S. Department of Energy’s Atmospheric Radiation Measurement (ARM) SGP site in Oklahoma. The goal of this campaign was to improve understanding of the sources and variability of ice-nucleating particles (INPs) at the SGP site. To this end, the key objectives of the campaign were (1) to produce a high-quality data set including measurements of atmospheric INP concentrations and aerosol particle properties relevant to the sources of INPs; and (2) to conduct a residual characterization experiment including offline and online analysis of the physical and chemical characteristics of INPs sampled in ambient air at SGP.

54 ENVIRONMENTAL SCIENCES↗

DOE OSTI2024

Data From Experiments on Bubbling Fluidization of Zeolite in a Rectangular Bubbling Fluidized Bed

Fluidization experiments were conducted in a lab-scale rectangular bubbling fluidized bed with the objective of generating a high-quality dataset for model validation and artificial intelligence/machine learning (AI/ML) training. Zeolite was chosen as the bed material, and the fluidizing medium was air as supplied by a compressor. Three different flow rates at the inlet were chosen such that the particles were fluidized but not elutriated from the system. The test matrix involved randomization and replicates to provide uncertainty estimates as well as four different batches of zeolite as the bed material. The quantities of interest obtained from this study were statistics of differential pressures, interface heights, and particle velocities. Considering all the components of the elaborate test plan, the results obtained were consistent and reproducible. Characterization tests were performed to estimate particle properties including size, density, coefficient of friction, coefficient of restitution, and minimum fluidization velocity. In addition, the angle of repose from granular discharge experiments has been reported to account for rolling friction, though its effect on the overall process is expected to be negligible.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

DOE OSTI2022

EPCAPE – Proton Transfer Reaction Mass Spectrometer Field Campaign Report

The Eastern Pacific Cloud Aerosol Precipitation Experiment – Proton Transfer Reaction Mass Spectrometer (EPCAPE-PTRMS) campaign was created in response to the urgent need expressed by EPCAPE co-investigators for measurements of volatile organic compounds (VOCs) during the EPCAPE intensive operational period. A proton transfer reaction time-of-flight mass spectrometer (PTR-ToF-MS, model 8000, Ionicon Analytik) was deployed to Mt. Soledad, San Diego, California, on 15 May 2023 for the measurement of VOCs. The instrument was installed in the same Atmospheric Radiation Measurement (ARM) user facility guest container that the Smith group used for the EPCAPE – Ultrafine Particle Properties (EPCAPE-UPP) campaign. The Smith group provided the sample inlet and operated and maintained the instrument. A complete VOC mass spectrum was recorded every 10 sec, continuously. Calibrations using a traceable VOC mixture were performed onsite at the end of the campaign.

54 ENVIRONMENTAL SCIENCES↗

DOE OSTI2026

Measurements of TRACER pre-convective conditions and mesoscale circulations using small unmanned aircraft systems (sUAS)

Improved comprehension of the physical processes governing convective cloud formation and lifecycle are of critical importance for understanding and predicting future climate states. The influence of these clouds on the planetary energy budget, including on precipitation, is significant. Things are particularly complex in coastal regimes, where gradients in aerosol particle properties, localized circulations such as sea breezes, and large population centers are found. To date, numerical models struggle to accurately represent these critical clouds and are therefore challenged to provide a realistic view on the planetary energy budget. Through the proposed research, we deployed two uncrewed aircraft systems (UAS) equipped with a variety of instruments alongside sensors deployed by the US Department of Energy Atmospheric Radiation Measurement (ARM) program for the TRACER (Tracking Aerosol Convection Interactions Experiment) field campaign. The two small UAS platforms consisted of a CU RAAVEN fixed-wing airplane and an OU CopterSonde system, with the copter collecting frequent vertical profiles of thermodynamic and kinematic variables such as temperature, pressure, wind and humidity. At the same time, the fixed-wing captured horizontal gradients of these quantities and aerosol size distribution. These systems were deployed south of the Houston metro area, in an area that is impacted by the Gulf of Mexico sea breeze on a daily basis. These observations offer enhanced and complementary perspectives to those provided by the DOE ARM Mobile Facility (AMF) which is was deployed in southeast Houston, and an ancillary site in a more rural location west of the urban Houston area. Quality-controlled versions of the UAS data were collected and posted on the DOE ARM data archive after the conclusion of the campaign where they are accessible by the research community and general public. The UAS perspective offers revolutionary insight into key spatial and temporal effects that have not been evaluated previously.

54 ENVIRONMENTAL SCIENCES↗

NASA NTRS1967

The Zodiacal Light and the Interplanetary Medium

Photometric and meteor observations, scattering properties, particle collection and impact, solar wind, and origin and evolution of zodiacal light in interplanetary medium - conference

Weinberg, J. L.↗

NASA NTRS1974

Interpretation of the polarization of Venus

The linear polarization of sunlight reflected by Venus is analyzed by comparing observations with extensive multiple scattering computations. The analysis establishes that Venus is veiled by a cloud or haze layer of spherical particles. The refractive index of the particles is about 1.44 at 0.55 microns with a normal dispersion, the refractive index decreasing from about 1.46 at 0.365 microns to 1.43 at 0.99 microns. The cloud particles have a narrow size distribution with a mean radius of about 1 micron; specifically, the effective radius of the size distribution is approximately 1.05 microns and the effective variance is about 0.07. The particles exist at a high level in the atmosphere, with the optical thickness unity occurring where the pressure is about 50 mb. The particle properties deduced from the polarization eliminate all but one of the cloud compositions which have been proposed for Venus. A concentrated solution of sulfuric acid provides good agreement with the polarization data.

Hansen, J. E.↗

NASA NTRS1974

Nature of the Venus clouds as derived from their polarization

The linear polarization of sunlight reflected by Venus is analyzed by comparing observations with extensive multiple scattering computations. The analysis establishes that Venus is veiled by a cloud or haze layer of particles which have a narrow size distribution with a mean radius of about 1 micron. The refractive index of the particles is 1.44 at 0.55 micron wavelength with a small normal dispersion, the refractive index decreasing from the ultraviolet toward the infrared. The particles exist at a high level in the atmosphere, with the optical thickness unity occurring where the pressure is about 50 mb. The particle properties deduced from the polarization eliminate all but one of the cloud compositions which have been proposed for Venus. A concentrated solution of sulfuric acid provides good agreement with the polarization data.

Hansen, J. E.↗

NASA NTRS1975

Chemically Reacting One-Dimensional Gas-Particle Flows

The governing equations for the one-dimensional flow of a gas-particle system are discussed. Gas-particle effects are coupled via the system momentum and energy equations with the gas assumed to be chemically frozen or in chemical equilibrium. A computer code for calculating the one-dimensional flow of a gas-particle system is discussed and a user's input guide presented. The computer code provides for the expansion of the gas-particle system from a specified starting velocity and nozzle inlet geometry. Though general in nature, the final output of the code is a startline for initiating the solution of a supersonic gas-particle system in rocket nozzles. The startline includes gasdynamic data defining gaseous startline points from the nozzle centerline to the nozzle wall and particle properties at points along the gaseous startline.

Tevepaugh, J. A.↗

NASA NTRS1975

Planetary isophotes as a clue to aerosol characteristics

A study was conducted to see how much information could be extracted from the Mariner 9 Mars isophotes taken at a phase angle of approximately 60 deg. It was found that the Minnaert functions and both isotropic and Rayleigh scattering could easily be ruled out, and that it was essential to use forward-peaked phase functions, which were computed from Mie theory. Isophotes similar to those observed assuming a semi-infinite dust cloud with a considerable variation in particle properties and size distribution could be obtained, so long as the ratio of the multiply- to singly-scattered light was held within certain limits. These conditions are met by micron-sized, moderatly absorbing mineral grains whose mean size should not be much larger than a micron. It was also found that a dust cloud of finite optical thickness bounded from below by a Lambert ground would fit the isophote data.

Kattawar, G. W.↗

NASA NTRS1977

Planetary isophotes as a clue to aerosol characteristics

A study was made to see how much information could be extracted from the Mariner 9 Mars isophotes taken at phase angle roughly 60 deg. Minnaert functions and both isotropic and Rayleigh scattering could easily be ruled out, and it was essential to use forward-peaked phase functions computed from Mie theory. Isophotes similar to those observed are plotted assuming a semi-infinite dust cloud with a considerable variation in particle properties and size distribution, so long as the ratio of the multiply to singly scattered light is held within certain limits. These conditions are met by micron-sized, moderately absorbing mineral grains whose mean size should not be much larger than a micron. It was also found that a dust cloud of finite optical thickness bounded from below by a Lambert ground would fit the isophote data.

Kattawar, G. W.↗

NASA NTRS1980

A macroscopic profile of the typical quasi-perpendicular bow shock - Isee 1 and 2

A macroscopic examination of field and particle properties of the bow shock recorded on November 5, 1977, identified earlier as stable features by comparison of Isee 1 and 2 data, is presented. Attention is given to the extent to which the shock was in a typical state, and multidiagnostic observations are combined to define the shock profile. It is found that the shock profile offered several unanticipated structural features, which include a variable directional profile of the reflected proton group passing through the front, an electrostatic boundary effect associated with the reflected protons upstream, and an oscillatory buildup of proton thermalization behind the overshoot portion of the shock signature.

Greenstadt, E. W.↗

NASA NTRS1989

The grand unified photon spectrum: A coherent view of the diffuse extragalactic background radiation

The spectrum of diffuse extragalactic background radiation (DEBRA) at wavelengths from 10(exp 5) to 10(exp -24) cm is presented in a coherent fashion. Each wavelength region, from the radio to ultra-high energy photons and cosmic rays, is treated both separately and as part of the grand unified photon spectrum (GUPS). A discussion of, and references to, the relevant literature for each wavelength region is included. This review should provide a useful tool for those interested in diffuse backgrounds, the epoch of galaxy formation, astrophysical/cosmological constraints to particle properties, exotic early Universe processes, and many other astrophysical and cosmological enterprises. As a worked example, researchers derive the cosmological constraints to an unstable-neutrino spies (with arbitrary branching ratio to a radiative decay mode) that follow from the GUPS.

Ressell, M. Ted↗

NASA NTRS1991

Second coefficient of viscosity in air

Acoustic attenuation measurements in air were analyzed in order to estimate the second coefficient of viscosity. Data over a temperature range of 11 C to 50 C and at relative humidities between 6 percent and 91 percent were used. This analysis showed that the second coefficient of viscosity varied between 1900 and 20,000 times larger than the dynamic or first coefficient of viscosity over the temperature and humidity range of the data. In addition, the data showed that the molecular relaxation effects, which are responsible for the magnitude of the second coefficient of viscosity, place severe limits on the use of time-independent, thermodynamic equations of state. Compressible flows containing large streamwise velocity gradients, like shock waves, which cause significant changes in particle properties to occur during time intervals shorter than hundredths of seconds, must be modeled using dynamic equations of state. The dynamic model approach is described briefly.

Ash, Robert L.↗

NASA NTRS1991

Planetary ring studies

The following topics are covered: (1) characterization of the fine scale structure in Saturn's A and B rings; (2) ballistic transport modeling and evolution of fine ring structure; (3) faint features in the rings of Saturn; (4) the Encke moonlet; (5) dynamics in ringmoon systems; (6) a nonclassical radiative transfer model; and (7) particle properties from stellar occultation data.

Cuzzi, Jeffrey N.↗

NASA NTRS1992

Mars: Correcting surface albedo observations for effects of atmospheric dust loading

We have developed a radiative transfer model which allows the effects of atmospheric dust loading on surface albedo to be investigated. This model incorporates atmospheric dust opacity, the single scattering albedo and particle phase function of atmospheric dust, the bidirectional reflectance of the surface, and variable lighting and viewing geometry. The most recent dust particle properties are utilized. The spatial and temporal variability of atmospheric opacity (Tan) strongly influences the radiative transfer modelling results. We are currently using the approach described to determine Tan for IRTM mapping sequences of selected regions. This approach allows Tan to be determined at the highest spatial and temporal resolution supported by the IRTM data. Applying the radiative transfer modelling and determination of Tan described, IRTM visual brightness observations can be corrected for the effects of atmospheric dust loading a variety of locations and times. This approach allows maps of 'dust-corrected surface albedo' to be constructed for selected regions. Information on the variability of surface albedo and the amount of dust deposition/erosion related to such variability results. To date, this study indicates that atmospheric dust loading has a significant effect on observations of surface albedo, amounting to albedo corrections of as much as several tens of percent. This correction is not constant or linear, but depends upon surface albedo, viewing and lighting geometry, the dust and surface phase functions, and the atmospheric opacity. It is clear that the quantitative study of surface albedo, especially where small variations in observed albedo are important (such as photometric analyses), needs to account for the effects of the atmospheric dust loading. Maps of 'dust-corrected surface albedo' will be presented for a number of regions.

Lee, S. W.↗

NASA NTRS1992

The Martian dust cycle

Martian dust plays a key role in determining the current climate of Mars, and is suspected of having had a major influence on the evolution of the surface and the history of climatic conditions on the planet. From spacecraft and ground-based observations, some understanding has been acquired of the styles and frequency of dust motion in the atmosphere and at the surface, of atmospheric dust loading, dust particle properties, and their variability. Limited constraints have also been derived for the volumes and ages of some potential dust reservoirs on the surface. These data are adequate to frame questions about the seasonal and long-term cycles of dust of Mars. Additional data are needed to place quantitative constraints on components of these cycles, on their possible linkage to one another, and to draw conclusions from the dust budget about the climate history of Mars.

Kahn, R. A.↗

NASA NTRS2001

Evaluation of NCAR Icing/SLD Forecasts, Tools and Techniques Used During The 1998 NASA SLD Flight Season

Supercooled Large Droplet (SLD) icing conditions were implicated in at least one recent aircraft crash, and have been associated with other aircraft incidents. Inflight encounters with SLD can result in ice accreting on unprotected areas of the wing where it can not be removed. Because this ice can adversely affect flight characteristics of some aircraft, there has been concern about flight safety in these conditions. The FAA held a conference on in-flight icing in 1996 where the state of knowledge concerning SLD was explored. One outcome of these meetings was an identified need to acquire SLD flight research data, particularly in the Great Lakes Region. The flight research data was needed by the FAA to develop a better understanding of the meteorological characteristics associated with SLD and facilitate an assessment of existing aircraft icing certification regulations with respect to SLD. In response to this need, NASA, the Federal Aviation Administration (FAA), and the National Center for Atmospheric Research (NCAR) conducted a cooperative icing flight research program to acquire SLD flight research data. The NASA Glenn Research Center's Twin Otter icing research aircraft was flown throughout the Great Lakes region during the winters of 1996-97 and 1997-98 to acquire SLD icing and meteorological data. The NASA Twin Otter was instrumented to measure cloud microphysical properties (particle size, LWC (Liquid Water Content), temperature, etc.), capture images of wing and tail ice accretion, and then record the resultant effect on aircraft performance due to the ice accretion. A satellite telephone link enabled the researchers onboard the Twin Otter to communicate with NCAR meteorologists. who provided real-time guidance into SLD icing conditions. NCAR meteorologists also provided preflight SLD weather forecasts that were used to plan the research flights, and served as on-board researchers. This document contains an evaluation of the tools and techniques NCAR forecasters used to predict the location of SLD icing conditions during the winter of 1997-1998. The objectives of this report are to: (1) assess the tools used to forecast in-flight icing. (2) assess the success/failure rate of the forecasts, and (3) discuss suggested changes to forecast techniques.

Bernstein, Ben C.↗