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DOE OSTI · 2920256

Robust Spin-Moiré-Superlattice-Driven Gap Opening in EuAg 4 Sb 2 under in-Plane Magnetic Field

Abstract

Moiré superlattices introduce new length and energy scales, enabling discoveries, such as unconventional superconductivity, in 2D systems. This concept has recently been extended to bulk materials with multiple-q spin textures, opening exciting opportunities for spin moiré physics. A notable example is EuAg 4 S b2 , where a spin moiré superlattice (SMS), manifested as a double-q spin modulation, induces a superzone gap opening. In this work, we investigate the tunability of this gap by an in-plane magnetic field in EuAg 4 Sb 2 by using neutron scattering, magnetization, and transport measurements. We reveal a cycloidal ground state and multiple spin-reoriented phases induced by the in-plane field, highlighting the critical role of in-plane components in driving magnetic transitions. Moreover, we demonstrate that a robust gap opening persists in the double-q phase, regardless of in-plane field orientation. Model calculations attribute this robustness to the stability of the SMS under tilted fields. Here, our results establish EuAg 4 Sb 2 as a tunable platform for exploring the spin-texture-driven superzone gap opening in electronic states.

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BibTeXRIS

Green, J. [University of California, Los Angeles, CA (United States)] (ORCID:0009000457270076), Arora, Arpit [University of California, Los Angeles, CA (United States)], Marshall, Madalynn [Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States); University of California, Los Angeles, CA (United States)], Shan, Wanfei [University of California, Los Angeles, CA (United States)], Udvarhelyi, Péter [University of California, Los Angeles, CA (United States)] (ORCID:0000000270731664), Morgan, Zachary [Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States)], Narang, Prineha [University of California, Los Angeles, CA (United States)] (ORCID:0000000339564594), Cao, Huibo [Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States)] (ORCID:0000000259704980), Ni, Ni [University of California, Los Angeles, CA (United States)]. 2025-09-02. Robust Spin-Moiré-Superlattice-Driven Gap Opening in EuAg 4 Sb 2 under in-Plane Magnetic Field. https://doi.org/10.1021/acs.nanolett.5c02167

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36 MATERIALS SCIENCE