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DOE OSTI · 3413786

Complex spin density wave ordering in La4Ni3O10

Abstract

The discovery of high-temperature superconductivity in layered nickelates under pressure has recently triggered enormous interest. Studies of these compounds have revealed a density-wave-like transition at ambient pressure, though its connection with superconductivity is still not well understood. Here, we report a detailed µ⁢SR study on single crystals of trilayer nickelate La4⁢Ni3⁢O10 at ambient pressure. We have identified a spin-density-wave (SDW) transition at the temperature of 𝑇N∼130K, as well as a broad crossover around 70–100 K. Based on the temperature dependence of the muon precession amplitudes and magnetic susceptibility, we attribute this additional crossover either to a spin reorientation, or to an inhomogeneous SDW ordering.

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BibTeXRIS

Gardner, Jason [ORNL] (ORCID:0000000278234072), Cao, Yantao [Songshan Lake Materials Laboratory, China], Liu, Andi [Songshan Lake Materials Laboratory, China], Wang, Bin [Songshan Lake Materials Laboratory, China], Zhang, Mingxin [ShanghaiTech University], Qi, Yanpeng [ShanghaiTech University,], Hickens, Thomas [Paul Scherrer Institut (PSI), Villigen, Switzerland], Leutkens, Hubertus [Paul Scherrer Institut (PSI), Villigen, Switzerland], Fu, Zhendong [Songshan Lake Materials Laboratory, China], Zhao, Jinkui [Songshan Lake Materials Laboratory, China], Guo, Hanjie [Songshan Lake Materials Laboratory, China]. 2025-11-01. Complex spin density wave ordering in La4Ni3O10. https://doi.org/10.1103/ncv2-7xnw

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