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Trkov, Andrej

Publications and source records attributed to Trkov, Andrej.

Low-Energy Reactions of the n+ 233 U Nuclear Compound System and Its Initial Validation

The strong negative gradient as a function of the epithermal fission fraction (FEPIT) observed in both Evaluated Nuclear Data File (ENDF)/B-VII.1 and ENDF/B-VIII.0 nuclear data libraries poses new challenges for the verification of the n+ 233 U nuclear compound system, especially in the low energy range. The aim of this paper is to summarize the steps forward to consistently update the 233 U evaluated nuclear data to attain improved performance in benchmark calculations; this work is described in detail in a forthcoming paper by Pigni et al.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Which nuclear data can be validated with LLNL pulsed-sphere experiments?

It is shown here that 14-MeV D+T LLNL pulsed-sphere experiments bring complementary information into the process of validating nuclear data compared to experiments that are traditionally used for this purpose—such as critical assemblies. To be more specific, the 14-MeV D+T LLNL pulsed-sphere neutron-leakage spectra enable to validate scattering and fission nuclear data up to 15 MeV (compared to approximately up to 5 MeV when using criticality experiments) and employ to this end simple compound targets containing only few isotopes. In this work, sensitivity profiles of the spectra to nuclear data are calculated in order to understand in detail which isotopes, observables, and energy ranges of nuclear data contribute significantly to their simulation. These profiles are presented for a few selected spheres containing 16 O, 12 C, 56 Fe, and 239 Pu. It is shown that the neutron-leakage spectra of spheres containing light elements are mostly sensitive to elastic- and inelastic-scattering cross sections on discrete levels and corresponding angular distributions. Spheres of structural materials are sensitive to elastic- and inelastic-scattering cross sections, including scattering on discrete levels and the continuum, and double-differential cross sections. Actinide spheres are also strongly sensitive to the fission observables, in particular to the total-fission neutron spectrum. Thin spheres (in which neutrons experience on average less than one scatter) are mostly sensitive to data near the elastic peak, in the energy range from 12–15 MeV, while thicker ones can be sensitive to data at lower incident-neutron energies due to multiple-scattering effects. This information is brought together with simulations of 71 pulsed-sphere neutron-leakage spectra using the ENDF/B-VII.1 and ENDF/B-VIII.0 nuclear-data libraries. This analysis highlights ENDF/B-VIII.0 data that could be further investigated for potential shortcomings ( 6 Li, 12 C, 16 O, 24-26 Mg, 27 Al, 48 Ti, 56 Fe, and 208 Pb) or are likely reliable ( 1,2 H, 7 Li, 9 Be, 14 N, 235,238 U, and 239 Pu) as indicated by validating with LLNL pulsed-sphere experiments.

14-MeV D+T LLNL pulsed-sphere neutron-leakage spec↗

Validation of Recent Changes in Actinide Evaluations U-235, U-233, Pu-239 [Slides]

This presentation discusses U-235 updates, including fluctuations in the fission cross section in the URR range that were refined to represent measured data following the Paradela et al. evaluation. There were small changes to the low-energy resonances to improve the fit to measured capture data from RPI (capture reduced by 5% from 0.06-7.8 eV, by 7.7% from 7.8-11 eV) and there was a very small change to the thermal nu-bar within uncertainties. Discrete level data are stored in MF=6 (format requirement, no impact on calculations) and issues leading to negative eigenvalues in cross-covariances in the RR have been sorted out. In conclusion, many improvements were made to evaluated nuclear data of actinides in the resonance region and above, such as minor changes to U-235 including assessment of changes that depend on the finalization of the O-16 evaluation. U-233 improvements show significant progress in performance and some further improvement might be needed at intermediate energies. Pu-239 ORNL/IAEA evaluation is promising; however, more work is needed.

07 ISOTOPE AND RADIATION SOURCES↗

Status of the RRR evaluations for 233,235 U and 239 Pu [Slides]

The presentation discusses the R -Matrix Analysis of 233 U, 235 U, and 239 Pu and how their interplay among PFNS, TNC, RRR, and neutron multiplicities has a significant impact on the benchmarks. The presentation also discusses the 233 U improved agreement on benchmarks, an additional investigation on the thickness of beryllium reflectors, work on URR (up to 40 keV) and/or extension of RRR (600 eV to 2 keV). Also discussed is how the 235 U progresses on understanding reactivity rates related to depletion calculations, improved agreement with measured (capture) data is quite insensitive to resolve the negative slope, and how the 239 Pu negative slope as a function of the temperature is not understood yet (bias over 2σ lower than measured).

07 ISOTOPE AND RADIATION SOURCES↗

INDEN Fissile Actinide Issues [Slides]

This presentation addresses the outlook for the International Nuclear Data Evaluation Network (INDEN), specifically regarding general issues that have been solved, including Thermal Neutron Constants (TNC) and Prompt Fission Neutron Spectra (PFNS). Other topics discussed include outstanding issues in fissile evaluations, comments on the RPI quasi-differential experiment, and reaction rate testing of trial evaluations in fast assemblies. The presentation concludes by discussing how INDEN interactions strongly helped to find deficiencies in existing evaluations and highlighted potential solutions to existing challenges, that updated trial evaluations for U-235, U-233, Pu-239 are available for testing, that further work is expected on U-235, Pu-239, and U-233, and that performance was tested on the ICSBEP and/or SINBAD benchmarks, during which significant improvement was demonstrated. The INDEN scheme of international collaboration on nuclear data evaluation is working well.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗