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Zhao, Chun

Publications and source records attributed to Zhao, Chun.

At least 37 records · Page 2

An overview of mineral dust modeling over East Asia

Dust aerosol, one of the most abundant aerosol species in the atmosphere, has significant impacts on the energy balance and climatic feedback of the Earth system through its influence on solar and terrestrial radiation as well as clouds. East Asia is the one of prominent regions of dust generation. The East Asia dust life cycle and associated radiative and climatic effects are the outstanding science issues in understanding climate change at regional and even global scale. In the past decades, numerous dust models have been developed and applied to comprehend a series of dust-related processes studies, including emission, transport, and deposition, and to understand the effects of dust aerosol on the radiation and climate over East Asian. In this paper, we review the recent achievements and progresses in East Asian dust modeling research and discuss the potential challenges in future studies.

climatic impact↗

Contribution of urbanization to the increase of extreme heat events in an urban agglomeration in east China

Abstract The urban agglomeration of Yangtze River Delta (YRD) is emblematic of China's rapid urbanization during the past decades. Based on homogenized daily maximum and minimum temperature data, the contributions of urbanization to trends of summer extreme temperature indices (ETIs) in YRD are evaluated. Dynamically classifying the observational stations into urban and rural, this study presents unexplored changes in temperature extremes during the past four decades in YRD and quantifies the amplification of the positive trends in ETIs by the urban heat island effect. Overall, urbanization contributes to more than one third of the increase of intensity of extreme heat events in the region, which is comparable to the contribution of greenhouse gases. Compared to rural stations, more notable shifts to the right in the probability distribution of temperature and ETIs are found in urban stations. The rapid urbanization in YRD has resulted in large increases in the risk of heat extremes.

Yang, Xuchao↗

Quantification of marine aerosol subgrid variability and its correlation with clouds based on high‐resolution regional modeling

Abstract One limitation of most global climate models (GCMs) is that with the horizontal resolutions they typically employ, they cannot resolve the subgrid variability (SGV) of clouds and aerosols, adding extra uncertainties to the aerosol radiative forcing estimation. To inform the development of an aerosol subgrid variability parameterization, here we analyze the aerosol SGV over the southern Pacific Ocean simulated by the high‐resolution Weather Research and Forecasting model coupled to Chemistry. We find that within a typical GCM grid, the aerosol mass subgrid standard deviation is 15% of the grid‐box mean mass near the surface on a 1 month mean basis. The fraction can increase to 50% in the free troposphere. The relationships between the sea‐salt mass concentration, meteorological variables, and sea‐salt emission rate are investigated in both the clear and cloudy portion. Under clear‐sky conditions, marine aerosol subgrid standard deviation is highly correlated with the standard deviations of vertical velocity, cloud water mixing ratio, and sea‐salt emission rates near the surface. It is also strongly connected to the grid box mean aerosol in the free troposphere (between 2 km and 4 km). In the cloudy area, interstitial sea‐salt aerosol mass concentrations are smaller, but higher correlation is found between the subgrid standard deviations of aerosol mass and vertical velocity. Additionally, we find that decreasing the model grid resolution can reduce the marine aerosol SGV but strengthen the correlations between the aerosol SGV and the total water mixing ratio (sum of water vapor, cloud liquid, and cloud ice mixing ratios).

Lin, Guangxing↗

Airborne observations reveal elevational gradient in tropical forest isoprene emissions

Terrestrial vegetation emits vast quantities of volatile organic compounds (VOCs) to he atmosphere1-3, which influence oxidants and aerosols leading to complex feedbacks on air quality and climate4-6. Isoprene dominates global non-methane VOC emissions with tropical regions contributing ~80% of global isoprene emissions2. Isoprene emission rates vary over several orders of magnitude for different plant species, and characterizing this immense biological chemodiversity is a challenge for estimating isoprene emission from tropical forests. Here we present the isoprene emission estimates from aircraft direct eddy covariance measurements over the pristine Amazon forest. We report isoprene emission rates that are 3 times higher than satellite top-down estimates and 35% higher than model predictions based on satellite land cover and vegetation specific emission factors (EFs). The results reveal strong correlations between observed isoprene emission rates and terrain elevations which are confirmed by similar correlations between satellite-derived isoprene emissions and terrain elevations. We propose that the elevational gradient in the Amazonian forest isoprene emission capacity is determined by plant species distributions and can explain a substantial degree of isoprene emission variability in tropical forests. Finally, we apply this approach over the central Amazon and use a model to demonstrate the impacts on regional air quality.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

Urbanization-induced urban heat island and aerosol effects on climate extremes in the Yangtze River Delta region of China

Abstract. The WRF-Chem model coupled with a single-layer urban canopy model (UCM) is integrated for 5 years at convection-permitting scale to investigate the individual and combined impacts of urbanization-induced changes in land cover and pollutant emissions on regional climate in the Yangtze River Delta (YRD) region in eastern China. Simulations with the urbanization effects reasonably reproduced the observed features of temperature and precipitation in the YRD region. Urbanization over the YRD induces an urban heat island (UHI) effect, which increases the surface temperature by 0.53 °C in summer and increases the annual heat wave days at a rate of 3.7 d yr−1 in the major megacities in the YRD, accompanied by intensified heat stress. In winter, the near-surface air temperature increases by approximately 0.7 °C over commercial areas in the cities but decreases in the surrounding areas. Radiative effects of aerosols tend to cool the surface air by reducing net shortwave radiation at the surface. Compared to the more localized UHI effect, aerosol effects on solar radiation and temperature influence a much larger area, especially downwind of the city cluster in the YRD. Results also show that the UHI increases the frequency of extreme summer precipitation by strengthening the convergence and updrafts over urbanized areas in the afternoon, which favor the development of deep convection. In contrast, the radiative forcing of aerosols results in a surface cooling and upper-atmospheric heating, which enhances atmospheric stability and suppresses convection. The combined effects of the UHI and aerosols on precipitation depend on synoptic conditions. Two rainfall events under two typical but different synoptic weather patterns are further analyzed. It is shown that the impact of urban land cover and aerosols on precipitation is not only determined by their influence on local convergence but also modulated by large-scale weather systems. For the case with a strong synoptic forcing associated with stronger winds and larger spatial convergence, the UHI and aerosol effects are relatively weak. When the synoptic forcing is weak, however, the UHI and aerosol effects on local convergence dominate. This suggests that synoptic forcing plays a significant role in modulating the urbanization-induced land-cover and aerosol effects on individual rainfall event. Hence precipitation changes due to urbanization effects may offset each other under different synoptic conditions, resulting in little changes in mean precipitation at longer timescales.

54 ENVIRONMENTAL SCIENCES↗

Examining the Hydrological Variations in an Aquaplanet World Using Wave Activity Transformation

Building on the recent advent of the concept of finite-amplitude wave activity, a contour-following diagnostics for column water vapor (CWV) is developed and applied to a pair of aquaplanet model simulations to understand and quantify the higher moments in the global hydrological cycle. The Lagrangian nature of the diagnostics leads to a more tractable formalism for the transient, zonally asymmetric component of the hydrological cycle, with a strong linear relation emerging between the wave activity and the wave component of precipitation minus evaporation ([Formula: see text]). The dry-versus-wet disparity in the transient hydrological cycle is measured by [Formula: see text], and it is found to increase at a super-Clausius–Clapeyron rate at the poleward side of the mean storm track in response to a uniform sea surface temperature (SST) warming and the meridional structure of the increase can be largely attributed to the change of the meridional stirring scale of the midlatitude Rossby waves. Further scaling for [Formula: see text] indicates that the rate of the wavy hydrological cycle, measured by the ratio of [Formula: see text] to the CWV wave activity, is subdued almost everywhere in the extratropics, implying an overall weakening of the transient circulation. Extending the CWV wave activity analysis to the transient moist regions helps reveal some unique characteristics of atmospheric rivers in terms of transport function, minimum precipitation efficiency, and maximum hydrological cycle rate, as well as an overall weakening of the hydrological cycle rate in the atmospheric river regions under SST warming.

Lu, Jian↗

Sensitivity of U.S. summer precipitation to model resolution and convective parameterizations across gray zone resolutions: Sensitivity Across Gray Zone Resolutions

Simulating summer precipitation is a significant challenge for climate models that rely on cumulus parameterizations to represent moist convection processes. Motivated by recent advances in computing that support very high-resolution modeling, this study aims to systematically evaluate the effects of model resolution and convective parameterizations across the gray zone resolutions. Simulations usingthe Weather Research and Forecasting model were conducted at grid spacings of 36 km, 12 km, and 4 km fortwo summers over the conterminous U.S. The convection-permitting simulations at 4 km grid spacing are most skillful in reproducing the observed precipitation spatial distributions and diurnal variability. Notable differences are found between simulations with the traditional Kain-Fritsch (KF) and the scale-aware Grell-Freitas (GF) convection schemes, with the latter more skillful in capturing the nocturnal timing in the Great Plains and North American monsoon regions. The GF scheme also simulates a smoother transition from convective to large-scale precipitation as resolution increases, resulting in reduced sensitivity to model resolution compared to the KF scheme. Nonhydrostatic dynamics has a positive impact on precipitation over complex terrain even at 12 km and 36 km grid spacings. With nudging of the winds toward observations, we show that the conspicuous warm biases in the Southern Great Plains are related to precipitation biases induced by large-scale circulation biases, which are insensitive to model resolution. Overall, notable improvements in simulating summer rainfall and its diurnal variability through convection-permitting modeling and scale-aware parameterizations suggest promising venues for improving climate simulations of water cycle processes.

54 ENVIRONMENTAL SCIENCES↗

An observationally constrained estimate of global dust aerosol optical depth

Here, the role of mineral dust in climate and ecosystems has been largely quantified using global climate and chemistry model simulations of dust emission, transport, and deposition. However, differences between these model simulations are substantial, with estimates of global dust aerosol optical depth (AOD) that vary by over a factor of 5. Here we develop an observationally based estimate of the global dust AOD, using multiple satellite platforms, in situ AOD observations and four state-of-the-science global models over 2004–2008. We estimate that the global dust AOD at 550 nm is 0.030 ± 0.005 (1σ), higher than the AeroCom model median (0.023) and substantially narrowing the uncertainty. The methodology used provides regional, seasonal dust AOD and the associated statistical uncertainty for key dust regions around the globe with which model dust schemes can be evaluated. Exploring the regional and seasonal differences in dust AOD between our observationally based estimate and the four models in this study, we find that emissions in Africa are often overrepresented at the expense of Asian and Middle Eastern emissions and that dust removal appears to be too rapid in most models.

54 ENVIRONMENTAL SCIENCES↗

Sources and pathways of the upscale effects on the Southern Hemisphere jet in MPAS-CAM4 variable-resolution simulations

Impacts of regional grid refinement on large-scale circulations (“upscale effects”) were detected in a previous study that used the Model for Prediction Across Scales-Atmosphere coupled to the physics parameterizations of the Community Atmosphere Model version 4. The strongest upscale effect was identified in the Southern Hemisphere jet during austral winter. This study examines the detailed underlying processes by comparing two simulations at quasi-uniform resolutions of 30 and 120 km to three variable-resolution simulations in which the horizontal grids are regionally refined to 30 km in North America, South America, or Asia from 120 km elsewhere. In all the variable-resolution simulations, precipitation increases in convective areas inside the high-resolution domains, as in the reference quasi-uniform high-resolution simulation. With grid refinement encompassing the tropical Americas, the increased condensational heating expands the local divergent circulations (Hadley cell) meridionally such that their descending branch is shifted poleward, which also pushes the baroclinically unstable regions, momentum flux convergence, and the eddy-driven jet poleward. This teleconnection pathway is not found in the reference high-resolution simulation due to a strong resolution sensitivity of cloud radiative forcing that dominates the aforementioned teleconnection signals. The regional refinement over Asia enhances Rossby wave sources and strengthens the upper level southerly flow, both facilitating the cross-equatorial propagation of stationary waves. Evidence indicates that this teleconnection pathway is also found in the reference high-resolution simulation. Lastly, the result underlines the intricate diagnoses needed to understand the upscale effects in global variable-resolution simulations, with implications for science investigations using the computationally efficient modeling framework.

54 ENVIRONMENTAL SCIENCES↗

Exploring the impacts of physics and resolution on aqua-planet simulations from a nonhydrostatic global variable-resolution modeling framework

Advances in computing resources are gradually moving regional and global numerical forecasting simulations towards sub-10 km resolution, but global high resolution climate simulations remain a challenge. The non-hydrostatic Model for Prediction Across Scales (MPAS) provides a global framework to achieve very high resolution using regional mesh refinement. Previous studies using the hydrostatic version of MPAS (H-MPAS) with the physics parameterizations of Community Atmosphere Model version 4 (CAM4) found notable resolution dependent behaviors. This study revisits the resolution sensitivity using the non-hydrostatic version of MPAS (NH-MPAS) with both CAM4 and CAM5 physics. A series of aqua-planet simulations at global quasi-uniform resolutions ranging from 240 km to 30 km and global variable resolution simulations with a regional mesh refinement of 30 km resolution over the tropics are analyzed, with a primary focus on the distinct characteristics of NH-MPAS in simulating precipitation, clouds, and large-scale circulation features compared to H-MPAS-CAM4. The resolution sensitivity of total precipitation and column integrated moisture in NH-MPAS is smaller than that in H-MPAS-CAM4. This contributes importantly to the reduced resolution sensitivity of large-scale circulation features such as the inter-tropical convergence zone and Hadley circulation in NH-MPAS compared to H-MPAS. In addition, NH-MPAS shows almost no resolution sensitivity in the simulated westerly jet, in contrast to the obvious poleward shift in H-MPAS with increasing resolution, which is partly explained by differences in the hyperdiffusion coefficients used in the two models that influence wave activity. With the reduced resolution sensitivity, simulations in the refined region of the NH-MPAS global variable resolution configuration exhibit zonally symmetric features that are more comparable to the quasi-uniform high-resolution simulations than those from H-MPAS that displays zonal asymmetry in simulations inside the refined region. Overall, NH-MPAS with CAM5 physics shows less resolution sensitivity compared to CAM4. These results provide a reference for future studies to further explore the use of NH-MPAS for high-resolution climate simulations in idealized and realistic configurations.

54 ENVIRONMENTAL SCIENCES↗

Coupling Spectral-bin Cloud Microphysics with the MOSAIC Aerosol Model in WRF-Chem: Methodology and Results for Marine Stratocumulus Clouds

Aerosol-cloud interaction processes can be represented more physically with bin cloud microphysics relative to bulk microphysical parameterizations. However, due to computational power limitations in the past, bin cloud microphysics was often run with very simple aerosol treatments. The purpose of this study is to represent better aerosol-cloud interaction processes in the Chemistry version of Weather Research and Forecast model (WRF-Chem) at convection-permitting scales by coupling spectral-bin cloud microphysics (SBM) with the MOSAIC sectional aerosol model. A flexible interface is built that exchanges cloud and aerosol information between them. The interface contains a new bin aerosol activation approach, which replaces the treatments in the original SBM. It also includes the modified aerosol resuspension and in-cloud wet removal processes with the droplet loss tendencies and precipitation fluxes from SBM. The newly coupled system is evaluated for two marine stratocumulus cases over the Southeast Pacific Ocean with either a simplified aerosol setup or full-chemistry. We compare the aerosol activation process in the newly-coupled SBM-MOSAIC against the SBM simulation without chemistry using a simplified aerosol setup, and the results show consistent activation rates. A longer time simulation reinforces that aerosol resuspension through cloud drop evaporation plays an important role in replenishing aerosols and impacts cloud and precipitation in marine stratocumulus clouds. Evaluation of the coupled SBM-MOSAIC with full-chemistry using aircraft measurements suggests that the new model works realistically for the marine stratocumulus clouds, and improves the simulation of cloud microphysical properties compared to a simulation using MOSAIC coupled with the Morrison two-moment microphysics.

Gao, Wenhua↗

Trans-Pacific transport and evolution of aerosols: Evaluation of quasi-global WRF-Chem simulation with multiple observations

A fully coupled meteorology-chemistry model (WRF-Chem, the Weather Research and Forecasting model coupled with chemistry) has been configured to conduct quasi-global simulation for 5 years (2010–2014) and evaluated with multiple observation data sets for the first time. The evaluation focuses on the simulation over the trans-Pacific transport region using various reanalysis and observational data sets for meteorological fields and aerosol properties. The simulation generally captures the overall spatial and seasonal variability of satellite retrieved aerosol optical depth (AOD) and absorbing AOD (AAOD) over the Pacific that is determined by the outflow of pollutants and dust and the emissions of marine aerosols. The assessment of simulated extinction Ångström exponent (EAE) indicates that the model generally reproduces the variability of aerosol size distributions as seen by satellites. In addition, the vertical profile of aerosol extinction and its seasonality over the Pacific are also well simulated. The difference between the simulation and satellite retrievals can be mainly attributed to model biases in estimating marine aerosol emissions as well as the satellite sampling and retrieval uncertainties. Compared with the surface measurements over the western USA, the model reasonably simulates the observed magnitude and seasonality of dust, sulfate, and nitrate surface concentrations, but significantly underestimates the peak surface concentrations of carbonaceous aerosol likely due to model biases in the spatial and temporal variability of biomass burning emissions and secondary organic aerosol (SOA) production. A sensitivity simulation shows that the trans-Pacific transported dust, sulfate, and nitrate can make significant contribution to surface concentrations over the rural areas of the western USA, while the peaks of carbonaceous aerosol surface concentrations are dominated by the North American emissions. Both the retrievals and simulation show small interannual variability of aerosol characteristics for 2010–2014 averaged over three Pacific sub-regions. Furthermore, the evaluation in this study demonstrates that the WRF-Chem quasi-global simulation can be used for investigating trans-Pacific transport of aerosols and providing reasonable inflow chemical boundaries for the western USA, allowing one to further understand the impact of transported pollutants on the regional air quality and climate with high-resolution nested regional modeling.

54 ENVIRONMENTAL SCIENCES↗

Sensitivity analysis of simulated SOA loadings using a variance-based statistical approach: SENSITIVITY ANALYSIS OF SOA

We investigate the sensitivity of secondary organic aerosol (SOA) loadings simulated by a regional chemical transport model to 7 selected tunable model parameters: 4 involving emissions of anthropogenic and biogenic volatile organic compounds, anthropogenic semi-volatile and intermediate volatility organics (SIVOCs), and NOx, 2 involving dry deposition of SOA precursor gases, and one involving particle-phase transformation of SOA to low volatility. We adopt a quasi-Monte Carlo sampling approach to effectively sample the high-dimensional parameter space, and perform a 250 member ensemble of simulations using a regional model, accounting for some of the latest advances in SOA treatments based on our recent work. We then conduct a variance-based sensitivity analysis using the generalized linear model method to study the responses of simulated SOA loadings to the tunable parameters. Analysis of SOA variance from all 250 simulations shows that the volatility transformation parameter, which controls whether particle-phase transformation of SOA from semi-volatile SOA to non-volatile is on or off, is the dominant contributor to variance of simulated surface-level daytime SOA (65% domain average contribution). We also split the simulations into 2 subsets of 125 each, depending on whether the volatility transformation is turned on/off. For each subset, the SOA variances are dominated by the parameters involving biogenic VOC and anthropogenic SIVOC emissions. Furthermore, biogenic VOC emissions have a larger contribution to SOA variance when the SOA transformation to non-volatile is on, while anthropogenic SIVOC emissions have a larger contribution when the transformation is off. NOx contributes less than 4.3% to SOA variance, and this low contribution is mainly attributed to dominance of intermediate to high NOx conditions throughout the simulated domain. The two parameters related to dry deposition of SOA precursor gases also have very low contributions to SOA variance. This study highlights the large sensitivity of SOA loadings to the particle-phase transformation of SOA volatility, which is neglected in most previous models.

Shrivastava, Manish↗

Mechanisms Contributing to Suppressed Precipitation in Mt. Hua of Central China. Part I: Mountain Valley Circulation

A significant reduction in precipitation in the past decades has been documented over many mountain ranges such as those in central and eastern China. Consistent with the increase of air pollution in these regions, it has been argued that the precipitation trend is linked to the aerosol microphysical effect on suppressing warm rain. Rigorous quantitative investigations on the reasons responsible for the precipitation reduction are lacking. In this study, an improved Weather Research and Forecasting (WRF) Model with online coupled chemistry (WRF-Chem) is applied and simulations are conducted at the convection-permitting scale to explore the major mechanisms governing changes in precipitation from orographic clouds in the Mt. Hua area in central China. It is found that anthropogenic pollution contributes to a ~40% reduction of precipitation over Mt. Hua during the 1-month summertime period. The reduction is mainly associated with precipitation events associated with valley–mountain circulation and a mesoscale cold-front event. In this paper (Part I), the mechanism leading to a significant reduction for the cases associated with valley–mountain circulation is scrutinized. It is found that the valley breeze is weakened by aerosols as a result of absorbing aerosol-induced warming aloft and cooling near the surface as a result of aerosol–radiation interaction (ARI). Here, the weakened valley breeze and the reduced water vapor in the valley due to reduced evapotranspiration as a result of surface cooling significantly reduce the transport of water vapor from the valley to mountain and the relative humidity over the mountain, thus suppressing convection and precipitation in the mountain

54 ENVIRONMENTAL SCIENCES↗

Quantifying the impact of sub-grid surface wind variability on sea salt and dust emissions in CAM5

This paper evaluates the impact of sub-grid variability of surface wind on sea salt and dust emissions in the Community Atmosphere Model version 5 (CAM5). The basic strategy is to calculate emission fluxes multiple times, using different wind speed samples of a Weibull probability distribution derived from model-predicted grid-box mean quantities. In order to derive the Weibull distribution, the sub-grid standard deviation of surface wind speed is estimated by taking into account four mechanisms: turbulence under neutral and stable conditions, dry convective eddies, moist convective eddies over the ocean, and air motions induced by mesoscale systems and fine-scale topography over land. The contributions of turbulence and dry convective eddy are parameterized using schemes from the literature. Wind variabilities caused by moist convective eddies and fine-scale topography are estimated using empirical relationships derived from an operational weather analysis data set at 15 km resolution. The estimated sub-grid standard deviations of surface wind speed agree well with reference results derived from 1 year of global weather analysis at 15 km resolution and from two regional model simulations with 3 km grid spacing. The wind-distribution-based emission calculations are implemented in CAM5. In terms of computational cost, the increase in total simulation time turns out to be less than 3 %. Simulations at 2° resolution indicate that sub-grid wind variability has relatively small impacts (about 7 % increase) on the global annual mean emission of sea salt aerosols, but considerable influence on the emission of dust. Among the considered mechanisms, dry convective eddies and mesoscale flows associated with topography are major causes of dust emission enhancement. With all the four mechanisms included and without additional adjustment of uncertain parameters in the model, the simulated global and annual mean dust emission increase by about 50 % compared to the default model. By tuning the globally constant dust emission scale factor, the global annual mean dust emission, aerosol optical depth, and top-of-atmosphere radiative fluxes can be adjusted to the level of the default model, but the frequency distribution of dust emission changes, with more contribution from weaker wind events and less contribution from stronger wind events. Lastly, in Africa and Asia, the overall frequencies of occurrence of dust emissions increase, and the seasonal variations are enhanced, while the geographical patterns of the emission frequency show little change.

58 GEOSCIENCES↗

Moist Process Biases in Simulations of the Madden–Julian Oscillation Episodes Observed during the AMIE/DYNAMO Field Campaign

Two Madden–Julian oscillation (MJO) episodes observed during the 2011 Atmospheric Radiation Measurement Program MJO Investigation Experiment (AMIE)/DYNAMO field campaign are simulated using a regional model with various cumulus parameterizations, a regional cloud-permitting model, and a global variable-resolution model with a high-resolution region centered over the tropical Indian Ocean. Model biases in relationships relevant to existing instability theories of MJO are examined and their relative contributions to the overall model errors are quantified using a linear statistical model. The model simulations capture the observed approximately log-linear relationship between moisture saturation fraction and precipitation, but precipitation associated with the given saturation fraction is overestimated especially at low saturation fraction values. This bias is a major contributor to the excessive precipitation during the suppressed phase of MJO. After accounting for this bias using a linear statistical model, the spatial and temporal structures of the model-simulated MJO episodes are much improved, and what remains of the biases is strongly correlated with biases in saturation fraction. The excess precipitation bias during the suppressed phase of the MJO episodes is accompanied by excessive column-integrated radiative forcing and surface evaporation. A large portion of the bias in evaporation is related to biases in wind speed, which are correlated with those of precipitation. Furthermore, these findings suggest that the precipitation bias sustains itself at least partly by cloud radiative feedbacks and convection–surface wind interactions.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

Sensitivity of biogenic volatile organic compounds to land surface parameterizations and vegetation distributions in California

Current climate models still have large uncertainties in estimating biogenic trace gases, which can significantly affect atmospheric chemistry and secondary aerosol formation that ultimately influences air quality and aerosol radiative forcing. These uncertainties result from many factors, including uncertainties in land surface processes and specification of vegetation types, both of which can affect the simulated near-surface fluxes of biogenic volatile organic compounds (BVOCs). In this study, the latest version of Model of Emissions of Gases and Aerosols from Nature (MEGAN v2.1) is coupled within the land surface scheme CLM4 (Community Land Model version 4.0) in the Weather Research and Forecasting model with chemistry (WRF-Chem). In this implementation, MEGAN v2.1 shares a consistent vegetation map with CLM4 for estimating BVOC emissions. This is unlike MEGAN v2.0 in the public version of WRF-Chem that uses a stand-alone vegetation map that differs from what is used by land surface schemes. This improved modeling framework is used to investigate the impact of two land surface schemes, CLM4 and Noah, on BVOCs and examine the sensitivity of BVOCs to vegetation distributions in California. The measurements collected during the Carbonaceous Aerosol and Radiative Effects Study (CARES) and the California Nexus of Air Quality and Climate Experiment (CalNex) conducted in June of 2010 provided an opportunity to evaluate the simulated BVOCs. Sensitivity experiments show that land surface schemes do influence the simulated BVOCs, but the impact is much smaller than that of vegetation distributions. This study indicates that more effort is needed to obtain the most appropriate and accurate land cover data sets for climate and air quality models in terms of simulating BVOCs, oxidant chemistry and, consequently, secondary organic aerosol formation.

Zhao, Chun↗

Observed variability of summer precipitation pattern and extreme events in East China associated with variations of the East Asian summer monsoon: VARIABILITY OF SUMMER PRECIPITATION AND EXTREME EVENT IN EAST CHINA

This paper presents a comprehensive analysis of interannual and interdecadal variations of summer precipitation and precipitation-related extreme events in China associated with variations of the East Asian summer monsoon (EASM) from 1979-2012. A high-quality daily precipitation dataset covering 2287 weather stations in China is analyzed. Based on the precipitation pattern analysis using empirical orthogonal functions, three sub-periods of 1979-1992 (period I), 1993-1999 (period II) and 2000-2012 (period III) are identified to be representative of the precipitation variability. Similar significant variability of the extreme precipitation indices is found across four sub-regions in eastern China. The spatial patterns of summer mean precipitation, the number of days with daily rainfall exceeding 95th percentile precipitation (R95p) and the maximum number of consecutive wet days (CWD) anomalies are consistent, but opposite to that of maximum consecutive dry days (CDD) anomalies during the three sub-periods. However, the spatial patterns of hydroclimatic intensity (HY-INT) are notably different from that of the other three extreme indices, but highly correlated to the dry events. The changes of precipitation anomaly patterns are accompanied by the change of the EASM regime and the abrupt shift of the position of the west Pacific subtropical high around 1992/1993 and 1999/2000, respectively, which influence the moisture transport that contributes most to the precipitation anomalies. Lastly, the EASM intensity is linked to sea surface temperature anomaly over the tropical Indian and Pacific Ocean that influences deep convection over the oceans.

EASM↗