Dynamic heterogeneity and nanophase separation in rubber-toughened amine-cured highly cross-linked polymer networks
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Engineering topics
Publications and source records attributed to Jones, B..
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The surface erosion of polyethylene is interrogated using pulsed x rays at the Z Machine (Sandia National Laboratories) and with proton beams at the Gamble II generator (Naval Research Laboratory) to validate a coupled model for volumetric thermal ablation, photoionization, finite-rate decomposition, and molecular recombination of radicals. The intense radiation pulses (up to ∼1014W/m2 over tens of nanoseconds) are used to generate one-dimensional vapor flows with low ionization fractions and a simplified geometry compared to typical laser ablation, allowing for evaluation of the model under local thermal equilibrium conditions. Areal momentum carried by the ensuing uniaxial hydrodynamic shock is used to indicate the extent of ablation. The threshold fluence for ablation is found to be in close correspondence with the bulk melt transition, and reasonable agreement with the model is obtained for peak temperatures in polyethylene up to 5500 K and heating rates up to 1011K/s where thermal decomposition reactions are also active.
A zero-dimensional magnetic implosion model with a coupled equivalent circuit for the description of an imploding nested wire array or gas puff is presented. Circuit model results have been compared with data from imploding stainless steel wire arrays, and good agreement has been found. The total energy coupled to the load, Ej×B, has been applied to a simple semi-analytic K-shell yield model, and excellent agreement with previously reported K-shell yields across all wire array and gas puff platforms is seen. Trade space studies in implosion radius and mass have found that most platforms operate near the predicted maximum yield. In some cases, the K-shell yield may be increased by increasing the mass or radius of the imploding array or gas puff.
Recoil imaging entails the detection of spatially resolved ionization tracks generated by particle interactions. This is a highly sought-after capability in many classes of detector, with broad applications across particle and astroparticle physics. However, at low energies, where ionization signatures are small in size, recoil imaging only seems to be a practical goal for micro-pattern gas detectors. This white paper outlines the physics case for recoil imaging, and puts forward a decadal plan to advance towards the directional detection of low-energy recoils with sensitivity and resolution close to fundamental performance limits. The science case covered includes: the discovery of dark matter into the neutrino fog, directional detection of sub-MeV solar neutrinos, the precision study of coherent-elastic neutrino-nucleus scattering, the detection of solar axions, the measurement of the Migdal effect, X-ray polarimetry, and several other applied physics goals. We also outline the R&D programs necessary to test concepts that are crucial to advance detector performance towards their fundamental limit: single primary electron sensitivity with full 3D spatial resolution at the $\sim$100 micron-scale. These advancements include: the use of negative ion drift, electron counting with high-definition electronic readout, time projection chambers with optical readout, and the possibility for nuclear recoil tracking in high-density gases such as argon. We also discuss the readout and electronics systems needed to scale-up such detectors to the ton-scale and beyond.
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The combination of the high intensity proton beam facilities and massive detectors for precision measurements of neutrino oscillation parameters including the charge-parity violating (CPV) phase will open the door to help make beyond the standard model (BSM) physics reachable even in low energy regimes in the accelerator-based experiments. Large-mass detectors with highly precise tracking and energy measurements, excellent timing resolution, and low energy thresholds will enable the searches for BSM phenomena from cosmogenic origin, as well. Therefore, it is also conceivable that BSM topics in the next-generation neutrino experiments could be the dominant physics topics in the foreseeable future, as the precision of the neutrino oscillation parameter and CPV measurements continue to improve. This paper reviews the current landscape of BSM theory in neutrino experiments in two selected areas of the BSM topics-dark matter and neutrino related BSM-and summarizes the current results from existing neutrino experiments to set benchmarks for both theory and experiment. This paper then provides a review of upcoming neutrino experiments throughout the next 10 to 15 year time scale and their capabilities to set the foundation for potential reach in BSM physics in the two aforementioned themes. An important outcome of this paper is to ensure theoretical and simulation tools exist to carry out studies of these new areas of physics, from the first day of the experiments, such as Deep Underground Neutrino Experiment in the U.S. and Hyper-Kamiokande Experiment in Japan.
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For this study, a proof-of-principle CR-39 based neutron-recoil-spectrometer was built and fielded on the Z facility. Data from this experiment match indium activation yields within a factor of 2 using simplified instrument response function (IRF) models. The data also demonstrates the need for neutron shielding in order to infer liner areal densities. A new shielded design has been developed. The spectrometer is expected to achieve signal-to-background greater than 2 for the down-scattered neutron signal and greater than 30 for the primary signal.
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With the advent of a new generation of neutrino experiments which leverage high-intensity neutrino beams for precision measurements, it is timely to explore physics topics beyond the standard neutrino-related physics. Given that the realm of beyond the standard model (BSM) physics has been mostly sought at high-energy regimes at colliders, such as the LHC at CERN, the exploration of BSM physics in neutrino experiments will enable complementary measurements at the energy regimes that balance that of the LHC. This is in concert with new ideas for high-intensity beams for fixed target and beam-dump experiments world-wide, e.g., those at CERN. The combination of the high intensity proton beam facilities and massive detectors for precision neutrino oscillation parameter measurements and for CP violation phase measurements will help make BSM physics reachable even in low energy regimes in accelerator based experiments. Large mass detectors with highly precise tracking and energy measurements, excellent timing resolution, and low energy thresholds will enable searches for BSM phenomena from cosmogenic origin, as well. Therefore, it is conceivable that BSM topics in the next generation neutrino experiments could be the dominant physics topics in the foreseeable future, as the precision of the neutrino oscillation parameter and CPV measurements continues to improve. In this spirit, this white paper provides a review of the current landscape of BSM theory in neutrino experiments in two selected areas of the BSM topics - dark matter and neutrino related BSM - and summarizes the current results from existing neutrino experiments to set benchmarks for both theory and experiment. This paper then provides a review of upcoming neutrino experiments throughout the next 10 - 15 year time scale and their capabilities to set the foundation for potential reach in BSM physics in the two aforementioned themes.
Here, the Magnetized Liner Inertial Fusion concept (MagLIF) [Slutz et al., Phys. Plasmas 17, 056303 (2010)] is being studied on the Z facility at Sandia National Laboratories. Neutron yields greater than 1012 have been achieved with a drive current in the range of 17–18 MA and pure deuterium fuel [Gomez et al., Phys. Rev. Lett. 113, 155003 (2014)]. We show that 2D simulated yields are about twice the best yields obtained on Z and that a likely cause of this difference is the mix of material into the fuel. Mitigation strategies are presented. Previous numerical studies indicate that much larger yields (10–1000 MJ) should be possible with pulsed power machines producing larger drive currents (45–60 MA) than can be produced by the Z machine [Slutz et al., Phys. Plasmas 23, 022702 (2016)]. To test the accuracy of these 2D simulations, we present modifications to MagLIF experiments using the existing Z facility, for which 2D simulations predict a 100-fold enhancement of MagLIF fusion yields and considerable increases in burn temperatures. Experimental verification of these predictions would increase the credibility of predictions at higher drive currents.
The apparent ion temperature and neutron-reaction history are important characteristics of a fusion plasma. Extracting these quantities from a measured neutron-time-of-flight signal requires accurate knowledge of the instrument response function (IRF). This paper describes a novel method for obtaining the IRF directly for single DT neutron interactions by utilizing n-alpha coincidence. The t(d,α)n nuclear reaction was produced at Sandia National Laboratories’ Ion Beam Laboratory using a 300 keV Cockcroft-Walton generator to accelerate a 2.5 μA beam of 175 keV D + ions into a stationary ErT 2 target. The average neutron IRF was calculated by taking a time-corrected average of individual neutron events within an EJ-228 plastic scintillator. The scintillator was coupled to two independent photo-multiplier tubes operated in the current mode: a Hamamatsu 5946 mod-5 and a Photek PMT240. Finally, the experimental setup and results will be discussed.
The one-dimensional imager of neutrons (ODIN) at the Sandia Z facility consists of a 10-cm block of tungsten with rolled edges, creating a slit imager with slit widths of either 250, 500, or 750 μm. Designed with a 1-m neutron imaging line of sight, we achieve about 4:1 magnification and 500-μm axial spatial resolution. The baseline inertial confinement fusion concept at Sandia is magnetized liner inertial fusion, which nominally creates a 1-cm line source of neutrons. ODIN was designed to determine the size, shape, and location of the neutron producing region, furthering the understanding of compression quality along the cylindrical axis of magnetized liner implosions. Challenges include discriminating neutrons from hard x-rays and gammas with adequate signal-to-noise in the 2 × 10 12 deuterium-deuterium (DD) neutron yield range, as well as understanding the point spread function of the imager to various imaging detectors (namely, CR-39). Modeling efforts were conducted with MCNP6.1 to determine neutron response functions for varying configurations in a clean DD neutron environment (without x-rays or gammas). Configuration alterations that will be shown include rolled-edge slit orientation and slit width, affecting the resolution and response function. The experiment to determine CR-39 neutron sensitivity, with and without a high density polyethylene (n, p) converter, an edge spread function, and resolution will be discussed.
Here, we investigate the potential of using deep learning techniques to reject background events in searches for neutrinoless double beta decay with high pressure xenon time projection chambers capable of detailed track reconstruction. The differences in the topological signatures of background and signal events can be learned by deep neural networks via training over many thousands of events. These networks can then be used to classify further events as signal or background, providing an additional background rejection factor at an acceptable loss of efficiency. The networks trained in this study performed better than previous methods developed based on the use of the same topological signatures by a factor of 1.2 to 1.6, and there is potential for further improvement.
Two Ar gas-puff experiments, each using loads consisting of two annuli and a center jet, were recently performed on Sandia National Laboratories' Z machine. These shots had the same load except that one of them (Z2603) employed a Xe dopant of 0.8% by number in the jet, which was not present in the otherwise identical Z2605. The extensive diagnostics deployed in these experiments reveal that the presence of this small fraction of Xe had a significant effect on the emitted K-shell radiation. Use of the Xe dramatically reduced the Ar K-shell yield from 373 ± 9% to 129 ± 9% kJ. However, the total yield increased, from 1.02 ± 17% to 1.14 ± 17% MJ. Also, the K-shell power pulse for Z2603 exhibited two nearly equal peaks separated by ∼5 ns, but that of Z2605 consisted of a more conventional single peak. Analysis of time- and space resolved K-shell spectra using a detailed atomic model for Ar ions indicates that a much greater fraction of the load mass was heated to the K-shell in the non-Xe shot Z2605. Previous average-ion atomic calculations of Xe cooling rates [Post et al., At. Data Nucl. Data Tables 20, 397 (1977)] show that the radiative cooling of the small 0.8% Xe fraction is nonetheless significant compared to that of the Ar and is therefore likely responsible for the differences in the shots.
A compact neutron spectrometer, based on a CH foil for the production of recoil protons and CR-39 detection, is being developed for the measurements of the DD-neutron spectrum at the NIF, OMEGA, and Z facilities. As a CR-39 detector will be used in the spectrometer, the principal sources of background are neutron-induced tracks and intrinsic tracks (defects in the CR-39). To reject the background to the required level for measurements of the down-scattered and primary DD-neutron components in the spectrum, the Coincidence Counting Technique (CCT) must be applied to the data. Using a piece of CR-39 exposed to 2.5-MeV protons at the MIT HEDP accelerator facility and DD-neutrons at Z, a significant improvement of a DD-neutron signal-to-background level has been demonstrated for the first time using the CCT. These results are in excellent agreement with previous work applied to DT neutrons.
We report that multi-keV X-ray radiation sources have a wide range of applications, from biomedical studies and research on thermonuclear fusion to materials science and astrophysics. The refurbished Z pulsed power machine at the Sandia National Laboratories produces intense multi-keV X-rays from argon Z-pinches, but for a krypton Z-pinch, the yield decreases much faster with atomic number Z A than similar sources on the National Ignition Facility (NIF) laser at the Lawrence Livermore National Laboratory. To investigate whether fundamental energy deposition differences between pulsed power and lasers could account for the yield differences, we consider the Kr plasma on the two machines. The analysis assumes the plasma not in local thermodynamic equilibrium, with a detailed coupling between the hydrodynamics, the radiation field, and the ionization physics. While for the plasma parameters of interest the details of krypton’s M-shell are not crucial, both the L-shell and the K-shell must be modeled in reasonable detail, including the state-specific dielectronic recombination processes that significantly affect Kr’s ionization balance and the resulting X-ray spectrum. We present a detailed description of the atomic model, provide synthetic K- and L-shell spectra, and compare these with the available experimental data from the Z-machine and from NIF to show that the K-shell yield behavior versus Z A is indeed related to the energy input characteristics. In conclusion, this work aims at understanding the probable causes that might explain the differences in the X-ray conversion efficiencies of several radiation sources on Z and