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Miller, D.

Publications and source records attributed to Miller, D..

At least 55 records · Page 3

Direct lifetime measurements of the excited states in Ni 72

The lifetimes of the first excited 2 + and 4 + states in 72 Ni were measured at the National Superconducting Cyclotron Laboratory with the recoil-distance Doppler-shift method, a model-independent probe to obtain the reduced transition probability. Excited states in 72 Ni were populated by the one-proton knockout reaction of an intermediate energy 73 Cu beam. γ-ray-recoil coincidences were detected with the γ-ray tracking array GRETINA and the S800 spectrograph. Our results provide evidence of enhanced transition probability B(E2;2 + → 0 + ) as compared to 68 Ni, but do not confirm the trend of large B(E2) values reported in the neighboring isotope 70 Ni obtained from Coulomb excitation measurement. The results are compared to shell model calculations. Here, the lifetime obtained for the excited 4 + 1 state is consistent with models showing decay of a seniority ν = 4, 4 + state, which is consistent with the disappearance of the 8+ isomer in 72 Ni.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Investigation of the role of 10 Li resonances in the halo structure of 11 Li through the 11 Li(p,d) 10 Li transfer reaction

Here, the first measurement of the one-neutron transfer reaction 11 Li(p,d) 10 Li performed using the IRIS facility at TRIUMF with a 5.7A MeV 11 Li beam interacting with a solid H 2 target is reported. The 10 Li residue was populated strongly as a resonance peak with energy E r = 0.62 ± 0.04 MeV having a total width Γ = 0.33 ± 0.07 MeV. The angular distribution of this resonance is characterized by neutron occupying the 1p 1/2 orbital. A DWBA analysis yields a spectroscopic factor of 0.67 ± 0.12 for p 1/2 removal strength from the ground state of 11 Li to the region of the peak.

10,11Li↗

Neutron and X-ray powder diffraction study of skutterudite thermoelectrics

N- and p-type filled-skutterudite materials prepared for thermoelectric power generation modules were analyzed by neutron diffraction at the POWGEN beam line of the Spallation Neutron Source (SNS) and X-ray diffraction (XRD). The skutterudite powders were processed by melt spinning, followed by ball milling and annealing. The n-type material consists of Ba–Yb–Co–Sb and the p-type material consists of Di–Fe–Ni–Sb or Di–Fe–Co–Sb (Di = didymium, an alloy of Pr and Nd). Powders for prototype module fabrication from General Motors and Marlow Industries were analyzed in this study. XRD and neutron diffraction studies confirm that both the n- and p-type materials have cubic symmetry. Structural Rietveld refinements determined the lattice parameters and atomic parameters of the framework and filler atoms. The cage filling fraction was found to depend linearly on the lattice parameter, which in turn depends on the average framework atom size. Ultimately, this knowledge may allow the filling fraction of these skutterudite materials to be purposefully adjusted, thereby tuning the thermoelectric properties.

36 MATERIALS SCIENCE↗

Structure of Sn 107 studied through single-neutron knockout reactions

The neutron-deficient nucleus Sn-107 has been studied by using the one-neutron knockout reaction. By measuring the decay gamma rays and momentum distributions of reaction residues, the spins of the ground, 5/2 + , and first-excited, 7/2 + , states of Sn-107 have been assigned by comparisons to eikonal-model reaction calculations. We also observed limits on the inclusive and exclusive cross sections and transitions due to neutron removals from below the N = 50 closed shell have been observed. New excited states up to 5.5 MeV in Sn-107 have been identified.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Saltstone 3QCY15 TCLP Toxicity and UTS Results

A Saltstone Disposal Facility (SDF) waste form was prepared in the Savannah River National Laboratory (SRNL) from a Tank 50H sample and Z-Area premix material for the third quarter of calendar year 2015 (3QCY15). After a 28 day cure, a sample of the SDF waste form was collected, and shipped to a certified laboratory for Toxic Characteristic and Universal Treatment Standards (UTS) analysis. The metals analysis is performed using the Toxic Characteristic Leaching Procedure (TCLP).1 The 3QCY15 saltstone sample results meet South Carolina Hazardous Waste Management Regulations (SCHWMR) R.61-79.261.24 and R.61-79.268.48(a) requirements for a nonhazardous waste form with respect to RCRA metals and underlying hazardous constituents (UHC).

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗

High Voltage Test-Stand Research Done on ICRF Antenna Elements of the High-Harmonic Fast-Wave System of NSTX

The twelve-strap high-harmonic fast-wave (HHFW) antenna on NSTX has exhibited a high-voltage standoff around 25 kV during previous experimental campaigns; this standoff needs to be improved for increased power coupling. During the recent NSTX-U upgrade period, a test-stand was set up with two antenna straps along with Faraday screens for testing purposes. Using a diagnostic suite consisting of a fast camera, a residual gas analyzer, a pressure gage, high-voltage probes, and an infrared camera, several interesting discoveries were made, leading to possible improvements of the antenna RF voltage operation level. First, arcing was observed outside the Faraday shields towards the low-voltage ("grounded") end of the straps (faraday shield box ends); this arcing was successfully eliminated by installing an additional grounding point between the Faraday shield box and the vessel wall. Second, considerable outgassing was observed during the RF pulse and the amount of outgassing was found to decrease with increasing RF power, possibly indicative of multipacting. Finally, infrared camera measurements of heating on the Faraday shield assembly suggest that the return currents on the Faraday shield box are highly localized at the box sides and possibly account for the pressure increase observed. Computations of these RF currents using Microwave Studio show qualitative agreement with the heated regions. New grounding points between the antenna box and the vessel have been implemented in NSTX-U, where future tests will be done to determine if the high-voltage standoff has improved. Further antenna improvements will be sought through future experiments on the test stand.

Perkins, R. J.↗

Experimental study of β and β - n decay of the neutron-rich N = 54 isotone As 87

The β-decay properties of neutron-rich 87 As produced in the proton-induced fission of 238 U were studied at the Holifield Radioactive Ion Beam Facility at Oak Ridge National Laboratory. The low-energy excited states in N = 53 87 Se and N = 52 86 Se were identified through β - γ and β-delayed neutron-γ decay of 87 As , respectively. In conclusion, the experimental systematics of low-energy levels of N = 53 isotones, Z = 34 87 Se, and Z = 32 85 Ge, and along with an analysis of shell-model calculations, allow us to discuss the main features of excited states expected for the next N = 53 isotone, 83 Zn .

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

β -decay properties of the very neutron-rich isotopes Ge 86 and As 86

For this research, the β -decay properties of very neutron rich nuclei 86 Ge and 86 As were measured at the Holifield Radioactive Ion Beam Facility at Oak Ridge National Laboratory. Spectroscopic information on new excited states in 86 As and in 86 Se was obtained and is interpreted within an advanced shell model approach. These calculations, previously explaining well the structure of 84 Ge and 85 Ge, are not able to reproduce all the experimentally determined features of the measured level schemes of 86 As and 86 Se. The Gamow-Teller decay of 86 Ge and 86 As is also investigated in a shell-model framework. The fission yield for 86 Ge is discussed.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Analogous intruder behavior near Ni, Sn, and Pb isotopes

Near shell closures, the presence of unexpected states at low energies provides a critical test of our understanding of the atomic nucleus. New measurements for the N = 42 isotones $69\atop{27}$Co and $71\atop{29}$Cu, along with recent data and calculations in the Ni isotopes, establish a full set of complementary, deformed, intruder states astride the closed-shell 28 Ni isotopes. In addition, nuclei with a one-proton hole or one-proton particle adjacent to Z = 28 were populated in β-decay experiments and in multinucleon transfer reactions. A β-decaying isomer, with a 750(250)-ms half-life, has been identified in $69\atop{27}$Co 42 . It likely has low spin and accompanies the previously established 7/2 - state. Complementary data for the levels of isotonic $71\atop{29}$Cu 42 support the presence of a deformed, ΔJ = 1 band built on the proton intruder 7/2 - level at 981 keV. Finally, these data, together with recent studies of lower-mass Co and Cu isotopes and extensive work near 68 Ni , support the view that intruder states based on particle-hole excitations accompany all closed proton shells with Z ≥ 28 .

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Evidence of Soft Dipole Resonance in 11 Li with Isoscalar Character

Here, the first conclusive evidence of a dipole resonance in 11 Li having isoscalar character observed from inelastic scattering with a novel solid deuteron target is reported. The experiment was performed at the newly commissioned IRIS facility at TRIUMF. The results show a resonance peak at an excitation energy of 1.03±0.03 MeV with a width of 0.51±0.11 MeV (FWHM). The angular distribution is consistent with a dipole excitation in the distorted-wave Born approximation framework. The observed resonance energy together with shell model calculations show the first signature that the monopole tensor interaction is important in 11 Li. The first ab initio calculations in the coupled cluster framework are also included.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Experimental Plan for Crystal Accumulation Studies in the WTP Melter Riser

This experimental plan defines crystal settling experiments to be in support of the U.S. Department of Energy – Office of River Protection crystal tolerant glass program. The road map for development of crystal-tolerant high level waste glasses recommends that fluid dynamic modeling be used to better understand the accumulation of crystals in the melter riser and mechanisms of removal. A full-scale version of the Hanford Waste Treatment and Immobilization Plant (WTP) melter riser constructed with transparent material will be used to provide data in support of model development. The system will also provide a platform to demonstrate mitigation or recovery strategies in off-normal events where crystal accumulation impedes melter operation. Test conditions and material properties will be chosen to provide results over a variety of parameters, which can be used to guide validation experiments with the Research Scale Melter at the Pacific Northwest National Laboratory, and that will ultimately lead to the development of a process control strategy for the full scale WTP melter. The experiments described in this plan are divided into two phases. Bench scale tests will be used in Phase 1 (using the appropriate solid and fluid simulants to represent molten glass and spinel crystals) to verify the detection methods and analytical measurements prior to their use in a larger scale system. In Phase 2, a full scale, room temperature mockup of the WTP melter riser will be fabricated. The mockup will provide dynamic measurements of flow conditions, including resistance to pouring, as well as allow visual observation of crystal accumulation behavior.

36 MATERIALS SCIENCE↗

Comparison of HLW Glass Melting Rate Between Frit and Glass Forming Chemicals Using X-Ray Computed Tomography

Efforts are being made to increase the loading of Hanford tank wastes in glass while meeting melter lifetime expectancies, as well as requirements for processing, regulatory compliance, and product quality. To achieve these goals, the Department of Energy – Office of River Protection (DOE-ORP) has requested that the Savannah River National Laboratory (SRNL) support the advancement of glass formulations and process control strategies in various key technical areas, which include melting rate studies. Numerous parameters influence cold cap melting and it is important to identify laboratory test methods to discern changes in melting rate. One of the primary screening tools being used at SRNL for melting rate comparisons is the dry-fed melt rate furnace (MRF). The MRF has been very effective in ranking relative melting rates of candidate frits for the Defense Waste Processing Facility (DWPF) on the laboratory-scale, which has successfully translated to facility operations.

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗

Observation of γ-vibrations and alignments built on non-ground-state configurations in ¹⁵⁶Dy

The exact nature of the lowest K π =2⁺ rotational bands in all deformed nuclei remains obscure. Traditionally they are assumed to be collective vibrations of the nuclear shape in the γ degree of freedom perpendicular to the nuclear symmetry axis. Very few such γ-bands have been traced past the usual back-bending rotational alignments of high-j nucleons. We have investigated the structure of positive-parity bands in the N=90 nucleus ¹⁵⁶Dy, using the ¹⁴⁸Nd(¹²C,4n)¹⁵⁶Dy reaction at 65 MeV, observing the resulting γ-ray transitions with the Gammasphere array. The even- and odd-spin members of the π =2⁺ γ-band are observed to 32⁺ and 31⁺ respectively. This rotational band faithfully tracks the ground-state configuration to the highest spins. The members of a possible γ-vibration built on the aligned yrast S-band are observed to spins 28⁺ and 27⁺. An even-spin positive-parity band, observed to spin 24⁺, is a candidate for an aligned S-band built on the seniority-zero configuration of the 0₂⁺ state at 676 keV. As a result, the crossing of this band with the 0₂⁺ band is at hw c = 0.28(1) MeV and is consistent with the configuration of the 0₂⁺ band not producing any blocking of the monopole pairing.

38 RADIATION CHEMISTRY, RADIOCHEMISTRY, AND NUCLEA↗

Saltstone 4QCY14 TCLP Toxicity and UTS Results

A Saltstone Disposal Facility (SDF) waste form was prepared in the Savannah River National Laboratory (SRNL) from a Tank 50H sample and Z-Area premix material for the fourth quarter of calendar year 2014 (4QCY14). After a 47 day cure, a sample of the SDF waste form was collected, and shipped to a certified laboratory for Toxic Characteristic and Universal Treatment Standards (UTS) analysis. The metals analysis is performed using the Toxic Characteristic Leaching Procedure (TCLP) . The 4QCY14 saltstone sample results show that the saltstone is Resource Conservation Recovery Act (RCRA) nonhazardous, but is greater than the universal treatment standard for land disposal. The Saltstone Production Facility (SPF) and SDF were in a maintenance outage during the 4QCY14. Thus no processing or disposal of saltstone, as characterized by this 4QCY14 sample, occurred.

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗

Beta decay of the most neutron-rich isotopes close to $^{78}$Ni

In an experiment at the HRIBF, Oak Ridge National Laboratory, USA, we have investigated excited states in 86 Se populated in the beta-decay of 86 As. Here, several new transitions were identified. Preliminary results are presented.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Extrapolating Accelerated UV Weathering Data: Perspective From PVQAT Task Group 5 (Presentation)

Taskgroup 5 (TG5) is concerned with a accelerated aging standard incorporating factors including ultraviolet radiation, temperature, and moisture. Separate experiments are being conducted in support of a test standard via the regional sub-groups in Asia, Europe, and the United States. The authors will describe the objectives and timeline for the TG5 interlaboratory study being directed out of the USA. Qualitative preliminary data from the experiment is presented. To date, the encapsulation transmittance experiment has: replicated behaviors of fielded materials (including specimen location- and formulation additive-specific discoloration); demonstrated coupling between UV aging and temperature; demonstrated that degradation in EVA results from UV- aging; and obtained good qualitative comparison between Xe and UVA-340 sources for EVA. To date, the encapsulation adhesion experiment (using the compressive shear test to quantify strength of attachment) has demonstrated that attachment strength can decrease drastically (>50%) with age; however, early results suggest significant factor (UV, T, RH) dependence. Much remains to be learned about adhesion.

14 SOLAR ENERGY↗