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X Liu

Publications and source records attributed to X Liu.

14 records
All sourcesNASA NTRSDOE OSTI
NASA NTRS2020

Aerosol-Ice Formation Closure Pilot Study (AEROICSTUDY) Field Campaign Report

The aerosol-ice formation closure pilot study (AEROICESTUDY) was a field campaign conducted at the U.S. Department of Energy Atmospheric Radiation Measurement (ARM) user facility at the Southern Great Plains (SGP) observatory from October 7 to 28, 2019. The purpose of this campaign was to test a field observational approach for conducting an aerosol-ice formation closure study. In other words, the goal was to predict the number of ice nucleating particles (INPs) from the measurements of physical and chemical aerosol properties and compare those to measured INP number concentrations. This project was motivated by the fact that the aerosol community has widely conducted aerosol radiative closure, aerosol-cloud condensation nuclei (CCN), and CCN-droplet closure studies to test the physical models and parameterizations that cloud-resolving and climate models rely on to perform reliable simulations of the Earth system and energy budget. However, very few closure studies related to INPs have been conducted, and to our knowledge, none using robust, size-resolved, ambient aerosol composition measurements as model inputs.

aerosol-ice formation↗
NASA NTRS2020

Aerosol-Ice Formation Closure Pilot Study (AEROICESTUDY) Field Campaign Report

The aerosol-ice formation closure pilot study (AEROICESTUDY) was a field campaign conducted at the U.S. Department of Energy Atmospheric Radiation Measurement (ARM) user facility at the Southern Great Plains (SGP) observatory from October 7 to 28, 2019. The purpose of this campaign was to test a field observational approach for conducting an aerosol-ice formation closure study. In other words, the goal was to predict the number of ice nucleating particles (INPs) from the measurements of physical and chemical aerosol properties and compare those to measured INP number concentrations. This project was motivated by the fact that the aerosol community has widely conducted aerosol radiative closure, aerosol-cloud condensation nuclei (CCN), and CCN-droplet closure studies to test the physical models and parameterizations that cloud-resolving and climate models rely on to perform reliable simulations of the Earth system and energy budget. However, very few closure studies related to INPs have been conducted, and to our knowledge, none using robust, size-resolved, ambient aerosol composition measurements as model inputs

AEROICESTUDY↗
NASA NTRS2016

Tropospheric Emissions: Monitoring of Pollution (TEMPO)

TEMPO (Tropospheric Emissions: Monitoring of Pollution) was selected in 2012 by NASA as the first Earth Venture Instrument, for launch between 2018 and 2021. It will measure atmospheric pollution for greater North America from space using ultraviolet and visible spectroscopy. TEMPO observes from Mexico City, Cuba, and the Bahamas to the Canadian oil sands, and from the Atlantic to the Pacific, hourly and at high spatial resolution (approximately 2.1 kilometers N/S by 4.4 kilometers E/W at 36.5 degrees N, 100 degrees W). TEMPO provides a tropospheric measurement suite that includes the key elements of tropospheric air pollution chemistry, as well as contributing to carbon cycle knowledge. Measurements are made hourly from geostationary (GEO) orbit, to capture the high variability present in the diurnal cycle of emissions and chemistry that are unobservable from current low-Earth orbit (LEO) satellites that measure once per day. The small product spatial footprint resolves pollution sources at sub-urban scale. Together, this temporal and spatial resolution improves emission inventories, monitors population exposure, and enables effective emission-control strategies. TEMPO takes advantage of a commercial GEO host spacecraft to provide a modest cost mission that measures the spectra required to retrieve ozone (O3), nitrogen dioxide (NO2), sulfur dioxide (SO2), formaldehyde (H2CO), glyoxal (C2H2O2), bromine monoxide (BrO), IO (iodine monoxide),water vapor, aerosols, cloud parameters, ultraviolet radiation, and foliage properties. TEMPO thus measures the major elements, directly or by proxy, in the tropospheric O3 chemistry cycle. Multi-spectral observations provide sensitivity to O3 in the lowermost troposphere, substantially reducing uncertainty in air quality predictions. TEMPO quantifies and tracks the evolution of aerosol loading. It provides these near-real-time air quality products that will be made publicly available. TEMPO will launch at a prime time to be the North American component of the global geostationary constellation of pollution monitoring together with the European Sentinel-4 (S4) and Korean Geostationary Environment Monitoring Spectrometer (GEMS) instruments.

tropospheric measurement suite↗
NASA NTRS2014

TPSAS-NF1676L-18357-DND

High-spectral resolution measurements (in the IR region) from space born infrared sensors can provide sufficient spectral information about cloud properties like cloud top pressure, cloud particle size and cloud optical thickness. Empirical orthogonal function (EOF) based regression scheme was used to retrieve cloud properties along with atmospheric state profiles. A channel based physical inversion scheme was also tried on cloud-contaminated radiances to improve retrieval accuracy achieved by regression scheme. Recently developed principle component (PC) based physical retrieval algorithm utilized the EOF transformation to compress both hyperspectral radiance spectra and atmospherical profiles into PC scores to greatly boost the computational speed while maintaining the information content. The accuracy of the (PC) based radiation transfer model (PCRTM) to simulate top-of the atmosphere(TOA) high-spectral resolution radiance spectra for both clear and cloudy sky conditions has been well tested by comparing with the other line-by-line radiation transfer model and using the observation data. The application of the PCRTM based physical inversion method on simulated IASI radiance under 'cloudy' conditions will be a good integrity test for the new algorithm.

X Liu↗
NASA NTRS2010

TPSAS-NF1676L-10761-DND

The presentation summarizes the NASA CLARREO mission to observe decadal climate change using high accuracy SI traceable reflected solar spectra, infrared emission spectra, and radio occultation from the Earth.

Bruce A Wielicki↗
NASA NTRSDate not supplied

TPSAS-NF1676L-29931-DND

The ACE science working group satellite concept calls for a combination of high spectral resolution aerosol lidar and a polarimeter able to determine vertical profiles of aerosol extinction and clouds. Here we discuss why an HSRL lidar is required to achieve these requirements. The primary advantage of an HSRL over an elastic backscatter lidar is that the HSRL channel allows for the independent retrieval of vertically resolved aerosol extinction without constraint. Not requiring a constraint means greater availability of retrievals in polar regions, on the night side, and in broken cloud situations, plus greater accuracy particularly in the lowest part of the atmosphere and in scenes with aerosol heterogeneity. Advantages go beyond the extinction products. Unlike attenuated backscatter, which is an integrated quantity, the aerosol backscatter coefficient depends only on the aerosol at a specific level in the atmosphere, making it preferable for use in quantitative applications. The aerosol backscatter coefficient is more accurate from an HSRL system compared to the retrieval from a single-channel system. This is because errors in both extinction and backscatter from a single-channel system increase with decreasing altitude, due to the need to accurately characterize the overlying attenuation. This means that an HSRL will also have more valid data in and near the boundary layer where aerosol is of primary interest for air quality and weather applications and for many climate objectives including aerosol-cloud interaction studies. Even cloud properties that do not directly use the HSRL capability (cloud phase and thin cirrus retrievals) benefit from the more accurate calibration of an HSRL system. The improved accuracy of backscatter and extinction also lead to better capabilities for aerosol typing, improved retrievals of aerosol radiative effect, and increased information content for combined lidar + polarimeter retrievals of profiles of microphysical properties such as vertically resolved effective radius.

S P Burton↗
NASA NTRSDate not supplied

Hyperspectral Radiatve Transfer Modeling and its Applications

We will describe a fast radiative transfer model that is specifically designed for hyperspectral remote sensing applications. The fast radiative transfer model is capable of performing efficient and accurate calculations under cloudy condition and in the presence of solar radiations. The model uses a Principal Component Analysis to speed up computational speed. The PCRTM model is capable of simulating top of atmospheric radiance or reflectance spectral from 50 wavenumber to 30000 wavenumber. The PCRTM has a very good accuracy relative to reference line-by-line radiative transfer models and it saves orders of magnitude computational time. We will show comparisons of the PCRTM model to AIRS, CrIS, IASI, NAST-I, and SCIAMACHY data. We will further show results of applying the PCRTM retrieval algorithm to these remote sensing data to retrieve atmospheric temperature and moisture profiles, CO2, CO, CH4, N2O, and O3 profiles, cloud optical depth, size, phase, and height. Surface properties such as surface emissivity spectra and surface skin temperatures are also retrieved simultaneously.

X Liu↗
NASA NTRSDate not supplied

TPSAS-NF1676L-27604-DND

Satellite-based hyperspectral observations provide high information content for the Earth's atmospheric and surface properties; however, in order to analyze hyperspectral data efficiently, fast and accurate radiative transfer model is needed. We have developed a Principal Component-based radiative transfer model (PCRTM) which can simulate radiative transfer in the cloudy atmosphere from far IR to visible and UV spectral regions quickly and accurately. Multi-scattering of multiple layers of clouds/aerosols is included in the model. The computation speed is 3 to 4 orders of magnitude faster than the medium speed correlated-k option MODTRAN5 and LBLRTM. The PCRTM calculated radiance spectra agree with the Modtran and LBLRTM within 0.02%. We will demonstrate the application of the PCRTM forward model for atmospheric and surface property inversions and for climate observation studies.

X Liu↗
NASA NTRSDate not supplied

Polar Vortex Outbreak Air Transport: Observation using Satellite IR Sounder Derived Ozone Product and Comparison with Model

The Single Field of View (SFOV) Sounder Atmospheric Products (SiFSAP) derived from Cross-track Infrared Sounder (CrIS) on SNPP and JPSS have a spatial resolution ( ~14.5 km) better than most global weather and climate models. Most recent significant improvement in the quality of these products enables us to use these high-resolution observation-based sounding data for weather studies and model evaluation. The aim of this study is to explore the value to use these SFOV products for studying the dynamic transport associated with polar vortex outbreak. In a few cases studies, we used SiFSAP products, especially ozone, as well as the data of wind, geopotential height (GPH) and potential velocity (PV) from the fifth-generation ECMWF reanalysis (ERA5) data, to analyze the variation of total ozone, relative humidity and ozone in different layers, as well as their correlation with GPH and PV. Some comparison of the retrieved temperature and water vapor with ERA5 data, and ozone with the Ozone Mapping and Profiler Suite (OMPS) measurements have also been made. It is found (1) the transport of O3-riched polar air accompanying the polar vortex breakup to lower latitude and lower atmosphere, and (2) the transport path of O3 agreeing well with the path of polar cold air (illustrated using the retrieved RH, wind fields and GPH). These results demonstrate the 3-D structure of O3 distribution as derived from CrIS measurements provides some insights of the cold air transport, and can be used to track the dynamic transport of polar cold air following the outbreak of polar vortex. The observed enhancement of O3 following the polar vortex outbreak also suggests some possible linkage between the tropospheric cold air advected with stratospheric air source.

Xiaozhen Xiong↗
NASA NTRSDate not supplied

All-sky Retrieval of Atmospheric Temperature, Water Vapor, Clouds, Trace Gases, and Surface Properties from Operational Hyperspectral IR Sounders

Operational IR sounders such AIRS, CrIS, and IASI provide high quality hyperspectral measurements for weather and climate applications. We will describe a new all-sky Single Field-of-view Sounder Atmospheric Product (SiFSAP). The uniqueness of this product is that it uses all available channels from hyperspectral sounders and the optimal estimation retrieval is done at a single FOV spatial resolution. The SiFSAP includes atmospheric temperature, water vapor, clouds, trace gases, surface skin, and surface emissivity and will be produced operationally at NASA GES DISC. We will describe the core component of the SiFSAP algorithm, which is the Principal Component-based Radiative Transfer Model (PCRTM), and will show example applications of the SiFSAP product for various atmospheric weather and dynamics studies. We also describe a new Climate Fingerprinting Sounder Product (ClimFiSP), which is derived from spatiotemporally averaged level-1 hyperspectral radiances directly. The ClimFiSP algorithm uses consistent radiative kernels and a robust spectral fingerprinting method. It provides fast and accurate data fusion products from multiple satellite sensors. We have applied this method to both AIRS and CrIS (on SNPP and on NOAA 20) data and generated two decades climate data records for atmospheric temperature, water vapor, cloud, trace gases, and surface skin temperature. The ClimFiSP are being transitioned to NASA data centers for routine generations level-3 products.

pcrtm↗
NASA NTRSDate not supplied

Preliminary Results from the HOTTech-2 Venus Weathering Experiment

Rocks exposed on the surface of Venus are subjected to extreme conditions. The most notable features of the planet’s atmosphere are its pressure (93 bars), its temperature (~460 degrees C), and the presence of oxidizing species such as SO 2 . In aggregate, these factors can be expected to alter exposed rocks over geologic timescales. Our understanding of the nature of this alteration is limited, as the conditions on the Venusian surface are unlike any encountered on the surface of Earth. Last summer, we initiated a multi-year experimental study of Venusian weathering processes. This project dovetails with the community’s Venus Exploration Roadmap, as it addresses priorities such as the study of Venus’ modern habitability and preparations for the upcoming VERITAS, DAVINCI+, and EnVision missions.

GEER↗
NASA NTRSDate not supplied

Reduced Dimensionality Analysis of TEMPO Ozone Profile Retrievals Using the Compact Phase Space (CPSR) Algorithm

TEMPO ozone (O 3 ) profile retrievals are expected to have fidelity in the troposphere due the sensitivities of the associated averaging kernels. However, those averaging kernels are severely rank deficiency meaning that a visual inspection of the vertical structure of the averaging kernel profile sensitivities is misleading due linear dependencies in the profile. The Compact Phase Space Retrieval (CPSR) algorithm use singular value decompositions of the averaging kernels and the ‘compressed’ retrieval solution error covariance to project the transformed averaging kernels into a space that removes the linear dependencies and accounts for the solution error uncertainties. In this oral presentation and poster, we apply the CPSR dimensional reduction analysis to TEMPO and TROPOMI O 3 profile retrievals for 13:45 UTC March 29, 2024 to study the phase space characteristics of the transformed averaging kernels as a function of latitude for North America. Our results show that TEMPO generally has more phase space vertical structure in the troposphere than TROPOMI. TEMPO has four to five dominant modes, and TROPOMI has five to six dominant modes. That means that dimensional reduction can reduce the TEMPO resource requirements by ~77% and the TROPOMI requirements by ~81%. Finally, we found that after removing linear dependences and after accounting for solution uncertainties TEMPO still has sensitivities throughout the troposphere.

TEMPO↗