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At least 181 records · Page 10

IER 268 CED-3b Report

The goal of IER 268 was to collect information from the operation of the Godiva IV super-prompt critical assembly to support multi-physics modeling efforts. There were two types of systems deployed. One was a Photo-Doppler Velocimetry (PDV) system which used the reflection of laser light on the surface of the Godiva IV core. The other consisted of an MHD 240 detector with two other detectors (an MHD-241 and an Eljen EJ-325A) used for reference as the MHD-240 detector was moved. The collection is referred to as the MHD Detector in the narrative log. There were two types of Godiva operations performed to gather data. A series of super-prompt critical bursts were performed and data collected on both systems, tied to a common trigger. Separately, a series of delayed critical operations at various power levels was performed for a combination of MHD detector distances from Godiva and the presence and absence of a shield in the line of sight between Godiva and the MHD detector. This data was collected to determine the contribution of room return during the burst measurements.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Constrained Bayesian Optimization of Criticality Experiments [Slides]

The design of criticality experiments is typically an iterative process that employs a Monte Carlo transport code. The goal is to find a design that optimizes some variable, like the sensitivity of a response to a cross section, while simultaneously ensuring criticality. The high fidelity of the Monte Carlo code is a great asset, but it makes exploring the design space computationally expensive. Herein, we present how a constrained Bayesian optimization algorithm can be used to efficiently design a criticality experiment. It uses Gaussian processes as a surrogate model to probe the design space and to reduce the number of code executions that are needed to find the optimum. We demonstrate constrained Bayesian optimization with a Pu-239/polyethylene solution system and a TEX experiment that is designed for criticality safety validation of a nuclear waste model at the Hanford Site. For both systems, a global optimum was found within 75 Monte Carlo simulations.

42 ENGINEERING↗

Data Testing with Zero Power Reactor (ZPR), Zero Power Physics Reactor (ZPPR), and New Thermal Epithermal eXperiments (TEX) Plutonium Benchmarks [Slides]

This presentation states that new TSLs in ENDF/B-VIII.0 will reduce the overprediction of the library for the most moderated cases. The differences between VII.1 and VIII.0 are driven by the 239 Pu changes and are consistently higher for all configurations. The VIII.0 239 Pu thermal cross sections were specifically adjusted lower to better predict plutonium thermal solutions criticality benchmarks, yet they overpredict the TEX thermal configurations, moderated by PE. Other, smaller differences have been seen for 240 Pu and 56 Fe. PMM-002 has shown utility in testing cross sections over a wide range of neutron energies.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Constrained Bayesian Optimization of Criticality Experiments at LLNL [Slides]

The design of criticality experiments is typically an iterative process that employs a Monte Carlo transport code. The goal is to find a design that optimizes some variable, like the sensitivity of a response to a cross section, while simultaneously ensuring criticality. The high fidelity of the Monte Carlo code is a great asset, but it makes exploring the design space computationally expensive. Herein, we present how a constrained Bayesian optimization algorithm can be used to efficiently design a criticality experiment. It uses Gaussian processes as a surrogate model to probe the design space and to reduce the number of code executions that are needed to find the optimum. We demonstrate constrained Bayesian optimization with a Pu-239/polyethylene solution system and a TEX experiment that is designed for critical ity safety validation of a nuclear waste model at the Hanford Site. For both systems, a global optimum was found within 75 Monte Carlo simulations.

42 ENGINEERING↗

Application of the Cohn-alpha Method on Bare Highly Enriched Uranium Using Organic Scintillators [Poster]

The prompt neutron decay constant (α), can be used to calculate the lifetime of prompt fission chains within a multiplying system and verify reactor startup and shutdown. We analyze a fast, bare system consisting of highly enriched uranium (93% 235 U) hemisphere shells known as the Measurements of Uranium Subcritical and Critical (MUSiC). We measured the system with a three by-four array of organic scintillators (OSCAR) to obtain the gamma-ray and fast neutron signals. Pulse shape discrimination was used to isolate the neutron time series data. The Cohn-α method was used to estimate α for 3 supercritical measurements of Configurations 8 MUSiC. We use these estimates to linearly extrapolate α at delayed critical. These values can be compared to highly detailed simulations in MCNP6.2.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Equivalent Fundamental-Mode Source Simulations for Spherical Uranium and Plutonium Systems

It is important in neutron noise measurements and reactor startup to understand how the source distribution in a system compares to the equivalent fundamental-mode (EFM) source. Deviation from the fundamental mode source distribution increases as the system $\kappa$ eff increases. A correction factor, g *, is a measure of this deviation, and is the focus of this work. Two methods were utilized to simulate g *. These methods are compared to each other and (where applicable) previous results. The effects associated with nuclear material inner radius, materials of reflectors, and reflector thickness are also investigated.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Sensitivity Coefficients Calculated for the Prompt Neutron Decay Constant At or Near Delayed Critical

The derivation of a non-invasive prompt neutron decay constant sensitivity coefficient is provided in this work. The computation of the sensitivity coefficient derived in this work does not require modification of Monte Carlo source code and is based on capabilities available in Monte Carlo N-Particle R© Code Version 6.2. The prompt neutron decay constant sensitivity coefficients are calculated for 44-group and 252-group energy structures for specific nuclide-reaction pairs in the Jezebel benchmark experiment. The nuclide-reaction pairs investigated in this work include Pu- 239(n,f), Pu-240(n,f), and Pu-241(n,f). Physical explanations of the sensitivity profiles exhibited by the 252-group energy structure are investigated for the prompt neutron multiplication factor, mean neutron lifetime, and prompt neutron decay constant. The prompt neutron decay constant sensitivity coefficients calculated for the 44-group and 252-group energy structure of Pu-239(n,f) are compared. Lastly, the 44-group energy structure sensitivity coefficients calculated are used for nuclear-data induced uncertainty quantification of the neutron multiplication factor. This work shows that a reduction in the nuclear data-induced uncertainty of the neutron multiplication factor is possible for all nuclide-reaction pairs investigated when prompt neutron decay constant sensitivity coefficients are utilized. This is important for new critical experiment design optimization studies of measurement configurations. This work provides a basis for more detailed sensitivity analysis and uncertainty quantification of nuclide, reaction, and energy-specific cross section data.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Sensitivity Coefficients Calculated for the Prompt Neutron Decay Constant at or Near Delayed Critical [Abstract]

Experimenters at Los Alamos National Laboratory (LANL) measure the prompt neutron decay constant for many experiments at the National Criticality Experiments Research Center (NCERC) to infer reactivity and the effective neutron multiplication factor. These quantities are very important for nuclear criticality safety and validating nuclear data. Uncertainty in measures of criticality of an experimental configuration can be determined prior to physically performing the experiment by applying first order perturbation theory to Monte Carlo codes, such as MCNP®. The first order perturbation theory produces first derivatives of some nuclear parameter to nuclear data (e.g., cross section data). This first derivative is commonly referred to as a sensitivity coefficient. Currently, the MCNP® software has the capability of computing effective neutron multiplication factor sensitivity coefficients to cross section data. This work builds off of this MCNP® capability and the first order perturbation theory to provide a method of calculating sensitivity coefficients for the prompt neutron decay constant at or near delayed critical to cross section data. The prompt neutron decay constant sensitivity coefficient calculated in this work does not depend on any modification of the MCNP® source code. Prompt neutron decay constant sensitivity coefficient calculations can be used to infer reactivity and effective neutron multiplication factor sensitivity coefficient values as well. By investigating the trends of prompt neutron decay constant sensitivity coefficients for nuclide-reaction pairs across energy spectra, experiments can be designed to maximize or minimize the uncertainty in the prompt neutron decay constant in a particular energy region, which can lead to further optimization studies. Prompt neutron decay constant sensitivity coefficients will be calculated for the Jezebel benchmark. Subsequently, these sensitivity coefficients will be used in a data assimilation process to determine if there is or are optimal experiments that can be performed to provide insight into adjustments of uncertain/inaccurate cross section data. Specifically, the effect of the prompt neutron decay constant sensitivity coefficients on the nuclear data-induced uncertainty in the effective neutron multiplication factor will be examined

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Equivalent Fundamental-Mode Source Simulations for Spherical Uranium and Plutonium Systems [Abstract]

The equivalent fundamental-mode source refers to a “source” which is identically distributed in space, energy, and angle as that of a fundamental-mode fission source distribution. It has previously been shown that the system fixed source multiplication ($M_{fs}$) relates to the effective multiplication factor ($\kappa_{eff}$) as $M_{fs} = \frac{g^*}{1-k_{eff}}$ The term $\mathcal{g}$* therefore relates the system source distribution to the system equivalent fundamental-mode source. As previously shown, the $\mathcal{g}$* term is approximately 1 for deeply subcritical systems and then diverges as the system multiplication increases. For a system with a point source located in the center of an assembly (such a sphere), $\mathcal{g}$* will be greater than 1; this happens because there is a higher probability of induced fission when all of the starter neutrons originate from the center of the sphere. For a uniform source, $\mathcal{g}$* is less than 1, but does not diverge from 1 as dramatically as seen by a point source. One reason that $\mathcal{g}$* is an important parameter is that it is used in measurement methods to infer reactor kinetics parameters ($β_{eff}$ being one example). This work will discuss multiple ways to simulate $\mathcal{g}$* using MCNP®6.2, which include use of traditional methods versus a single input file method that was recently published. A discussion related to methods to simulate $M_{fs}$ will be presented. Spherical systems of Highly Enriched Uranium (HEU) will be compared with previous works. In addition, results of plutonium including multiple reflector materials will be investigated. Simulated systems will include both parametric studies as well as configurations used in recent experiments performed at the National Criticality Experiments Research Center (NCERC). These studies will include subtleties associated with system geometry that have not been previously shown. Last, this work will investigate the relationship between $\mathcal{g}$* and reactor kinetics parameters (such as $β_{eff}$).

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

High-Fidelity Measurements for Flattop-HEU Benchmark Reevaluation

Flattop was first built in the 1950’s at Los Alamos National Laboratory. Flattop-HEU is composed of a sphere of highly enriched uranium (HEU) surrounded by a thick spherical natural uranium (NU) reflector. The reflector is composed of three parts: a stationary hemisphere and two movable quarter spheres. For fine control of the reactivity of the system, there are three control rods of natural uranium located in voids in the stationary hemisphere. The final components that make Flattop a useful critical assembly are the glory hole and mass adjustment pieces. These pieces can be loaded in various configurations into the glory hole and the core pedestal to control the known worth of the system. The glory hole and mass adjustment pieces are mostly small pieces of HEU with some mass adjustment pieces fabricated from NU. This allows for the irradiation of samples to a specified level. To better document the system, Flattop was evaluated and included in the International Criticality Safety Benchmark Evaluation Project (ICSBEP) handbook. The original benchmark evaluation of Flattop-HEU was written in 1999 based on an experiment completed in the 1960’s. This original evaluation was written to provide a single diameter that defined critical mass; however, as computational capabilities have increased, the focus for benchmark evaluations has shifted to include detailed modelswith all physical dimensions. Thus, as Flattop is a lynchpin in critical experiment work, the benchmark is being reevaluated at current standards. This summary discusses some of the largest known uncertainties from the evaluation and the high-fidelity measurements taken to reduce these uncertainties.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Sensitivity Studies, Gap Analysis, and Benchmark Experiment Optimization for Reactor Applications

In regards to nuclear data, some reactor applications may lack validation experiments, which reduces confidence in predicted results. This is especially true for emerging advanced reactor, micro reactor, and Accelerator Driven System (ADS) designs. This work presents an approach to design new criticality experiments that have similar k eff cross section sensitivities to an application of interest. This process involves simulations to generate cross-section sensitivities to a parameter of interest (such as k eff ), a gap analysis to determine which existing benchmarks are most similar to the application, and an experiment optimization. This work focuses on cross-section sensitives and gap analysis for three examples relevant to the reactor physics community including a Travelling Wave Reactor (TWR) type-design, Kilopower (a space reactor design), and a lead-bismuth eutectic cooled accelerator-driven system (ADS) to transmute minor actinides.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

IER 501: Pulsed Neutron Die-Away Experiments at LLNL [Slides]

This presentation notes the purpose of Pulsed Neutron Die Away (PNDA) for Thermal Neutron Scattering Law (TSL) validation. PNDA for TSL validation does not require fissile material. It consists of simple target shapes and compositions and is only sensitive to absorption and scattering of target medium. Well conducted experiments have uncertainties of 0.1% - 0.5%. This presentation also covers Pulsed Neutron Die Away Experiments, while noting previous experiments such as the FY22 PNDA Experiments. The presentation concludes with FY23 benchmarking efforts and a timeline to FY24.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Future of the MUSiC Experiment Data

The Measurements of Uranium Subcritical and Critical (MUSiC) experiment was a highly enriched uranium (HEU) experiment performed at the National Criticality Experiments Research Center (NCERC) executed between December 2020 and April 2021. The experiment intended to measure criticality and reactor kinetics parameters in a bare HEU system. The experiment concurrently measured radiation signatures from the system while utilizing different neutron source types. This was an attempt to benchmark both detectors and analysis techniques against one another for identical measurements. The experiment consisted of the Rocky Flats HEU hemi-shells constructed into ten configurations spanning between deeply subcritical (about 14 kgs) to supercritical (about 60 kgs). Two of the ten configurations were supercritical and the other eight were subcritical. The two supercritical configurations, often referred to as the critical configurations, were documented into an International Criticality Safety Benchmark Evaluation Project (ICSBEP) benchmark evaluation and submitted to the technical review group (TRG). The subcritical configurations of the MUSiC experiment were examined using three different detection systems. The systems include: the NoMAD He-3 neutron detector which consists of 15 He-3 tubes surrounded by a polyethylene matrix, a liquid scintillator system called the Rossi-α Measurement Rapid Organic Discriminating Detector (RAM-RODD), and a trans-stilbene organic scintillator array (OSCAR) provided by the University of Michigan. The NoMAD and RAM-RODD data are planned to be evaluated in two separate ICSBEP evaluations utilizing neutron noise methods such as Feynman Variance-to-Mean, Rossi-α and the pulsed neutron source method. Each of the subcritical configurations were examined using three different source types including: a Cf-252 source in the center, with only the intrinsic neutron source in the HEU, and with an external D-T neutron generator.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

High Multiplication Neutron Noise Measurements Using the 7uPCX Assembly

The Seven Percent Critical Experiment, or 7uPCX, is a system that mimics the physics of light water nuclear reactor systems by using uranium dioxide fuel pins at an enrichment of approximately 7%. 7uPCX is often used for benchmarking and nuclear data purposes. As part of a collaboration between Lawrence Livermore National Laboratory, Los Alamos National Laboratory, Sandia National Laboratories, and the Institut de Radioprotection et de Sûreté Nucléaire, measurements were performed in support of a high-multiplication, subcritical benchmark candidate for a thermal system. The measurements were completed by making subcritical configurations using the fuel loading pattern of a well-documented configuration of the Seven Percent Critical Experiment at Sandia National Laboratories, which exists as a benchmark in the International Criticality Safety Benchmark Evaluation Project handbook. These measurements, which aimed to capture multiplications ranging from approximately 10 to 1,000, also serve as an intercomparison between both the fielded detector systems and analysis methodologies with the goal of better characterizing the detectors and their ability to capture the state of the criticality these types of systems. Los Alamos National Laboratory’s measurements for this collaboration were made with five linked helium-3 based neutron multiplicity detectors placed on the periphery of the reactor tank beyond the infinite reflector thickness of water, and four organic scintillators placed in dry-wells in-reactor near the edge of the upper fuel grid plate. This work captures the Los Alamos National Laboratory measurements, the Rossi-α and Feynman-Y results, provides an intercomparison between the results of the 3 He neutron detectors and the organic scintillators, compares to simulation where possible, and expands on future work.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

EUCLID: Experiments Underpinned by Computational Learning for Improvements in Nuclear Data [Slides]

EUCLID will design validation experiments optimized to resolve compensating errors and adjust nuclear data to experiments. A big part of the success of the EUCLID proposal was due to previous work supported by NCSP (MCNP, nuclear data, and NCERC capabilities). The work performed under EUCLID will similarly benefit the NCSP mission. It will lead to new MCNP capabilities, improved nuclear data and nuclear data capabilities, and new methodology and tools that will have large impact on future NCERC experiments.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

KRUSTY Experiment: Reactivity Insertion Accident Analysis

The centerpiece of the Kilopower Project, i.e., the Kilowatt Reactor Using Stirling TechnologY (KRUSTY) test, consists of the development and testing of a ground technology demonstration of a small fission power system based on a 1-kW(electric) space science power requirement. The KRUSTY test was authorized by the U.S. Department of Energy’s (DOE’s) National Nuclear Security Administration Nevada Field Office. Authorization was obtained by adding an amendment to the existing regulatory documents for the National Criticality Experiments Research Center to cover the KRUSTY experiment. This amendment was reviewed and approved by the DOE. The most important safety question for the experiment was the addition of over 2 $ of excess reactivity to the reactor system. This amount of excess reactivity meant that the analyst could postulate accidents where the reactor went prompt critical, leading to physical shock or melting of the fuel. This paper analyzes these accidents using computer calculations and examines the controls used to mitigate them. The estimation of the impacts both on accident progression and consequences of reactivity insertion events was a significant part of obtaining approval for the KRUSTY experiment. The regulatory approval of KRUSTY was one of the first to be obtained for a completely new reactor concept in many decades.

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

Foreword Special issue on the Kilopower Project, Kilowatt Reactor Using Stirling TechnologY (KRUSTY) Test

This special issue of Nuclear Technology contains full-length, peer-reviewed papers describing the design work leading up to and the results of the Kilowatt Reactor Using Stirling TechnologY (KRUSTY) test. KRUSTY was the centerpiece of the National Aeronautics and Space Administration (NASA) Kilopower Project to design, build, and test a space nuclear reactor. This test was the first such test since the end of the Space Nuclear Auxiliary Power (SNAP) project at the end of the 1960s. In this issue, the introduction paper presents the goals of the Kilopower Project and the potential missions this reactor concept could serve in NASA. Kilopower was intended to serve both human exploration needs on planetary surfaces as well as science needs for deep-space exploration. The design work for the experiment by Poston and the power conversion development by Gibson present the pre-work required to perform the eventual KRUSTY test. A paper on regulatory analysis follows, to show the path used to gain approval of the proposed experiment. Then, the early zero-power critical experiments are presented by Sanchez and Grove. These experiments were essential data used to enhance model predictions prior to the high-temperature test. Next, Poston presents the three experiments (warm criticals) that increase the temperature in an incremental fashion prior to the final experiment. These experiments were used to achieve final regulatory approval of the final high-temperature experiment. The last paper by Poston presents the results of the steady-state and transient testing of the reactor at full power and at the design temperature. These results show that the reactor design and as-built experiment met all of the requirements that NASA had developed for the system. Any experiment of this magnitude was accomplished only because of the hard work and dedication of a large number of people at multiple institutions, including the NASA Glenn Research Center, NASA Marshall Space Flight Center, Y-12 National Security Site, Los Alamos National Laboratory, and the Nevada National Security Site prime contractor (formerly National Security Technologies and now the Mission Support and Test Services). The project was jointly funded by the Space Technology Mission Directorate at NASA and the Criticality Safety Program at the National Nuclear Security Administration (NNSA). A special thanks to Jerry McKamy and Angela Chambers at the NNSA and Lee Mason and Don Palac at NASA for their support and guidance. For the authors and multitude of staff that performed this work, the passion for space nuclear reactors was the key to making this experiment a reality.

99 GENERAL AND MISCELLANEOUS↗