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Hebden, Andrew

Publications and source records attributed to Hebden, Andrew.

The University of Missouri Research Reactor (MURR) LEU Fuel Element Flow Test Preliminary Design

As part of the U.S. National Nuclear Security Administration’s (NNSA) mission to eliminate or minimize the civilian use of weapons-grade highly enriched uranium (HEU, ≥ 20 wt% U-235) fuels, the NNSA Material Management and Minimization (M3) Office of Reactor Conversion and Uranium Supply is collaborating with six U.S. high performance research reactors (USHPRR), including one critical facility, to convert from the use of HEU to low-enriched uranium (LEU, < 20 wt% U-235) fuel. Primary conversion objectives for the USHPRR are to develop LEU fuel element designs that will ensure safe reactor operations and maintain the existing experimental facilities performance. The work is being conducted through many interrelated activities by stakeholders across organizations.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Massachusetts Institute of Technology Reactor LEU Fuel Element Flow Test Preliminary Design

As part of the U.S. National Nuclear Security Administration’s (NNSA) mission to minimize the civilian use of weapon-grade highly enriched uranium (HEU) fuels, the NNSA Office of Material Management and Minimization Conversion Program is collaborating with six U.S. High Performance Research Reactors (USHPRR), including one critical facility, to convert from the use of HEU to low-enriched uranium (LEU) fuel. The conversion objectives for the USHPRR are to develop LEU fuel element designs that will ensure safe reactor operations and maintain the existing experimental facilities performance. The work is being conducted through many interrelated activities that are being completed by stakeholders across organizations. Within the Reactor Conversion (RC) Pillar of the USHPRR Project, four of the USHPRR, including the Massachusetts Institute of Technology Reactor (MITR-II, also referred to as MITR), have progressed through preliminary fuel element design using the proposed monolithic alloy of uranium- 10 wt% molybdenum (U-10Mo). Preliminary fuel element design and safety analyses have been completed for MITR. This work has relied on preliminary data for properties, performance, and fabrication tolerances for the fuel systems that have been produced by the Fuel Qualification (FQ), Fuel Fabrication (FF), and RC Pillars of the USHPRR Project.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

National Bureau of Standards Reactor LEU Fuel Element Flow Test Conceptual Design

As part of the U.S. National Nuclear Security Administration’s (NNSA’s) mission to eliminate or minimize the civilian use of weapon-grade highly enriched uranium (HEU) fuels, the NNSA Office of Material Management and Minimization (M 3 ) Reactor Conversion Program is collaborating with six U.S. High Performance Research Reactors (USHPRR), including one critical facility, to convert from the use of HEU to low-enriched uranium (LEU) fuel. The M3 conversion objectives for the USHPRR are to develop LEU fuel element designs that will ensure safe reactor operations and maintain the existing experimental performance of each facility. The work is being conducted through many interrelated activities that are being completed by stakeholders across organizations.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Massachusetts Institute of Technology Reactor LEU Fuel Element Flow Test Conceptual Design

As part of the U.S. National Nuclear Security Administration’s (NNSA’s) mission to minimize the civilian use of weapon-grade highly enriched uranium (HEU) fuels, the NNSA Office of Material Management and Minimization (M 3 ) Conversion Program is collaborating with six U.S. High Performance Research Reactors (USHPRR), including one critical facility, to convert from the use of HEU to low-enriched uranium (LEU) fuel. The M 3 conversion objectives for the USHPRR are to develop LEU fuel element designs that will ensure safe reactor operations and maintain the existing experimental performance of each facility. The work is being conducted through many interrelated activities that are being completed by stakeholders across organizations.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

University of Missouri Research Reactor LEU Fuel Element Flow Test Conceptual Design

As part of the U.S. National Nuclear Security Administration’s (NNSA’s) mission to eliminate or minimize the civilian use of weapon-grade highly enriched uranium (HEU) fuels, the NNSA Office of Material Management and Minimization (M 3 ) Conversion Program is collaborating with six U.S. High Performance Research Reactors (USHPRR), including one critical facility, to convert from the use of HEU to low-enriched uranium (LEU) fuel. The M 3 conversion objectives for the USHPRR are to develop LEU fuel-element designs that will ensure safe reactor operations, as well as maintain the existing experimental performance of each facility. The work is being conducted through many interrelated activities that are being completed by stakeholders across organizations.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Massachusetts Institute of Technology Reactor LEU Fuel Element Flow Test Conceptual Design – Hydraulic Reactor Design Parameters

The Massachusetts Institute of Technology Reactor (MITR-II, also referred to as MITR) is one of six U.S. high performance research reactors (USHPRR), including one critical facility, that is actively collaborating with the U.S. National Nuclear Security Administration (NNSA) Material Management and Minimization (M 3 ) Reactor Conversion Program to convert to the use of low-enriched uranium (LEU, < 20 wt% 235 U) fuel. The MIT Nuclear Reactor Laboratory has been working with the USHPRR Reactor Conversion (RC) Pillar at Argonne National Laboratory to perform fuel element design and fuel cycle performance analyses, steady-state thermal hydraulics safety analyses, and accident safety analyses in preparation for the conversion of MITR and support a preliminary Safety Analysis Report (SAR) for conversion to LEU fuel.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

University of Missouri Research Reactor LEU Fuel Element Flow Test Conceptual Design—Hydraulic Reactor Design Parameters

The University of Missouri-Columbia Research Reactor (MURR®) is one of five U.S. high performance research reactors (USHPRR), plus one critical facility, that actively collaborates with the National Nuclear Security Administration (NNSA) Material Management and Minimization(M 3 ) Reactor Conversion Program to convert to the use of low-enriched uranium (LEU, < 20 wt.% U-235) fuel. A new type of LEU fuel with very high density, based on an alloy of uranium and 10 weight percent molybdenum (U-10Mo), is expected to allow the conversion to LEU of USHPRR that have been found unable to be converted with previously qualified uranium silicide-aluminum (U 3 Si 2 -Al) dispersion fuel. MURR has been working with the USHPRR Reactor Conversion (RC) Pillar at Argonne National Laboratory to perform fuel element design and fuel cycle performance analyses, steady-state thermal hydraulics safety analyses, and accident safety analyses in preparation for the conversion of MURR and to support a preliminary Safety Analysis Report (SAR) for conversion to LEU fuel. This work is performed in preparation for the flow test campaign that will be conducted by the USHPRR RC Pillar. The purpose of the hydraulic performance evaluation of the MURR LEU fuel element designed by the RC Pillar is to test a prototypic commercially fabricated LEU fuel element to determine whether any failure modes are observed or predicted in the fuel element, including significant deformations such as plate bending, twisting, or plate detachment from the side plate under selected safety-basis limits for reactor hydraulic conditions. To support the design of the flow test for MURR LEU fuel element hydraulic performance evaluation, design parameters for hydraulic testing of the LEU fuel element are laid out in this report.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Developments of solid materials for UF 6 sampling

This project demonstrated that a device using majority Commercial Off the Shelf (COTS) components could be used to collect uranium hexafluoride samples safely from gaseous or solid sources. The device was based on the successful Cristallini method developed by ABACC over the past 10 years. The system was designed to capture and store the UF 6 as an inert fluoride salt to ease transportation regulations. In addition, the method was considerably faster than traditional cryogenic methods, collected enough material to perform analyses without undue waste, and could be used either inside a facility or in the storage yard.

36 MATERIALS SCIENCE↗

Development of solid materials for UF 6 sampling: FY16 Annual Report

A handheld implementation of the ABACC-developed Cristallini method, which captures uranium hexafluoride samples as an inert salt, was organized in FY17 and succeeded in demonstrating the handheld sampler concept with reactive hexafluoride gases. The Cristallini method relies on the use of a hydrated substrate to react the incoming hexafluoride resulting in the formation of a stable uranyl fluoride salt. The Cristallini method has been demonstrated as a facility modification installed near the sampling tap of a gas centrifuge enrichment plant. While very successful in reducing the hazards of uranium hexafluoride sample, the method still takes a considerable amount of time and can only be used in facilities where the apparatus has been installed; this arrangement generally prohibits the sampling of filled cylinders that have already exited the facility and have been deposited in the on-site tank storage yard. The handheld unit under development will allow the use of the Cristallini method at facilities that have not been converted as well as tanks in the storage yard. The handheld system utilizes an active vacuum system, rather than a passive vacuum system in the facility setup, to drive the uranium hexafluoride onto the adsorbing media. The handheld unit will be battery operated for fully autonomous operation and will include onboard pressure sensing and flushing capability. To date, the system concept of operations was demonstrated with tungsten hexafluoride that showed the active vacuum pump with multiple cartridges of adsorbing media was viable. Concurrently, the hardened prototype system was developed and tested; removable sample cartridges were developed (the only non-COTS component to date); and preparations were made for uranium tests and a domestic field test.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Compendium of Phase-I Mini-SHINE Experiments

Argonne National Laboratory is assisting SHINE Medical Technologies in their efforts to develop the technology to become a domestic Mo-99 producer using low-enriched uranium (LEU). Mini-SHINE experiments are being performed with the high-current electron linear accelerator (linac) at Argonne. The target solution is a 90-150 g-U/L LEU uranyl sulfate at pH 1. In Phase 1, the convertor was tantalum with a maximum beam power on the convertor of 10 kW, and the target solution was limited to 5 L. This configuration generated a peak fission power density of 0.05 W/mL. Nine experiments were performed between February and October 2015. Results are reported and discussed for each experiment regarding the off-gas analysis system, the sampling and Mo-recovery operation, and the Mo-product concentration and purification system. In Phase 2, the convertor will be depleted uranium; beam power will increase to 20 kW; and the solution volume will be 18 L. This configuration will generate a fission power density of up to 1 W/mL.

43 PARTICLE ACCELERATORS↗

Cristallini Material Review and Selection

The creation of a handheld unit to utilize the Cristallini method of uranium hexafluoride sampling requires the identification and qualification of suitable substrate materials. These materials will need to quickly and completely react with the process gas, resist vapor locking under vacuum, while being relatively inexpensive and homogeneous. Two forms of powdered alumina have been chosen for a head-to-head comparison during upcoming uranium hexafluoride tests. Both materials have shown ideal uptake characteristics during tungsten hexafluoride tests with a high loading capacity and no measureable breakthrough. They have also been shown to work well at vacuums below 10 Torr, are commercially available and inexpensive. In addition, two possible hydrogen fluoride trapping materials, sodium fluoride and saturated calcium carbonate, have been identified for further testing.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Low-enriched uranium high-density target project. Compendium report

At present, most 99 Mo is produced in research, test, or isotope production reactors by irradiation of highly enriched uranium targets. To achieve the denser form of uranium needed for switching from high to low enriched uranium (LEU), targets in the form of a metal foil (~125-150 µm thick) are being developed. The LEU High Density Target Project successfully demonstrated several iterations of an LEU-fission-based Mo-99 technology that has the potential to provide the world’s supply of Mo-99, should major producers choose to utilize the technology. Over 50 annular high density targets have been successfully tested, and the assembly and disassembly of targets have been improved and optimized. Two target front-end processes (acidic and electrochemical) have been scaled up and demonstrated to allow for the high-density target technology to mate up to the existing producer technology for target processing. In the event that a new target processing line is started, the chemical processing of the targets is greatly simplified. Extensive modeling and safety analysis has been conducted, and the target has been qualified to be inserted into the High Flux Isotope Reactor, which is considered above and beyond the requirements for the typical use of this target due to high fluence and irradiation duration.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Argonne Mockup of the Two Frontend Processes for the Hot-Cell Demonstrations to be Run at Oak Ridge National Laboratory

The Global Threat Reduction Initiative (GTRI) Conversion Program develops technology necessary to convert civilian facilities that use high enriched uranium (HEU) to low enriched uranium (LEU) fuels and targets. The conversion of conventional HEU dispersion targets to LEU for the production of Mo-99 requires approximately five times the uranium in a target to maintain the Mo-99 yield per target; therefore, processes involving high-density metal LEU foil targets are a primary focus of this research and development effort.

Vandegrift, George F.↗

FY-12 Results of Phase-1 Mini-SHINE/MIPS Experiments

This report describes Fiscal Year 2012 (FY-12) results for the first part of the phase 1 mini-SHINE/Medical Isotope Production System (MIPS) experiments, water irradiation. Water irradiation experiments were implemented to shake down/test equipment that will be used in the mini-SHINE/MIPS experiment with uranyl-salt solutions without the potential hazard of producing radioactive solutions and gases.

Chemerisov, Sergey↗