Thermodynamics and transport in molten chloride salts and their mixtures

Cockrell, C. [Nuclear Futures Institute, Bangor University, Bangor LL57 1UT, UK, School of Physical and Chemical Sciences, Queen Mary University of London, Mile End Road, London E1 4NS, UK] (ORCID:0000000285017287); Withington, M. [School of Physical and Chemical Sciences, Queen Mary University of London, Mile End Road, London E1 4NS, UK]; Devereux, H. L. [School of Physical and Chemical Sciences, Queen Mary University of London, Mile End Road, London E1 4NS, UK] (ORCID:0000000194497350); Elena, A. M. [Scientific Computing Department, Science and Technology Facilities Council, Daresbury Laboratory, Keckwick Lane, Daresbury WA4 4AD, UK]; Todorov, I. T. [Scientific Computing Department, Science and Technology Facilities Council, Daresbury Laboratory, Keckwick Lane, Daresbury WA4 4AD, UK] (ORCID:0000000172751784); Liu, Z. K. [Department of Materials Science and Engineering, The Pennsylvania State University, University Park, PA 16802, USA]; Shang, S. L. [Department of Materials Science and Engineering, The Pennsylvania State University, University Park, PA 16802, USA]; McCloy, J. S. [School of Mechanical and Materials Engineering, Washington State University, Pullman, WA, USA] (ORCID:0000000174767771); Bingham, P. A. [Materials and Engineering Research Institute, Sheffield Hallam University, Sheffield S1 1WB, UK]; Trachenko, K. [School of Physical and Chemical Sciences, Queen Mary University of London, Mile End Road, London E1 4NS, UK]

doi:10.1039/d4cp04180a

DOE OSTI · 2483641

Thermodynamics and transport in molten chloride salts and their mixtures

Cockrell, C. [Nuclear Futures Institute, Bangor University, Bangor LL57 1UT, UK, School of Physical and Chemical Sciences, Queen Mary University of London, Mile End Road, London E1 4NS, UK] (ORCID:0000000285017287)·Withington, M. [School of Physical and Chemical Sciences, Queen Mary University of London, Mile End Road, London E1 4NS, UK]·Devereux, H. L. [School of Physical and Chemical Sciences, Queen Mary University of London, Mile End Road, London E1 4NS, UK] (ORCID:0000000194497350)·Elena, A. M. [Scientific Computing Department, Science and Technology Facilities Council, Daresbury Laboratory, Keckwick Lane, Daresbury WA4 4AD, UK]·Todorov, I. T. [Scientific Computing Department, Science and Technology Facilities Council, Daresbury Laboratory, Keckwick Lane, Daresbury WA4 4AD, UK] (ORCID:0000000172751784)·Liu, Z. K. [Department of Materials Science and Engineering, The Pennsylvania State University, University Park, PA 16802, USA]·Shang, S. L. [Department of Materials Science and Engineering, The Pennsylvania State University, University Park, PA 16802, USA]·McCloy, J. S. [School of Mechanical and Materials Engineering, Washington State University, Pullman, WA, USA] (ORCID:0000000174767771)·Bingham, P. A. [Materials and Engineering Research Institute, Sheffield Hallam University, Sheffield S1 1WB, UK]·Trachenko, K. [School of Physical and Chemical Sciences, Queen Mary University of London, Mile End Road, London E1 4NS, UK]

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Abstract

Relationship between thermophysical properties and phonon mean free path. Heat capacity, viscosity, and thermal conductivity in ionic liquids decrease as mean free path decreases and dynamics become less “solid-like” and collect motion diminishes.

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Cockrell, C. [Nuclear Futures Institute, Bangor University, Bangor LL57 1UT, UK, School of Physical and Chemical Sciences, Queen Mary University of London, Mile End Road, London E1 4NS, UK] (ORCID:0000000285017287), Withington, M. [School of Physical and Chemical Sciences, Queen Mary University of London, Mile End Road, London E1 4NS, UK], Devereux, H. L. [School of Physical and Chemical Sciences, Queen Mary University of London, Mile End Road, London E1 4NS, UK] (ORCID:0000000194497350), Elena, A. M. [Scientific Computing Department, Science and Technology Facilities Council, Daresbury Laboratory, Keckwick Lane, Daresbury WA4 4AD, UK], Todorov, I. T. [Scientific Computing Department, Science and Technology Facilities Council, Daresbury Laboratory, Keckwick Lane, Daresbury WA4 4AD, UK] (ORCID:0000000172751784), Liu, Z. K. [Department of Materials Science and Engineering, The Pennsylvania State University, University Park, PA 16802, USA], Shang, S. L. [Department of Materials Science and Engineering, The Pennsylvania State University, University Park, PA 16802, USA], McCloy, J. S. [School of Mechanical and Materials Engineering, Washington State University, Pullman, WA, USA] (ORCID:0000000174767771), Bingham, P. A. [Materials and Engineering Research Institute, Sheffield Hallam University, Sheffield S1 1WB, UK], Trachenko, K. [School of Physical and Chemical Sciences, Queen Mary University of London, Mile End Road, London E1 4NS, UK]. 2025-01-15. Thermodynamics and transport in molten chloride salts and their mixtures. https://doi.org/10.1039/d4cp04180a

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