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At least 181 records · Page 10

Estimating UV-B, UV-Erithemic, and UV-A Irradiances From Global Horizontal Irradiance and MERRA-2 Ozone Column Information

The ground ultraviolet (UV) solar radiation is relevant due to its impacts on plastics degradation (mainly UVA) and on human health (UVB and erithemic UV (UVE)). UV ground measurements are not as ubiquitous as the relatively common global horizontal irradiance (GHI) measurements. Three simple models that estimate the UVA, UVB, and UVE components of solar irradiance from GHI and ozone column information are locally adjusted and validated. Five one-minute datasets from three sites in southeastern South America and two in the United States are used for simultaneous solar irradiance and UV data. All sites correspond to temperate mid-latitude regions. Simultaneous atmospheric total ozone column information is obtained from the reanalysis modern-era retrospective analysis for research and applications (MERRA-2) database for each site. Aside from locally adjusted models, average models with a single set of coefficients are also evaluated. For instance, the best average model is able to estimate UVE with a typical uncertainty below 12% and mean biases between +-3%, relative to the average of the measurements. Similar results are reported for the UVB and UVA components. These results, which can be useful in regions with similar climate and geography, provide a simple way to estimate UV irradiance under all-sky conditions with known uncertainty. This is an alternative to global satellite-based UV estimates, which can have high uncertainties at specific locations. Because MERRA-2 information has a global coverage, when coupled with good satellite-based estimates for GHI, UV irradiances can be estimated by this method over a large territory.

environmental UV radiation↗

Irradiated stainless steel 347 and irradiated, welded, and hydrogen charged Zircaloy-4 property data for the target solution vessel and support lines of SHINE

In support of the reactor-vessel development effort of SHINE medical technologies, irradiation of its structural materials and post-irradiation testing have been performed in the High Flux Isotope Reactor at Oak Ridge National Laboratory. This irradiation was performed on welded and unwelded AISI 347 steel and Zircaloy-4 samples at low temperature (~60°C) in contact with the reactor coolant. Hardness, Charpy, and tensile data have been taken from all cases of unirradiated specimens, while post-irradiation tensile and hardness data have been taken from AISI 347 base metal and Zircaloy-4 base metal and weld specimens so far. Additionally, 3-point bend data have been taken from explosion-welded specimens. The expected changes to hardness, yield strength, ultimate tensile strength, uniform elongation, and total elongation as a result of the low temperature and low dose neutron irradiation are reported here.

36 MATERIALS SCIENCE↗

AFC FY 2023 HFIR Irradiation Test Matrix – Supported by the Design of a Ring Specimen Irradiation Vehicle

The development and deployment of accident-tolerant cladding materials in light water nuclear reactors requires the collection of neutron-irradiated properties of these materials with specific consideration to the material properties orientation (i.e., tube geometry). To that end, a test plan to irradiate several cladding tube and ring specimens in the High Flux Isotope Reactor (HFIR) at Oak Ridge National Laboratory (ORNL) was proposed, along with the development of a new capsule design that features ring specimens with a preexisting gauge section. This ring specimen geometry removes the need to machine a gauge section on the irradiated specimen and thus allows for direct application of a ring-pull test post-irradiation. The test matrix includes uncoated and chromium-coated Zircaloy-4 and advanced zirconium alloy cladding specimens, pre-characterized at ORNL. Plans are to irradiate the specimens at about 4 and 10 dpa—corresponding to two and five cycles at the HFIR centerline—with a target specimen gauge section temperature of 330°C.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Correlation of irradiation data using activation fluences and irradiation temperature.

Nil-ductility transition temperature data for A302-B ferritic steel were analyzed by using multiple regression. Four independent variables were used - i.e., specimen temperature during irradiation, and time-integrated specific activations (activation fluences) of fast-, intermediate-, and thermal-neutron detectors. The results of these analyses were predictive equations having the increase in transition temperature as the dependent variable. For a reference point, a similar analysis was also performed using the flux integral above 1 MeV and the irradiation temperature as independent variables. Also, the effect of excluding irradiation temperature from these analyses was studied. The results of the analyses showed that excellent correlation was achieved by using activation fluences and irradiation temperature as the independent variables. Irradiation temperature was found to account for from 29 to 46% of the data variability depending on the model used.

Lynch, J. H.↗

Irradiation effects in rapidly and conventionally solidified alloys. Phase stability in rapidly solidified N i-Nb under Ni ion irradiation

Two alloy compositions in the Ni-Nb system (Ni60Nb40 and Ni85Nb15) were produced by rapidly quenching from the melt with the piston anvil technique. The Ni60Nb40 was transformed to a metastable, partially crystalline state by heat treatment in a differential scanning calorimeter. The Ni85Nb15 was fully crystalline, with the majority of the grains composed of collections of primary dendrite arms. Both compositions were irradiated with 4 MeV Ni++ ions. The irradiation induced microstructures were examined by transmission electron microscopy and compared with thermally aged samples. The thermal evolution was arrested by ion irradiation in the temperature range studied, by inhibiting the nucleation of the NiNb phase. No irradiation induced voids were observed. It is found that the ion irradiation drives the microstructure along a different path than thermal evolution.

Source record↗

Response of thyroid follicular cells to gamma irradiation compared to proton irradiation: II. The role of connexin 32

The objective of this study was to determine whether connexin 32-type gap junctions contribute to the "contact effect" in follicular thyrocytes and whether the response is influenced by radiation quality. Our previous studies demonstrated that early-passage follicular cultures of Fischer rat thyroid cells express functional connexin 32 gap junctions, with later-passage cultures expressing a truncated nonfunctional form of the protein. This model allowed us to assess the role of connexin 32 in radiation responsiveness without relying solely on chemical manipulation of gap junctions. The survival curves generated after gamma irradiation revealed that early-passage follicular cultures had significantly lower values of alpha (0.04 Gy(-1)) than later-passage cultures (0.11 Gy(-1)) (P < 0.0001, n = 12). As an additional way to determine whether connexin 32 was contributing to the difference in survival, cultures were treated with heptanol, resulting in higher alpha values, with early-passage cultures (0.10 Gy(-1)) nearly equivalent to untreated late-passage cultures (0.11 Gy(-1)) (P > 0.1, n = 9). This strongly suggests that the presence of functional connexin 32-type gap junctions was contributing to radiation resistance in gamma-irradiated thyroid follicles. Survival curves from proton-irradiated cultures had alpha values that were not significantly different whether cells expressed functional connexin 32 (0.10 Gy(-1)), did not express connexin 32 (0.09 Gy(-1)), or were down-regulated (early-passage plus heptanol, 0.09 Gy(-1); late-passage plus heptanol, 0.12 Gy(-1)) (P > 0.1, n = 19). Thus, for proton irradiation, the presence of connexin 32-type gap junctional channels did not influence their radiosensitivity. Collectively, the data support the following conclusions. (1) The lower alpha values from the gamma-ray survival curves of the early-passage cultures suggest greater repair efficiency and/or enhanced resistance to radiation-induced damage, coincident with the expression of connexin 32-type gap junctions. (2) The increased sensitivity of FRTL-5 cells to proton irradiation was independent of their ability to communicate through connexin 32 gap junctions. (3) The fact that the beta components of the survival curves from both gamma rays and proton beams were similar (average 0.022 +/- 0.008 Gy(-2), P > 0.1, n = 39) suggests that at higher doses the loss of viability occurs at a relatively constant rate and is independent of radiation quality and the presence of functional gap junctions.

Non-NASA Center↗

High energy X-ray diffraction study of the relationship between the macroscopic mechanical properties and microstructure of irradiated HT-9 steel

Samples harvested from an HT-9 fuel test assembly (ACO-3) irradiated for six years in the Fast Flux Test Facility (FFTF) reaching 2–147 dpa at 382–504°C were deformed in-situ while collecting high-energy X-ray diffraction data to monitor microstructure evolution. With the initiation of plastic deformation, all samples exhibited a clear load transfer from the ferrite matrix to carbide particulate. This behavior was confirmed by modeling of the control material. The evolution of dislocation density in the material as a result of deformation was characterized through full pattern line profile analysis. The dislocation densities increased substantially after deformation, the level of dislocation evolution observed was highly dependent upon the irradiation temperature of the sample. The differences in both the yield and hardening behavior between samples irradiated at higher and lower temperatures suggest the existence of a transition in tensile behavior at an irradiation temperature near 420°C dividing regions of distinct damage effects.

36 MATERIALS SCIENCE↗

Model for Deriving the Direct Normal and Diffuse Horizontal Irradiance from the Global Tilted Irradiance

We developed a separation model for deriving the direct normal irradiance (DNI) and the diffuse horizontal irradiance (DHI) from the global tilted irradiance (GTI). The model is based on the DIRINT model, but substitutes the use of the GTI in place of the global horizontal irradiance (GHI) for determining the global clearness index (Kt). Additionally, an iterative method is used to adjust Kt to improve the derived values of the DNI and the DHI. The model is referred to as the GTI-DIRINT model. When using for model input the GTI measured with a pyranometer tilted at a small angle from the horizontal (10°), the deviations between the measured DNI and DHI and the GTI-DIRINT-modeled DNI and DHI were essentially the same as those for the DIRINT model when using the GHI for model input. Increasing the tilt angle from horizontal (as great as 44° for Eugene, Oregon) increased the deviations between the modeled and measured DNI and DHI, but our results were still reasonable. The GTI-DIRINT model provides reasonable values of DNI and DHI from the GTI, and if they are subsequently used with the Perez tilted surface model to model the GTI for orientations within 30° of the azimuth and tilt of the GTI used for model input, the result is as good or better than may be obtained when using a measured DNI and DHI, and without their significant instrumentation cost.

14 SOLAR ENERGY↗

Structure and band gap determination of irradiation-induced amorphous nano-channels in LiNbO{sub 3}

The irradiation of lithium niobate with swift heavy ions results in the creation of amorphous nano-sized channels along the incident ion path. These nano-channels are on the order of a hundred microns in length and could be useful for photonic applications. However, there are two major challenges in these nano-channels characterization: (i) it is difficult to investigate the structural characteristics of these nano-channels due to their very long length and (ii) the analytical electron microscopic analysis of individual ion track is complicated due to electron beam sensitive nature of lithium niobate. Here, we report the first high resolution microscopic characterization of these amorphous nano-channels, widely known as ion-tracks, by direct imaging them at different depths in the material, and subsequently correlating the key characteristics with electronic energy loss of ions. Energetic Kr ions ({sup 84}Kr{sup 22} with 1.98 GeV energy) are used to irradiate single crystal lithium niobate with a fluence of 2 × 10{sup 10} ions/cm{sup 2}, which results in the formation of individual ion tracks with a penetration depth of ∼180 μm. Along the ion path, electron energy loss of the ions, which is responsible for creating the ion tracks, increases with depth under these conditions in LiNbO{sub 3}, resulting in increases in track diameter of a factor of ∼2 with depth. This diameter increase with electronic energy loss is consistent with predictions of the inelastic thermal spike model. We also show a new method to measure the band gap in individual ion track by using electron energy-loss spectroscopy.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Offline multiple adaptive planning strategy for concurrent irradiation of the prostate and pelvic lymph nodes

Purpose: Concurrent irradiation of the prostate and pelvic lymph nodes (PLNs) can be challenging due to the independent motion of the two target volumes. To address this challenge, the authors have proposed a strategy referred to as Multiple Adaptive Planning (MAP). To minimize the number of MAP plans, the authors’ previous work only considered the prostate motion in one major direction. After analyzing the pattern of the prostate motion, the authors investigated a practical number of intensity-modulated radiotherapy (IMRT) plans needed to accommodate the prostate motion in two major directions simultaneously. Methods: Six patients, who received concurrent irradiation of the prostate and PLNs, were selected for this study. Nine MAP-IMRT plans were created for each patient with nine prostate contours that represented the prostate at nine locations with respect to the PLNs, including the original prostate contour and eight contours shifted either 5 mm in a single anterior-posterior (A-P), or superior-inferior (S-I) direction, or 5 mm in both A-P and S-I directions simultaneously. From archived megavoltage cone beam CT (MV-CBCT) and a dual imaging registration, 17 MV-CBCTs from 33 available MV-CBCT from these patients showed large prostate displacements (>3 mm in any direction) with respect to the pelvic bones. For each of these 17 fractions, one of nine MAP-IMRT plans was retrospectively selected and applied to the MV-CBCT for dose calculation. For comparison, a simulated isocenter-shifting plan and a reoptimized plan were also created for each of these 17 fractions. The doses to 95% (D95) of the prostate and PLNs, and the doses to 5% (D5) of the rectum and bladder were calculated and analyzed. Results: For the prostate, D95 > 97% of the prescription dose was observed in 16, 16, and 17 of 17 fractions for the MAP, isocenter-shifted, and reoptimized plans, respectively. For PLNs, D95 > 97% of the prescription doses was observed in 10, 3, and 17 of 17 fractions for the three types of verification plans, respectively. The D5 (mean ± SD) of the rectum was 45.78 ± 5.75, 45.44 ± 4.64, and 44.64 ± 2.71 Gy, and the D5 (mean ± SD) of the bladder was 45.18 ± 2.70, 46.91 ± 3.04, and 45.67 ± 3.61 Gy for three types of verification plans, respectively. Conclusions: The MAP strategy with nine IMRT plans to accommodate the prostate motions in two major directions achieved good dose coverage to the prostate and PLNs. The MAP approach can be immediately used in clinical practice without requiring extra hardware and software.

62 RADIOLOGY AND NUCLEAR MEDICINE↗

Survival and Neurocognitive Outcomes After Cranial or Craniospinal Irradiation Plus Total-Body Irradiation Before Stem Cell Transplantation in Pediatric Leukemia Patients With Central Nervous System Involvement

Purpose: To evaluate survival and neurocognitive outcomes in pediatric acute lymphoblastic leukemia (ALL) patients with central nervous system (CNS) involvement treated according to an institutional protocol with stem cell transplantation (SCT) and a component of craniospinal irradiation (CSI) in addition to total-body irradiation (TBI) as preparative regimen. Methods and Materials: Forty-one pediatric ALL patients underwent SCT with TBI and received additional cranial irradiation or CSI because of CNS leukemic involvement. Prospective neurocognitive testing was performed before and after SCT in a subset of patients. Cox regression models were used to determine associations of patient and disease characteristics and treatment methods with outcomes. Results: All patients received a cranial radiation boost; median total cranial dose was 24 Gy. Eighteen patients (44%) received a spinal boost; median total spinal dose for these patients was 18 Gy. Five-year disease-free survival (DFS) for all patients was 67%. Those receiving CSI had a trend toward superior DFS compared with those receiving a cranial boost alone (hazard ratio 3.23, P=.14). Patients with isolated CNS disease before SCT had a trend toward superior DFS (hazard ratio 3.64, P=.11, 5-year DFS 74%) compared with those with combined CNS and bone marrow disease (5-year DFS 59%). Neurocognitive testing revealed a mean post-SCT overall intelligence quotient of 103.7 at 4.4 years. Relative deficiencies in processing speed and/or working memory were noted in 6 of 16 tested patients (38%). Pre- and post-SCT neurocognitive testing revealed no significant change in intelligence quotient (mean increase +4.7 points). At a mean of 12.5 years after transplant, 11 of 13 long-term survivors (85%) had completed at least some coursework at a 2- or 4-year college. Conclusion: The addition of CSI to TBI before SCT in pediatric ALL with CNS involvement is effective and well-tolerated. Craniospinal irradiation plus TBI is worthy of further protocol investigation in children with CNS leukemia.

62 RADIOLOGY AND NUCLEAR MEDICINE↗

Comparative post-irradiation examination of high burnup U-19Pu-10Zr: Assessing steady-state irradiation behavior against historical and modeled fuel performance

Here, the development of next-generation sodium-cooled fast reactors necessitates comprehensive research on metallic fuels to maximize economic performance while ensuring safe operation. In this study, we investigated the steady-state irradiation behavior of two high burnup U-19Pu-10Zr fuel pins, DP-36 and DP-40, in preparation for planned safety testing. Post-irradiation examination (PIE) was performed to quantify fuel column elongation, regions of low-density at the top of the fuel column, pin deformation, fission product distribution, fractional fission gas release, microstructural evolution, and fuel constituent redistribution. Benchmarking against existing PIE data from U-19Pu-10Zr fuel pins irradiated in EBR-II revealed consistent patterns in fuel column elongation and cladding diametral strain. However, both pins exhibited longer low-density structures, and destructive examination of DP-36 revealed more complex constituent redistribution patterns compared to previously reported data for ternary fuel pins. The steady-state irradiation of both pins was also modeled using BISON. Comparisons of PIE results with modeled predictions showed overall agreement in fractional fission gas release but consistent overestimation of axial and radial swelling due to gaseous and solid swelling models. These findings underscore the critical importance of pre-test characterization on test and sibling pins to accurately capture steady-state fuel behavior ahead of transient testing, thus establishing a baseline for post-test comparison. Additionally, these analyses identified key data gaps that warrant further investigation to improve the understanding and prediction of fuel swelling, thereby enhancing the synergy between modeling and experimental efforts in supporting accident testing.

BISON↗

Irradiation-induced grain boundary migration in an ion irradiated Fe-Ni-Cr-Mn alloy

Irradiation-induced grain boundary migration (RIGM) has previously been observed in different metallic systems. However, the mechanisms and dependence on irradiation conditions remained unclear. Here, we report on radiation-induced GB migration (RIGM) in a coarse-grain Fe-Ni-Cr-Mn austenitic alloy irradiated with Fe ions at 400 °C to 15, 35, and 70 dpa. Grain boundary migration is only observed in the irradiated regions and exhibits a linear dependence on the locally delivered dose, as estimated from SRIM calculations. Notably, the same linear dependence is noted across the nominal doses. Furthermore, the evidence points to grain boundary migration being mediated by the flux of point defects to grain boundaries and motivates additional systematic studies of RIGM in these systems.

Grain boundary↗

K{sub α} x-ray imaging of laser-irradiated, limited-mass zirconium foils

X-ray fluorescence measurements to determine the effect of target heating on imaging efficiency, at a photon energy of 15.7 keV corresponding to the K{sub α} line of zirconium, have been carried out using limited-mass foils irradiated by the Texas Petawatt Laser. Zirconium foils that ranged in volume from 3000 × 3000 × 21 μm{sup 3} to 150 × 150 × 6 μm{sup 3} were irradiated with 100 J, 8 ps-long pulses and a mean intensity of 4 × 10{sup 19} W/cm{sup 2}. The K{sub α} emission was measured simultaneously using a highly ordered pyrolytic graphite crystal spectrometer and a curved quartz imaging crystal. The measured ratio of the integrated image signal to the integrated spectral signal was, within the experimental error, constant, indicating that the imaging efficiency's dependence on temperature is weak throughout the probed range. Based on our experience of target heating under similar conditions, we estimate a temperature of ∼200 eV for the smallest targets. The successful imaging of K{sub α} emission for temperatures this high represents an important proof of concept for Zr K{sub α} imaging. At these temperatures, the imaging of K{sub α} emission from lower-Z materials (such as Cu) is limited by temperature-dependent shifts in the K{sub α} emission energy.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗