Level densities for Ga 69 , 71 nuclei using a particle-evaporation technique
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Engineering topics
Publications and source records attributed to Grimes, S. M..
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The spin cutoff parameter for 59 Ni has been studied from different types of experimental data, including neutron angular distributions from the 56 Fe(α,n) 59 Ni reaction, spin of discrete levels, the level density from the proton evaporation spectrum of the 54 Fe( 6 Li,p) 59 Ni reaction and neutron resonance spacing. Experimental data points were compared with calculations using models widely used in literature. It was found that the available empirical models overestimate data points in the energy region below the neutron separation energy, while microscopic calculations which take into account pairing correlations within Hartree-Fock +Bardeen-Cooper-Schrieffer approach are consistent with data. As a result, it confirmed earlier findings that pairing correlations play an important role and need to be taken into account when the spin cutoff parameter is calculated below the neutron separation energy.
The 10 B + n system has been studied by measuring charged particles from neutron-induced reactions in the 1 to 20 MeV energy range. Protons, deuterons, tritons, and α particles were measured at four angles using the pulsed white neutron spectrum at the Los Alamos Neutron Science Center Weapons Neutron Research facility. Differential cross sections for each species are reported. These new data are combined with literature data in an R-matrix analysis of the 11 B compound system. Furthermore, a comparison is made to the molecular and cluster states candidates observed in these reactions.
The effect of the isovector imaginary optical potential has been studied experimentally by using the particle-evaporation technique for the 11 B + 48 Ca reaction with a 21.8 MeV 11 B beam. Spectra of neutron, proton, and α particles emitted from the neutron-rich compound nucleus 59 Mn have been measured and analyzed with traditional optical model potentials with their original parametrizations as well as with adjusted isovector imaginary components. It is shown that the isovector component of the imaginary potential is indispensable in the reproduction of proton and α-particle yields from this reaction and even needs to be enhanced compared with the suggestions of the original model parametrizations. Furthermore, this can lead to important consequences for astrophysical reaction-rate calculations.
Nuclear reactions of interest for astrophysics and applications often rely on statistical model calculations for nuclear reaction rates, particularly for nuclei far from β stability. However, statistical model parameters are often poorly constrained, where experimental constraints are particularly sparse for exotic nuclides. For example, our understanding of the breakout from the NiCu cycle in the astrophysical rp-process is currently limited by uncertainties in the statistical properties of the proton-rich nucleus 60 Zn. We have determined the nuclear level density of 60 Zn using neutron evaporation spectra from 58 Ni( 3 He,n) measured at the Edwards Accelerator Laboratory. We compare our results to a number of theoretical predictions, including phenomenological, microscopic, and shell-model-based approaches. Notably, we find the 60 Zn level density is somewhat lower than expected for excitation energies populated in the 59 Cu(p,γ) 60 Zn reaction under rp-process conditions. This includes a level density plateau from roughly 5 to 6 MeV excitation energy, which is counter to the usual expectation of exponential growth and all theoretical predictions that we explore. Here, a determination of the spin distribution at the relevant excitation energies in 60 Zn is needed to confirm that the Hauser-Feshbach formalism is appropriate for the 59 Cu(p,γ) 60 Zn reaction rate at x-ray burst temperatures
Bethe wrote a pivotal paper providing the formalism for the theory of nuclear level densities. At that time, there were no known deformed nuclei, so Bethe made the assumption that all nuclei are spherical. After deformed nuclei were discovered, theorists predicted that the level density for such nuclei should be substantially enhanced over the level density for neighboring spherical nuclei. Despite these results, two comprehensive level density compilations based on neutron resonances counting at low neutron energy failed to find significant enhancement in level density for deformed nuclei. A recent paper has concluded that the Bethe spin distribution for nuclear levels is not appropriate for deformed nuclei. When a more accurate spin distribution is used in resonance analysis, it is found that an enhancement of approximately the predicted magnitude is observed.
The level densities of 74,76 Ge nuclei are studied with 68,70 Zn( 7 Li , Xp ) reactions. Proton evaporation spectra are measured at backward angles in a wide energy region, from about 2 to 25 MeV. The analysis of spectra allows for the testing of level density models used in modern reaction codes for practical cross-section calculations. Our results show that at excitation energies above the discrete level region, all level density models tested in this work overestimate the level densities that are needed to reproduce proton spectra from these reactions. The Gilbert and Cameron model, which includes the constant-temperature energy dependence of the level density, shows the best agreement with experiment, however, its parameters need to be adjusted to reflect the observed reduction of the level density at higher excitation energies.