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McDonald, Benjamin S

Publications and source records attributed to McDonald, Benjamin S.

Phase Contrast X-ray Imaging Signatures for Security Applications

Abstract: Differential phase contrast imaging with a grating interferometer is a promising new radiographic technique providing three distinct contrast mechanisms - absorption, phase, and scatter (or dark field) - using a conventional x-ray tube source. We investigate the signatures available in these three contrast mechanisms with attention towards potential security applications. We find that the scatter mode in particular is sensitive to textured materials, enabling lowered detection limits than absorption for materials such as powders. We investigate the length scales to which our imaging system is sensitive.

Environmental Molecular Sciences Laboratory↗

Characterization of a New Lead Slowing Down Spectrometer

There is considerable interest in developing direct measurement methods to determine the plutonium content of spent nuclear fuel within a fuel assembly. One technique that may prove successful is lead slowing-down spectroscopy. Lead Slowing Down Spectroscopy (LSDS) has been used for decades to make cross-section measurements on relatively small isotopic samples of well know masses. For spent fuel assembly measurements, LSDS will be applied in reverse; unknown masses will be determined using well-know cross-sections. In the LSDS, a pulse of neutrons (on the order of 10-100 MeV) is injected into a large lead stack (~ 1m3). The neutrons quickly down-scatter but exhibit little spread in energy about the average, continually-decreasing neutron energy making for a strong correlation between the elapsed time from the initial pulse and the average energy of the neutron. By measuring this elapsed time, it is possible to measure interactions of the neutrons with the fuel in the 0.1 to 1,000 eV range. Many of the actinides have strong resonances in this region, making it possible, through careful measurements and analysis, to extract isotopic masses from LSDS measurements. Pacific Northwest National Laboratory is actively conducting research on both LSDS measurement and data analysis techniques. This paper will present results of the effort to construct and characterize a new lead slowing down spectrometer. The spectrometer was designed to begin testing both experimental measurement and data analysis techniques for determining the plutonium content of spent fuel. To characterize the spectrometer, a series of (n,γ) experiments were conducted to measure the correlation between the time after the neutrons enter the lead and the energy of the interaction. Results from these measurements as well as plans for future development of the spectrometer will be discussed.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Low-Intrusion Techniques and Sensitive Information Management for Warhead Counting and Verification: FY2011 Annual Report

Future arms control treaties may push nuclear weapons limits to unprecedented low levels and may entail precise counting of warheads as well as distinguishing between strategic and tactical nuclear weapons. Such advances will require assessment of form and function to confidently verify the presence or absence of nuclear warheads and/or their components. Imaging with penetrating radiation can provide such an assessment and could thus play a unique role in inspection scenarios. Yet many imaging capabilities have been viewed as too intrusive from the perspective of revealing weapon design details, and the potential for the release of sensitive information poses challenges in verification settings. A widely held perception is that verification through radiography requires images of sufficient quality that an expert (e.g., a trained inspector or an image-matching algorithm) can verify the presence or absence of components of a device. The concept of information barriers (IBs) has been established to prevent access to relevant weapon-design information by inspectors (or algorithms), and has, to date, limited the usefulness of radiographic inspection. The challenge of this project is to demonstrate that radiographic information can be used behind an IB to improve the capabilities of treaty-verification weapons-inspection systems.

98 NUCLEAR DISARMAMENT, SAFEGUARDS, AND PHYSICAL P↗

Non-Invertible Transforms for Image-Based Verification

Imaging may play a unique role in verifying the presence and distribution of warhead components in warhead counting and dismantlement settings where image information content can distinguish among shapes, forms, and material composition of items. However, a major issue with imaging is the high level of intrusiveness, and in particular, the possible need to store sensitive comparison images in the inspection system that would violate information barrier (IB) principles. Reducing images via transformations or feature extraction can produce image features (e.g. attributes) for verification, but with enough prior information about structure the reduced information itself may be sufficient to deduce sensitive details of the original image. Further reducing resolution of the transformed image information is an option, but too much reduction destroys the quality of the attribute. We study the possibility of a one-way transform that allows storage of non-sensitive reference information and analysis to enable comparison of transformed images within IB constraints. In particular, we consider the degree to which images can be reconstructed from image intensity histograms depending on the number of pixel intensity bins and the degree of frequency data quantization, as well as assumed knowledge of configuration of objects in the images. We also explore the concept of a 'perceptual hash' as a class of transforms that may enable verification with provable non-invertibility, leading to an effective one-way transform that preserves the nature of the image feature data without revealing sufficient information to reconstruct the original image.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

MODEL AND ALGORITHM EVALUATION FOR THE HYBRID UF6 CONTAINER INSPECTION SYSTEM

ABSTRACT Pacific Northwest National Laboratory (PNNL) is developing an automated UF6 cylinder verification station concept based on the combined collection of traditional enrichment-meter (186 keV photons from U-235) data and non-traditional, neutron-induced, high-energy gamma-signatures (3-8.5 MeV) with an array of collimated, medium-resolution scintillators. Previous (2010) work at PNNL demonstrated proof-of-principle that this hybrid method yields accurate, full-volume assay of the cylinder enrichment, reduces systematic errors when compared to several other enrichment assay methods, and provides simplified instrumentation and algorithms suitable for long-term unattended operations. We used Monte Carlo modeling with MCNP5 to support system design (e.g., number and configuration of detector arrays, and design of iron/poly collimators for enhanced (n,γ) conversion) and enrichment algorithm development. We developed a first-generation modeling framework in 2010. These tools have since been expanded, refined and benchmarked against field measurements with a prototype system of a 30B cylinder population (0.2 to 4.95 weight % U-235). The MCNP5 model decomposes the radiation transport problem into a linear superposition of “basis spectra” representing contributions from the different uranium isotopes and gamma-ray generation mechanisms (e.g. neutron capture). This scheme accommodates fast generation of “virtual assay signatures” for arbitrary enrichment, material age, and fill variations. Ongoing (FY-2011) refinements to the physics model include accounting for generation of bremsstrahlung photons, arising primarily from the beta decay of Pa-234m, a U-238 daughter. We are using the refined model to optimize collimator design for the hybrid method. The traditional assay method benefits from a high degree of collimation (to isolate each detector’s field-of-view) and relatively small detector area, while the non-traditional method benefits from a wide field-of-view, i.e. less collimation and larger detectors. We implement the enrichment-meter method by applying a square-wave digital filter to a raw spectrum and extracting the 186-keV peak area directly from the convolute spectrum. Ongoing enhancements to this approach include mitigating a systematic peak-area measurement deficit arising from curvature in the spectrum continuum shape. An optimized system prototype based on model results is utilized in a new set of 2011 field measurements, and model and measurement enrichment assay uncertainties are compared.

MODEL AND ALGORITHM EVALUATION FOR THE HYBRID UF6 ↗

Phase Contrast X-ray Imaging Signatures for Homeland Security Applications

Gratings-based phase contrast imaging is a promising new radiographic technique providing three distinct contrast mechanisms, absorption, phase, and scatter, using a conventional x-ray tube source. We investigate the signatures available in these three contrast mechanisms with particular attention towards potential homeland security applications. We find that the scatter mode in particular is sensitive to textured materials, enabling lowered detection limits than absorption for materials such as powders. We investigate the length scales to which our imaging system is sensitive.

99 GENERAL AND MISCELLANEOUS↗

IMAGE-BASED VERIFICATION: SOME ADVANTAGES, CHALLENGES, AND ALGORITHM-DRIVEN REQUIREMENTS

ABSTRACT Imaging technologies may be a particularly useful technique that supports monitoring and verification of deployed and stockpiled nuclear weapons and dismantlement components. However, protecting the sensitive design information requires processing the image behind an information barrier and reporting only non-sensitive attributes related to the image. Reducing images to attributes may destroy some sensitive information, but the challenge remains. For example, reducing the measurement to an attribute such as defined shape and X-ray transmission of an edge might reveal sensitive information relating to shape, size, and material composition. If enough additional information is available to analyze with the attribute, it may still be possible to extract sensitive design information. In spite of these difficulties, the implementation of new treaty requirements may demand image technology as an option. Two fundamental questions are raised: What (minimal) information is needed from imaging to enable verification, and what imaging technologies are appropriate? PNNL is currently developing a suite of image analysis algorithms to define and extract attributes from images for dismantlement and warhead verification and counting scenarios. In this talk, we discuss imaging requirements from the perspective of algorithms operating behind information barriers, and review imaging technologies and their potential advantages for verification. Companion talks will concentrate on the technical aspects of the algorithms.

IMAGE-BASED VERIFICATION: SOME ADVANTAGES, CHALLEN↗