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Schmidt, K. Sebastian

Publications and source records attributed to Schmidt, K. Sebastian.

Influence of Aerosol Embedded in Shallow Cumulus Cloud Fields on the Surface Solar Irradiance

Ubiquitous shallow cumulus clouds are associated with complex variability in surface solar irradiance (SSI). Aerosol embedded in the cloud field typically has a much smaller overall radiative effect, but can significantly perturb the shape of the SSI probability density function (PDF). These perturbations have important implications for several applications that utilize SSI, but are poorly quantified and are the subject of this study. Multiple cases of shallow cumulus cloud fields with embedded aerosol are simulated at the Southern Great Plains Atmospheric Observatory using large eddy simulation (LES). The LES-derived cloud and aerosol fields are then ingested into Monte Carlo three-dimensional (3D) radiative transfer to simulate SSI. We find a variety of perturbations to the SSI PDF that depend on aerosol presence and optical properties. The processes leading to these perturbations include extinction of the direct beam that often increases from the clear-sky region toward cloud edge due to aerosol hygroscopic growth, and scattering of radiation by aerosol into cloud shadows. The ability to predict the SSI PDF in the presence of aerosol is assessed by adding three representative aerosol optical properties into an existing machine learning framework. We show that machine learning accurately predicts the SSI PDF across a wide range of conditions with negligible computational expense. Importance metrics reveal the relatively high influence of aerosol optical properties in making the predictions. These new findings highlight the important role that aerosol plays in SSI variability for highly 3D cloud-aerosol environments and provides a computationally efficient route forward for its simulation.

3D radiative transfer↗

An overview of the ORACLES (ObseRvations of Aerosols above CLouds and their intEractionS) project: aerosol–cloud–radiation interactions in the southeast Atlantic basin

Southern Africa produces almost a third of the Earth's biomass burning (BB) aerosol particles, yet the fate of these particles and their influence on regional and global climate is poorly understood. ORACLES (ObseRvations of Aerosols above CLouds and their intEractionS) is a 5-year NASA EVS-2 (Earth Venture Suborbital-2) investigation with three intensive observation periods designed to study key atmospheric processes that determine the climate impacts of these aerosols. During the Southern Hemisphere winter and spring (June-October), aerosol particles reaching 3-5 km in altitude are transported westward over the southeast Atlantic, where they interact with one of the largest subtropical stratocumulus (Sc) cloud decks in the world. The representation of these interactions in climate models remains highly uncertain in part due to a scarcity of observational constraints on aerosol and cloud properties, as well as due to the parameterized treatment of physical processes. Three ORACLES deployments by the NASA P-3 aircraft in September 2016, August 2017, and October 2018 (totaling ~350 science flight hours), augmented by the deployment of the NASA ER-2 aircraft for remote sensing in September 2016 (totaling ~100 science flight hours), were intended to help fill this observational gap. ORACLES focuses on three fundamental science themes centered on the climate effects of African BB aerosols: (a) direct aerosol radiative effects, (b) effects of aerosol absorption on atmospheric circulation and clouds, and (c) aerosol–cloud microphysical interactions. This paper summarizes the ORACLES science objectives, describes the project implementation, provides an overview of the flights and measurements in each deployment, and highlights the integrative modeling efforts from cloud to global scales to address science objectives. Significant new findings on the vertical structure of BB aerosol physical and chemical properties, chemical aging, cloud condensation nuclei, rain and precipitation statistics, and aerosol indirect effects are emphasized, but their detailed descriptions are the subject of separate publications. The main purpose of this paper is to familiarize the broader scientific community with the ORACLES project and the dataset it produced.

54 ENVIRONMENTAL SCIENCES↗

On the Relationship Between Shallow Cumulus Cloud Field Properties and Surface Solar Irradiance

Abstract Shallow cumulus clouds exhibit highly three‐dimensional (3‐D) spatial structure leading to complex variability in the surface solar irradiance (SSI) beneath. This variability is captured by the typically bimodal shape of the SSI probability density function (PDF). Using large eddy simulation to generate well‐resolved cloud fields and Monte Carlo 3‐D radiative transfer to reproduce realistic associated SSI PDFs, we seek direct relationships between the cloud field properties and the SSI PDF shape. Applying both random forest and artificial neural network algorithms, we find variations in the two modes of the SSI PDF are well predicted by just a handful of cloud field properties. The two algorithms utilize cloud properties similarly, with indistinguishable performance despite their different architectures. These results offer a marked improvement in realism relative to one‐dimensional radiative transfer while bypassing computationally expensive 3‐D radiative transfer, with immediate application to renewable energy assessments, and potential for several other geophysical applications.

58 GEOSCIENCES↗

Observation of the Spectrally Invariant Properties of Clouds in Cloudy-to-Clear Transition Zones During the MAGIC Field Campaign

We use the spectrally invariant method to study the variability of cloud optical thickness τau and droplet effective radius r(sub eff) in transition zones (between the cloudy and clear sky columns) observed from Solar Spectral Flux Radiometer (SSFR) and Shortwave Array Spectroradiometer-Zenith (SASZe) during the Marine ARM GPCI Investigation of Clouds (MAGIC) field campaign. The measurements from the SSFR and the SASZe are different, however inter-instrument differences of self-normalized measurements (divided by their own spectra at a fixed time) are small. The spectrally invariant method approximates the spectra in the cloud transition zone as a linear combination of definitely clear and cloudy spectra, where the coefficients, slope and intercept, characterize the spectrally invariant properties of the transition zone. Simulation results from the SBDART (Santa Barbara DISORT Atmospheric Radiative Transfer) model demonstrate that (1) the slope of the visible band is positively correlated with the cloud optical thickness τ while the intercept of the near-infrared band has high negative correlation with the cloud drop effective radius r(sub eff)even without the exact knowledge of τau; (2) the above relations hold for all Solar Zenith Angle (SZA) and for cloud-contaminated skies. In observations using redundant measurements from SSFR and SASZe, we find that during cloudy-to-clear transitions, (a) the slopes of the visible band decrease, and (b) the intercepts of the near-infrared band remain almost constant near cloud edges. The findings in simulations and observations suggest that, while the optical thickness decreases during the cloudy-to-clear transition, the cloud drop effective radius does not change when cloud edges are approached. These results support the hypothesis that inhomogeneous mixing dominates near cloud edges in the studied cases.

spectral invariance↗

Characterizing a New Surface-Based Shortwave Cloud Retrieval Technique, Based on Transmitted Radiance for Soil and Vegetated Surface Types

This paper presents an approach using the GEneralized Nonlinear Retrieval Analysis (GENRA) tool and general inverse theory diagnostics including the maximum likelihood solution and the Shannon information content to investigate the performance of a new spectral technique for the retrieval of cloud optical properties from surface based transmittance measurements. The cumulative retrieval information over broad ranges in cloud optical thickness (tau), droplet effective radius (r(sub e)), and overhead sun angles is quantified under two conditions known to impact transmitted radiation; the variability in land surface albedo and atmospheric water vapor content. Our conclusions are: (1) the retrieved cloud properties are more sensitive to the natural variability in land surface albedo than to water vapor content; (2) the new spectral technique is more accurate (but still imprecise) than a standard approach, in particular for tau between 5 and 60 and r(sub e) less than approximately 20 nm; and (3) the retrieved cloud properties are dependent on sun angle for clouds of tau from 5 to 10 and r(sub e) less than 10 nm, with maximum sensitivity obtained for an overhead sun.

Shannon information content↗

Directly Measured Heating Rates of a Tropical Subvisible Cirrus Cloud

We present the first direct measurements of the infrared and solar heating rates of a tropical subvisible cirrus (SVC) cloud sampled off the east coast of Nicaragua on 25 July 2007 by the NASA ER-2 aircraft during the Tropical Composition, Cloud and Climate Coupling Experiment (TC4). On this day a persistent thin cirrus layer, with mostly clear skies underneath, was detected in real time by the cloud lidar on the ER-2, and the aircraft was directed to profile down through the SVC. Measurements of the net broadband infrared irradiance and spectrally integrated solar irradiance above, below, and through the SVC are used to determine the infrared and solar heating rates of the cloud. The lidar measurements show that the variable SVC layer was located between approximately 13 and 15 km. Its midvisible optical depth varied from 0.01 to 0.10 with a mean of 0.034 +/- 0.033. Its depolarization ratio was approximately 0.4, indicative of ice clouds. From the divergence of the measured net irradiances the infrared heating rate of the SVC was determined to be approximately 2.50 - 3.24 K/d and the solar heating rate was found to be negligible. These values are consistent with previous indirect observations of other SVC and with model-generated heating rates of SVC with similar optical depths. This study illustrates the utility and potential of the profiling sampling strategy employed here. A more fully instrumented high-altitude aircraft that also included in situ cloud and aerosol probes would provide a comprehensive data set for characterizing both the radiative and microphysical properties of these ubiquitous tropical clouds

Bucholtz, Anthongy↗