Discovery of the Origin of the Enormous Zr 88 Neutron-Capture Cross Section and Quantifying Its Impact on Applications
Not Available
Stamatopoulos, Athanasios (ORCID:0000000196071185)↗
Engineering topics
Koehler, Paul E.
Publications and source records attributed to Koehler, Paul E..
DICER: A new instrument at LANSCE to constrain neutron capture rates on radionuclides [Slides]
Abstract not provided.
73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
Study of 149 Sm Capture and Total Cross Sections for Burnup Credit Applications [Slides]
This presentation highlights how capture and transmission measurements were performed with the DANCE (Detector for Advanced Neutron Capture Experiments) instrument with capture data from 8 eV – 1 keV, and DICER (Device for Indirect Capture Experiments on Radionuclides) instruments with transmission data from 1meV – 1 keV. There were additional measurements of 147 Sm which had contaminant in the samples, 3.4 eV strong resonance, interesting abnormalities. The data analysis is complete and the R-Matrix analysis almost (90%) complete.
46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
The LANSCE experimental program: accelerator requirements
The LANSCE accelerator complex exploits a flexible, high power 800 MeV proton linear accelerator to enable a broad swath of experimental work supporting multiple scientific programs. The beam requirements for these programs are diverse and change over time. The purpose of this document is to record, at a high level, the experimental requirements driving the beam delivery requirements for each experimental facility at LANSCE. Revision 0 serves to baseline the current set of experiments, and we expect to revise the document on an as-needed basis when either the experimental requirements change or are found to require a more complete definition.
43 PARTICLE ACCELERATORS↗
Production of zirconium-88 via proton irradiation of metallic yttrium and preparation of target for neutron transmission measurements at DICER
Abstract A process for the production of tens to hundreds of GBq amounts of zirconium-88 ( 88 Zr) using proton beams on yttrium was developed. For this purpose, yttrium metal targets (≈20 g) were irradiated in a ~16 to 34 MeV proton beam at a beam current of 100–200 µA at the Los Alamos Isotope Production Facility (IPF). The 88 Zr radionuclide was produced and separated from the yttrium targets using hydroxamate resin with an elution yield of 94(5)% (1σ). Liquid DCl solution in D 2 O was selected as a suitable 88 Zr sample matrix due to the high neutron transmission of deuterium compared to hydrogen and an even distribution of 88 Zr in the sample matrix. The separated 88 Zr was dissolved in DCl and 8 µL of the obtained solution was transferred to a tungsten sample can with a 1.2 mm diameter hole using a syringe and automated filling station inside a hot cell. Neutron transmission of the obtained 88 Zr sample was measured at the Device for Indirect Capture Experiments on Radionuclides (DICER).
73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
Constraining the nuclear spin distribution using improved 197 Au neutron resonance parameters
New neutron transmission data at resonance energies using a 197 Au sample were measured using an early version of the Device for Indirect Capture Experiments on Radionuclides (DICER), which is under development at the Los Alamos Neutron Science Center (LANSCE). These data were combined with previous neutron transmission and capture data in a simultaneous R-matrix analysis to extract improved neutron resonance parameters for this nuclide. As a result, total radiation widths, Γ γ , were obtained for 33 J=1 and 44 J=2 197 Au+n resonances. Γ γ distributions for these two spins states were compared to distributions calculated according to the nuclear statistical model using published nuclear level density (NLD) and photon strength functions (PSF) measured using the Oslo technique. The calculated distributions were found to be narrower and the average values for the two spins states closer together than the data. The calculation can be brought into agreement with the data by substantial modifications to the spin distribution in 198 Au as a function of excitation energy. As far as we know, the spin distribution currently is otherwise poorly constrained. The modified spin distribution changes the shapes of the NLD and PSF extracted using the Oslo technique and so could have broad implications.
73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗