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Newman, P. A.

Publications and source records attributed to Newman, P. A..

At least 55 records · Page 3

Chance Encounter with a Stratospheric Kerosene Rocket Plume from Russia over California

During a routine ER-2 aircraft high-altitude test flight on April 18, 1997, an unusual aerosol cloud was detected at 20 km altitude near the California coast at about 370 degrees N latitude. Not visually observed by the ER-2 pilot, the cloud was characterized bv high concentration of soot and sulfate aerosol in a region over 100 km in horizontal extent indicating that the source of the plume was a large hydrocarbon fueled vehicle, most likely a launch vehicle powered only by rocket motors burning liquid oxygen and kerosene. Two Russian Soyuz rockets could conceivably have produced the plume. The first was launched from the Baikonur Cosmodrome, Kazakhstan on April 6th; the second was launched from Plesetsk, Russia on April 9. Air parcel trajectory calculations and long-lived tracer gas concentrations in the cloud indicate that the Baikonur rocket launch is the most probable source of the plume. The parcel trajectory calculations do not unambiguously trace the transport of the Soyuz plume from Asia to North America, illustrating serious flaws in the point-to-point trajectory calculations. This chance encounter represents the only measurement of the stratospheric effects of emissions from a rocket powered exclusively with hydrocarbon fuel.

Newman, P. A.↗

Dehydration and Denitrification in the Arctic Polar Vortex During the 1995-1996 Winter

Dehydration of more than 0.5 ppmv water was observed between 18 and 19 km (theta about 450-465 K) at the edge of the Arctic polar vortex on February 1, 1996. More than half the reactive nitrogen (NO(sub y)) had also been removed, with layers of enhanced (sub y) at lower altitudes. Back trajectory calculations show that air parcels sampled inside the vortex had experienced temperatures as low as 188 K within the previous 12 days, consistent with a small amount of dehydration. The depth of the dehydrated layer (about 1 km) and the fact that trajectories passed through the region of ice saturation in one day imply selective growth of a small fraction of particles to sizes large enough (>10 micron) to be irreversibly removed on this timescale. Over 25% of the Arctic vortex in a 20-30 K range of theta is estimated to have been dehydrated in this event.

Hintsa, E. J.↗

Dehydration and Denitrification in the Arctic Polar Vortex During the 1995-1996 Winter

Dehydration of more than 0.5 ppmv water was observed between 18 and 19 km (0-450-465 K) at the edge of the Arctic polar vortex on February 1, 1996. More than half the reactive nitrogen (NO(y)) had also been removed, with layers of enhanced NO(y) at lower altitudes. Back trajectory calculations show that air parcels sampled inside the vortex had experienced temperatures as low as 188 K within the previous 12 days, consistent with a small amount of dehydration. The depth of the dehydrated layer (approximately 1 km) and the fact that trajectories passed through the region of ice saturation in one day imply selective growth of a small fraction of particles to sizes large enough (>10 microns) to be irreversibly removed on this timescale. Over 25% of the Arctic vortex in a 20-30 K range of 0 is estimated to have been dehydrated in this event.

Hintsa, E. J.↗

Dehydration and Denitrification in the Arctic Polar Vortex During the 1995-1996 Winter

Dehydration of more than 0.5 ppmv water was observed between 18 and 19 km (theta approximately 450-465 K) at the edge of the Arctic polar vortex on February 1, 1996. More than half the reactive nitrogen (NO(y)) had also been removed, with layers of enhanced NO(y) at lower altitudes. Back trajectory calculations show that air parcels sampled inside the vortex had experienced temperatures as low as 188 K within the previous 12 days, consistent with a small amount of dehydration. The depth of the dehydrated layer (approximately 1 km) and the fact that trajectories passed through the region of ice saturation in one day imply selective growth of a small fraction of particles to sizes large enough (>10 micrometers) to be irreversibly removed on this timescale. Over 25% of the Arctic vortex in a 20-30 K range Transport of theta is estimated to have been dehydrated in this event.

Hintsa, E. J.↗

Dehydration and Denitrification in the Arctic Polar Vortex During the 1995-1996 Winter

Dehydration of more than 0.5 ppmv water was observed between 18 and 19 km (theta = 450-465 K) at the edge of the Arctic polar vortex on February 1, 1996. More than half the reactive nitrogen (NOy) had also been removed, with layers of enhanced NOy at lower altitudes. Back trajectory calculations show that air parcels sampled inside the vortex had experienced temperatures as low as 188 K within the previous 12 days, consistent with a small amount of dehydration. The depth of the dehydrated layer (approx. 1 km) and the fact that trajectories passed through the region of ice saturation in one day imply selective growth of a small fraction of particles to sizes large enough (>10 micrometers) to be irreversibly removed on this timescale. Over 25% of the Arctic vortex in a 20-30 K range of theta is estimated to have been dehydrated in this event.

Hintsa, E. J.↗

Ozone Budgets from a Global Chemistry/Transport Model and Comparison to Observations from POLARIS

The objective of the Photochemistry of Ozone Loss in the Arctic Region in Summer (POLARIS) field mission was to obtain data to better characterize the summertime seasonal decrease of ozone at mid to high latitudes. The decrease in ozone occurs mainly in the lower stratosphere and is expected to result from in situ chemical destruction. Instrumented balloons and aircraft were used in POLARIS, along with satellites, to measure ozone and chemical species which are involved with stratospheric ozone chemistry. In order to close the seasonal ozone budget, however, ozone transport must also be estimated. Comparison to a global chemistry and transport model (CTM) of the stratosphere indicates how well the summertime ozone loss processes are simulated and thus how well we can predict the ozone response to changing amounts of chemical source gases. Moreover, the model gives insight into the possible relative magnitude of transport contributions to the seasonal ozone decline. Initial comparison to the Goddard CTM, which uses transport winds and temperatures from meteorological data assimilation, shows a high ozone bias in the model and an attenuated summertime ozone loss cycle. Comparison of the model chemical partitioning and ozone catalytic loss rates to those derived from measurements shows fairly close agreement both at ER-2 altitudes (20 km) and higher. This suggests that the model transport is too active in resupplying ozone to the high latitude region, although chemistry failings cannot be completely ruled out. Comparison of ozone and related species will be shown along with a full diagnosis of the model ozone budget and its possible sources of error.

Kawa, S. Randolph↗

Ozone Change from 1992 to 1993 as Observed from SSBUV on the ATLAS-1 and ATLAS-2 Missions

The Shuttle SBUV (SSBUV) conducted its fourth and fifth flights in late March 1992 and early April 1993 along with the ATLAS-1 and ATLAS-2 Shuttle missions, respectively. The two successive SSBUV flights yielded ozone data nearly one year apart. An analysis of the meteorological conditions, namely temperature and winds, during the two flight periods indicate that the conditions in the stratosphere were very similar. The temperatures had significantly warmed from winter throughout most of the stratosphere and the circulation was approaching normal summertime conditions for both periods. SSBUV-4, flown in 1992, measured ozone from approximately 30S to 60N while SSBUV-5, flown in 1993, measured ozone from approximately 55S to 60N. Zonal average column ozone amounts were derived from the two flights and compared to determine if a systematic change in ozone could be detected despite the fact that only a few days from each year were sampled. The comparison indicates that in the latitude range 30N to 60N total ozone was lower in 1993 than in 1992 by about 12%. This change is larger than the observational errors and the expected interannual variations. This result verifies similar data taken from ground and satellites.

Hilsenrath, E.↗

Meteor 3/total ozone mapping spectrometer observations of the 1993 ozone hole

The development of the springtime (September-November) Antarctic ozone hole was observed by the Meteor 3/total ozone mapping spectromter (TOMS) to result in the lowest ozone value, 85 DU (Dobson units) on October 8, 1993, ever measured by TOMS. During late September and early October the region of extremely low ozone values was centered on the geographical pole between 85 deg S and 90 deg S. The geographical extent of the ozone hole region, the area within the 220-DU contour, reached a maximum during the first week in October at a near-circular area covering 24 x 10(exp 6) sq km reaching to the southern tip of South America. This approximately matched the 1992 area record. After the maximum area was reached in early October, the 1993 ozone hole region was significantly larger than during 1992 throughout the remainder of the month of October. The very low ozone values over the Antarctic continent have been confirmed by independent ground-based data. Unlike 1992, the formation of the 1993 Antarctic ozone hole does not coincide with unusually low ozone values observed over most of the globe for the past 2 years. The most recent ozone data from Meteor 3/TOMS show that there has been a recovery at all latitudes from the extraordinarily low values observed during 1992 and part of 1993 after the June 1991 eruption of Mount Pinatubo. Meteor 3/TOMS is described and compared with Nimbus 7/TOMS during the 1991 to May 1993 overlap period. Observations of the 1992 ozone hole are presented from both instruments and are shown to agree within 5 DU.

Herman, J. R.↗

Fine-scale, poleward transport of tropical air during AASE 2

The poleward transport of tropical air in the lower stratosphere during the winter period of the second Airborne Arctic Stratospheric Expedition (AASE 2) (December 1991-March 1992) is examined using contour advection calcutions. These calculations show that filaments of tropical air extend into mid-latitudes, and are wrapped around the equatorward edge of the polar jet. Simultaneously filaments are drawn from the polar vortex and are intermingled with the filaments of tropical air. The tropical filaments are consistent with measurements of chemical tracers taken aboard the ER-2 and DC-8 aircraft which show localized regions, in mid-latitudes, of air with the characteristics of tropical air.

Waugh, D. W.↗

UARS MILS O3 soundings compared with lidar measurements using the conservative coordinates reconstruction technique

A technique based on conservative properties of certain meteorological fields is used to compare ozone measurements from the Microwave Limb Sounder (MLS) on the Upper Atmosphere Research Satellite (UARS) with soundings from a lidar system operated at midlatitudes by the University of L'Aquila, Italy. A few typical cases are analyzed in connection with the position of the vortex relative to the observing station, and it is shown that in general lidar observations taken within the vortex compare well with the UARS data, regardless of whether they are coincident with a satellite overpass. It is shown that such analysis may be useful for comparing measurements of the same quantity taken at different sites using different measurement techniques.

Redaelli, G.↗

Transport out of the lower stratospheric Arctic vortex by Rossby wave breaking

The fine-scale structure in lower stratospheric tracer transport during the period of the two Arctic Airborne Stratospheric Expeditions (January and February 1989; December 1991 to March 1992) is investigated using contour advection with surgery calculations. These calculations show that Rossby wave breaking is an ongoing occurrence during these periods and that air is ejected from the polar vortex in the form of long filamentary structures. There is good qualitative agreement between these filaments and measurements of chemical tracers taken aboard the NASA ER-2 aircraft. The ejected air generally remains filamentary and is stretched and mixed with midlatitude air as it is wrapped around the vortex. This process transfers vortex air into midlatitudes and also produces a narrow region of fine-scale filaments surrounding the polar vortex. Among other things, this makes it difficult to define a vortex edge. The calculations also show that strong stirring can occur inside as well as outside the vortex.

Waugh, D. W.↗

Intrusions into the lower stratospheric Arctic vortex during the winter of 1991-1992

Investigations of the kinematics of the lower stratospheric Arctic vortex during the winter of 1991-1992 using the contour advection with surgery technique reveal three distinct events in which there was substantial intrusion of midlatitude air into the vortex, in apparent contradiction of the view that the polar vortex constitutes an isolated air mass. Two of these events, in late January and mid-February, were well documented. They were predicted in high-resolution forecasts by the European Centre for Medium-Range Weather Forecasts, most clearly in experimental forecasts with reduced diffusion. Direct confirmation of the presence of the intrusions and of their calculated locations was provided by aerosol observations from the airborne differential absorption laser lidar aboard the NASA DC-8, taken as part of the second Airborne Arctic Stratospheric Expedition campaign; aerosol-rich air of midlatitude origin was seen in the expected position of the intrusions. The reality of the February event was also confirmed by in situ measurements from the NASA ER-2. Such events may be significant for the chemical processes taking place within the winter vortex. The intrusions were evidently related to the meteorology of the northern stratosphere during this winter and in particular to persistent tropospheric blocking over the northeastern Atlantic Ocean and western Europe and concomitant ridging into the lower stratospheric vortex in this region. Nevertheless, preliminary investigations have indicated that such events are not uncommon in other northern hemisphere winters, although no such events were found in the southern hemisphere during the Antarctic winter of 1987.

Plumb, R. A.↗

MLS CLO observations and arctic polar vortex temperatures

Analysis of Upper Altmosphere Research Satellite (UARS) Microwave Limb Sounder (MLS) observations in early January 1992 shows a clear relationship between predicted polar stratospheric cloud formation along the back trajectory and elevated ClO amounts. These findings are in good agreement with aircraft observations. The MLS observed variation of ClO amounts within the vortex also fits the pattern of ClO change as a result of air parcel solar exposure and nitric acid photolysis. Outside the polar vortex, the occasional highly elevated ClO appear statistically consistent with MLS measurement noise.

Schoeberl, M. R.↗

Interpretation of NO(x)/NO(y) observations from AASE-2 using a model of chemistry along trajectories

In situ measurements of NO and NO(y) are used to derive the ratio NO(x)/NO(y) along the flight track of the NASA ER-2 aircraft. Data are presented for two flights at midlatitudes in October 1991 during the Airborne Arctic Stratospheric Expedition-2 (AASE-2). Aerosol particle surface area was concurrently measured. The observations are compared with a photochemical model integrated along back trajectories from the aircraft flight track. Comparison of observations with the model run along trajectories and at a fixed position clearly and quantitatively demonstrates the importance of an air parcel's dynamic history in interpretation of local chemical observations. Comparison of the data with model runs under different assumptions regarding heterogeneous chemistry further reinforces the case for occurrence of the reaction of N2O5 + H2O on sulfate aerosol surfaces in the atmosphere. Finally, comparisons for which relative changes in the model and the data are not consistent caution that our ability to resolve all the observations is not yet complete.

Kawa, S. R.↗

The evolution of ClO and NO along air parcel trajectories

Back trajectory analysis of Arctic and Antarctic aircraft data reveals that high ClO concentrations are associated with predicted polar stratospheric cloud (PSCs) encounters. The ClO concentrations within the Arctic and Antarctic polar vortices vary widely but appear to be inversely related to parcel solar exposure since the last PSC interaction. These results imply that production of NO(x) from HNO3 photolysis and reaction with OH is the mechanism for the loss of chlorine radicals through the reformation of chlorine nitrate. Highly denitrified air parcels show no change in ClO with solar exposure. The recovery process is quantitatively duplicated using a model of chemistry along trajectories. Although PSC processing is the primary mechanism for producing elevated ClO amounts, back trajectories apparently unperturbed by PSC's also show slightly elevated ClO levels in 1992 compared to Arctic 1989 and Antarctic 1987 measurements presumably due to the presence of Pinatubo aerosol.

Schoeberl, M. R.↗

New observations of the NOy/N2O correlation in the lower stratosphere

During the Airborne Arctic Stratospheric Expedition 2 (AASE 2), September 1991 through March 1992, in situ measurements of reactive nitrogen (NO(y) and N20 were made in the Northern Hemisphere lower stratosphere. We present an analysis of this new data and compare it with results from similar data taken during AASE in the winter of 1989. In the Northern Hemisphere there is consistent linear correlation of N2O and NO(y) which shows no interannual variation. Cases of departure from a linear correlation are examined and classified as being due to denitrification (NO(y) loss) or sampling air from a region where the photochemical lifetime of NO(y) is decreased. The latter case was observed for the first time in the winter of 1992.

Loewenstein, M.↗

Post-Pinatubo optical depth spectra vs. latitude and vortex structure: Airborne tracking sunphotometer measurements in AASE 2

In January and March 1992, DC-8-measured stratospheric particle optical depth spectra, tau(sub P)(lambda), peaked broadly at midvisible or longer wavelenghts. At mid-to-high northern latitudes outside the vortex, tau(sub p)(526 nm) above about 11 km was as large as 0.22 in both January and March, reflecting continued Pinatubo volcanic influence. In both months, in-vortex tau(sub p)(lambda) above 11 km was smaller than outside-vortex values by a factor of two or more, and in January a strong anticorrelation was observed between tau(sub p)(lambda) and HF column content (an indicator of vortex penetration). In late January at 18-20S, near the edge of the southern subtropical jet, tau(sub p)(526 nm) above 12 km was only about 0.07-0.09, with a flatter spectral shape than northern mid- to high-latitude measurements in both January and March. Occasional high-latitude vertical profiles indicate 6-11-km slab optical depths, Delta tau(sub p)(526 nm), of 0.05 to 0.1, which should be added to the above-11-km values to yield values above 6 km.

Russell, P. B.↗

Post-Pinatubo Optical Depth Spectra VS. Latitude and Vortex Structure: Airborne Tracking Sunphotometer Measurements in AASE 2

In January and March 1992, DC-8-measured stratospheric particle optical depth spectra, (tau)(sub p)(lambda), peaked broadly at midvisible or longer wavelengths. At mid-to-high northern latitudes outside the vortex, tau(sub p)(526 microns) above about 11 km was as large as 0.22 in both January and March, reflecting continued Pinatubo volcanic influence. In both months, in-vortex tau(sub p) above 11 km was smaller than outside-vortex values by a factor of two or more, and in January a strong anticorrelation was observed between tau(sub p)(lambda) and HF column content (an indicator of vortex penetration). In late January at 18-20S, near the edge of the southern subtropical jet, tau(sub p)(526 microns) above 12 km was only about 0.07- 0.09, with a flatter spectral shape than northern mid-to high-latitude measurements in both January and March. Occasional high-latitude vertical profiles indicate 6-1 km slab optical depths, delta(tau)(sub p)(526 micron), of 0.05 to 0.1, which should be added to the above-11-km values to yield values above 6 km.

Russell, P. B.↗