Transient convective delayed neutron precursors of 235U for the Molten Salt Reactor Experiment
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Engineering topics
Publications and source records attributed to Taylor, Zack.
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A numerical framework for modeling depletion and mass transport in liquid-fueled molten salt reactions is presented based on exponential time differencing. The solution method involves using the finite volume method to transform the system of partial differential equations (PDEs) into a much larger system of ordinary differential equations. The key part of this method involves solving for the exponential of a matrix. We explore six different algorithms to compute the exponential in a series of progression problems that explore physical transport phenomena in molten salt reactors. This framework shows good results for solving linear parabolic PDEs with each of the six matrix exponential algorithms. For large problems, the series solvers such as Padé and Taylor have large run times, which can be mitigated by using the Krylov subspace.
Molten salt reactors (MSRs) are a class of next-generation nuclear reactors that have received recent industrial and research interest. A generalized species transport solver was implemented in the Virtual Environment for Reactor Applications (VERA) computing suite to extend this tool to analyze liquid-fueled MSRs. This core simulator has been extended to model the transport of fission product gases into a collection of circulating gas bubbles with the purpose of removing the gases. This paper presents the governing species transport equation, along with various nuclear source terms. Development of the source term for phase migration is discussed, along with a simplified interfacial area tracking method. Finally, a case study on a simplified MSR loop is presented in which modeling parameters were varied to assess their impact on gas removal. The steady state results show that parameters such as bubble diameter, gas injection rate and mass transfer coefficient have a low to moderate effect on the fraction of xenon in the core region. Removal efficiency has the greatest effect on the fraction in the core region. After the pump bowl, bubble diameter has a minor effect on the fraction of xenon in the gas void. Finally, these results point out that increasing parameters such as mass transfer coefficient, gas injection rate, and removal efficiency drives the xenon into the circulating gas void, while decreasing bubble diameter also drives xenon into the gas void by increasing interfacial area.
The objective of the integration roadmap is to describe the necessary physics required and a plan for modeling and simulation approach for predicting mass accountancy in molten salt reactors on an engineering scale. The thermophysical properties and the underlying thermodynamics are fundamental inputs. Therefore, the modeling will span length scales from first principles calculations to the engineering scale. The intention is to predict where material accumulates in a reactor core and loop and to understand perturbations on the systems level, for example the downstream effects from a turbine failure
With the resurgence of interest in molten salt reactors, there is a need for new experiments and modeling capabilities to characterize the unique phenomena present in this fluid fuel system. A Versatile Experimental Salt Irradiation Loop (VESIL) is currently under investigation at Idaho National Laboratory to be placed in the Advanced Test Reactor (ATR). One of the key phenomena this proposed experiment plans to elucidate is fission product speciation in the fuel-salt and the subsequent effects this has on the fuel-salt properties, source term generation, and corrosion control. Specifically, noble gases (Xe & Kr) will bubble out to a plenum or off-gas system, and noble metals (Mo, Tc, Te, etc.) will precipitate and deposit in specific zones in the loop. This work extends the mass transfer and species interaction models in CTF (Coolant-Boiling in Rod Arrays—Two Fluids) and applies these models to give a preliminary estimation of fission product behavior in the proposed VESIL design. A noble metal–helium bubble mass transfer model is coupled with the thermal-hydraulic results from CTF to determine the effectiveness of this insoluble fission product (IFP) extraction method for VESIL. Amounts of IFP species extracted to the off-gas system and species distributions in VESIL after a 60-day ATR cycle are reported.
New multiphysics coupling capabilities for molten salt reactor (MSR) analysis have been developed in the Virtual Environment for Reactor Applications (VERA). This development consisted of two main efforts. First, a generic species transport module was added in the CTF code, which is the thermal-hydraulics (TH) code for VERA. This module uses the velocity fields for which CTF solves during the TH calculation to transport species through the core and around the primary loop. Additionally, a gas sparging model has been added to CTF to model the movement of certain species, namely, fission products such as xenon gas, to transport between the molten salt and gas bubbles present in the salt. The second effort in this development was coupling this capability to VERA’s neutron transport code MPACT. This effort focused on coupling the detailed TH transport models in CTF to MPACT to account for feedback effects in the neutron transport calculations. Finally, the thermochemistry code Thermochimica has also been coupled to VERA. Thermochimica performs pointwise calculations for chemical potential and Gibbs free energy and determines what phases are produced by the temperature, pressure, and elemental concentrations at different locations in the primary loop. These capabilities are demonstrated using a model of the Molten Salt Reactor Experiment (MSRE). Furthermore, this reactor operated at Oak Ridge National Laboratory in the 1960s, providing sources of experimental data that were used to develop the model. Various combinations of species were modeled using VERA’s new multiphysics coupling capabilities. Species distributions and reactivity effects behaved as expected for the MSRE model, demonstrating that the coupling is behaving correctly and causing appropriate feedback. The results of these calculations show the potential for VERA to be used for a wide variety of MSR analyses.