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Sun, Ning

Publications and source records attributed to Sun, Ning.

83 records · Page 5
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DOE OSTI2020

Bioprocessing Separations Consortium Three-Year Overview: Technical Advances Process Economics Influence, and State of the Science

The Bioprocessing Separations Consortium solves separations challenges that are unique to bioprocessing. To do this, the Consortium uses two methods: applying existing technologies to new challenges and developing new technologies that may address these unique challenges better than today’s commercial technologies. In its research and development, the Consortium leverages its three core capabilities: materials development and evaluation, process development, and analysis and computation. In its first three years, from 2016 to 2019, the Consortium addressed four critical challenges in biochemical and thermochemical processing. First, the Consortium targeted the fractionation of lignin to enable valorization of this portion of biomass that offers diverse, complex, and valuable building blocks and products. Second, Consortium researchers developed technologies to enable process intensification, which can reduce equipment needs, energy consumption, and waste generation, thereby cutting bioprocessing capital costs and rendering processes more efficient. Third, the Consortium sought to recover carbon from dilute aqueous streams that are common to bioprocessing; recovering dilute carbon can improve process efficiency and economics. Finally, Consortium researchers designed and developed new materials and catalysts to reduce targeted foulants and poisons in bioprocessing streams that can limit the lifetime of downstream catalysts or fermenting microorganisms. Table 1 lists the technologies that were examined and places them in the context of the Consortium’s capabilities, types of bioprocesses, and critical challenges in bioprocessing separations. Overall, across these projects, we have developed separations technologies for 10 bioprocesses, addressed 9 target compounds in bioprocessing, developed 10 materials, and evaluated 4 processes for cost and sustainability.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2020

Bioprocessing Separations Consortium: Three-Year Overview - Technical Advances, Process Economics Influence, and State of the Science

The Bioprocessing Separations Consortium solves separations challenges that are unique to bioprocessing. To do this, the Consortium uses two methods: applying existing technologies to new challenges and developing new technologies that may address these unique challenges better than today’s commercial technologies. In its research and development, the Consortium leverages its three core capabilities: materials development and evaluation, process development, and analysis and computation. In its first three years, from 2016 to 2019, the Consortium addressed four critical challenges in biochemical and thermochemical processing. First, the Consortium targeted the fractionation of lignin to enable valorization of this portion of biomass that offers diverse, complex, and valuable building blocks and products. Second, Consortium researchers developed technologies to enable process intensification, which can reduce equipment needs, energy consumption, and waste generation, thereby cutting bioprocessing capital costs and rendering processes more efficient. Third, the Consortium sought to recover carbon from dilute aqueous streams that are common to bioprocessing; recovering dilute carbon can improve process efficiency and economics. Finally, Consortium researchers designed and developed new materials and catalysts to reduce targeted foulants and poisons in bioprocessing streams that can limit the lifetime of downstream catalysts or fermenting microorganisms. Table 1 lists the technologies that were examined and places them in the context of the Consortium’s capabilities, types of bioprocesses, and critical challenges in bioprocessing separations. Overall, across these projects, we have developed separations technologies for 10 bioprocesses, addressed 9 target compounds in bioprocessing, developed 10 materials, and evaluated 4 processes for cost and sustainability.

09 BIOMASS FUELS↗
DOE OSTI2019

Roles of irrigation and reservoir operations in modulating terrestrial water and energy budgets in the Indian subcontinental river basins

Water management activities affect the terrestrial water cycle by increasing water supply and hence changing the partitioning of surface water and energy budgets over irrigated agricultural land, as well as modifying streamflow seasonality through reservoir operations (for irrigation, hydropower generation, and other purposes). Indian sub-continental basins are strongly influenced by human activities. However, the dynamics of how anthropogenic activities interact with the terrestrial water cycle have not been sufficiently studied over Indian sub-continental Basins. In this study, we applied a well-evaluated water management model, coupled with a large-scale land surface hydrological model with irrigation and reservoir operation schemes to examine the impacts of irrigation and reservoir operations on terrestrial water budgets over the Indian sub-continental basins. We conducted two simulations: one NATURAL (i.e., no irrigation and no reservoirs) and water management scenario (i.e., with irrigation and with reservoir regulations, referred to as MANAGED) over 18 basins from 1951 to 2012. The water management impacts were evaluated by comparing a number of key water and energy budget terms such as evapotranspiration (ET), total runoff (TR), land surface temperature (LST), reservoir storage, and discharge. Our results show that water management activities have significant (p-value < 0.05) impacts on ET and LST in most of the river basins during the pre-monsoon season (February-May). Comparing to the NATURAL scenario, ET under the MANAGED scenario is significantly increased in most basins during pre- and post-monsoon seasons especially in semi-arid regions, and LST is reduced predominately in the pre-monsoon season when irrigation water demand is high.

Shah, Harsh L.↗
DOE OSTI2019

Evaluating next-generation intensity–duration–frequency curves for design flood estimates in the snow-dominated western United States

Civil infrastructure such as culverts and bridges are commonly designed using precipitation-based intensity-duration-frequency (PREC-IDF) curves, which assume that the occurrence of precipitation is in the form of rainfall and immediately available for the rainfall-runoff process. In snow-dominated regions, where most winter precipitation occurs as snow that melts during spring to early summer, the use of standard PREC-IDF curves may lead to substantial underestimation of design floods and high failure risk of infrastructure. In this context, we developed next-generation IDF (NG-IDF) curves that characterize the actual water reaching the land surface (i.e., rainfall plus snowmelt) to enhance standard infrastructure design in snow-dominated regions. This study evaluates the performance of NG-IDF curves coupled with U.S. Department of Agriculture Technical Release 55 hydrologic model in estimating design floods for 246 snowy locations in different hydroclimate regimes of the western United States. Design flood estimates from a well-validated continuous simulation using a physics-based hydrologic model, the Distributed Hydrology Soil Vegetation Model (DHSVM), were used as the performance benchmark. Compared with the benchmark estimates, the standard PREC-IDF curves led to substantial errors in design flood estimates while the NG-IDF curves significantly reduced these errors. For example, the averaged error in the 50-year design flood estimates over the 246 locations was reduced from 31% with the use of PREC-IDF curves to 12% with the use of NG-IDF curves. Despite the different model structures, the single-event NG-IDF approach versus the continuous simulation DHSVM did not exhibit statistically significant differences in 91% of the 246 locations for the 50-year design flood estimates. We find this indicates a satisfactory performance of NG-IDF curves to estimate design flow under the conditions tested in the snow-dominated western United States. This article also presents technical suggestions and the limitations of infrastructure design using NG-IDF curves for regulatory agencies and practicing engineers.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2019

Incorporating Climate Nonstationarity and Snowmelt Processes in Intensity–Duration–Frequency Analyses with Case Studies in Mountainous Areas

In this work, downscaled high-resolution climate simulations were used to provide inputs to the physics-based Distributed Hydrology Soil Vegetation Model (DHSVM), which accounts for the combined effects of snowmelt and rainfall processes, to determine spatially distributed available water for runoff (AWR). After quasi-stationary time windows were identified based on model outputs extracted for two different mountainous field sites in Colorado and California, intensity–duration–frequency (IDF) curves for precipitation and AWR were generated and evaluated at each numerical grid to provide guidance on hydrological infrastructure design. Impacts of snowmelt are found to be spatially variable due to spatial heterogeneity associated with topography according to geostatistical analyses. AWR extremes have stronger spatial continuity compared to precipitation. Snowmelt impacts on AWR are more pronounced at the wet California site than at the semiarid Colorado site. The sensitivities of AWR and precipitation IDFs to increasing greenhouse gas emissions are found to be localized and spatially variable. In subregions with significant snowfall, snowmelt can result in an AWR (e.g., 6-h 100-yr events) that is 70% higher than precipitation. For comparison, future greenhouse gas emissions may increase 6-h 100-yr precipitation and AWR by up to 50% and 80%, respectively, toward the end of this century.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2019

Assessing the Impacts of Hydrologic and Land Use Alterations on Water Temperature in the Farmington River Basin in Connecticut

Aquatic ecosystems can be significantly altered by the construction of dams and modification of riparian buffers and the effects are often reflected in spatial and temporal changes to water temperature. To investigate the implications for water temperature of spatially and temporally varying riparian buffers and dam-induced hydrologic alterations, we have implemented a modeling system (DHSVM-RBM) that couples a spatially distributed land surface hydrologic model, DHSVM, with the distributed stream temperature model, RBM. The basic modeling system has been applied previously to several similar-sized watersheds. However, we have made enhancements to DHSVM-RBM that simulate spatial heterogeneity and temporal variation (i.e. seasonal changes in canopy cover) in riparian vegetation, and we included additional features in DHSVM-RBM that provide the capability for simulating the impacts of reservoirs that may develop thermal stratification. We have tested the modeling system in the Farmington River basin in the Connecticut River system that includes varying types of watershed development (e.g. deforestation and reservoirs) that can alter the streams’ hydrologic regime and thermal energy budget. We evaluated streamflow and stream temperature simulations against all available observations distributed along the Farmington River basin. Results based on metrics recommended for model evaluation compare well to those obtained in similar studies. We demonstrate the way in which the model system can provide decision support for watershed planning by simulating a limited number of scenarios associated with hydrologic and land use alterations.

Freshwater Ecosystem, Water Temperature, Riparian ↗
DOE OSTI2019

Parallel Distributed Hydrology Soil Vegetation Model (DHSVM) using global arrays

The Distributed Hydrology Soil Vegetation Model (DHSVM) code was parallelized for distributed memory computers using Global Arrays (GA). To analyze parallel performance, DHSVM was used to simulate two significantly sized river basins located in northwest continental United States and southwest Canada at 90~m resolution: (1) Clearwater (25,000~km2) and (2) Columbia (668,000~km2). Meteorological forcing applied to both basins was dynamically down-scaled from a global circulation model using the Weather Research and Forecasting (WRF) model and read into DHSVM as 2D maps each time step. We report parallel code speed up was significant. Run times for 1-year simulations were reduced by an order of magnitude for both test basins. A maximum speed up of 105 was attained with 480 processors while simulating the Columbia basin. Speed up was limited by input dominated tasks, particularly the input of meteorological forcing data.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2019

Methyl Ketones from Municipal Solid Waste Blends by One‐Pot Ionic‐Liquid Pretreatment, Saccharification, and Fermentation

Abstract The conversion of municipal solid waste (MSW) and lignocellulosic biomass blends to methyl ketones (MKs) was investigated by using bioderived ionic liquid (bionic liquid)‐based hydrolysates followed by fermentation with an engineered Escherichia coli strain. The hydrolysates were produced by a one‐pot process using six types of MSW–biomass blends, choline‐based bionic liquids, and commercial enzymes. Based on the sugar yields, one blend (corn stover/MSW=95:5, w / w ) and two bionic liquids {cholinium lysinate ([Ch][Lys]) and cholinium aspartate ([Ch] 2 [Asp])} were selected for scale‐up studies. Maximum yields of 82.3 % glucose and 54.4 % xylose were obtained from the selected blend in the scale‐up studies (6 L), which was comparable with 83.6 % glucose and 52.8 % xylose obtained at a smaller scale (0.2 L). Comparable or higher yields of medium‐chain (C 11 –C 17 ) MKs were achieved by using the MSW–biomass blend‐derived hydrolysates, relative to the sugar controls (glucose and xylose) with similar sugar feeding concentrations. Up to 1145 mg L −1 of MKs was produced by using MSW–biomass‐derived hydrolysates, and the MK titer decreased to 300 mg L −1 when the bionic‐liquid concentration in the hydrolysate increased from 1 to 2 %, indicative of bionic‐liquid inhibition. Technoeconomic analysis was conducted to investigate the economic potential of using the selected MSW–biomass blend as a feedstock to produce MKs.

Yan, Jipeng↗
DOE OSTI2019

Sugar extraction and ionic liquid recycling using alkaline solutions

The present invention provides a method for obtaining a monosaccharide from a lignocellulosic material in a form suitable for use as a carbon source in a reaction. In some embodiments, the monosaccharide is in a form suitable for use in a fermentation reaction, e.g., to produce an alcohol such as ethanol.

Sun, Ning↗
DOE OSTI2019

Next-Generation Intensity–Duration–Frequency Curves to Reduce Errors in Peak Flood Design

Precipitation-based intensity–duration–frequency (PREC-IDF) curves are a standard tool used to derive design floods for hydraulic infrastructure worldwide. In snow-dominated regions where a large percentage of flood events are caused by snowmelt and rain-on-snow events, the PREC-IDF design approach can lead to substantial underestimation or overestimation of design floods and associated infrastructure. In this study, next-generation IDF (NG-IDF) curves, which characterize the actual water reaching the land surface, are introduced into the design process to improve hydrologic design. The authors compared peak design flood estimates from the National Resource Conservation Service TR-55 hydrologic model driven by NG-IDF and PREC-IDF curves at 399 Snowpack Telemetry (SNOTEL) stations across the western United States, all of which had at least 30 years of high-quality records. They found that about 70% of the stations in the western United States showed the potential for underdesign, for which the PREC-IDF curves underestimated peak design floods by as much as 324%. These results demonstrated the need to update the use of PREC-IDF curves to the use of NG-IDF curves for hydrologic design in snow-dominated regions.

Yan, Hongxiang↗