Engineering Papers⌕ Search

Engineering topics

Youinou, G.

Publications and source records attributed to Youinou, G..

Laser Ablation Positive-Ion AMS of Neutron Activated Actinides

At Argonne we have enhanced the AMS capabilities of the Argonne Tandem Linac Accelerator System (ATLAS) to attempt to minimize crosstalk between samples and to quickly move from one (M/Q) setting to another in order to make measurements on a large number of samples provided by the MANTRA (Measurement of Actinide Neutron Transmutation Rates by Accelerator mass spectrometry) project. Those improvements include the use of a picosecond laser to ablate actinide material into the source, a new 20- sample holder that can switch samples within 1-2 minutes, and a number of accelerator configuration improvements that allow quick and precise switching between species. In principle, AMS can provide production yields of actinide isotopes produced during the irradiation period at a sensitivity exceeding other mass spectrometry techniques. A total of 27 irradiated samples of a variety of actinides have been provided for measurement. We discuss our experience with these facility improvements and how well we have met our performance goals. In addition, we present preliminary results on a number of the irradiated actinide samples with this approach and compare those results to Multi- Collector ICPMS measurements.

Pardo, R. C.↗

A Versatile Coupled Test Reactor Concept

A Versatile Coupled Test Reactor (VCTR) is a highly reconfigurable, sodium-cooled, coupled fast and thermal spectrum test reactor, which provides (1) a fast flux irradiation environment prototypical of potential fast reactor designs, (2) thermal and epithermal flux irradiation environments complementary to those of ATR and HFIR, and (3) other possibilities, including beam tubes for scientific experiments, irradiation vehicles for isotope production, etc. The ongoing design of a new versatile coupled thermal-fast test reactor at INL that can accommodate both fast and thermal irradiation, technology and safety features tests is described in this paper. A coupled reactor is defined as a reactor with two distinct spectral zones (Fast and Thermal), which are neutronically coupled to each other: some neutrons born in zone F cause fission in zone T and vice-versa. Only fast neutrons are allowed to go from one zone to the other, which is assured by a thermal neutron filter. A distinction of coupling can be made depending on the main purpose of using fuel assemblies with some level of neutron moderation (thermal zone) together with fuel assemblies with as little moderation as possible (fast zone). It can be used mainly to minimize the core power and fissile inventory, or it can be used mainly to provide additional control of the irradiation conditions in the thermal zone. The steady-state neutronics calculations were performed using the three-dimensional continuous-energy Monte Carlo reactor physics burnup calculation code Serpent2. Although, a few changes were necessary to support the Serpent code in calculating the coupling coefficients. Steady state and transient thermal analyses were performed with RELAP5-3D. RELAP5-3D is the latest in the RELAP5 code series developed at INL. One of the core configurations using only low enriched uranium fuel could provide both a high fast neutron flux and a high thermal neutron flux—respectively 3.5E15 n/s.cm2 and 1E15 n/s.cm2—in large volumes while maintaining core power below 300 MW. The use of plutonium in the fast zone provides more flexibility in fuel assembly design than when low enriched uranium is used, the designer has more degrees of freedom to work with; in particular it could provide additional control of the irradiation conditions in the thermal zone. The results showed that the current design fulfills most R&D needs requirements providing high thermal and fast fluxes and wide possibilities for diversified future reactor features test in appropriate loops, both in steady state and during transients.

coupled spectrum↗

VCTR: A Versatile Coupled Test Reactor Concept

The United States has currently no domestic fast neutron test and irradiation capabilities necessary to pursue a strong research and development program related to fast neutron reactors. This lack prevents the testing of fast reactor fuels in a prototypic environment, the testing of new safety features and of new coolants. A new irradiation test reactor is a costly investment that will operate for several decades and the initial specifications are crucial to ensure the relevance of such a facility in the long run. This new test reactor should be highly reconfigurable and allow operation as a fast test reactor or a thermal test reactor or a cou-pled fast-thermal test reactor. This report presents the on-going effort at Idaho National Laboratory (INL) to design a versatile coupled test reactor (VCTR—pronounced Victor) that could fulfill the R&D needs requiring high fast neutron fluxes but also high thermal neutron fluxes in configurations that could not be met in current thermal neutron test reactors such as ATR. The objective of this report is to summarize the efforts undertaken at INL from May 2015 to March 2016 aimed at understanding the main options for designing and building a versatile test reactor, with a primary mission to provide thermal and fast neutrons for irradiation of fuels and materials in a manner complementary to the ATR and HFIR reactors. Other missions can also be considered, including the validation of computer codes and the development of specific reactor technologies.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

Preliminary neutronic study of D{sub 2}O-Cooled high conversion PWRs

This paper presents a preliminary neutronics analysis of tight-pitch D{sub 2}O-cooled high-conversion pressurised water reactors (HPWR) loaded with MOX fuel aiming at high Pu conversion and negative void coefficient. SCALE6.1 code has been exclusively utilized for this study. The analyses are performed in two separate parts. The first part of this paper investigates the performance of axial and internal blankets and seeks break-even or near-breeder core even without the presence of radial blankets. The analyses showed that the relative Pu mass balance was effectively increased by the addition of the axial blanket. The addition of only 4 cm of blanket resulted in the 4000 pcm increase in the void coefficient. Thus, the presence of the axial blanket made the void coefficient hardly negative. The second part of this paper performs sensitivity and uncertainty analyses of integral parameters (k{sub eff} and void coefficient) for selected systems in order to analyze the characters of this high-conversion PWR from different aspects. The uncertainty analysis of k{sub eff} showed that its breakup contributions for D{sub 2}O-HPWR were very similar to other fast systems (SFR and H{sub 2}O-HPWR) such that the key contributors were {sup 238}U inelastic and {sup 239}Pu ν-bar. However, breakup uncertainties of void coefficients showed that while those of D{sub 2}O-HPWR resembled to H{sub 2}O-HPWR, Na elastic became the significant contributor of the void coefficient uncertainty of SFR. Also sensitivity profiles of {sup 238}U inelastic and {sup 239}Pu ν-bar to the void coefficient revealed that those of SFR were quite dissimilar to both HPWRs. The study also found that while the absolute values of void coefficient uncertainty for D{sub 2}O-HPWR were invariant through the burnup, its percentage uncertainty was significantly increased.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Reactor physics behavior of transuranic-bearing TRISO-particle fuel in a pressurized water reactor

Calculations have been performed to assess the neutronic behavior of pins of Fully-Ceramic Micro-encapsulated (FCM) fuel in otherwise-conventional Pressurized Water Reactor (PWR) fuel pins. The FCM fuel contains transuranic (TRU) - only oxide fuel in tri-isotropic (TRISO) particles with the TRU loading coming from the spent fuel of a conventional LWR after 5 years of cooling. Use of the TRISO particle fuel would provide an additional barrier to fission product release in the event of cladding failure. Depletion calculations were performed to evaluate reactivity-limited burnup of the TRU-only FCM fuel. These calculations showed that due to relatively little space available for fuel, the achievable burnup with these pins alone is quite small. Various reactivity parameters were also evaluated at each burnup step including moderator temperature coefficient (MTC), Doppler, and soluble boron worth. These were compared to reference UO{sub 2} and MOX unit cells. The TRU-only FCM fuel exhibits degraded MTC and Doppler coefficients relative to UO{sub 2} and MOX. Also, the reactivity effects of coolant voiding suggest that the behavior of this fuel would be similar to a MOX fuel of very high plutonium fraction, which are known to have positive void reactivity. In general, loading of TRU-only FCM fuel into an assembly without significant quantities of uranium presents challenges to the reactor design. However, if such FCM fuel pins are included in a heterogeneous assembly alongside LEU fuel pins, the overall reactivity behavior would be dominated by the uranium pins while attractive TRU destruction performance levels in the TRU-only FCM fuel pins is retained. From this work, it is concluded that use of heterogeneous assemblies such as these appears feasible from a preliminary reactor physics standpoint. (authors)

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗