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Read, W. G.

Publications and source records attributed to Read, W. G..

At least 19 records

Variability in the Speed of the Brewer-Dobson Circulation as Observed by Aura/MLS

We use Aura/MLS stratospheric water vapour (H2O) measurements as tracer for dynamics and infer interannual variations in the speed of the Brewer-Dobson circulation (BDC) from 2004 to 2011. We correlate one-year time series of H2O in the lower stratosphere at two subsequent pressure levels (68 hPa, approx.18.8 km and 56 hPa, approx 19.9 km at the Equator) and determine the time lag for best correlation. The same calculation is made on the horizontal on the 100 hPa (approx 16.6 km) level by correlating the H2O time series at the Equator with the ones at 40 N and 40 S. From these lag coefficients we derive the vertical and horizontal speeds of the BDC in the tropics and extra-tropics, respectively. We observe a clear interannual variability of the vertical and horizontal branch. The variability reflects signatures of the Quasi Biennial Oscillation (QBO). Our measurements confirm the QBO meridional circulation anomalies and show that the speed variations in the two branches of the BDC are out of phase and fairly well anti-correlated. Maximum ascent rates are found during the QBO easterly phase. We also find that transport of H2O towards the Northern Hemisphere (NH) is on the average two times faster than to the Southern Hemisphere (SH) with a mean speed of 1.15m/s at 100 hPa. Furthermore, the speed towards the NH shows much more interannual variability with an amplitude of about 21% whilst the speed towards the SH varies by only 10 %. An amplitude of 21% is also observed in the variability of the ascent rate at the Equator which is on the average 0.2mm/s.

Brewer-Dobson circulation

Correlation among Cirrus Ice Content, Water Vapor and Temperature in the TTL as Observed by CALIPSO and Aura-MLS

Water vapor in the tropical tropopause layer (TTL) has a local radiative cooling effect. As a source for ice in cirrus clouds, however, it can also indirectly produce infrared heating. Using NASA A-Train satellite measurements of CALIPSO and Aura/MLS we calculated the correlation of water vapor, ice water content and temperature in the TTL. We find that temperature strongly controls water vapor (correlation r =0.94) and cirrus clouds at 100 hPa (r = −0.91). Moreover we observe that the cirrus seasonal cycle is highly (r =−0.9) anticorrelated with the water vapor variation in the TTL, showing higher cloud occurrence during December-January-February. We further investigate the anticorrelation on a regional scale and find that the strong anticorrelation occurs generally in the ITCZ (Intertropical Convergence Zone). The seasonal cycle of the cirrus ice water content is also highly anticorrelated to water vapor (r = −0.91) and our results support the hypothesis that the total water at 100 hPa is roughly constant. Temperature acts as a main regulator for balancing the partition between water vapor and cirrus clouds. Thus, to a large extent, the depleting water vapor in the TTL during DJF is a manifestation of cirrus formation.

Flury, T.

Validation of Aura Microwave Limb Sounder HCl Measurements

The Earth Observing System (EOS) Microwave Limb Sounder (MLS) aboard the Aura satellite has provided daily global HCl profiles since August 2004. We provide a characterization of the resolution, random and systematic uncertainties, and known issues for the version 2.2 MLS HCl data. The MLS sampling allows for comparisons with many (~1500 to more than 3000) closely matched profiles from the Halogen Occultation Experiment (HALOE) and Atmospheric Chemistry Experiment Fourier Transform Spectrometer (ACE-FTS). These data sets provide HCl latitudinal distributions that are, overall, very similar to those from (coincident) MLS profiles, although there are some discrepancies in the upper stratosphere between the MLS and HALOE gradients. As found in previous work, MLS and ACE HCl profiles agree very well (within approximately 5%, on average), but the MLS HCl abundances are generally larger (by 10-20%) than HALOE HCl. The bias versus HALOE is unlikely to arise mostly from MLS, as a similar systematic bias (of order 15%) is not observed between average MLS and balloon-borne measurements of HCl, obtained over Fort Sumner, New Mexico, in 2004 and 2005. At the largest pressure (147 hPa) for MLS HCl, a high bias (approximately 0.2 ppbv) is apparent in analyses of low to midlatitude data versus in situ aircraft chemical ionization mass spectrometry (CIMS) HCl measurements from the Aura Validation Experiment (AVE) campaigns in 2004, 2005, and 2006; this bias is also observed in comparisons of MLS and aircraftHCl/O3 correlations. Good agreement between MLS and CIMS HCl is obtained at 100 to 68 hPa. The recommended pressure range for MLS HCl is from 100 to 0.15 hPa.

Earth Observing System (EOS)

Validation of Aura Microwave Limb Sounder O3 and CO Observations in the Upper Troposphere and Lower Stratosphere

Global satellite observations of ozone and carbon monoxide from the Microwave Limb Sounder (MLS) on the EOS Aura spacecraft are discussed with emphasis on those observations in the 2 15 - 100 hPa region (the upper troposphere and lower stratosphere). The precision, resolution and accuracy of the data produced by the MLS "version 2.2" processing algorithms are discussed and quantified. O3 accuracy is estimated at approx.40 ppbv +5% (approx.20 ppbv +20% at 215 hPa) while the CO accuracy is estimated at approx.30 ppbv +30% for pressures of 147 hPa and less. Comparisons with expectations and other observations show good agreements for the O3 product, generally consistent with the systematic errors quoted above. In the case of COY a persistent factor of approx.2 high bias is seen at 215 hPa. However, the morphology is shown to be realistic, consistent with raw MLS radiance data, and useful for scientific study. The MLS CO data at higher altitudes are shown to be consistent with other observations.

Livesey, N. J.

Validation of Aura Microwave Limb Sounder Ozone by Ozonesonde and Lidar Measurements

We present validation studies of MLS version 2.2 upper tropospheric and stratospheric ozone profiles using ozonesonde and lidar data as well as climatological data. Ozone measurements from over 60 ozonesonde stations worldwide and three lidar stations are compared with coincident MLS data. The MLS ozone stratospheric data between 150 and 3 hPa agree well with ozonesonde measurements, within 8% for the global average. MLS values at 215 hPa are biased high compared to ozonesondes by approximately 20% at middle to high latitude, although there is a lot of variability in this altitude region.

validation studies

Validation of the Aura Microwave Limb Sounder middle atmosphere water vapor and nitrous oxide measurements

The quality of the version 2.2 (v2.2) middle atmosphere water vapor and nitrous oxide measurements from the Microwave Limb Sounder (MLS) on the Earth Observing System (EOS) Aura satellite is assessed. The impacts of the various sources of systematic error are estimated by a comprehensive set of retrieval simulations. Comparisons with correlative data sets from ground-based, balloon and satellite platforms operating in the UV/visible, infrared and microwave regions of the spectrum are performed. Precision estimates are also validated, and recommendations are given on the data usage. The v2.2 H2O data have been improved over v1.5 by providing higher vertical resolution in the lower stratosphere and better precision above the stratopause. The single-profile precision is ~0.2–0.3 ppmv (4–9%), and the vertical resolution is ~3–4 km in the stratosphere. The precision and vertical resolution become worse with increasing height above the stratopause. Over the pressure range 0.1–0.01 hPa the precision degrades from 0.4 to 1.1 ppmv (6–34%), and the vertical resolution degrades to ~12–16 km. The accuracy is estimated to be 0.2–0.5 ppmv (4–11%) for the pressure range 68–0.01 hPa. The scientifically useful range of the H2O data is from 316 to 0.002 hPa, although only the 82–0.002 hPa pressure range is validated here. Substantial improvement has been achieved in the v2.2 N2O data over v1.5 by reducing a significant low bias in the stratosphere and eliminating unrealistically high biased mixing ratios in the polar regions. The single-profile precision is ~13–25 ppbv (7–38%), the vertical resolution is ~4–6 km and the accuracy is estimated to be 3–70 ppbv (9–25%) for the pressure range 100–4.6 hPa. The scientifically useful range of the N2O data is from 100 to 1 hPa.

Atlas, E.

Effects of the 2004 El Nino on Tropospheric Ozone and Water Vapor

The global effects of the 2004 El Nino on tropospheric ozone and H2O based on Aura OM1 and MLS measurements are analyzed. Although it was a weak El Nino from a historical perspective, it produced significant changes in these parameters in tropical latitudes. Tropospheric ozone increased by 10-20% over most of the western Pacific region and decreased by about the same amount over the eastern Pacific region. H2O in the upper troposphere showed similar changes but with opposite sign. These zonal changes in tropospheric ozone and H2O are caused by the eastward shift in the Walker circulation in the tropical pacific region during El Nino. For the 2004 El Nino, biomass burning did not have a significant effect on the ozone budget in the troposphere unlike the 1997 El Nino. Zonally averaged tropospheric column ozone did not change significantly either globally or over the tropical and subtropical latitudes.

Chandra, S.

Validation of the Aura Microwave Limb Sounder Temperature and Geopotential Height Measurements

This paper describes the retrievals algorithm used to determine temperature and height from radiance measurements by the Microwave Limb Sounder on EOS Aura. MLS is a "limbscanning" instrument, meaning that it views the atmosphere along paths that do not intersect the surface - it actually looks forwards from the Aura satellite. This means that the temperature retrievals are for a "profile" of the atmosphere somewhat ahead of the satellite. Because of the need to view a finite sample of the atmosphere, the sample spans a box about 1.5km deep and several tens of kilometers in width; the optical characteristics of the atmosphere mean that the sample is representative of a tube about 200-300km long in the direction of view. The retrievals use temperature analyses from NASA's Goddard Earth Observing System, Version 5 (GEOS-5) data assimilation system as a priori states. The temperature retrievals are somewhat deperrde~zt on these a priori states, especially in the lower stratosphere. An important part of the validation of any new dataset involves comparison with other, independent datasets. A large part of this study is concerned with such comparisons, using a number of independent space-based measurements obtained using different techniques, and with meteorological analyses. The MLS temperature data are shown to have biases that vary with height, but also depend on the validation dataset. MLS data are apparently biased slightly cold relative to correlative data in the upper troposphere and slightly warm in the middle stratosphere. A warm MLS bias in the upper stratosphere may be due to a cold bias in GEOS-5 temperatures.

Schwartz, M. J.

Temporal Decrease in Upper Atmospheric Chlorine

We report a steady decrease in the upper stratospheric and lower mesospheric abundances of hydrogen chloride (HCl) from August 2004 through January 2006, as measured by the Microwave Limb Sounder (MLS) aboard the Aura satellite. For 60(deg)S to 60(deg)N zonal means, the average yearly change in the 0.7 to 0.1 hPa (approx.50 to 65 km) region is -27 +/- 3 pptv/year, or -0.78 +/- 0.08 percent/year. This is consistent with surface abundance decrease rates (about 6 to 7 years earlier) in chlorine source gases. The MLS data confirm that international agreements to reduce global emissions of ozone-depleting industrial gases are leading to global decreases in the total gaseous chlorine burden. Tracking stratospheric HCl variations on a seasonal basis is now possible with MLS data. Inferred stratospheric total chlorine (CITOT) has a value of 3.60 ppbv at the beginning of 2006, with a (2-sigma) accuracy estimate of 7%; the stratospheric chlorine loading has decreased by about 43 pptv in the 18-month period studied here. We discuss the MLS HCl measurements in the context of other satellite-based HCl data, as well as expectations from surface chlorine data. A mean age of air of approx. 5.5 years and an age spectrum width of 2 years or less provide a fairly good fit to the ensemble of measurements.

chlorine

Observation of Night OH in the Mesosphere

Satellite measurements from the Aura MLS instrument show a layer of OH near 82 km in the night. This layer confirms earlier measurements by ground-based LIDAR. The MLS and LIDAR observations measure OH in the lowest vibrational state and are distinct, but related chemically, from vibrationally-excited emission from the OH Meinel bands in the near infrared. The Caltech 1-D model has been extended to include vibrational dependence of OH reactions and shows good agreement with MLS OH data and with observations of the Meinel bands. The model shows a chemical lifetime of HO(x) that increases from less than a day at 80 km to over a month at 87 km. Above this altitude transport processes become an important part of HOx chemistry. The model predicts that ground state OH represents 99% of the total OH up to 84 km.

hydroxyl

EOS Microwave Limb Sounder observations of the Antarctic polar vortex breakup in 2004

New observations from the Microwave Limb Sounder (MLS) on NASA’s Aura satellite give a detailed picture of the spring Antarctic polar vortex breakup throughout the stratosphere, with the first daily global HCl profiles providing an unprecedentedly clear view of transport in the lower stratosphere. Poleward transport at progressively lower levels, filamentation, and mixing are detailed in MLS HCl, N2O, H2O, and O3 as the 2004 Antarctic vortex broke up from the top down in early October through late December. Improved MLS H2O data show the subvortex, below the tropical tropopause, breaking up almost simultaneously with the lower stratospheric vortex in December. Vortex remnants persisted in MLS tracers for over a month after the breakup in the midstratosphere, but no more than a week in the lower stratosphere. MLS observations show diabatic descent continuing throughout November, but weak ascent after late October in the lower stratospheric vortex core. Our results extend previous observational transport studies and show consistency with mixing and vortex evolution in meteorological analyses, and with model studies

Pawson, S.

Polar processing and development of the 2004 Antarctic ozone hole : first results from MLS on Aura

The Microwave Limb Sounder (MLS) on Aura is providing an extensive data set on stratospheric winter polar processing, including the first daily global observations of HCl, together with simultaneous measurements of ClO, HNO3, H2O, O3, N2O, and temperature (among others). We present first results charting the evolution of these quantities during the 2004 Antarctic late winter. MLS observations of chlorine deactivation and ozone loss during this period are shown to be consistent with results from the SLIMCAT chemical transport model.

Microwave Limb Sounder (MLS)

EOS Microwave Limb Sounder Observations of the Antarctic Polar Vortex Breakup in 2004

Observations from the Microwave Limb Sounder (MLS) on NASA's new Aura satellite give an unprecedentedly detailed picture of the spring Antarctic polar vortex breakup throughout the stratosphere. HCl is a particularly valuable tracer in the lower stratosphere after chlorine deactivation. MLS HCl, N2O, H2O broke up in the upper stratosphere by early October, in the midstratosphere by early November, and in the lower stratosphere by late December. The subvortex broke up just a few days later than the lower stratospheric vortex. Vortex remnants persisted in the midstratosphere through December, but only through early January 2005 in the lower stratosphere. MLS N2O observations show diabatic descent continuing throughout November, with evidence of weak ascent after late October in the lower stratospheric vortex core.

Manney, G. L.