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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 181 records · Page 10

Bubble Behavior in a Vertically Vibrating Enclosed, Liquid-Filled Cylinder

When subjected to certain harmonic oscillations, the gas bubble in a partially liquid-filled, closed, vertical cylinder will break up. Under certain conditions, some of the gas will migrate to the bottom due to Bjerknes forces. At sufficiently large amplitudes, the bubble will break up into gas bubbles at the top and bottom ends of the cylinder. High-speed imaging captured the dynamics of bubble breakup and gas migration. Several parameters were investigated: oscillation frequency, oscillation acceleration, gas volume fraction, and liquid viscosity.

42 ENGINEERING↗

Search for inelastic dark matter-nucleus scattering with the PICO-60 CF$_{3}$I and C$_{3}$F$_{8}$ bubble chambers

PICO bubble chambers have exceptional sensitivity to inelastic dark matter-nucleus interactions due to a combination of their extended nuclear recoil energy detection window from a few keV to $O$(100 keV) or more and the use of iodine as a heavy target. Inelastic dark matter-nucleus scattering is interesting for studying the properties of dark matter, where many theoretical scenarios have been developed. This study reports the results of a search for dark matter inelastic scattering with the PICO-60 bubble chambers. The analysis reported here comprises physics runs from PICO-60 bubble chambers using CF$_{3}$I and C$_{3}$F$_{8}$. The CF$_{3}$I run consisted of 36.8 kg of CF$_{3}$I reaching an exposure of 3415 kg-day operating at thermodynamic thresholds between 7 and 20 keV. The C$_{3}$F$_{8}$ runs consisted of 52 kg of C$_{3}$F$_{8}$ reaching exposures of 1404 kg-day and 1167 kg-day running at thermodynamic thresholds of 2.45 keV and 3.29 keV, respectively. The analysis disfavors various scenarios, in a wide region of parameter space, that provide a feasible explanation of the signal observed by DAMA, assuming an inelastic interaction, considering that the PICO CF$_{3}$I bubble chamber used iodine as the target material.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Benchmarking and Exploring Parameter Space of the 2-Phase Bubble Tracking Model for Liquid Mercury Target Simulation

High intensity proton pulses strike the Spallation Neutron Source (SNS)’s mercury target to provide bright neutron beams. These strikes deposit extensive energy into the mercury and its steel vessel. Prediction of the resultant loading on the target is difficult when helium gas is intentionally injected into the mercury to reduce the loading and to mitigate the pitting damage on the vessel. A 2-phase material model that incorporates the Rayleigh-Plesset (R-P) model is expected to address this complex multi-physics dynamics problem by including the bubble dynamics in the liquid mercury. We present a study comparing the measured target strains in the SNS target station with the simulation results of the solid mechanics simulation framework. We investigate a wide range of various physical model parameters, including the number of bubble families, bubble size distribution, viscosity, surface tension, etc. to understand their impact on simulation accuracy. Our initial findings reveal that using 8-10 bubble families in the model renders a simulation strain envelope that covers the experimental ones. Further optimization studies are planned to predict the strain response more accurately.

Lin, Lianshan↗

Chiral-Bubble-Induced Topological Hall Effect in Ferromagnetic Topological Insulator Heterostructures

In this letter, we report compelling evidence of emergent topological Hall effect (THE) from chiral bubbles in a two-dimensional uniaxial ferromagnet, V-doped Sb 2 Te 3 heterostructure. The sign of THE signal is determined by the net curvature of domain walls in different domain configuration, and the strength of THE signal is correlated with the density of nucleation or pinned bubble domains. The experimental results are in good agreement with the integrated linear transport and Monte Carlo simulations, corroborating the emergent gauge field at chiral magnetic bubbles. Lastly, our findings not only reveal a general mechanism of THE in two-dimensional ferromagnets, but also pave the way for the creation and manipulation of topological spin textures for spintronic applications.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Electrical breakdown dynamics in an argon bubble submerged in conductive liquid for nanosecond pulsed discharges

Abstract This study delves into the dynamics of cold atmospheric plasma and their interaction within conductive solutions under the unique conditions of nanosecond pulsed discharges (22 kV peak voltage, 10 ns FWHM, 4.5 kV ns −1 rate-of-rise). The research focuses on the electrical response, breakdown, and discharge propagation in an argon bubble, submerged in a NaCl solution of varying conductivity. Full or partial discharges were observed at conductivities of 1.5 µ S cm −1 (deionized water) to 1.6 mS cm −1 , but no breakdown was observed at 11.0 mS cm −1 when reducing the electrode gap. It is demonstrated that at higher conductivity electric breakdown is observed only when the gas bubble comes into direct contact with the electrode and multiple emission nodes were observed at different timescales. These nodes expanded in the central region of the bubble over timescales longer than the initial high-voltage pulse. This work offers a temporal resolution of 2 ns exposure times over the first 30 ns of the initial voltage pulse, and insight into plasma formation over decaying reflected voltage oscillations over 200 ns.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Freestanding Ferroelectric Bubble Domains

Bubble-like domains, typically a precursor to the electrical skyrmions, arise in ultrathin complex oxide ferroelectric-dielectric-ferroelectric heterostructures epitaxially clamped with flat substrates. Here, it is reported that these specially ordered electric dipoles can also be retained in a freestanding state despite the presence of inhomogeneously distributed structural ripples. By probing local piezo and capacitive responses and using atomistic simulations, this study analyzes these ripples, sheds light on how the bubbles are stabilized in the modified electromechanical energy landscape, and discusses the difference in morphology between bubbles in freestanding and as-grown states. Furthermore, these results are anticipated to be the starting point of a new paradigm for the exploration of electric skyrmions with arbitrary boundaries and physically flexible topological orders in ferroelectric curvilinear space.

36 MATERIALS SCIENCE↗

Phase distribution in Fischer-Tropsch mimicked slurry bubble column via computed tomography

This study aims to investigate the phases distribution and hydrodynamics in an air-Therminol LT-glass beads slurry bubble column reactor in bubbly and churn-turbulent flow regimes by implementing a gamma-ray computed tomography. It is found that gas holdup increases with increasing superficial gas velocity and operating pressure while increasing solids loading has an opposite effect on gas holdup measurements. It is noticed that the pressure effect is more significant at high solids loading and the solids loading is relatively more substantial at lower pressure. Solids loading has the most significant a stronger effect on the solids holdup profile than on the gas holdup profile. Current results were compared with the Sedimentation-Dispersion Model (SDM) predictions. Overall, the findings of this study advance the knowledge of the true behavior of phases distribution in FT mimicked slurry bubble columns which are pertinent in designing such reactors.

42 ENGINEERING↗

Early self-organization of fission gas bubble superlattice formation in neutron-irradiated monolithic U-10Mo fuels

Self-organization of defect superlattices in far-from-equilibrium systems presents a promising way to mitigate swelling concerns in nuclear materials. The gas bubble superlattice (GBS) is a highly ordered, three-dimensional complex defect structure that can retain fission gasses in Uranium-Molybdenum (U-Mo) fuels. Transmission electron microscopy (TEM) investigation of monolithic U-10Mo fuel irradiated to 1.15 × 10 21 fissions/cm 3 and 1.30 × 10 21 fissions/cm 3 revealed that early-stage ordering preferentially occurs at the grain boundaries (GB) and that the critical bubble size for complete ordering is ~3 nm. Once formed at the GB, the GBS extends towards the grain interior; however, the spread in distance from the GB varies likely depending on the type and strength of the GB sink. TEM results also showed a possible correlation between the growth and evolution of the intragranular disordered bubbles and large dislocation networks. The fission product distribution in and outside of the GBS was also investigated confirming the presence of xenon in the GBS, as well as other fission products including cesium, barium, lanthanum, and cerium.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Understanding fission gas bubble distribution, lanthanide transportation, and thermal conductivity degradation in neutron-irradiated α-U using machine learning

U—10Zr based metallic nuclear fuel is the leading candidate for next-generation sodium-cooled fast reactors in the United States. US research reactors have used and tested this fuel type since the 1960s and accumulated considerable experience and knowledge about the fuel performance. Most of the knowledge, however, remains empirical. The lack of mechanistic understanding of fuel performance puts a large burden on proof through experimental verification for the qualification of U—10Zr fuel for commercial use. Further, this paper proposes an image data-driven machine learning approach, coupled with domain knowledge provided by advanced post irradiation examination, to provide unprecedented quantified insights into the morphology, size, density and the connectivity of fission gas bubbles and their effects on the fission product transportation and thermal conductivity. Specifically, we developed a method to automatically detect, extract statistics, and classify ~19,000 fission gas bubbles into different categories, and quantitatively link the data to lanthanide transportation through connected bubbles and degradation of thermal conductivity along the radial temperature gradient in a neutron irradiated U—10Zr annular fuel. Results indicate the approach can be modified to study other irradiation effects, such as secondary phase redistribution and gaseous fuel swelling in other irradiated nuclear fuels.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Corrigendum and Addendum: Helium flux effects on bubble growth and surface morphology in plasma-facing tungsten from large-scale molecular dynamics simulations (2019 Nucl. Fusion 59 066035)

Two of the simulations discussed in a prior article (Hammond et al 2019 Nucl. Fusion 59 066035) were affected by a simulation glitch. We repeated the affected calculations and discuss them here. Here, the overall conclusions are essentially unchanged, though the details are different. In particular, observations that we referred to as ‘concerted bursting’ were caused primarily by non-physical heating and cooling applied by the thermostat after most atoms’ velocities were deleted (for reasons that are not known for certain). The phenomenon of one bubble bursting and causing another nearby bubble to burst does exist, though its effects are much less spectacular in the absence of non-physical driving forces. The observation of an interconnected network of sub-surface cavities formed by burst bubbles is real, and the observation of holes on the surface 1–2 nm in diameter is also confirmed.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

MHD simulations of cold bubble formation from 2/1 tearing mode during massive gas injection in a tokamak

Massive gas injection (MGI) experiments have been carried out in many tokamaks to study disruption dynamics and mitigation schemes. Two events often observed in those experiments are the excitation of the m = 2, n = 1 magnetohydrodynamic mode, and the formation of cold bubble structure in the temperature distribution before the thermal quench (TQ). Here m is the poloidal mode number, n the toroidal mode number. The physics mechanisms underlying those phenomena, however, have not been entirely clear. In this work, our recent NIMROD simulations of the MGI process in a tokamak have reproduced the main features of both events, which has allowed us to examine and establish the causal relation between them. In these simulations, the 3/1 and 2/1 islands are found to form successively after the arrival of impurity ion cold front at the corresponding q = 3 and q = 2 rational surfaces. At the interface between impurity and plasma, a local thin current sheet forms due to an enhanced local pressure gradient and moves inward following the gas cold front, this may contribute to the formation of a dominant 2/1 mode. Following the growth of the 2/1 tearing mode, the impurity penetration into the core region inside the q = 2 surface gives rise to the formation of the cold bubble temperature structure and initiates the final TQ. Here, a subdominant 1/1 mode developed earlier near the q = 1 surface alone does not cause such a cold bubble formation, however, the exact manner of the preceding impurity penetration depends on the nature of the 1/1 mode: kink-tearing or quasi-interchange.

2/1 tearing mode↗

Feasibility of the LAMMPS SPH Package for Simulating Bubble Motion in Vibrating Containers

The Smoothed Particle Hydrodynamics (SPH) package within LAMMPS is explored as a possible tool for simulating the motion of bubbles in a vibrating liquid-filled container. As an initial test case, the unphysical but computationally less intense situation of a two-dimensional single bubble rising in a quiescent liquid under the influence of gravity is considered herein. Although physically plausible behavior was obtained under certain conditions, this behavior depends strongly on the system parameters. Moreover, the large density ratio between the liquid and bubble requires extremely small timesteps, which make the simulations undesirably computationally expensive. Ultimately, it was determined that this method is not feasible for providing quantitatively accurate results for the desired application.

42 ENGINEERING↗

Bubble-Free Frontal Polymerization of Acrylates via Redox-Initiated Free Radical Polymerization

Thermal frontal polymerization (FP) of acrylate monomers mixed with conventional peroxide initiators leads to significant bubble formation at the polymerizing front, limiting their practical applications. Redox initiators present a promising alternative to peroxide initiators, as they prevent the formation of gaseous byproducts during initiator decomposition and lower the front temperature, thereby enabling bubble-free FP. In this study, we investigate the FP of acrylate monomers of varying functionalities, including methyl methacrylate (MMA), 1,6-hexanediol diacrylate (HDDA), and trimethylolpropane triacrylate (TMPTA), using N,N -dimethylaniline/benzoyl peroxide (DMA/BPO) redox couple at room temperature and compare their front behavior, pot life, and bubble formation with those of same resin systems mixed with a conventional peroxide initiator, Luperox 231. The use of redox couples in FP of acrylates shows promise for rapid, energy-efficient manufacturing of polyacrylates and can enable new applications such as 3D printing and composite manufacturing.

36 MATERIALS SCIENCE↗

Scintillating Bubble Chambers for Rare Event Searches

The Scintillating Bubble Chamber (SBC) collaboration is developing liquid-noble bubble chambers for the detection of sub-keV nuclear recoils. These detectors benefit from the electron recoil rejection inherent in moderately-superheated bubble chambers with the addition of energy reconstruction provided from the scintillation signal. The ability to measure low-energy nuclear recoils allows the search for GeV-scale dark matter and the measurement of coherent elastic neutrino-nucleus scattering on argon from MeV-scale reactor antineutrinos. The first physics-scale detector, SBC-LAr10, is in the commissioning phase at Fermilab, where extensive engineering and calibration studies will be performed. In parallel, a functionally identical low-background version, SBC-SNOLAB, is being built for a dark matter search underground at SNOLAB. SBC-SNOLAB, with a 10 kg-yr exposure, will have sensitivity to a dark matter–nucleon cross section of 2×10 –42 cm 2 at 1 GeV/c 2 dark matter mass, and future detectors could reach the boundary of the argon neutrino fog with a tonne-yr exposure. In addition, the deployment of an SBC detector at a nuclear reactor could enable neutrino physics investigations including measurements of the weak mixing angle and searches for sterile neutrinos, the neutrino magnetic moment, and the light Z’ gauge boson.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Understanding grain refinement and intergranular gas bubble evolution in U-10Mo fuel using phase-field modeling

Monolithic U-10Mo fuel undergoes significant microstructural changes in the form of grain refinement and gas bubble formation during burnup, which degrades its mechanical properties. In this talk, I present a phase-field model for microstructure evolution in U-10Mo developed using the Multiphysics Object-Oriented Simulation Environment (MOOSE) framework. Simulations demonstrate that grain refinement initiates at pre-existing grain boundaries (GBs) to eliminate the lattice distortion energy caused by the accumulation of self-interstitial loops. By employing an equation of state for xenon gas, we simulate the evolution of gas bubbles in the polycrystal microstructure. Large, interconnected bubbles are found to form along the triple junctions. The effects of defect production rate, diffusivities and GB mobility on the microstructure evolution are systematically studied. Homogenization is employed on the microstructures to obtain effective elastic constants and diffusivity as a function of fission density. The simulations provide critical insights on microstructure and property degradation in U-10Mo fuel.

11 - NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Backpack electrofishing does not contribute to external signs of gas bubble trauma in sculpins

Abstract We exposed prickly sculpin Cottus asper and reticulate sculpin Cottus perplexus to electroshock and sham treatments in a controlled laboratory setting to determine if backpack electrofishing contributed to or exacerbated external signs of gas bubble trauma (GBT) in fish exposed to elevated total dissolved gas (TDG) levels. Fish were exposed to 115, 120 and 125% TDG (measured as percent of saturation) for various amounts of time (24–144 h) then subjected to a 5‐s electroshock or sham treatment of no electroshock. Fish were examined to determine the incidence of GBT pre‐ and post‐treatment, and all aspects (i.e., dorsal, ventral, left and right sides) of each fish were photographed. Across all TDG levels in all trials, no sculpin showed any change in GBT incidence following treatment. Analysis of GBT signs evident in photographs of 68 fish found no evidence of change in mean pre‐ and post‐treatment gas bubble sizes in fish in any TDG trial, nor were any new gas bubbles found following treatment. We are aware of no physiological mechanism by which backpack electrofishing can cause GBT in sculpin, and as such, we believe using this gear should not increase GBT incidence rates in sculpin.

Tiffan, Kenneth F.↗

Axion interactions with domain and bubble walls

We show that interactions between axion-like particles (ALPs) and co-dimension one defects, such as phase-transition bubble walls and solitonic domain walls, can lead to important changes in the evolution of both walls and ALPs. The leading effect arises from the change in the ALP decay constant across the interface, which naturally follows from shift-symmetric interactions with the corresponding order parameter. Specifically, we show that for thin walls moving relativistically, an ALP background — such as e.g. axion dark matter — gives rise to a frictional force on the interface that is proportional to γ 2 , with γ the Lorentz factor of the wall, and that this effect is present in both the oscillating and frozen axion regimes. We explore the broader consequences of this effect for bubble and domain walls in the early universe, and show that this source of friction can be present even in the absent of a conventional medium such as radiation or matter. Possible implications include modifications to the dynamics of bubble and domain walls and their corresponding gravitational wave signatures, as well as the generation of a dark radiation component of ALPs in the form of ultra-relativistic ‘axion shells’ with Lorentz factor γ shell ≃ 2γ 2 ≫ 1 that may remain relativistic until the present day.

Axions and ALPs↗

Neutralizing topological obstructions to bubbles of nothing

Theories with compact extra dimensions can exhibit a vacuum instability known as a bubble of nothing. These decay modes can be obstructed if the internal manifold is stabilized by fluxes, or if it carries Wilson lines for background gauge fields, or if the instanton is incompatible with the spin structure. In each of these cases the decay can proceed by adding dynamical charged membranes or gauge fields. We give a general, bottom-up procedure for constructing approximate bubble of nothing solutions in models with internal spheres stabilized by flux and study the influence of the brane tension on the tunneling exponent, finding two branches of solutions that merge at a minimal superextremal value of the tension. In the case of Wilson operators and incompatible fermions, the relevant bubble is shown to be the Euclidean Reissner-Nordstrom black hole, and the ordinary decay exponent is modified by 1/g 2 effects. We examine the Dirac operator on this background and comment on the relevance for models of supergravity with gauged R-symmetry.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗