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Greenquist, Ian

Publications and source records attributed to Greenquist, Ian.

High-Burnup BWR LOCA Burst Analysis Framework Development and Demonstration

Nuclear power currently contributes approximately 20% of total electricity generation in the United States and more than 10% globally. Given the increasing reliance on nuclear energy to achieve our nation’s goal of reaching net-zero carbon emissions by 2050, there is significant pressure on the existing nuclear industry to extend plant operational licenses and improve efficiency. This is crucial as the existing nuclear fleet serves as a vital bridge until new light water and advanced reactors can be developed and deployed, bolstering the supply of carbon-free energy to meet domestic demands. Operational costs primarily consist of plant operation and maintenance and fuel costs, influenced by materials and reactor core designs. These factors, coupled with heavily subsidized renewable energy markets, create a challenging economic environment for the existing light water reactor fleet, as well as for new build projects. To address these economic challenges, the nuclear industry has developed a strategic blueprint aimed at enhancing nuclear power’s economic sustainability. Past initiatives, such as efforts to eliminate fuel failures by 2010 and reduce operating costs by 30% before 2020, have laid the groundwork. Optimizing core design parameters, including burnup limits and enrichment levels, can lengthen cycles, reduce outages, reduce batch reload batch fractions and spent fuel storage requirements, and lower maintenance and operating expenses, thereby enhancing economic viability. In the United States, boiling water reactors (BWRs) comprise approximately one-third of the fleet, although much of the research and development focus has traditionally been on pressurized water reactors (PWRs). Advances in modeling and simulation, particularly through the Nuclear Energy Advanced Modeling and Simulation (NEAMS) program, are crucial to the long-term viability of BWRs, just as they are for PWRs. A key research area of the high burnup/increased enriched fuel initiative is focused on addressing loss-of-coolant-accident (LOCA)-related issues. NEAMS has dedicated significant effort to enhancing tools to better support BWRs, with a current focus on showcasing the BWR framework for high-burnup LOCA analysis. This high-fidelity work will demonstrate a best estimate pin-by-pin high-burnup BWR LOCA analysis to assess full-core cladding rupture behavior. This modeling capability will help with better understanding and realistic evaluation of fuel fragmentation, relocation, and dispersal (FFRD) phenomena at BWRs, which then could be used to prevent FFRD at BWRs without penalizing operational parameters. In addition, the results of this work will help identify strategies to identify additional margins or to potentially limit cladding rupture through core design optimizations.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

Fuel Performance Calculations of Tagged UO 2 MiniFuel Disks

Isotopic taggants are being considered as a novel form of forensic identifiers for nuclear fuels. As part of this effort, eighteen tagged MiniFuel disks were irradiated in the High Flux Isotope Reactor at Oak Ridge National Laboratory. In this work, the BISON fuel performance code was used to recreate the pellets and predict their behavior and their post-irradiation material properties. These predictions are to serve as a baseline to help investigators identify results of interest during post-irradiation examination of actual MiniFuel disks. The simulation methodology and models are described herein, along with the individual disk predictions. Several general trends were identified in this analysis. Based on the models, it is predicted that the pellets’ internal temperatures will rise over time, fission gas release will remain constant at around 1%, regardless of the burnup, and no grain growth will occur in any of the disks. The reasons for these predictions are discussed below. Probable shortcomings in the BISON predictions are addressed, and future work is proposed.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

NEAMS Burnup Extension Accomplishments and Remaining Modeling Gaps

The economic viability of light-water reactors (LWRs) in the United States is declining in heavily subsidized markets, and as a result, the nuclear industry is looking for opportunities to enhance the economic competitiveness of nuclear power. This is not a foreign concept to the nuclear industry: in the mid-2000s, the nuclear industry set out to achieve zero fuel failures by 2010. The goal in this effort was to drive down the cost of reactor shut down by replacing a pin or bundle in response to fuel rod failure. 2010 brought about the initiative to deliver the nuclear promise to reduce operating cost by 30% to improve nuclear energy’s economic competitiveness before 2020. The emergence of accident-tolerant fuel also offers the nuclear industry an opportunity to build on these past successes and deliver affordable, clean energy. Accident-tolerant fuel has been shown to provide superior performance compared to traditional Zircaloy/UO2 fuel concepts, offering the unique ability to remove operational limitations that inhibit the economic viability of nuclear power. This has led the industry to begin building a technical case to extend the peak rod average burnup beyond 62 GWd/tU to extend pressurized water reactor cycle lengths to 24 months and to develop more efficient boiling water reactor core designs. The Nuclear Energy Advanced Modeling and Simulation (NEAMS) program mission is to develop advanced modeling and simulation tools and capabilities to accelerate the deployment of advanced nuclear energy technologies. The primary safety concern inhibiting the nuclear industry from extending burnup is related to high-burnup fuel fragmentation, relocation, and dispersal. Therefore, the NEAMS program developed a targeted 5-year plan to support the industry’s efforts to extend burnup. This milestone report summarizes the 5-year plan that was enacted in FY20, followed by a discussion of the ongoing activates required to fulfill the 5-year plan, as well as the approach to address the current modeling gaps. Additionally, an LWR stakeholder meeting was held to communicate work performed in the NEAMS program over the past three years, to assess the LWR community’s perspective on the impact of the program, and to identify remaining significant gaps in the NEAMS suite of capabilities. This engagement will be documented by the Electric Power Research Institute and used by NEAMS to redirect current LWR scope as needed and to develop the next phase for LWR research and development.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

UO 2 -Liquid Metal Suspension Fuel Concept: Alloy Selection and Depletion Calculations

A novel nuclear fuel was recently proposed that consists of UO 2 particles suspended in a liquid metal mixture. Two liquid metal candidates were identified: BiPbSn and PbSn. Scoping simulations were performed on an over-simplified reactor core that showed a potential limit on achievable burnup. Those findings led to two questions that needed to be addressed: What is the corrosion behavior of the liquid metals toward Zircaloy-4 (Zr4)? And what level of burnup can the fuel be expected to achieve? This report documents efforts to answer both of those questions. First, corrosion experiments were performed between the liquid metal candidates and Zr4 coupons. Second, the previous scoping simulations were expanded to include depletion analyses so that maximum burnups could be estimated. At 400°C, neither PbSn nor BiPbSn caused significant corrosion to the Zr4 coupons. At 600°C, BiPbSn did not cause significant corrosion, but PbSn did. In addition, pure bismuth and pure tin were both highly corrosive, whereas pure lead was non-corrosive. The depletion simulations found that low-enriched fuel could maintain light-water reactor operating temperatures but achieve a burnup of only about one-third of existing reactors. Higher enrichments could achieve burnups equal to or higher than those of existing reactors but at the expense of higher operating temperatures.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Effects of transient fission gas release on rod balloon burst behavior during a loss-of-coolant accident

The US nuclear energy industry is investigating strategies to increase the reactor operating cycle to 24 months, which would result in rod average burnups exceeding the current limit of 62 GWd/tU. To support this goal, multiphysics simulations tools and methodologies are being developed to predict the effects of this change during transient events such as loss-of-coolant accidents (LOCAs). In this work, two cladding burst correlations were used to predict cladding failure. Here, these were coupled with three transient fission gas release (tFGR) models and were implemented in the BISON fuel performance code to quantify any changes in cladding burst behavior during a large-break LOCA. First, a simple linear model was used to perform a sensitivity analysis of a single fuel rod. Second, a tFGR model available in BISON was applied to 281 fuel rods throughout the core. The third model examined was an empirical correlation based on data from the literature.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

MOOSE-Python Binder

This code is a wrapper for Python code so that it can be accessed by MOOSE and the two can pass variables back and forth. Since this code was developed by ORNL, it must be independently approved before being added to the MOOSE repository.

Cheniour, Amani↗