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Kinne, Stefan

Publications and source records attributed to Kinne, Stefan.

At least 19 records

Comparison of Radiative Energy Flows in Observational Datasets and Climate Modeling

This study examines radiative flux distributions and local spread of values from three major observational datasets (CERES, ISCCP, and SRB) and compares them with results from climate modeling (CMIP3). Examinations of the spread and differences also differentiate among contributions from cloudy and clear-sky conditions. The spread among observational datasets is in large part caused by noncloud ancillary data. Average differences of at least 10Wm(exp -2) each for clear-sky downward solar, upward solar, and upward infrared fluxes at the surface demonstrate via spatial difference patterns major differences in assumptions for atmospheric aerosol, solar surface albedo and surface temperature, and/or emittance in observational datasets. At the top of the atmosphere (TOA), observational datasets are less influenced by the ancillary data errors than at the surface. Comparisons of spatial radiative flux distributions at the TOA between observations and climate modeling indicate large deficiencies in the strength and distribution of model-simulated cloud radiative effects. Differences are largest for lower-altitude clouds over low-latitude oceans. Global modeling simulates stronger cloud radiative effects (CRE) by +30Wmexp -2) over trade wind cumulus regions, yet smaller CRE by about -30Wm(exp -2) over (smaller in area) stratocumulus regions. At the surface, climate modeling simulates on average about 15Wm(exp -2) smaller radiative net flux imbalances, as if climate modeling underestimates latent heat release (and precipitation). Relative to observational datasets, simulated surface net fluxes are particularly lower over oceanic trade wind regions (where global modeling tends to overestimate the radiative impact of clouds). Still, with the uncertainty in noncloud ancillary data, observational data do not establish a reliable reference.

Raschke, Ehrhard↗

Aerosol Comparisons Between Observations and Models: AeroCom and ABC

I will represent the AeroCom community to the Atmospheric Brown Cloud (ABC) workshop. I will summarize the activities and results from AeroCom Phase I activities in the past 8 years and introduce the new results and activities in the current AeroCom Phase II. We hope to coordinate some activities with the ABC community to share model output and data access for model evaluations, comparisons, and assessment.

Chin, Mian↗

Aerosol Absorption and Radiative Forcing

We present a comprehensive examination of aerosol absorption with a focus on evaluating the sensitivity of the global distribution of aerosol absorption to key uncertainties in the process representation. For this purpose we extended the comprehensive aerosol-climate model ECHAM5-HAM by effective medium approximations for the calculation of aerosol effective refractive indices, updated black carbon refractive indices, new cloud radiative properties considering the effect of aerosol inclusions, as well as by modules for the calculation of long-wave aerosol radiative properties and instantaneous aerosol forcing. The evaluation of the simulated aerosol absorption optical depth with the AERONET sun-photometer network shows a good agreement in the large scale global patterns. On a regional basis it becomes evident that the update of the BC refractive indices to Bond and Bergstrom (2006) significantly improves the previous underestimation of the aerosol absorption optical depth. In the global annual-mean, absorption acts to reduce the shortwave anthropogenic aerosol top-of-atmosphere (TOA) radiative forcing clear-sky from -0.79 to -0.53 W m(sup -2) (33%) and all-sky from -0.47 to -0.13W m(sup -2 (72%). Our results confirm that basic assumptions about the BC refractive index play a key role for aerosol absorption and radiative forcing. The effect of the usage of more accurate effective medium approximations is comparably small. We demonstrate that the diversity in the AeroCom land-surface albedo fields contributes to the uncertainty in the simulated anthropogenic aerosol radiative forcings: the usage of an upper versus lower bound of the AeroCom land albedos introduces a global annual-mean TOA forcing range of 0.19W m(sup -2) (36%) clear-sky and of 0.12W m(sup -2) (92%) all-sky. The consideration of black carbon inclusions on cloud radiative properties results in a small global annual-mean all-sky absorption of 0.05W m(sup -2) and a positive TOA forcing perturbation of 0.02W m(sup -2). The long-wave aerosol radiative effects are small for anthropogenic aerosols but become of relevance for the larger natural dust and sea-salt aerosols.

Stier, Philip↗

Impact of Nonabsorbing Anthropogenic Aerosols on Clear-Sky Atmospheric Absorption

Absorption of solar radiation by atmospheric aerosol has become recognized as important in regional and global climate. Nonabsorbing, hydrophilic aerosols, such as sulfate, potentially affect atmospheric absorption in opposing ways: first, decreasing absorption through aging initially hydrophobic black carbon (BC) to a hydrophilic state, enhancing its removal by wet scavenging, and consequently decreasing BC lifetime and abundance, and second, increasing absorption through enhancement of the BC absorption efficiency by internal mixing as well as through increasing the amount of diffuse solar radiation in the atmosphere. On the basis of General Circulation Model studies with an embedded microphysical aerosol module we systematically demonstrate the significance of these mechanisms both on the global and regional scales. In remote transport regions, the first mechanism prevails, reducing atmospheric absorption, whereas in the vicinity of source regions, despite enhanced wet scavenging, absorption is enhanced owing to the prevalence of the second mechanisms. Our findings imply that the sulfur to BC emission ratio plays a key role in aerosol absorption.

Stier, Philip↗

Dust in the Sky: Atmospheric Composition. Modeling of Aerosol Optical Thickness

Aerosol is any small particle of matter that rests suspended in the atmosphere. Natural sources, such as deserts, create some aerosols; consumption of fossil fuels and industrial activity create other aerosols. All the microscopic aerosol particles add up to a large amount of material floating in the atmosphere. You can see the particles in the haze that floats over polluted cities. Beyond this visible effect, aerosols can actually lower temperatures. They do this by blocking, or scattering, a portion of the sun's energy from reaching the surface. Because of this influence, scientists study the physical properties of atmospheric aerosols. Reliable numerical models for atmospheric aerosols play an important role in research.

Chin, Mian↗

Cirrus Cloud Radiative and Microphysical Properties from Ground Observations and In Situ Measurements During FIRE 1991 and Their Application to Exhibit Problems in Cirrus Solar Radiative Transfer Modeling

Measurements from the FIRE 1991 cirrus cloud field experiment in the central United States are presented and analyzed. The first part focuses on cirrus microphysical properties. Aircraft 2D-probe in situ data at different cloud altitudes were evaluated for cirrus cases on four different days. Also presented are simultaneous data samples from balloonborne videosondes. Only these balloonsondes could detect the smaller crystals. Their data suggest (at least for midlatitude altitudes below 10 km) that ice crystals smaller than 15 microns in size are rare and that small ice crystals not detected by 2D-probe measurements are radiatively of minor importance, as overlooked 2D-probe crystals account for about 10% of the total extinction. The second part focuses on the link between cirrus cloud properties and radiation. With cloud macrophysical properties from surface remote sensing added to the microphysical data and additional radiation measurements at the surface, testbeds for radiative transfer models were created. To focus on scattering processes, model evaluations were limited to the solar radiative transfer by comparing calculated and measured transmissions of sunlight at the surface. Comparisons under cloud-free conditions already reveal a model bias of about +45 W/sq m for the hemispheric solar downward broadband flux. This discrepancy, which is (at least in part) difficult to explain, has to be accounted for in comparisons involving clouds. Comparisons under cirrus cloud conditions identify as the major obstacle in cirrus solar radiative transfer modeling the inability of one-dimensional radiative transfer models to account for horizontal inhomogeneities. The successful incorporation of multidimensional radiative transfer effects will depend not only on better models but critically on the ability to measure and to define characteristic inhomogeneity scales of cloud fields. The relative minor error related to the microphysical treatment is in part a reflection of the improved understanding on solar scattering on ice crystals over the last decade and of the available wealth on ice-crystal size and shape data for this study. In absence of this information, uncertainties from microphysical cirrus model assumptions will remain high.

Kinne, Stefan↗

Microphysical modeling of cirrus. 1: Comparison with 1986 FIRE IFO measurements

We have used a one-dimensional model of cirrus formation to study the development of cirrus clouds during the 1986 First ISCCP (International Satellite Cloud Climatology Project) Regional Experiment (FIRE) intensive field observations (IFO). The cirrus model includes microphysical, dynamical, and radiative processes. Sulfate aerosols, solution drops, ice crystals, and water vapor are all treated as interactive elements in the model. Ice crystal size distributions are fully resolved based on calculations of homogeneous freezing nucleation, growth by water vapor deposition, evaporation, coagulation, and vertical transport. We have focused on the cirrus observed on November 1, 1986. Vertical wind speed for the one-dimensional simulation is taken from a mesoscale model simulation for the appropriate time period. The mesoscale model simulation suggested that strong upward motions over Wyoming and subsequent horizontal transport of upper level moisture were responsible for the cirrus observed over Wisconsin on this date. We assumed that our one-dimensional model could be used to represent a vertical column moving from Wyoming to Wisconsin over a period of several hours. Ice crystal nucleation occurs in our model in the 8 to 10-km region as a result of the strong updrafts (and cooling) early in the simulation. Growth, coagulation, and sedimentation of these ice crystals result in a broad cloud region (5-10 km thick) with an optical depth of 1-2 after a few hours, in agreement with the FIRE measurements. Comparison with aircraft microphysical measurements made over Wisconsin indicates that the simulation generated reasonable ice water content, but the predicted ice number densities are too low, especially for radii less than about 50 microns. Sensitivity tests suggest that better agreement between simulated and observed microphysical properties is achieved if the nucleation rate is higher or stronger vertical mixing (perhaps associated with multidimensional motions) is present.

Jensen, Eric J.↗

Microphysical modeling of cirrus. 2: Sensitivity studies

The one-dimensional cirrus model described in part 1 of this issue has been used to study the sensitivity of simulated cirrus microphysical and radiative properties to poorly known model parameters, poorly understood physical processes, and environmental conditions. Model parameters and physical processes investigated include nucleation rate, mode of nucleation (e.g., homogeneous freezing of aerosols and liquid droplets or heterogeneous deposition), ice crystal shape, and coagulation. These studies suggest that the leading sources of uncertainty in the model are the phase change (liquid-solid) energy barrier and the ice-water surface energy which dominate the homogeneous freezing nucleation rate and the coagulation sticking efficiency at low temperatures which controls the production of large ice crystals (radii greater than 100 mcirons). Environmental conditions considered in sensitivity tests were CN size distribution, vertical wind speed, and cloud height. We found that (unlike stratus clouds) variations in the total number of condensation nuclei (NC) have little effect on cirrus microphysical and radiative properties, since nucleation occurs only on the largest CN at the tail of the size distribution. The total number of ice crystals which nucleate has little or no relationship to the number of CN present and depends primarily on the temperature and the cooling rate. Stronger updrafts (more rapid cooling) generate higher ice number densities, ice water content, cloud optical depth, and net radiative forcing. Increasing the height of the clouds in the model leads to an increase in ice number density, a decrease in effective radius, and a decrease in ice water content. The most prominent effect of increasing cloud height was a rapid increase in the net cloud radiative forcing which can be attributed to the change in cloud temperature as well as change in cloud ice size distributions. It has long been recognized that changes in cloud height or cloud area have the greatest potential for causing feedbacks on climate change. Our results suggest that variations in vertical velocity or cloud microphysical changes associatd with cloud height changes may also be important.

Jensen, Eric J.↗

Airborne brightness temperature measurements of the polar winter troposphere as part of the Airborne Arctic Stratosphere Experiment 2 and the effect of brightness temperature variations on the diabatic heating in the lower stratosphere

In this paper we report radiometric measurements of tropospheric brightness temperatures obtained during the AASE 2 experiment. These measurements represent the first attempt to characterize effective radiative temperatures as seen from above the troposphere during the Arctic winter. The reported measurements include brightness temperatures at 6.7 and 10.5 microns as seen from the NASA DC-8 aircraft flying at about 11 km altitude. We also present radiative transfer calculations to estimate the effect of tropospheric brightness temperature on the lower stratospheric heating rates. Because of the recent massive eruption of the Pinatubo volcano, we also discuss the effects of a volcanic aerosol layer. It is concluded that small particles like the volcanic aerosol or polar stratospheric clouds (PSCs) type 1 do not affect stratospheric heating rates by much; on the other hand, larger particles, PSCs types 2 and 3, may have significant effects on heating rates and consequently on dynamics of the lower stratosphere. The dynamical effects of local stratospheric temperature variations are briefly discussed.

Valero, Francisco P. J.↗

Airborne Brightness Temperature Measurements of the Polar Winter Troposphere as Part of the Airborne Arctic Stratosphere Experiment 2 and the Effect of Brightness Temperature Variations on the Diabatic Heating in the Lower Stratosphere

In this paper we report radiometric measurements of tropospheric brightness temperatures obtained during the AASE 2 experiment. These measurements represent the first attempt to characterize effective radiative temperatures as seen from above the troposphere during the Arctic winter. The reported measurements include brightness temperatures at 6.7 and 10.5 micrometers as seen from the NASA DC-8 aircraft flying at about 11 km altitude. We also present radiative transfer calculations to estimate the effect of tropospheric brightness temperature on the lower stratospheric heating rates. Because of the recent massive eruption of the Pinatubo volcano, we also discuss the effects of a volcanic aerosol layer. It is concluded that small particles like the volcanic aerosol or PSCs type 1 do not affect stratospheric heating rates by much; on the other hand, larger particles, PSCs types 2 and 3, may have significant effects on heating rates and consequently on dynamics of the lower stratosphere. The dynamical effects of local stratospheric temperature variations are briefly discussed.

Valero, Francisoco P. J.↗

Cirrus microphysics and radiative transfer - Cloud field study on 28 October 1986

An analysis of remote-sensing measurements which had detected an inhomogeneous cloud structure, at 6-11 km altitude, in the data acquired during the FIRE 86 experiment in a 75 x 50 km cirrus cloud field, has derived fluxes whose comparison with modeled fluxes imply a modeling-based underestimation of both solar reflectivity/attenuation and downward IR fluxes. Reconciliation of model results with measurements can be achieved either by adding large concentrations of ice crystals or by altering the backscattering properties of ice crystals.

Kinne, Stefan↗

The 27-28 October 1986 FIRE Cirrus case study - Retrieval of cloud particle sizes and optical depths from comparative analyses of aircraft and satellite-based infrared measurements

Infrared radiance measurements were acquired from a narrow-field nadir-viewing radiometer based on the NASA ER-2 aircraft during a coincident Landsat 5 overpass on October 28, 1986 as part of the FIRE Cirrus IFO in the vicinity of Lake Michigan. The spectral bandpasses are 9.90-10.87 microns for the ER-2-based radiometer and 10.40-12.50 microns for the Landsat thematic mapper band. After adjusting for spatial and temporal differences, a comparative study using data from these two instruments is undertaken in order to retrieve cirrus cloud ice-crystal sizes and optical depths. Retrieval is achieved by analysis of measurement correlations between the two spectral bands and comparison to multistream radiative transfer model calculations. The results indicate that the equivalent sphere radii of the cirrus ice crystals were typically less than 30 microns. Such particles were too small to be measured by the available in situ instrumentation. Cloud optical depths at a reference wavelength of 11.4 microns ranged from 0.3 to 2.0 for this case study. Supplemental results in support of this study are described using radiation measurements from the King Air aircraft, which was also in near coincidence with the Landsat overpass.

Hammer, Philip D.↗

Cirrus microphysics and radiative transfer: Cloud field study on October 28, 1986

The radiative properties of cirrus clouds present one of the unresolved problems in weather and climate research. Uncertainties in ice particle amount and size and, also, the general inability to model the single scattering properties of their usually complex particle shapes, prevent accurate model predictions. For an improved understanding of cirrus radiative effects, field experiments, as those of the Cirrus IFO of FIRE, are necessary. Simultaneous measurements of radiative fluxes and cirrus microphysics at multiple cirrus cloud altitudes allows the pitting of calculated versus measured vertical flux profiles; with the potential to judge current cirrus cloud modeling. Most of the problems in this study are linked to the inhomogeneity of the cloud field. Thus, only studies on more homogeneous cirrus cloud cases promises a possibility to improve current cirrus parameterizations. Still, the current inability to detect small ice particles will remain as a considerable handicap.

Kinne, Stefan↗

A comparative study of infrared radiance measurements by an ER-2 based radiometer and the LANDSAT 5 Thematic Mapper (TM-6)

Infrared radiance measurements were acquired from a radiometer on the NASA ER-2 during a coincident LANDSAT 5 overpass on 28 Oct. 1986 as part of the FIRE Cirrus IFO in the vicinity of Lake Michigan. A comparative study is made to infer microphysical properties of the cirrus cloud field. Radiances are derived from the image by convolving the ER-2 radiometer's effective field of view along the flight path. A multistream radiative transfer model is used to account for the differences in spectral bandwidths, 10.40 to 12.50 microns for the LANDSAT band and 9.90 to 10.87 microns for the radiometer.

Hammer, Philip D.↗

Retrieval of cirrus cloud properties from comparative analyses of aircraft and satellite measurements made during the 1986 FIRE IFO

Results are presented of a comparison of cirrus cloud properties obtained from aircraft measurements made during the FIRE Intensive Field Observations and Landsat 5 and NOAA-9 observations carried out during several near coincident overpasses by these satellites. Results of the analyses of these measurements and a comparison between measurements and model calculations were used to determine particle sizes within cirrus clouds and the IR optical depths.

Hammer, Philip D.↗

The effects of the nonsphericity and size distribution of ice crystals on the radiative properties of cirrus clouds

Hexagonal ice crystal and equivalent ice spheres have significantly different single-scattering properties. Although the extinction cross-section for spheres with equivalent surface areas is about the same as that for nonspherical ice crystals randomly oriented in space, equivalent spheres produce more forward scattering and have smaller single-scattering albedos. On the basis of broad-band radiative transfer calculations, in this note we will illustrate that the assumption that ice particles are spheres with equivalent surface areas leads to an underestimate to the solar albedo of cirrus clouds. Furthermore, we show that, for a given optical thickness, small ice particles reflect more solar flux than large ice particles. This implies that the ice crystal size distribution could be extremely important in the determination of the solar albedo of cirrus clouds due to external radiative forcing in climatic perturbation experiments. In the thermal infrared region, absorption by ice crystals predominates and the effects of the nonsphericity and size distribution of ice crystals on infrared radiative transfer appear to be secondary.

Kinne, Stefan↗

On the size and composition of particles in polar stratospheric clouds

Attenuation measurements of the solar radiation between 1.5 and 15 micron wavelengths were performed with the airborne (DC-8) JPL MARK 4 interferometer during the 1987 Antarctic Expedition. The opacities not only provide information about the abundance of stratospheric gases but also about the optical depths of polar stratospheric clouds (PSCs) at wavelengths of negligible gas absorption (windows). The optical depth of PSCs can be determined for each window once the background attenuation, due to air-molecules and aerosol has been filtered out with a simple extinction law. The ratio of optical thicknesses at different wavelengths reveals information about particle size and particle composition. Among the almost 700 measured spectra only a few PSC cases exist. PSC events are identified by sudden reductions in the spectrally integrated intensity value and are also verified with backscattering data from an upward directed lidar instrument, that was mounted on the DC-8. For the selected case on September 21st at 14.40 GMT, lidar data indicate an optically thin cloud at 18k and later an additional optically thick cloud at 15 km altitude. All results still suffer from: (1) often arbitrary definitions of a clear case, that often already may have contained PSC particles and (2) noise problems that restrict the calculations of optical depths to values larger than 0.001. Once these problems are handled, this instrument may become a valuable tool towards a better understanding of the role PSCs play in the Antarctic stratosphere.

Kinne, Stefan↗

Effects of cirrus composition on atmospheric radiation budgets

A radiative transfer model that can be used to determine the change in solar and infrared fluxes caused by variations in the composition of cirrus clouds was used to investigate the importance of particle size and shape on the radiation budget of the Earth-atmosphere system. Even though the cloud optical thickness dominates the radiative properties of ice clouds, the particle size and nonsphericity of ice crystals are also important in calculations of the transfer of near-IR solar wavelengths. Results show that, for a given optical thickness, ice clouds composed of larger particles would produce larger greenhouse effects than those composed of smaller particles. Moreover, spherical particles with equivalent surface areas, frequently used for ice crystal clouds, would lead to an overestimation of the greenhouse effect.

Kinne, Stefan↗