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At least 181 records · Page 10

Development and Optimization of a Purification Process to Recover 99 Mo from Low-enriched Uranium

Supported by the DOE-NNSA Office of Material Management & Minimization (M3), a number of domestic entities are pursuing non-highly enriched uranium (non-HEU) production of 99 Mo. As the production technologies of 99Mo pivot toward low-enriched uranium (LEU) or molybdenum targets, new reaction channels and accelerators are being evaluated. Superconducting electron linear accelerators (LINACs) with high-Z converter targets can generate bremsstrahlung photons and neutron fluxes that are capable of inducing photonuclear reactions and LEU fission. A particular advantage of a LINAC is that it does not rely on HEU-fueled reactor cores (which are currently slated for LEU conversion) and can operate on an almost continuous basis. Regarding the chemical purification of 99 Mo from irradiated uranium targets under acidic digestion, there exists a procedure known as Cintichem or modifications thereof with respect to LEU (LEU Modified Cintichem process, LMC). The process relies on a number of selective precipitation steps and column chromatography to purify Mo. It is important to note that LMC prescribes the addition of stable Mo to carry 99 Mo on alpha benzoin oxime, which reduces the specific activity of 99 Mo. This is especially important for processing 99 Mo batches with lower activities (~33 Ci of 99 Mo per batch).

07 ISOTOPE AND RADIATION SOURCES↗

Metal Bellows Valve Reliability Testing - Copper Stem Tip Testing

SRNL was funded in Mid-Year FY20 by NNSA NA-231 to continue evaluation of alternate valves for use in tritium service to support domestic Mo-99 production. The focus of the effort was to identify valve cycle life as a function of actuator size and stem tip material. Using the minimum size actuator to reliability open and close valves can reduce glovebox size and thus support domestic companies to “come to market” faster in supplying Mo-99 to the US market. This report serves as a continuation to the FY19 report and summarizes the task activities completed in FY20 after authorization to start work was obtained on May 5 th , 2020. Copper stem tips were tested on the Swagelok 1C and 5C actuated metal bellows valves. With ambitions to cycle each set 150,000 times, both 1C and 5C valves were met with high failure rates. The smaller 1C actuated valves required additional closing pressure to form a seal with the Cu stem tips installed however, excessive stem tip deformation may be the root cause of the majority of the valves failing before 500 cycles. The larger 5C actuated valves were cycled 150,000 times but still resulted in 80% failure rate, suspected of metal fatigue in the bellows due to high cycling frequencies.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Los Alamos National Laboratory Floodplain Assessment for the West Road Maintenance Project

The National Nuclear Security Administration (NNSA), a semi-autonomous agency within the U.S. Department of Energy (DOE), is proposing to take action at Los Alamos National Laboratory (LANL) and do maintenance on West Road at locations along its entirety from the intersection with West Jemez Road/New Mexico State Road 501 (NM 501) to the intersection with Dulce Street through Los Alamos Canyon. The proposed West Road Maintenance Project is intended to improve vehicular and pedestrian safety on West Road by reducing traffic hazards associated with poor road conditions and unsafe roadside parking. Proposed road maintenance and improvement activities throughout the length of West Road include asphalt milling and resurfacing of approximately 2.06 miles (mi.) of the road. West Road crosses approximately 0.35 mi. (1,900 feet (ft.)) of the Los Alamos Canyon floodplain at the bottom of Los Alamos Canyon. Project activities within the floodplain include: 1) mill and resurface the roadway, 2) replace existing guardrails, 3) block access to the informal roadside parking along either side of West Road in Los Alamos Canyon, 4) install trail signage and perform trail maintenance, and 5) restore habitat and reduce wildland fire risk through invasive species removal.

54 ENVIRONMENTAL SCIENCES↗

High Flux Isotope Reactor Low-Enriched Uranium Low Density Silicide Fuel Design Parameters

High Flux Isotope Reactor (HFIR) highly enriched uranium (HEU) to low-enriched uranium (LEU) conversion activities are ongoing as part of the Department of Energy (DOE) National Nuclear Security Administration (NNSA)’s nuclear nonproliferation mission. Design activities studying the conversion of HFIR from HEU to LEU fuel explored different fuel design features and shapes with a low density uranium-silicide dispersion (U 3 Si 2 -Al) fuel, which has a uranium density of 4.8 gU/cm 3 . The goal of these studies is to generate several HFIR LEU fuel designs of varying fuel fabrication complexity that meet the current HEU performance metrics and safety requirements. The documented designs will serve as references for fuel fabrication and qualification activities. Recent advancements in modeling and simulation tools enable quick prototyping of fuel designs. Shift, a Monte Carlo neutron transport and depletion tool optimized for high-performance computing (HPC) architectures, is used for efficient fuel cycle and performance metrics calculations. The HFIR Steady State Heat Transfer Code (HSSHTC) is used to vet the thermal safety margin. Also, a new automation tool that connects all fuel design analysis steps, named Python HFIR Analysis and Measurement Engine (PHAME), has been developed to expedite the design study in an efficient and reproducible manner. Leveraging these tools, several candidate fuel designs were selected for varying fabrication complexity. This report provides design feature details for four selected HFIR LEU low density U 3 Si 2 -Al fuel designs and their corresponding performance and safety metrics. Nominal, best-estimate design parameters and irradiation conditions, including fission rate densities, power densities, heat fluxes, and cumulative fission densities are provided for candidate fuel designs relevant to framing irradiation experiments to support fuel qualification efforts. Simulations show that the low density U 3 Si 2 -Al, with design features to enhance safety, can meet HEU core performance metrics and safety requirements if the reactor power is increased from 85 MW (HEU) to 95 MW (LEU) and if the active fuel length is increased from 50.80 cm (HEU) to 55.88 cm (LEU).

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

FY2020 LDRD Annual Report

The Laboratory Directed Research and Development (LDRD) program funds scientific efforts to build upon the unique knowledge base of Savannah River National Laboratory (SRNL). The program yields foundational scientific research and development (R&D) essential to SRNL’s core business areas, while aligning optimally and continuously with SRNL’s Strategic Plan and providing long-term benefits to DOE and the National Nuclear Security Administration (NNSA), other customers, and stakeholders. While fiscal year (FY) 2020 presented unprecedented challenges due to the COVID-19 global pandemic, the SRNL research team continued to advance science and further technology through the support of the LDRD program.

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Assessment of Modeling and Nuclear Data Needs for Active Neutron Interrogation

This document is the primary deliverable for a scoping study proposed to DOE National Laboratory Announcement Number LAB 19-2114 in the NNSA research area. The study supports user applications employing active neutron interrogation by providing a science plan to improve the modeling capability and the nuclear data that radiation transport codes use. Users rely on the accuracy of the elastic scattering and non-elastic cross-sections spanning thermal energies to 14 MeV (and higher in some cases) for modeling the neutron transport through complex geometries of materials potentially composed of many elements. While the elastic scattering cross-section data are accepted for all commonly occurring elements, the non-elastic cross-section data and the associated emission data include reaction channels that require attention. The study focused on the non-elastic reactions that emit secondary, also known as prompt, gammas with the premise that many users would benefit from improved modeling of these reactions. Many users develop material assay technologies based upon gamma signatures from radiative capture, inelastic scattering, and reactions on low-Z isotopes emitting multiple particles, so the nuclear data gaps, modeling deficiencies, and recommendations for addressing the shortfalls were assessed for these reactions. Fission gammas were excluded from this study because there are other efforts underway to address known shortfalls. Follow-on efforts that successfully execute the recommendations will tangibly improve to the ability to model gamma signatures and backgrounds for user applications, such as controlled substance detection, oil-well logging, and space exploration.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Systems Engineering Approach for Design and Implementation of a Gas Breech for Actinide Experiments at the JASPER Facility

The Joint Actinide Shock Physics Experimental Research (JASPER) Facility is located approximately 65 miles north of Las Vegas, Nevada at the Nevada National Security Site (NNSS). The primary mission is to conduct shock physics research on actinide materials in support of NNSA’s Stockpile Stewardship Program. JASPER experiment uses a two-stage light gas gun to accelerate projectiles into targets at velocities up to 8 km/s (17,000 mph). The first stage uses an ignited propellent to drive a piston to compress gas in the pump tube. At the second stage, the gas compression exceeds a specified pressure and a rupture valve at the end of the pump tube opens. This launches a projectile to impact the target. The target is housed inside the target assembly and the debris field is contained inside the primary target chamber (PTC). The PTC is placed inside the secondary confinement chamber (SCC) as an added protection against possible contamination. These major components are illustrated in Figure 1.JASPER is capable of generating and measuring data on the properties of radioactive chemical elements at high shock pressures, temperatures, and strain rates approximating the conditions in nuclear weapons by using a two-stage gas gun. The data is used to determine material equations-of-state and validate computer models of material response. The work advances predictive capability, thus ensuring confidence in the nuclear stockpile.

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AMPP Newsletter (Jun 2021)

Welcome to our June 2021 issue of the AMPP newsletter. I hope the information you find within this newsletter allows you, as either a new addition to AMPP or as a long-term AMPP family member, to gain a better understanding of our organization and how we are working to meet not just our mission deliverables of today, but preparing for our future. In this newsletter issue the articles are dedicated to the principle of how we do work is as important as what we do. AMPP is known for excellence in our NNSA and DOE Missions execution. In this issue we are highlighting our Heat Source Final Assembly (HSFA) manufacturing efforts. Although what we produce for our HSFA customer is important their faith in us as an organization is just as much based on how we perform work to ensure that we safely and securely produce a quality product. We have added a new section to the newsletter called the “Group Leader Corner” where in this issues Chasity Kolar, the Group Leader for AMPP-3, discusses what it means to have a questioning attitude.

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Request for Proposal: MSI Workforce Program Funding Opportunity

Los Alamos National Laboratory is a multidisciplinary research institution engaged in strategic science on behalf of national security. The Laboratory strives to enhance national security and make the world safer through research and advances in innovative science and technology. The Lab inspires the talent of its workforce and the region to solve problems related to defense, energy, environment, infrastructure, health, and global security concerns. LANL currently employs 11,700 and anticipates hiring 1000 plus people this year. The LANL mission is critical to meeting military requirements to ensure the U.S. nuclear deterrent is modern, responsive, and resilient. LANL is designated by NNSA as the nation’s Plutonium Center of Excellence. LANL has an experienced and skilled workforce, high-hazard nuclear facilities and associated infrastructure, and unique plutonium processing, fabrication, and experimental capabilities.

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NNSA/CEA Workflow Workshop Report 2021

Researchers from three NNSA labs plus CEA recently met for a half-day workshop on scientific and engineering workflows in March of 2021. Tools, projects and use cases from each institution were described. A wide range of unique capabilities and requirements were represented. The workshop highlights the fact that the CEA/NNSA workflows space mirrors the broader open science workflows community, with multiple technologies under development in a number of science domains and under a number of funding streams, with differing capabilities and focuses. Despite the number of tools, presentations and discussions have shown that these tools cover specific mission spaces at the four labs, each with distinctive capabilities that do not completely overlap with each other. We believe there is a strong interest in the short term for sharing lessons learned and collaborating on benchmarks and site evaluation of projects. This report, prepared by the NNSA/CEA Workflows Working Group, briefly summarizes the presentations in the areas of domain specific workflows, end user environments, data management, job and resource management, and infrastructure, and then identifies six broad areas for potential collaboration. A key finding is that users could benefit from greater interoperability, compatibility, and composability of the workflow technologies under development and that point-to-point collaboration opportunities should be identified to explore these aspects.

97 MATHEMATICS AND COMPUTING↗

Soil Sampling Results for Closure of a Portion of Solid Waste Management Unit #16

The U.S. Department of Energy/National Nuclear Security Administration (DOE/ NNSA) and National Technology & Engineering Solutions of Sandia, LLC (NTESS), the management and operating contractor for Sandia National Laboratories/California (SNL/CA), has prepared this soil sampling results report for closure of a portion of Solid Waste Management Unit (SWMU) #16. The entire network of SNL/CA sanitary sewer lines, including building laterals, was identified as SWMU #16 under a Resource Conservation and Recovery Act (RCRA) Facility Assessment conducted for SNL/CA in April 1991 (DOE 1992). Along with the previous SWMU #16 investigation results (SNL/CA 2019), the results of this investigation are intended to support closure decisions by the San Francisco Bay Regional Water Quality Control Board (RWQCB), as discussed below. SNL/CA personnel completed upgrading its sanitary sewer discharge network in 2019. These upgrades included installing new sections of underground lines and decommissioning certain sections of the old piping system by capping in place. To date, several sections of the sewer line have been abandoned-in-place by capping as new sewer lines were installed or flow was rerouted to other existing lines. To formally close these abandoned sections of the sewer line, the RWQCB required that SNL/CA personnel collect soil samples to be analyzed for contaminants potentially released from the sewer lines. SNL/CA personnel hired Weiss Associates (Weiss) of Emeryville, California to prepare a sampling and analysis plan, implement the sampling plan and report the results of the investigation under Purchase Order #2166257. The Sampling and Analysis Plan for Partial Closure of Solid Waste Management Unit #16 (SAP) was submitted to the RWQCB on August 14, 2020 by Weiss on behalf of SNL/CA. The RWQCB approved the SAP on September 30, 2020 after Weiss updated the method detection limit and reporting limits for total polychlorinated biphenyls (PCBs) and individual aroclors. Soil sampling was conducted in accordance with the SAP except that fewer locations were sampled due to site constraints, as discussed below. This report presents the results of the sampling effort and documents all associated field activities including borehole clearing, soil sample collection, storage and transportation to the analytical laboratories, borehole backfilling and surface restoration, and storage of investigation-derived waste (IDW) for future profiling and disposal by SNL/CA waste management personnel.

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Gleaming new facility delivers expertise now and into the future

On Tuesday, July 27, leadership from the Prototype Fabrication (PF) division welcomed a band of machinists, managers, project managers, members of Lab leadership, and NNSA to celebrate the official opening of a facility like no other at the Laboratory, and unique across the globe. The Mark Quality Manufacturing Center (MQMC) was developed throughout 2020 in support of weapons production capabilities, and is the Lab’s new home for high-precision non-nuclear components manufacturing. Work has been occurring there for several months, but with pandemic restrictions easing, it was finally time to celebrate.

45 MILITARY TECHNOLOGY, WEAPONRY, AND NATIONAL DEF↗

Towards Predictive Plasma Science and Engineering through Revolutionary Multi-Scale Algorithms and Models (Final Report)

This report describes the high-level accomplishments from the Plasma Science and Engineering Grand Challenge LDRD at Sandia National Laboratories. The Laboratory has a need to demonstrate predictive capabilities to model plasma phenomena in order to rapidly accelerate engineering development in several mission areas. The purpose of this Grand Challenge LDRD was to advance the fundamental models, methods, and algorithms along with supporting electrode science foundation to enable a revolutionary shift towards predictive plasma engineering design principles. This project integrated the SNL knowledge base in computer science, plasma physics, materials science, applied mathematics, and relevant application engineering to establish new cross-laboratory collaborations on these topics. As an initial exemplar, this project focused efforts on improving multi-scale modeling capabilities that are utilized to predict the electrical power delivery on large-scale pulsed power accelerators. Specifically, this LDRD was structured into three primary research thrusts that, when integrated, enable complex simulations of these devices: (1) the exploration of multi-scale models describing the desorption of contaminants from pulsed power electrodes, (2) the development of improved algorithms and code technologies to treat the multi-physics phenomena required to predict device performance, and (3) the creation of a rigorous verification and validation infrastructure to evaluate the codes and models across a range of challenge problems. These components were integrated into initial demonstrations of the largest simulations of multi-level vacuum power flow completed to-date, executed on the leading HPC computing machines available in the NNSA complex today. These preliminary studies indicate relevant pulsed power engineering design simulations can now be completed in (of order) several days, a significant improvement over pre-LDRD levels of performance.

42 ENGINEERING↗

ADAM Program Execution Plan LANL Inputs (FY2022)

The National Security Research Center (NSRC) is Los Alamos National Laboratory’s classified library. There are two groups associated with the NSRC, both of who work for LANL’s Weapons Research Services (WRS) division (WRS-SIS and WRS-WMT). These groups are funded in part by the NNSA Archives Program. The NSRC’s collections include tens of millions of documents from the Manhattan Project era through today. It is staffed with an expert, highly trained staff of librarians, archivists, digitizers, historians, and communications specialists. The NSRC traces its lineage to the wartime Technical Library created by J. Robert Oppenheimer during in 1943. Today, it supports a broad range of researchers within the LANL Weapons Program and beyond. The NSRC also has customers across other National Nuclear Security Administration labs and sites, and partners in the Department of Defense. This report highlights LANL accomplishments through NSRC.

45 MILITARY TECHNOLOGY, WEAPONRY, AND NATIONAL DEF↗

Atomic Ejecta Source Optical Probe (AESOP) (L3 Milestone Report FY2021 Work Package)

As part of its mission to ensure the reliability of the nation's nuclear weapons stockpile, the NNSA has funded a broad range of projects to characterize the mass of material ejected from shocked metal surfaces with special emphasis placed on determining the size distribution of macroscopic "ejecta" particles. Substantial work has been done for particles with diameters down to roughly 1 μm, but little data is available for smaller particles, and no data exist for the amount of atomic-scale ejecta produced in such dynamic environments. Such data are important due to the implications for weapons systems behavior but also for distinguishing between different potential ejecta production mechanisms, such as Rayleight-Taylor instability or the shallow-bubble-collapse phenomenon recently proposed by G. Maskally.

36 MATERIALS SCIENCE↗

Nuclear Enterprise Science & Technology (NEST) [Slides]

The NEST Certificate Program is designed to provide students with the skills and experience to qualify for entry-level positions in nuclear facilities as Fissile Material Handler and/or Glovebox Operator. The program goal is to provide for a technically qualified workforce who can execute a variety of programmatic work in modern nuclear materials handling and processing facilities. The program is designed to be completed in a minimum of 1 year (2 semesters) of university level courses (30 credit hours). A certificate will be offered and awarded through the University of New Mexico – Los Alamos (UNM-LA). NEST is unique in that it is an immersive education program. The NNSA-required training for nuclear material handlers and fissionable material handlers has been cross-walked with the educational Core Curricula. Academic content will be delivered that provides background scientific and engineering understanding of the fundamental concepts behind this training. It will be offered as a Pilot Program to an incumbent cohort to ensure that the Certificate meets programmatic needs. NEST is modelled after a Wharton County Junior College (Texas) program to attract and produce nuclear reactor operators.

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Development of a Neutron List Mode Collar (LMCL) and a List Mode Response Matrix Analysis Concept

This report was prepared for the Safeguards Program of the US Department of Energy’s (DOE’s) National Nuclear Security Administration (NNSA), Office of Defense Nuclear Nonproliferation Research and Development (DNN R&D). The report presents the development of the neutron nondestructive assay system, the List Mode Collar (LMCL) for the project OR16-List Mode for Collar-PD1La “List Mode Response Matrix for Advanced Correlated Neutron Analysis for Nuclear Safeguards.” The new list mode electronics developed under this project, and a spatial analysis concept called the List Mode Response Matrix are also described in this report. Analysis algorithms based on classification methods are published in a separate report. This research addresses the need to expand the capabilities of current nondestructive assay systems used for nuclear safeguards applications and considers the sustainability of safeguards technologies by the development of a “retrofit” concept using electronics based on modern standards. Furthermore, employing list mode data acquisition enabled the development of a spatial analysis concept and empirical measurement of a spatial response not previously used for safeguards neutron counting applications or measured in a traditional neutron collar detector and, therefore, provides new capability.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Safeguards Technology for Thorium Fuel Cycles: Research and Development Needs Assessment and Recommendations

This report presents Safeguards Technology for Thorium Fuel Cycles: Research and Development Needs Assessment and Recommendations prepared for the National Nuclear Security Administration (NNSA) Office of Defense Nuclear Nonproliferation Research and Development (DNN R&D) Safeguards Program by a multilaboratory team from Oak Ridge National Laboratory, Los Alamos National Laboratory, and Y-12 National Security Complex. It documents key findings of a 2-year scoping study on “Safeguards Technology Needs Assessment for Leading Thorium Fuel Cycles” (project OR18-V-SG Tec Needs Th Fuel Cycles-PD1Lb).

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