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At least 181 records · Page 10

Efficient simulations of charge density waves in the transition metal Dichalcogenide TiSe 2

Charge density waves (CDWs) in transition metal dichalcogenides are the subject of growing scientific interest due to their rich interplay with exotic phases of matter and their potential technological applications. Here, using density functional theory with advanced meta-generalized gradient approximations (meta-GGAs) and linear response time-dependent density functional theory (TDDFT) with state-of-the-art exchange-correlation kernels, we investigate the electronic, vibrational, and optical properties in 1T-TiSe 2 with and without CDW. In both bulk and monolayer TiSe 2 , the electronic bands and phonon dispersions in either normal or CDW (semiconducting) phase are described well via meta-GGAs, which separate the valence and conduction bands just as HSE06 does but with significantly more computational feasibility. The experimentally observed humps of electron energy loss spectroscopy are successfully reproduced in TDDFT. Our work opens the door to simulating these complexities in CDW compounds from first principles by revealing meta-GGAs as an accurate low-cost alternative to HSE06.

Electronic properties and materials↗

Bi-2212/1T-TaS 2 Van der Waals junctions: Interplay of proximity induced high-T c superconductivity and CDW order

Understanding the coexistence, competition and/or cooperation between superconductivity and charge density waves (CDWs) in the transition metal dichalcogenides (TMDs) is an elusive goal which, when realized, promises to reveal fundamental information on this important class of materials. Here in this paper, we use four-terminal current-voltage measurements to study the Van der Waals interface between freshly exfoliated flakes of the high-T c superconductor, Bi-2212, and the CDW-dominated TMD layered material, 1T-TaS 2 . For highly transparent barriers, there is a pronounced Andreev reflection feature providing evidence for proximity-induced high-Tc superconductivity in 1T-TaS 2 with a surprisingly large energy gap (~20 meV) equal to half that of intrinsic Bi-2212 (~40 meV). Our systematic study using conductance spectroscopy of junctions with different transparencies also reveals the presence of two separate boson modes, each associated with a “dip-hump” structure. Finally, we infer that the proximityinduced high-T c superconductivity in the 1T-TaS 2 is driven by coupling to the metastable metallic phase coexisting within the Mott commensurate CDW (CCDW) phase and associated with a concomitant change of the CCDW order parameter in the interfacial region.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Candidate spin-liquid ground state in CsNdSe 2 with an effective spin-1/2 triangular lattice

Rare-earth-based triangular lattice materials are extremely attractive for studying unconventional magnetism. Here, we report the magnetic properties of layered CsNdSe 2 based on direct current (DC) and alternating current (AC) susceptibility measurements down to 0.04 K. While the AC susceptibility at the zero DC field shows a broad hump below 0.5 K, there is no sign of any long-range magnetic ordering. Quantitative analysis of the DC magnetic susceptibility gives the negative Curie-Weiss (CW) temperature θ CW < 0 in all directions, indicating antiferromagnetic interaction between Nd ions. Of particular interest is the low temperature magnetic susceptibility, which reflects the effective spin-1/2 state with $\theta^a_{\text {cw}}/\theta^c_{\text {cw}}$ > 3. The estimated exchange interactions are J a /k B = 1.42 K (in-plane) and J c /k B = 0.44 K (out-of-plane), pointing to the anisotropic magnetism. First-principles calculations that include spin-orbit coupling and Coulomb correlations reveal multiple states with zero net magnetization for CsNdSe 2 . Both experiment and simulation strongly suggest CsNdSe 2 has the spin liquid ground state with effective spin-1/2. Application of a magnetic field can induce long-range antiferromagnetic ordering with the maximum transition temperature around 0.3 K, in further support of the zero-field spin liquid state.

36 MATERIALS SCIENCE↗

Discovery of hard-spectrum γ -ray emission from the BL Lacertae object 1ES 0414+009

1ES 0414 + 009 (z = 0.287) is a distant high-frequency-peaked BL Lac object, and has long been considered a likely emitter of very-high-energy (VHE, E > 100 GeV) γ-rays due to its high X-ray and radio flux. Observations in the VHE γ-ray band and across the electromagnetic spectrum can provide insights into the origin of highly energetic particles present in the source and the radiation processes at work. Because of the distance of the source, the γ-ray spectrum might provide further limits on the level of the extragalactic background light (EBL). Methods. We report observations made between October 2005 and December 2009 with H.E.S.S., an array of four imaging atmospheric Cherenkov telescopes. Observations at high energies (HE, 100 MeV–100 GeV) with the Fermi-LAT instrument in the first 20 months of its operation are also reported. To complete the multi-wavelength picture, archival UV and X-ray observations with the Swift satellite and optical observations with the ATOM telescope are also used. Based on the observations with H.E.S.S., 1ES 0414 + 009 is detected for the first time in the VHE band. An excess of 224 events is measured, corresponding to a significance of 7.8σ. The photon spectrum of the source is well described by a power law, with photon index of ΓVHE = 3.45 ± 0.25stat ± 0.20syst. The integral flux above 200 GeV is (1.88 ± 0.20stat ± 0.38syst) × 10-12 cm-2 s-1. Observations with the Fermi-LAT in the first 20 months of operation show a flux between 200 MeV and 100 GeV of (2.3 ± 0.2stat) × 10-9 erg cm-2 s-1, and a spectrum well described by a power-law function with a photon index ΓHE = 1.85 ± 0.18. Swift/XRT observations show an X-ray flux between 2 and 10 keV of (0.8-1) × 10-11 erg cm-2 s-1, and a steep spectrum ΓX = (2.2-2.3). Combining X-ray with optical-UV data, a fit with a log-parabolic function locates the synchrotron peak around 0.1 keV. Although the GeV–TeV observations do not provide better constraints on the EBL than previously obtained, they confirm a low density of the EBL, close to the lower limits from galaxy counts. The absorption-corrected HE and VHE γ-ray spectra are both hard and have similar spectral indices (≈1.86), indicating no significant change of slope between the HE and VHE γ-ray bands, and locating the γ-ray peak in the SED above 1–2 TeV. As for other TeV BL Lac objects with the γ-ray peak at such high energies and a large separation between the two SED humps, this average broad-band SED represents a challenge for simple one-zone synchrotron self-Compton models, requiring a high Doppler factor and very low B-field.

79 ASTRONOMY AND ASTROPHYSICS↗

Faraday cup with nanosecond response and adjustable impedance for fast electron beam characterization

A movable Faraday cup design with simple structure and adjustable impedance is described in this work. This Faraday cup has external adjustable shunt resistance for self-biased measurement setup and 50 {Omega} characteristic impedance to match with 50 {Omega} standard BNC coaxial cable and vacuum feedthroughs for nanosecond-level pulse signal measurements. Adjustable shunt resistance allows self-biased measurements to be quickly acquired to determine the electron energy distribution function. The performance of the Faraday cup is validated by tests of response time and amplitude of output signal. When compared with a reference source, the percent difference of the Faraday cup signal fall time is less than 10% for fall times greater than 10 ns. The percent difference of the Faraday cup signal pulse width is below 6.7% for pulse widths greater than 10 ns. A pseudospark-generated electron beam is used to compare the amplitude of the Faraday cup signal with a calibrated F-70 commercial current transformer. The error of the Faraday cup output amplitude is below 10% for the 4-14 kV tested pseudospark voltages. The main benefit of this Faraday cup is demonstrated by adjusting the external shunt resistance and performing the self-biased method for obtaining the electron energy distribution function. Results from a 4 kV pseudospark discharge indicate a ''double-humped'' energy distribution.

43 PARTICLE ACCELERATORS↗

A study of the role of various reactions on the density distribution of hydrogen, silylene, and silyl in SiH{sub 4}/H{sub 2} plasma discharges

Fluid model has been used to study the effect of pressure on the distribution of hydrogen (H), silylene (SiH{sub 2}), and silyl (SiH{sub 3}) in hydrogen silane plasma discharges used for deposition of hydrogenated microcrystalline silicon ({mu}c-Si:H) or hydrogenated amorphous silicon (a-Si:H) thin films for solar cells. Time averaged reaction rates have been calculated to study the influence of various reactions on the density distributions of hydrogen, silylene, and silyl. Change in the distributions of hydrogen and silylene from bell shaped distribution at low pressure (1 Torr) to double humped distribution at high pressure (5 Torr) is explained with the help of time averaged reaction rates. Important reactions have been identified that contribute to the production and consumption of hydrogen (H), silylene (SiH{sub 2}), and silyl (SiH{sub 3}). The hydrogen consumption reactions SiH{sub 4} + H {yields} SiH{sub 3} + H{sub 2} and SiH{sub 3} + H {yields} SiH{sub 2} + H{sub 2} are found to play a central role in deciding the distribution of hydrogen. On the other hand, silylene consumption reaction SiH{sub 2} + H{sub 2}{yields} SiH{sub 4} is found to play a central role in determining the distribution of silylene. The distribution of these species at high pressure has been explained by using time averaged continuity equation. The code has been optimized by identifying 33 reactions (out of 53 reactions which contribute in the production and consumption of H, SiH{sub 2}, and SiH{sub 3}) that have no net effect on the density and distribution of these species. It is observed that dropping of 33 reactions has insignificant effect on the density of all the thin film deposition precursors such as Si, SiH, SiH{sub 2}, SiH{sub 3}, and Si{sub 2}H{sub 5}. This reduced set of 20 reactions can be used instead of 53 reactions to calculate the density and distribution of H, SiH{sub 2}, and SiH{sub 3} in the fluid simulation of SiH{sub 4}/H{sub 2} plasma discharges.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Arbitrary amplitude kinetic Alfven solitons in a plasma with a q-nonextensive electron velocity distribution

Arbitrary amplitude solitary kinetic Alfven waves (KAWs) in a plasma with q-nonextensive electrons are investigated by the conventional Sagdeev pseudopotential method, through which the existence of solitary KAWs is analyzed theoretically and numerically. It is shown only solitons with density hump can exist, the amplitude of which depends sensitively on the parameter q and the plasma {beta}. There is an upper limit for the amplitude of solitary wave which decreases with the increase of q and {beta}. The results obtained in the framework of Maxwellian distribution are reproduced when q {yields} 1.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Nuclear photofission studies with monochromatic {gamma} ray beams

Two new research facilities will be ready for operation very soon (MEGa-Ray at Liver-more National Laboratory) or start construction (ELI-Nuclear Physics in Bucharest), both providing highly brilliant {gamma} beams with so far unprecedented properties via Compton backscattering of laser photons from a high-quality, relativistic electron beam. With these intense, monochromatic {gamma} beams, a new era of photonuclear physics will be enabled. A new research campaign is proposed to exploit the unprecedented properties of these highly-brilliant, novel {gamma} beams on highly-selective studies of extremely deformed nuclei in the multiple-humped potential energy landscape of the actinides via photofission. With the unique {gamma} beam bandwidth of {Delta}E/E = 10{sup -3}, we can aim at resolving individual resonances which could never be achieved so far due to the limited {gamma} bandwidth of bremsstrahlung beams. Exploratory, non-bremsstrahlung photofission experiments are going to be performed very soon at the HI{gamma}S facility (Duke University, USA) to investigate the fine structure of the sub-barrier transmission resonances of the actinides.

43 PARTICLE ACCELERATORS↗

Correlation between Ga-O signature and midgap states at the Al{sub 2}O{sub 3}/In{sub 0.53}Ga{sub 0.47}As interface

Al{sub 2}O{sub 3}/In{sub 0.53}Ga{sub 0.47}As gate stacks were fabricated using different concentrations of NH{sub 4}OH as a pre-deposition treatment. Increased NH{sub 4}OH concentrations significantly reduced the C-V weak inversion hump and the measured near midgap interface states density (D{sub it}). X-ray photoelectron spectroscopy (XPS) studies revealed that these changes in the electrical properties were accompanied by a reduction in the amount of the Ga-O bonding while As-As dimers as well as other XPS detected InGaAs surface species did not correlate with the observed D{sub it} trend. Possible explanations for these findings are suggested.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Dissipative ion-cyclotron oscillitons in a form of solitons with chirp in Earth's low-altitude ionosphere

In this paper, we consider theoretically nonlinear ion-cyclotron gradient-drift dissipative structures (oscillitons) in low ionospheric plasmas. Similar to Nonlinear Optics and Condensed Matter Physics, the Ginzburg-Landau equation for the envelope of electric wave fields is derived, and solutions for oscillitons in the form of solitons with chirp are examined. The whole dissipative structure constitutes a soliton with a moving charge-neutral density hump. Conditions for excitation and properties of the structures are considered.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Higher order nonlinear equations for the dust-acoustic waves in a dusty plasma with two temperature-ions and nonextensive electrons

The nonlinear propagation of dust-acoustic waves in a dusty plasma whose constituents are negatively charged dust, Maxwellian ions with two distinct temperatures, and electrons following q-nonextensive distribution, is investigated by deriving a number of nonlinear equations, namely, the Korteweg-de-Vries (K-dV), the modified Korteweg-de-Vries (mK-dV), and the Gardner equations. The basic characteristics of the hump (positive potential) and dip (negative potential) shaped dust-acoustic (DA) Gardner solitons are found to exist beyond the K-dV limit. The effects of two temperature ions and electron nonextensivity on the basic features of DA K-dV, mK-dV, and Gardner solitons are also examined. It has been observed that the DA Gardner solitons exhibit negative (positive) solitons for q q{sub c}) (where q{sub c} is the critical value of the nonextensive parameter q). The implications of our results in understanding the localized nonlinear electrostatic perturbations existing in stellar polytropes, quark-gluon plasma, protoneutron stars, etc. (where ions with different temperatures and nonextensive electrons exist) are also briefly addressed.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Growth of tungsten nanoparticles in direct-current argon glow discharges

The growth of nanoparticles from the sputtering of a tungsten cathode in DC argon glow discharges is reported. The study was performed at fixed argon pressure and constant discharge current. The growth by successive agglomerations is evidenced. First, tungsten nanocrystallites agglomerate into primary particles, the most probable size of which being {approx}30 nm. Primary particles of this size are observed for all plasma durations and always remain the most numerous in the discharge. Primary particles quickly agglomerate to form particles with size up to {approx}150 nm. For short plasma duration, log-normal functions describe accurately the dust particle size distributions. On the contrary, for long discharge durations, a second hump appears in the distributions toward large particle sizes. In the meantime, the discharge voltage, electron density, and emission line intensities strongly evolve. Their evolutions can be divided in four separate phases and exhibit unusual distinctive features compared to earlier observations in discharges in which particles were growing. The evolution of the different parameters is explained by a competition between the surface state of the tungsten cathode and the influence of the growing nanoparticles. The differences with sputtering glow discharges and chemically active plasmas suggest that the nanoparticle growth and its influence on discharge parameters is system and material dependent.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Analysing organic transistors based on interface approximation

Temperature-dependent characteristics of organic transistors are analysed thoroughly using interface approximation. In contrast to amorphous silicon transistors, it is characteristic of organic transistors that the accumulation layer is concentrated on the first monolayer, and it is appropriate to consider interface charge rather than band bending. On the basis of this model, observed characteristics of hexamethylenetetrathiafulvalene (HMTTF) and dibenzotetrathiafulvalene (DBTTF) transistors with various surface treatments are analysed, and the trap distribution is extracted. In turn, starting from a simple exponential distribution, we can reproduce the temperature-dependent transistor characteristics as well as the gate voltage dependence of the activation energy, so we can investigate various aspects of organic transistors self-consistently under the interface approximation. Small deviation from such an ideal transistor operation is discussed assuming the presence of an energetically discrete trap level, which leads to a hump in the transfer characteristics. The contact resistance is estimated by measuring the transfer characteristics up to the linear region.

36 MATERIALS SCIENCE↗

Experimental evidence of intermittent chaos in a glow discharge plasma without external forcing and its numerical modelling

Intermittent chaos was observed in a glow discharge plasma as the system evolved from regular type of relaxation oscillations (of larger amplitude) to an irregular type of oscillations (of smaller amplitude) as the discharge voltage was increased. Floating potential fluctuations were analyzed by different statistical and spectral methods. Features like a gradual change in the normal variance of the interpeak time intervals, a dip in the skewness, and a hump in the kurtosis with variation in the control parameter have been seen, which are strongly indicative of intermittent behavior in the system. Detailed analysis also suggests that the intrinsic noise level in the experiment increases with the increasing discharge voltage. An attempt has been made to model the experimental observations by a second order nonlinear ordinary differential equation derived from the fluid equations for an unmagnetized plasma. Though the experiment had no external forcing, it was conjectured that the intrinsic noise in the experiment could be playing a vital role in the dynamics of the system. Hence, a constant bias and noise as forcing terms were included in the model. Results from the theoretical model are in close qualitative agreement with the experimental results.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Ion-acoustic cnoidal waves in plasmas with warm ions and kappa distributed electrons and positrons

Electrostatic ion-acoustic periodic (cnoidal) waves and solitons in unmagnetized electron-positron-ion (EPI) plasmas with warm ions and kappa distributed electrons and positrons are investigated. Using the reductive perturbation method, the Korteweg-de Vries (KdV) equation is derived with appropriate boundary conditions for periodic waves. The corresponding analytical and various numerical solutions are presented with Sagdeev potential approach. Differences between the results caused by the kappa and Maxwell distributions are emphasized. It is revealed that only hump (compressive) structures of the cnoidal waves and solitons are formed. It is shown that amplitudes of the cnoidal waves and solitons are reduced in an EPI plasma case in comparison with the ordinary electron-ion plasmas. The effects caused by the temperature variations of the warm ions are also discussed. It is obtained that the amplitude of the cnoidal waves and solitons decreases for a kappa distributed (nonthermal) electrons and positrons plasma case in comparison with the Maxwellian distributed (thermal) electrons and positrons EPI plasmas. The existence of kappa distributed particles leads to decreasing of ion-acoustic frequency up to thermal ions frequency.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Standing electromagnetic solitons in hot ultra-relativistic electron-positron plasmas

Using a one-dimensional self-consistent fluid model, we investigate standing relativistic bright solitons in hot electron-positron plasmas. The positron dynamics is taken into account. A set of nonlinear coupled differential equations describing the evolution of electromagnetic waves in fully relativistic two-fluid plasma is derived analytically and solved numerically. As a necessary condition for the existence of standing solitons the system should be relativistic. For the case of ultra-relativistic plasma, we investigate non-drifting bright solitary waves. Detailed discussions of the acceptable solutions are presented. New single hump non-trivial symmetric solutions for the scalar potential were found, and single and multi-nodal symmetric and anti-symmetric solutions for the vector potential are presented. It is shown that for a fixed value of the fluid velocity excited modes with more zeros in the profile of the vector potential show a higher magnitude for the scalar potential. An increase in the plasma fluid velocity also increases the magnitude of the scalar potential. Furthermore, the Hamiltonian and the first integral of the system are given.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Dynamics of Johari-Goldstein β relaxation and its universal relation to α relaxation in bulk metallic glasses by mechanical spectroscopy

The dynamics of the Johari–Goldstein (JG) β relaxation and the α relaxation in bulk metallic glasses (MGs) has been investigated by using mechanical spectroscopy combined with the Coupling Model. The β relaxations of MGs exhibit different behaviors such as peaks, humps, and excess wings due to the different fluctuations of the chemical interactions among the constituting atoms. A universal correlation between the β relaxation and the α relaxation is generally found by their activation energies and relaxation times as well as the non-exponentiality parameter of the α relaxation, which can be predicted quantitatively from the Coupling Model. Based on the quasi-point defects theory, a correlation factor χ shows a broad peak along with the β relaxation, suggesting that the concentration and the correlation degree of the string-like configurations involved in the β relaxation vary with increasing temperature, which challenges the previous view that the system is in an iso-configuration state below T{sub g} and may shed new light on the nature of the JG β relaxation in metallic glasses.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Nonlinear space charge dynamics in mixed ionic-electronic conductors: Resistive switching and ferroelectric-like hysteresis of electromechanical response

We performed self-consistent modelling of nonlinear electrotransport and electromechanical response of thin films of mixed ionic-electronic conductors (MIEC) allowing for steric effects of mobile charged defects (ions, protons, or vacancies), electron degeneration, and Vegard stresses. We establish correlations between the features of the nonlinear space-charge dynamics, current-voltage, and bending-voltage curves for different types of the film electrodes. A pronounced ferroelectric-like hysteresis of the bending-voltage loops and current maxima on the double hysteresis current-voltage loops appear for the electron-transport electrodes. The double hysteresis loop with pronounced humps indicates a memristor-type resistive switching. The switching occurs due to the strong nonlinear coupling between the electronic and ionic subsystems. A sharp meta-stable maximum of the electron density appears near one open electrode and moves to another one during the periodic change of applied voltage. Our results can explain the nonlinear nature and correlation of electrical and mechanical memory effects in thin MIEC films. The analytical expression proving that the electrically induced bending of MIEC films can be detected by interferometric methods is derived.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗