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DOE OSTI Β· 3017459

Enhancement of antiferromagnetic spin fluctuations in UTe2 under pressure revealed by 125 Te NMR

Abstract

Characterizing magnetic fluctuations is one of the keys to understanding the origin of superconductivity in the spin-triplet superconductor UTe 2 , which exhibits two superconducting (SC) phases (SC1 and SC2) under pressure: SC1 where the superconducting transition temperature of 𝑇c decreases with pressure, whereas 𝑇c of SC2 rises with pressure. Previously, D. Ambika et al. [Phys. Rev. B 105, L220403 (2022)] reported the possible coexistence of ferromagnetic (FM) and antiferromagnetic (AFM) spin fluctuations in UTe2 under pressure from their nuclear magnetic resonance (NMR) measurements. To delve into the relationship between the magnetic fluctuations and the two SC phases, we have carried out detailed 125 Te NMR measurements on a single crystal of UTe2 with 𝑇c=1.6K at various pressures ranging from 0 to 2.05 GPa. By comparing the temperature 𝑇 dependence of nuclear spin-lattice relaxation rates divided by temperature 1/𝑇1⁒𝑇 with that of the Knight shift 𝐾 for magnetic fields along the π‘Ž, 𝑏, and 𝑐 directions, we evidence the enhancement of AFM spin fluctuations with increasing pressure. Based on the results, we suggest that FM spin fluctuations are more favorable for SC1 and AFM spin fluctuations are crucial for SC2. Our work will inspire further study on this material to understand the peculiar SC phases in detail.

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BibTeXRIS

Vijayan Ambika, Devi [Ames Laboratory (AMES), Ames, IA (United States); Iowa State Univ., Ames, IA (United States)], Ding, Qing-Ping [Ames Laboratory (AMES), Ames, IA (United States)] (ORCID:000000017488066X), Frank, Corey E. [Univ. of Maryland, College Park, MD (United States); National Inst. of Standards and Technology (NIST), Gaithersburg, MD (United States)] (ORCID:0000000326387795), Ran, Sheng [Washington Univ., St. Louis, MO (United States)], Butch, Nicholas P. [Univ. of Maryland, College Park, MD (United States); National Inst. of Standards and Technology (NIST), Gaithersburg, MD (United States)] (ORCID:0000000260838388), Furukawa, Yuji [Ames Laboratory (AMES), Ames, IA (United States); Iowa State Univ., Ames, IA (United States)]. 2026-01-20. Enhancement of antiferromagnetic spin fluctuations in UTe2 under pressure revealed by 125 Te NMR. https://doi.org/10.1103/4gcm-mbl7

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