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DOE OSTI · 2587868

Chiral flat-band optical cavity with atomically thin mirrors

Abstract

A fundamental requirement for photonic technologies is the ability to control the confinement and propagation of light. Widely used platforms include two-dimensional (2D) optical microcavities in which electromagnetic waves are confined in either metallic or distributed Bragg reflectors. Recently, transition metal dichalcogenides hosting tightly bound excitons with high optical quality have emerged as promising atomically thin mirrors. In this work, we propose and experimentally demonstrate a subwavelength 2D nanocavity using two atomically thin mirrors with degenerate resonances. Angle-resolved measurements show a flat band, which sets this system apart from conventional photonic cavities. We demonstrate how the excitonic nature of the mirrors enables the formation of chiral and tunable optical modes upon the application of an external magnetic field. Moreover, we show the electrical tunability of the confined mode. Our work demonstrates a mechanism for confining light with high-quality excitonic materials, opening perspectives for spin-photon interfaces, and chiral cavity electrodynamics.

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Suárez-Forero, Daniel G. [Univ. of Maryland, College Park, MD (United States). Joint Quantum Inst. (JQI)] (ORCID:0000000227576320), Ni, Ruihao [Univ. of Maryland, College Park, MD (United States)] (ORCID:0000000199238809), Sarkar, Supratik [Univ. of Maryland, College Park, MD (United States). Joint Quantum Inst. (JQI)] (ORCID:0000000326452307), Jalali Mehrabad, Mahmoud [Univ. of Maryland, College Park, MD (United States). Joint Quantum Inst. (JQI)] (ORCID:0000000298099998), Mechtel, Erik [Univ. of Maryland, College Park, MD (United States). Joint Quantum Inst. (JQI)], Simonyan, Valery [Univ. of Maryland, College Park, MD (United States). Joint Quantum Inst. (JQI)] (ORCID:0000000225773240), Grankin, Andrey [Univ. of Maryland, College Park, MD (United States). Joint Quantum Inst. (JQI)], Watanabe, Kenji [National Inst. for Materials Science (Japan)] (ORCID:0000000337018119), Taniguchi, Takashi [National Inst. for Materials Science (Japan)] (ORCID:0000000214673105), Park, Suji [Brookhaven National Laboratory (BNL), Upton, NY (United States). Center for Functional Nanomaterials (CFN)] (ORCID:0000000222697705), Jang, Houk [Brookhaven National Laboratory (BNL), Upton, NY (United States). Center for Functional Nanomaterials (CFN)], Hafezi, Mohammad [Univ. of Maryland, College Park, MD (United States). Joint Quantum Inst. (JQI)] (ORCID:0000000316794880), Zhou, You [Univ. of Maryland, College Park, MD (United States). Maryland Quantum Materials Center] (ORCID:000000029854545X). 2024-12-18. Chiral flat-band optical cavity with atomically thin mirrors. https://doi.org/10.1126/sciadv.adr5904

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