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NASA NTRS1974

Spin projection of single-determinant wavefunctions

The components of the one- and two-particle density matrices resulting from spin projection of a single-determinant wave function are rederived by the method of expansion in terms of the natural orbitals of charge density, and the results are found to diverge from those given by Harriman and Sando for the two-particle case. The theory is generalized to include molecules with unequal numbers of electrons and basis orbitals and is applied to a number of organic molecules and ions. The correctness and internal consistency of the results argue in favor of the modification described.

Phillips, D. H.↗

NASA NTRS1989

Neutron starquakes and the nature of gamma-ray bursts

The possibility that gamma-ray bursts originate from quakes deep in the solid crust of a neutron star is investigated. Seismic waves are radiated if shear stress is relieved by brittle fracture. However they cannot propagate directly to the surface but are temporarily trapped below a reflecting layer. The shaking of the stellar surface couples the seismic waves to Alfven waves which propagate out into the magnetosphere. The crust-magnetosphere transmission coefficient strongly increases with wave frequency and magnetic field strength. Alfven wave luminosities sufficient to power galactic gamma-ray bursts are possible if magnetic fields greater than 100 billion G cover at least part of the stellar surface. As the Alfven waves propagate out into the low density magnetosphere, they become increasingly charge starved, thereby accelerating particles to relativistic energies.

Madau, P.↗

DOE OSTI2026

Frieze charge-stripes in a correlated kagome superconductor

In kagome metals, geometric frustration, electronic correlations and band topology combine to produce a wide range of intriguing phenomena. Among them, CsCr$_3$Sb$_5$ offers an opportunity to investigate unconventional superconductivity in a strongly correlated kagome system, with indications of frustrated magnetism and quantum criticality. Here, we demonstrate a cascade of density-wave transitions with distinct symmetries in bulk single crystals of CsCr$_3$Sb$_5$. Using spectroscopic imaging scanning tunneling microscopy, we uncover a unidirectional density wave that breaks all mirror symmetries -- resembling a chiral density wave -- but that also retains a mirror glide symmetry. We refer to this as a frieze charge stripe order phase, as its symmetry properties correspond to one of the fundamental frieze symmetry groups. A combination of high-resolution imaging, Fourier analysis and theoretical simulations reveal the key role of sublattice degrees of freedom in stabilizing this phase, characterized by internal chiral textures of opposite handedness. These findings suggest that superconductivity in CsCr$_3$Sb$_5$ emerges from this distinct density wave state and provide fresh insight into realizing electronic phases governed by frieze symmetry groups in quantum materials.

Cheng, Siyu [Boston College, Chestnut Hill, MA (Un↗

NASA NTRS1989

Dusty plasmas in the solar system

The processes that lead to charging of dust grains in a plasma are briefly reviewed. Whereas for single grains the results have been long known, the reduction of the average charge on a grain by 'Debye screening' has only recently been discovered. This reduction can be important in the Jovian ring and in the rings of Uranus. The emerging field of gravitoelectrodynamics which deals with the motion of charged grains in a planetary magnetosphere is then reviewed. Important mechanisms for distributing grains in radial distance are due to stochastic fluctuations of the grain charge and a systematic variation due to motion through plasma gradients. The electrostatic levitation model for the formation of spokes is discussed, and it is shown that the radial transport of dust contained in the spokes may be responsible for the rich radial structure in Saturn's rings. Finally, collective effects in dusty plasmas are discussed which affect various waves, such as density waves in planetary rings and low-frequency plasma waves. The possibility of charged grains forming a Coulomb lattice is briefly described.

Goertz, C. K.↗

NASA NTRS1985

Formation and detection of high latitude ionospheric irregularities

Measurements of Total Electron Content (TEC) and airglow variations show that large scale plasma patches appearing in the high-latitude ionsophere have irregular structures evidenced by the satellite phase and amplitude scintillations. Whistler waves, intense quasi-DC electric field, and atmospheric gravity waves can become potential sources of various plamsa instabilities. The role of thermal effects in generating ionospheric irregularities by these sources is discussed. Meter-scale irregularities in the ionospheric E and F regions can be excited parametrically with lower hybrid waves by intense whistler waves. Ohmic dissipation of Pedersen current in the electron gas is able to create ionospheric F region irregularities in plasma blobs or plasma patches (i.e., high ambient plasma density environment) with broad scale lengths ranging from tens of meters to a few kilometers. Through the neutral-charged particle collisions, gravity waves can excite large-scale (less than tens of kilometers) ionospheric irregularities simultaneously with forced ion acoustic modes in the E region. The large-scale ionospheric density fluctuations produced in the E region can extend subsequently alogn the earth's magnetic field to the F region and the topside ionospheric regions. These mechanisms characterized by various thermal effects can contribute additively with other processes to the formation of ionospheric irregularities in the high latitude region.

Lee, M. C.↗

NASA NTRS1987

A laboratory investigation of potential double layers

In a triple plasma device, the injection of electron current from the source chamber to the target chamber causes the formation of a potential double layer. At a low current density, the space charge of the injected current produces a virtual cathode-type potential double layer. This double layer is stable, and various wave instabilities are observed to associate with this double layer. As the current density is increased, the double layer becomes unstable, and a moving double layer results. As the current density is increased further, the enhanced ionization causes the neutralization of the space charge of the electron beam, and the beam plasma discharge is ignited.

Leung, Philip↗

NASA NTRS1987

A laboratory investigation of potential double layers

In a triple plasma device, the injection of electron current from the source chamber to the target chamber causes the formation of a potential double layer. At a low current density, the space charge of the injected current produces a virtual cathode-type potential double layer. This double layer is stable and various wave instabilities are observed to associate with this double layer. As the current density is increased, the double layer becomes unstable and a moving double layer results. As the current density is increased further, the enhanced ionization causes the neutralization of the space charge of the electron beam and the 'beam plasma discharge' is ignited.

Leung, Philip↗

DOE OSTI2025

Competing pair density wave and uniform 𝑑-wave superconductivity in phase-separated 214 cuprates at the 1/8 anomaly

Compelling evidence exists for electronic phase separation in cuprate high-𝑇𝑐 superconductors, emerging near 1/8 hole doping. At these dopings and low temperatures, intertwined charge and spin stripes coexist with more uniformly doped regions in the two-dimensional (2D) copper-oxide planes. Each region is capable of developing superconducting pairing, either as a pair density wave (PDW) within the stripes or as a uniform 𝑑-wave condensate (𝑑-SC) in the more homogeneous regions. Using neutron scattering on single crystals of La1.875−𝑦⁢Nd𝑦⁢Sr0.125⁢CuO4, we demonstrate that the onset temperatures for spin stripe order (𝑇𝑁) and superconductivity (𝑇𝑐) merge as the average ordered moment vanishes in LSCO (𝑦=0), whereas Nd doping stabilizes static stripe order and suppresses 𝑇𝑐. Because the spin stripes possess the same in-plane periodicity (8⁢𝑎) as the PDW and establish the framework within which the PDW resides, the stabilization of spin stripe order enhances PDW correlations. Thus, the competition between 𝑑-wave pairing in the uniform regions and PDW pairing in the stripe-ordered regions can be controlled by the Nd concentration in La1.875−𝑦⁢Nd𝑦⁢Sr0.125⁢CuO4, allowing the superconducting 𝑇𝑐 to vary by nearly an order of magnitude at a fixed 1/8-hole doping.

Aczel, Adam [ORNL] (ORCID:0000000319641943)↗

NASA NTRS1993

Solar-Driven Neutral Density Waves

Interstellar neutral hydrogen atoms flowing into the solar system are attracted by the solar gravitational force, repelled by solar hydrogen Ly-alpha radiation pressure, and are ionized, primarily, through charge exchange with the solar wind protons. The solar cycle variation of the radiation pressure causes the net central solar force to fluctuate between attraction and repulsion resulting in the modulation of the neutral hydrogen density about the usual time independent model. The calculation presented here shows that the time dependent downstream density is strongly modulated by a large number of travelling neutral density waves. The waves possess a continuous range of wavelengths as is to be expected for a Maxwellian gas subjected to several eleven year cycle variations during its journey through the solar system. The amplitudes of the density modulation were found to be quite large. The backscattered glow was found to depend on the position of the detector and the phase of the solar cycle. At the most favorable condition a deviation of the order of 25% from the time dependent glow might be observed.

Blum, P.↗

NASA NTRS1972

Dynamics of stratified liquids in the presence of space charge.

The dispersion characteristics of small signal electrohydrodynamic space charge and polarization waves in continuously and discretely stratified liquids are developed. The liquids, modeled as incompressible, inviscid, and perfectly insulating have distributions of mass density, charge density, permittivity, and electric field. A general set of relations for perturbation field and flow variables defined for a prototype layer are used to describe the dynamics of many superposed planar layers. It is shown that the general relations can be used to represent systems of coupled layers which approximate continuous distributions by a series of step functions. Specific examples of weak gradient and exponential distributions are presented showing that the solution found directly from the distributed theory is approached by the system of coupled layers, if the limit is taken in which the number of layers become large while each layer thickness approaches zero.

Zahn, M.↗

NASA NTRS1994

The dynamics of charged particles in turbulent astrophysical plasmas

We consider the resonant interaction of energetic charged particles and transverse plasma wave propagating parallel and/or antiparallel to the uniform magnetic field B(sub 0) in an underlying background plasma of density n. The coupling of the plasma waves and the energetic particles will be controlled by the ratio n/(the absolute value of B(sub 0)(exp 2). A variation of this ratio leads to a strong variation of the dynamics of the energetic particles. By taking into account the whole transverse plasma branch for the resonant interaction we discuss the influence of the background plasma density, the background magnetic field, the cross helicity, and the magnetic helicities on the dynamics of charged particles in astrophysical plasmas. It is shown that low-energy electrons can be accelerated efficiently by the higher electromagnetic waves and short-wavelength whistlers for low values of the ratio n/(the absolute value of B(sub 0)(exp 2), which means for low values of the ratio of plasma frequency to gyrofrequency.

Dung, Rudiger↗

NASA NTRS1986

Parallel electric fields in extragalactic jets - Double layers and anomalous resistivity in symbiotic relationships

After examining the properties of Coulomb-collision resistivity, anomalous (collective) resistivity, and double layers, a hybrid anomalous-resistivity/double-layer model is introduced. In this model, beam-driven waves on both sides of a double layer provide electrostatic plasma-wave turbulence that greatly reduces the mobility of charged particles. These regions then act to hold open a density cavity within which the double layer resides. In the double layer, electrical energy is dissipated with 100 percent efficiency into high-energy particles, creating conditions optimal for the collective emission of polarized radio waves.

Borovsky, J. E.↗

NASA NTRS1989

Effects of unequal particle number densities on Alfven waves

Analytic plasma theory and numerical solutions of the dispersion equation are used to show that the assumption that the linear properties of the waves are determined by a charge-neutral plasma in the absence of the nonthermal particles, while the nonthermal particles cause growth or additional damping superposed onto the background, is seriously flawed even for stable plasmas. Even when the nonthermal particles do not contribute significantly to the dispersion equation, unequal thermal electron and ion number densities (due to the presence of the nonthermal particles) may cause fundamental low wave number modifications to the Alfven modes, including the creation of a new resonance and severely modified dispersion. These results are found for both cold and warm plasmas. Previous work on Alfven waves should be reevaluated in view of these results.

Cairns, I. H.↗

DOE OSTI2026

Understanding cold electron impact on parallel-propagating whistler chorus waves via moment-based quasilinear theory

Earth's magnetosphere hosts a wide range of collisionless particle populations that interact through various wave-particle processes. Among these, cold electrons, with energies below 100 eV, often dominate the plasma density but remain poorly characterized due to measurement challenges such as spacecraft charging and photoelectron contamination. Understanding the contribution of these cold populations to wave–particle interaction is of significant interest. Recent kinetic simulations identified a secondary drift-driven instability, in which parallel-propagating whistler-mode chorus waves excite oblique electrostatic whistler waves near the resonance cone and Bernstein-mode turbulence. These secondary modes enable a new channel of energy transfer from the parallel-propagating whistler wave to the cold electrons. In this work, we develop a moment-based quasilinear theory of the secondary instabilities to quantify such energy exchange. Our results show that these secondary instabilities persist for a wide range of parameters and, in many cases, lead to nearly complete damping of the primary wave. Such secondary instability might limit the amplitude of parallel-propagating whistler waves in Earth's magnetosphere and might explain why high-amplitude oblique whistler or electron Bernstein waves are rarely observed simultaneously with high-amplitude field-aligned whistler waves in the inner magnetosphere.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

DOE OSTI2025

Quantum Nonlinear Acoustic Hall Effect and Inverse Acoustic Faraday Effect in Dirac Insulators

Here, we propose to realize the quantum nonlinear Hall effect and the inverse Faraday effect through the acoustic wave in a time-reversal invariant but inversion broken Dirac insulator. We focus on the acoustic frequency much lower than the Dirac gap such that the interband transition is suppressed and these effects arise solely from the intrinsic valley-contrasting band topology. The corresponding acoustoelectric conductivity and magnetoacoustic susceptibility are both proportional to the quantized valley Chern number and independent of the quasiparticle lifetime. The linear and nonlinear components of the longitudinal and transverse topological currents can be tuned by adjusting the polarization and propagation directions of the surface acoustic wave. The static magnetization generated by a circularly polarized acoustic wave scales linearly with the acoustic frequency as well as the strain-induced charge density. Our results unveil a quantized nonlinear topological acoustoelectric response of gapped Dirac materials, like hexagonal boron nitride and transition-metal dichalcogenide, paving the way toward room-temperature acoustoelectric devices due to their large band gaps.

36 MATERIALS SCIENCE↗

NASA NTRS1984

Measurements of plasma, plasma waves, and suprathermal charged particles in Saturn's inner magnetosphere

The Pioneer 11 and Voyager 1, 2 traversals of Saturn's inner magnetosphere provided direct information on the complex and highly structured distributions of plasma and suprathermal charged particles present in this region. The Voyager wave intruments also yielded absolute electron density measurements in certain inner magnetosphere locations; the wave data were used to evaluate the magnitudes of several wave-particle interactions. The plasma and wave measurements for 24-hr periods centered around closest approach, are summarized, pitch-angle scattering effects possibly associated wtih measured whistler mode turbulence are evaluated, and the effects of wave-particle interactions associated with electrostatic waves are discussed.

Scarf, F. L.↗

DOE OSTI2025

Revisiting the assignment of atomic charges in metal oxides based on core-level x-ray photoelectron spectra: The case of Ti in SrTiO3(001)

We demonstrate that assigning formal charges to transition metal (TM) cations based on core-level (CL) x-ray photoemission binding energies in oxides leads to physically inconsistent pictures of electronic structure. O 2p–TM 3d hybridization is well known to result in significant covalency in TM–O bonds, thereby reducing TM cation charges from their fully ionic values. However, the ionic bonding model remains the working paradigm for assigning TM CL features, and the resulting cation charges are often taken to be representative of the material under study. Here, we show that a more physically meaningful way to assign charges is to extract information about charge distributions utilizing Dirac–Hartree–Fock theory to calculate CL spectra from first principles and then use the resulting wave functions to determine charges based on orbital occupancies. TM cation charges can also be determined using density functional theory and Bader population analysis. We illustrate these two methods using the Ti 2p spectrum for SrTiO3(001) and show that the agreement between them is excellent. Significantly, the resulting Ti charge is considerably lower than the formal charge. The high degree of similarity between the Ti 2p spectrum for SrTiO3 and those for the rutile and anatase polymorphs of TiO2 suggests that the charge densities surrounding Ti in the latter materials are similar to that in SrTiO3. Taking a broader perspective, oxides containing other first-row transition metals also exhibit covalent character, leading to TM cation charges lower than the analogous fully ionic values in these materials as well.

Chambers, Scott A. (ORCID:000000025415043X)↗

NASA NTRS1972

Space-charge dynamics of liquids.

The propagation and instability characteristics of small-signal electro-fluid-mechanical space-charge and polarization waves in nonhomogeneous fluids are developed. Stratified equilibrium configurations with fluid properties and space-charge density constant within planar, cylindrical, and spherical surfaces, are emphasized. Equilibrium electric fields due both to charges in the fluid and to externally imposed potentials are normal to these surfaces. The liquid is modeled as incompressible, inviscid, and perfectly insulating, with domains of sufficiently high frequency or growth rate to validate the last assumption defined in terms of electrical conductivity or mobility. A general set of relations for perturbation field and flow variables on the perturbed surfaces of fluid layers having constant properties and space charge are derived in each of the configurations.

Zahn, M.↗