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Loewenstein, Max

Publications and source records attributed to Loewenstein, Max.

At least 19 records

Airborne Observations of Carbon Dioxide and Methane Emission Ratios from the Yosemite Rim Wildfire, California

This paper presents airborne in situ measurements of carbon dioxide (CO2) and methane (CH4) downwind of an exceptionally large wildfire, the Rim Fire, near Yosemite, California, during two flights. Data analyses are discussed in terms of emission ratios (ER) and emission factors (EF) and are compared to previous studies. CH4 ER’s were 7.5-7.9 parts per billion (ppb) CH4 for every 1 part per million (ppm) of CO2 (ppb CH4 (ppm CO2)(exp.-1)) on 29 August 2013 and 14.2-16.7 ppb CH4 (ppm CO2)(exp. -1) on 10 September 2013. This study measured only CO2 and CH4; however, estimated emission factors (EEF’s) are used as rough estimates of EF’s of CO2 and CH4 and are in close agreement with EF’s reported in previous studies. In the western US, wildfires dominate over prescribed fires, contributing to atmospheric trace gas budgets and regional and local air pollution. Limited sampling of emissions from wildfires means western US emission estimates rely largely on data from prescribed fires, which may not be a suitable proxy for wildfire emissions. Given the magnitude of the Yosemite Rim wildfire, the impacts it had on regional air quality and the limited sampling of wildfire emissions in the western US to date, this study provides a valuable measurement dataset and may have important implications for forestry and regional air quality management.

Yates, Emma L.

Comparison Of Downscaled CMIP5 Precipitation Datasets For Projecting Changes In Extreme Precipitation In The San Francisco Bay Area.

Water resource managers planning for the adaptation to future events of extreme precipitation now have access to high resolution downscaled daily projections derived from statistical bias correction and constructed analogs. We also show that along the Pacific Coast the Northern Oscillation Index (NOI) is a reliable predictor of storm likelihood, and therefore a predictor of seasonal precipitation totals and likelihood of extremely intense precipitation. Such time series can be used to project intensity duration curves into the future or input into stormwater models. However, few climate projection studies have explored the impact of the type of downscaling method used on the range and uncertainty of predictions for local flood protection studies. Here we present a study of the future climate flood risk at NASA Ames Research Center, located in South Bay Area, by comparing the range of predictions in extreme precipitation events calculated from three sets of time series downscaled from CMIP5 data: 1) the Bias Correction Constructed Analogs method dataset downscaled to a 1/8 degree grid (12km); 2) the Bias Correction Spatial Disaggregation method downscaled to a 1km grid; 3) a statistical model of extreme daily precipitation events and projected NOI from CMIP5 models. In addition, predicted years of extreme precipitation are used to estimate the risk of overtopping of the retention pond located on the site through simulations of the EPA SWMM hydrologic model. Preliminary results indicate that the intensity of extreme precipitation events is expected to increase and flood the NASA Ames retention pond. The results from these estimations will assist flood protection managers in planning for infrastructure adaptations.

Storm

TES Carbon Monoxide Validation during the Two AVE Campaigns using the Argus and ALIAS Instruments on NASA's WB-57F

The Aura Validation Experiment (AVE) focuses on validating Aura satellite measurements of important atmospheric trace gases using ground-based, aircraft, and balloon-borne instruments. Global satellite observations of CO from the Tropospheric Emission Spectrometer (TES) on the EOS Aura satellite have been ongoing since September 2004. This paper discusses CO validation experiments during the Oct-AVE (2004 Houston, Texas) and CR-AVE (2006 San Jose, Costa Rica) campaigns. The coincidences in location and time between the satellite observations and the available in situ profiles for some cases are not ideal. However, the CO distribution patterns in the two validation flight areas are shown to have very little variability in the aircraft and satellite . observations, thereby making them suitable for validation comparisons. TES CO profiles, which typically have a retrieval uncertainty of 10-20%, are compared with in situ CO measurements from NASA Ames Research Center's Argus instrument taken on board the WB-57F aircraft during Oct-AVE. TES CO retrievals during CR-AVE are compared with in situ measurements from Jet Propulsion Laboratory's Aircraft Laser Infrared Absorption Spectrometer (ALIAS) instrument as well as with the Argus instrument, both taken on board the WB-57F aircraft. During CR-AVE, the average overall difference between ALIAS and Argus CO was 4%, with the ALIAS measurement higher. During individual flights, 2-min time-averaged differences between the two in situ instruments had standard deviation of 14%. The TES averaging kernels and a priori constraint profiles for CO are applied to the in situ data for proper comparisons to account for the reduced vertical resolution and the influence of the a priori in the satellite-derived profile. In the TES sensitive pressure range, approx.700-200 hPa, the in situ profiles and TES profiles agree within 5-10%, less than the variability in CO distributions obtained by both TES and the aircraft instruments in the two regions. TES CO is slightly lower than in situ measurements in the Houston area (midlatitudes) and slightly higher than in situ CO measurements in the Costa Rica region (tropical).

Lopez, Jinena P.

Transport in the Subtropical Lowermost Stratosphere during CRYSTAL-FACE

We use in situ measurements of water vapor (H2O), ozone (O3), carbon dioxide (CO2), carbon monoxide (CO), nitric oxide (NO), and total reactive nitrogen (NO(y)) obtained during the CRYSTAL-FACE campaign in July 2002 to study summertime transport in the subtropical lowermost stratosphere. We use an objective methodology to distinguish the latitudinal origin of the sampled air masses despite the influence of convection, and we calculate backward trajectories to elucidate their recent geographical history. The methodology consists of exploring the statistical behavior of the data by performing multivariate clustering and agglomerative hierarchical clustering calculations, and projecting cluster groups onto principal component space to identify air masses of like composition and hence presumed origin. The statistically derived cluster groups are then examined in physical space using tracer-tracer correlation plots. Interpretation of the principal component analysis suggests that the variability in the data is accounted for primarily by the mean age of air in the stratosphere, followed by the age of the convective influence, and lastly by the extent of convective influence, potentially related to the latitude of convective injection [Dessler and Sherwuud, 2004]. We find that high-latitude stratospheric air is the dominant source region during the beginning of the campaign while tropical air is the dominant source region during the rest of the campaign. Influence of convection from both local and non-local events is frequently observed. The identification of air mass origin is confirmed with backward trajectories, and the behavior of the trajectories is associated with the North American monsoon circulation.

Pittman, Jasna V.

CO Signatures in Subtropical Convective Clouds and Anvils during CRYSTAL-FACE: An Analysis of Convective Transport and Entrainment using Observations and a Cloud-Resolving Model

Convective systems are an important mechanism in the transport of boundary layer air into the upper troposphere. The Cirrus Regional Study of Tropical Anvils and Cirrus Layers-Florida Area Cirrus Experiment (CRYSTAL-FACE) campaign, in July 2002, was developed as a comprehensive atmospheric mission to improve knowledge of subtropical cirrus systems and their roles in regional and global climate. In situ measurements of carbon monoxide (CO), water vapor (H2Ov), and total water (H2Ot) aboard NASA's WB-57F aircraft and CO aboard the U.S. Navy's Twin Otter aircraft were obtained to study the role of convective transport. Three flights sampled convective outflow on 11, 16 and 29 July found varying degrees of CO enhancement relative to the free troposphere. A cloud-resolving model used the in situ observations and meteorological fields to study these three systems. Several methods of filtering the observations were devised here using ice water content, relative humidity with respect to ice, and particle number concentration as a means to statistically sample the model results to represent the flight tracks. A weighted histogram based on ice water content observations was then used to sample the simulations for the three flights. In addition, because the observations occurred in the convective outflow cirrus and not in the storm cores, the model was used to estimate the maximum CO within the convective systems. In general, anvil-level air parcels contained an estimated 20-40% boundary layer air in the analyzed storms.

Lopez, Jimena P.

CO Signatures in Subtropical Convective Clouds and Anvils During CRYSTAL-FACE: An Analysis of Convective Transport and Entertainment Using Observations and a Cloud-Resolving Model

Convective systems are an important mechanism in the transport of boundary layer air into the upper troposphere. The Cirrus Regional Study of Tropical Anvils and Cirrus Layers-Florida Area Cirrus Experiment (CRYSTAL-FACE) campaign, in July 2002, was developed as a comprehensive atmospheric mission to improve knowledge of subtropical cirrus systems and their roles in regional and global climate. In situ measurements of carbon monoxide (CO), water vapor (H20v), and total water (H20t) aboard NASA's . WB-57F aircraft and CO aboard the U.S. Navy's Twin Otter aircraft were obtained to study the role of convective transport. Three flights sampled convective outflow on 11, 16 and 29 July found varying degrees of CO enhancement relative to the fiee troposphere. A cloud-resolving model used the in situ observations and meteorological fields to study these three systems. Several methods of filtering the observations were devised here using ice water content, relative humidity with respect to ice, and particle number concentration as a means to statistically sample the model results to represent the flight tracks. A weighted histogram based on ice water content observations was then used to sample the simulations for the three flights. In addition, because the observations occurred in the convective outflow cirrus and not in the storm cores, the model was used to estimate the maximum CO within the convective systems. In general, anvil-level air parcels contained an estimated 20-40% boundary layer air in the analyzed storms.

Lopez, Jimena P.

In-situ Observations of Mid-latitude Forest Fire Plumes Deep in the Stratosphere

We observed a plume of air highly enriched in carbon monoxide and particles in the stratosphere at altitudes up to 15.8 km. It can be unambiguously attributed to North American forest fires. This plume demonstrates an extratropical direct transport path from the planetary boundary layer several kilometers deep into the stratosphere, which is not fully captured by large-scale atmospheric transport models. This process indicates that the stratospheric ozone layer could be sensitive to changes in forest burning associated with climatic warming.

Jost, Hans-Juerg

Tracer-based Determination of Vortex Descent in the 1999/2000 Arctic Winter

A detailed analysis of available in situ and remotely sensed N2O and CH4 data measured in the 1999/2000 winter Arctic vortex has been performed in order to quantify the temporal evolution of vortex descent. Differences in potential temperature (theta) among balloon and aircraft vertical profiles (an average of 19-23 K on a given N2O or CH4 isopleth) indicated significant vortex inhomogeneity in late fall as compared with late winter profiles. A composite fall vortex profile was constructed for 26 November 1999, whose error bars encompassed the observed variability. High-latitude extravortex profiles measured in different years and seasons revealed substantial variability in N2O and CH4 on theta surfaces, but all were clearly distinguishable from the first vortex profiles measured in late fall 1999. From these extravortex-vortex differences we inferred descent prior to 26 November: as much as 397 plus or minus 15 K (lsigma) at 30 ppbv N2O and 640 ppbv CH4, and falling to 28 plus or minus 13 K above 200 ppbv N2O and 1280 ppbv CH4. Changes in theta were determined on five N2O and CH4 isopleths from 26 November through 12 March, and descent rates were calculated on each N2O isopleth for several time intervals. The maximum descent rates were seen between 26 November and 27 January: 0.82 plus or minus 0.20 K/day averaged over 50- 250 ppbv N2O. By late winter (26 February to 12 March), the average rate had decreased to 0.10 plus or minus 0.25 K/day. Descent rates also decreased with increasing N2O; the winter average (26 November to 5 March) descent rate varied from 0.75 plus or minus 0.10 K/day at 50 ppbv to 0.40 plus or minus 0.11 K/day at 250 ppbv. Comparison of these results with observations and models of descent in prior years showed very good overall agreement. Two models of the 1999/2000 vortex descent, SLIMCAT and REPROBUS, despite theta offsets with respect to observed profiles of up to 20 K on most tracer isopleths, produced descent rates that agreed very favorably with the inferred rates from observation.

Greenblatt, Jeffrey B.

Argus: a new instrument for the measurement of the stratospheric dynamical tracers, N2O and CH4

We describe here a new instrument for the simultaneous, in situ measurement of the stratospheric tracer molecules, nitrous oxide (N2O) and methane (CH4). Argus is unique in its small size making it well suited for limited payload atmospheric research platforms. Argus employs second harmonic spectroscopy using tunable lead-salt diode lasers emitting in the mid-infrared. We first explain the Argus design philosophy followed by detailed descriptions of the instrument's optical, mechanical, and thermal sub-systems. Argus employs an in-flight calibration system providing real time calibrations and tightly constrained uncertainty estimates of the returned data. Data analysis is carried out using non-linear least-squares model fits to the acquired second harmonic spectra. A sampling of Argus data acquired on a recent stratospheric research campaign in the Arctic winter is presented.

Methane/analysis

Defining the Polar Vortex Edge from a N20: Potential Temperature Correlation

A prerequisite to studying phenomena in the winter stratospheric polar vortex is the separation of measurements inside and outside the dynamical barrier of the vortex edge. We describe a technique to accurately determine the inner edge of the vortex boundary region from measurements of potential temperature and a trace gas, such as N2O, and apply it to in situ aircraft and balloon measurements from the SOLVE/THESEO 2000 Arctic campaign. The method may be used to refine the Nash algorithm, which, due to the inherently coarser resolution of potential vorticity on which it is dependent, may misidentify the inner edge by more than 400 km and omit the identification of small, extravortex filaments within the vortex.

Greenblatt, Jeffery B.

Defining the Polar Vortex Edge Using an N2O: Potential Temperature Correlation Versus the Nash Criterion: A Comparison

A prerequisite to study phenomena in the winter stratospheric polar vortex is the separation of measurements inside and outside the dynamical barrier of the vortex edge. We describe a technique to accurately determine the inner edge of the vortex boundary region from measurements of potential temperature and a trace gas, such as N2O, and apply it to in situ aircraft and balloon measurements from the SOLVE/THESE02000 Arctic campaign. The method may be used to refine the Nash algorithm, which, due to the inherently coarser resolution of potential vorticity on which it is dependent, may misidentify the inner edge by up to 466 km, and omit the identification of small, extra-vortex filaments within the vortex.

Greenblatt, Jeffery B.

Tracer-Based Determination of Vortex Descent in the 1999-2000 Arctic Winter

A detailed analysis of available in situ and remotely sensed N2O and CH4 data measured in the 1999-2000 winter Arctic vortex has been performed in order to quantify the temporal evolution of vortex descent. Differences in potential temperature (theta) among balloon and aircraft vertical profiles (an average of 19-23 K on a given N2O or CH4 isopleth) indicated significant vortex inhomogeneity in late fall as compared with late winter profiles. A composite fall vortex profile was constructed for November 26, 1999, whose error bars encompassed the observed variability. High-latitude, extravortex profiles measured in different years and seasons revealed substantial variability in N2O and CH4 on theta surfaces, but all were clearly distinguishable from the first vortex profiles measured in late fall 1999. From these extravortex-vortex differences, we inferred descent prior to November 26: 397+/-15 K (1sigma) at 30 ppbv N2O and 640 ppbv CH4, and 28+/-13 K above 200 ppbv N2O and 1280 ppbv CH4. Changes in theta were determined on five N2O and CH4 isopleths from November 26 through March 12, and descent rates were calculated on each N2O isopleth for several time intervals. The maximum descent rates were seen between November 26 and January 27: 0.82+/-0.20 K/day averaged over 50-250 ppbv N2O. By late winter (February 26-March 12), the average rate had decreased to 0.10+/-0.25 K/day. Descent rates also decreased with increasing N2O; the winter average (November 26-March 5) descent rate varied from 0.75+/-0.10 K/day at 50 ppbv to 0.40+/-0.11 K/day at 250 ppbv. Comparison of these results with observations and models of descent in prior years showed very good overall agreement. Two models of the 1999-2000 vortex descent, SLIMCAT and REPROBUS, despite theta offsets with respect to observed profiles of up to 20 K on most tracer isopleths, produced descent rates that agreed very favorably with the inferred rates from observation.

Greenblatt, Jeffery B.

Quantifying Subsidence in the 1999-2000 Arctic Winter Vortex

Quantifying the subsidence of the polar winter stratospheric vortex is essential to the analysis of ozone depletion, as chemical destruction often occurs against a large, altitude-dependent background ozone concentration. Using N2O measurements made during SOLVE on a variety of platforms (ER-2, in-situ balloon and remote balloon), the 1999-2000 Arctic winter subsidence is determined from N2O-potential temperature correlations along several N2O isopleths. The subsidence rates are compared to those determined in other winters, and comparison is also made with results from the SLIMCAT stratospheric chemical transport model.

Greenblatt, Jeffery B.

Defining the Vortex Boundary Using N2O Measurements

Defining the stratospheric vortex boundary is typically done using; the Nash criterion,(a) which determines the maximum gradient of Ertel's potential vorticity (EPV) in the vicinity of maximum zonal winds. However, such a procedure is insensitive to small-scale variations near the boundary, because EPV maps rely on interpolation from sparse data, and are therefore only accurate over large areas. An examination was made of high-speed N2O measurements during SOLVE, from Argus ER-2 flights across the vortex boundary in the 1999-2000 Arctic winter, to see whether sharp changes in N2O concentrations co-occur sufficiently well with the Nash definition of the vortex edge to serve as a reliable alternate definition.

Greenblatt, Jeffery

Stratospheric Horizontal Wavenumber Spectra of Winds, Potential Temperature, and Atmospheric Tracers Observed by High-Altitude Aircraft

Horizontal wavenumber power spectra of vertical and horizontal wind velocities, potential temperatures, and ozone and N(2)O mixing ratios, as measured in the mid-stratosphere during 73 ER-2 flights (altitude approx. 20km) are presented. The velocity and potential temperature spectra in the 100 to 1-km wavelength range deviate significantly from the uniform -5/3 power law expected for the inverse energy-cascade regime of two-dimensional turbulence and also for inertial-range, three-dimensional turbulence. Instead, steeper spectra approximately consistent with a -3 power law are observed at horizontal scales smaller than 3 km for all velocity components as well as potential temperature. Shallower spectra are observed at scales longer than 6 km. For horizontal velocity and potential temperature the spectral indices at longer scales are between -1.5 and -2.0. For vertical velocity the spectrum at longer scales become flat. It is argued that the observed velocity and potential temperature spectra are consistent with gravity waves. At smaller scales, the shapes are also superficially consistent with a Lumley-Shur-Weinstock buoyant subrange of turbulence and/or nonlinear gravity waves. Contemporaneous spectra of ozone and N(sub 2)O mixing ratio in the 100 to 1-km wavelength range do conform to an approximately uniform -5/3 power law. It is argued that this may reflect interactions between gravity wave air-parcel displacements and laminar or filamentary structures in the trace gas mixing ratio field produced by enstropy-cascading two-dimensional turbulence.

TRACE GAS MIXING RATIO FIELDS

SPADE H2O measurements and the seasonal cycle of statospheric water vapor

We present measurements of lower statospheric water vapor obtained during the Stratospheric Phototchemistry, Aerosols and Dynamics Expedition (SPADE) mission with a new high precision, fast response, Lyman-alpha hygrometer. The H2O data show a distinct seasonal cycle. For air that recently entered the statosphere, data collected during the fall show much more water vapor than data from the spring. Fast quasi-horizontal mixing causes compact relationships between water and N2O to be established on relatively short time scales. The measurements are consistent with horizontal mixing times of a few months or less. Vertical mixing appears to cause the seasonal variations in water vapor to propagate up to levels corresponding to air that has been in the stratosphere approximately one year.

Hintsa, Eric J.

Tracer-tracer relationships and lower stratospheric dynamics: CO2 and N2O correlations during SPADE

Simultaneous measurements of CO2 and N2O from the NASA ER-2 aircraft during SPADE deployments in November 1992, April/May 1993, and October 1993 provide new information on transport rates in the lower stratosphere. The tropospheric seasonal cycle in CO2, superimposed on the long-term trend, is observed to propagate into the statosphere. The compact correlations observed between CO2 and N2O indicate that meridional transport is sufficiently rapid to create a uniform set of relationships over the northern hemisphere up to at least 21 km even though CO2 changes significantly on a time scale of 8 to 12 weeks. the observed seasonal dependence of the correlations indicates that vertical transport above 20 km is slower in northern summer than in winter and slow throughout the year between 19 km and the tropopause. The inferred amplitude of the seasonal CO2 oscillation in the statopshere, viewed relative to N2O, places constraints on the mean latitude for air entering the statosphere.

Boering, Kristie A.

Vertical transport rates in the statosphere in 1993 from observations of CO2, N2O, and CH4

Measurements of CO2, N2O, and CH4 are analyzed to define hemispheric average vertical exchange rates in the lower stratosphere from November 1992 to October 1993. Effective vertical diffusion coefficients were small in summer, less than or equal to 1 sq m/s at altitudes below 25 km; values were similar near the tropopause in winter, but increased markedly with altitude. The analysis suggests possible longer residence times for exhaust from stratospheric aircraft, and more efficient transport from 20 km to the middle stratosphere, than predicted by many current models. Seasonally-resolved measurements of stratospheric CO2 and N2O provide significant new constraints on rates for global-scale vertical transport.

Wofsy, Steven C.