Engineering PapersSearch

DOE OSTI · 2574959

Homomorphic data compression for real time photon correlation analysis

Abstract

The construction of highly coherent X-ray sources, combined with next-generation detectors that are larger and faster, has enabled new research opportunities across the scientific landscape. Among the techniques that benefit most from these advancements is X-ray photon correlation spectroscopy (XPCS), where faster acquisition unlocks the ability to study faster dynamics within samples. However, faster acquisition on larger detectors also introduces unprecedented challenges for online data processing and offline data storage. Such challenges are particularly prominent for XPCS, where real time analyses require simultaneous calculation of all the previously acquired data in the time series. We present a homomorphic compression scheme to effectively reduce the computational time and memory space required for XPCS analysis. Leveraging similarities in the mathematical expression between a matrix-based compression algorithm and the correlation calculation, our approach allows direct operation on the compressed data without their decompression. The offline compression scheme extends storage capacity by a factor of 40 while preserving key features in the lossy compressed data. Meanwhile, the online compression scheme reduces the computational time to below 1 ms, enabling real time calculation of the correlation functions at kHz framerate. Our demonstration of a homomorphic compression of scientific data provides an effective solution to the big data challenge at coherent light sources. Beyond the example shown in this work, the framework can be extended to facilitate real-time operations directly on a compressed data stream for other techniques.

Explore related subjects

Keep this discovery

Explore connections, maps & timelines

BibTeXRIS

Strempfer, Sebastian [Argonne National Laboratory (ANL), Argonne, IL (United States)], Di, Zichao Wendy [Argonne National Laboratory (ANL), Argonne, IL (United States)], Yoshii, Kazutomo [Argonne National Laboratory (ANL), Argonne, IL (United States)], Cao, Yue [Argonne National Laboratory (ANL), Argonne, IL (United States)], Zhang, Qingteng [Argonne National Laboratory (ANL), Argonne, IL (United States)], Dufresne, Eric M. [Argonne National Laboratory (ANL), Argonne, IL (United States)], Cherukara, Mathew [Argonne National Laboratory (ANL), Argonne, IL (United States)] (ORCID:0000000214756998), Narayanan, Suresh [Argonne National Laboratory (ANL), Argonne, IL (United States)], Holt, Martin V. [Argonne National Laboratory (ANL), Argonne, IL (United States)], Miceli, Antonino [Argonne National Laboratory (ANL), Argonne, IL (United States)], Zhou, Tao [Argonne National Laboratory (ANL), Argonne, IL (United States)] (ORCID:0000000280937666). 2025-03-07. Homomorphic data compression for real time photon correlation analysis. https://doi.org/10.1364/oe.543404

Cite the original work for its findings. Save a collection to share your selection of sources.

KEEP EXPLORING

Related reports

Cyclic moisture reactivation of calcium sorbents for long duration thermochemical energy storage

The transition to a flexible and reliable energy infrastructure, using electro-thermal energy generation technologies such as geothermal, concentrated solar power, and nuclear, usually demands simultaneous advancement of thermal energy storage (TES) to support on-demand electricity generation and industrial applications while mitigating the inherent intermittency of renewable energy sources and power outages from direct energy generation. Among TES technologies, thermochemical energy storage (TCES) based on calcium looping emerges as a compelling high-power energy storage candidate due to its high reaction enthalpy, compatibility with elevated operating temperatures, and abundance of low-cost materials. However, the long-term durability of calcium-based sorbents for TCES is hindered by surface sintering and particle aggregation, leading to performance degradation over repeated thermal cycles. This study explores a moisture hydration-based strategy to regenerate a degraded calcium sorbent and mitigate performance degradation for long duration TCES. The addition of moisture transforms calcium oxide into calcium hydroxide and produces intercalation water layers, associated with a regenerated surface area and reduced calcium oxide crystallite size. Both these effects are beneficial in restoring the sorbents' reactivity for carbonization. Additionally, an optimized hydration-assisted reactivation protocol balances the recovered energy storage capacity with heating penalty required for moisture removal from hydrated samples, resulting in an enhanced energy storage capacity up to 176% compared to benchmark sorbents that undergo cycling without reactivation after 60 cycles. In conclusion, these results highlight the potential of hydration-assisted reactivation to enhance the long-term performance of TCES, providing an effective pathway to advancing electro-thermal storage technologies.

36 MATERIALS SCIENCE