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Froidevaux, Lucien

Publications and source records attributed to Froidevaux, Lucien.

29 records · Page 2

Large-scale variations in ozone from the first two years of UARS MLS data

Two years of stratospheric measurements of ozone from the Upper Atmosphere Research Satellite (UARS) Microwave Limb Sounder (MLS) are examined in order to characterize large horizontal scale wave variations. The use of Fourier analysis allows the detection of variations from daily through seasonal and interannual timescales. High-latitude winter variations at 10 hPa often have very large amplitudes, but smaller midlatitude variations are more ubiquitous. Some variations have the characteristics of locally generated instabilities. Correlations of wave features with changes in the zonal-mean ozone at 10 hPa suggest the presence of significant horizontal motions during strong wintertime polar warming events. Such correlations are not evident at other levels. Spectral analysis of the large-scale variations show most waves to be slowly propagating. In contrast to some past observations, equatorial regions are shown to lack large amplitude wave events.

Elson, Lee S.↗

The tropical semiannual oscillations in temperature and ozone as observed my the MLS

The first two years of Microwave Limb Sounder (MLS) temperature and ozone data are used to examine the tropical upper-stratospheric semiannual oscillation (SAO). Time series analysis revealed that the strongest amplitudes of the SAO occurred near the equator at 2 mb for temperature and 5 mb for ozone, consistent with previous observations. The first cycle of each calendar year was observed to have a much higher amplitude than the second cycle except for the warm phase in late 1991. Interannual variability in the strength of the SAO, such as the much stronger warm phase of late 1991 as compared to late 1992, was significant and could be partly attributed to the Quasi-Biennial Oscillation (QBO) in zonal wind.

Ray, Eric A.↗

Equatorial Kelvin waves: A UARS MLS view

Data from the Microwave Limb Sounder (MLS) instrument on the Upper Atmosphere Research Satellite (UARS) are used to compare two periods of Kelvin wave activity during different stages of the equatorial quasi-biennial oscillation. The analysis is carried out using an asynoptic mapping technique. A wide bandpass filter is used to isolate the frequency bands where Kelvin waves have been identified in previous studies. Time-height and time-latitude plots of the bandpassed data are used to identify Kelvin wave activity in the temperature and ozone fields. Frequency spectra of temperature and ozone amplitudes are constructed to further analyze the latitudinal and meridional distribution of Kelvin wave activity in zonal wavenumbers 1 and 2. The characteristics identified in these plots agree well with theoretical predictions and previous observations of middle atmosphere Kelvin waves. The time-height and time-latitude plots support the existence of Kelvin waves in discrete frequency bands; the slow, fast, and ultrafast Kelvin modes are all identified in the data. The characteristics of these modes do not vary much despite different mean flow conditions in the two periods examined. For the Kelvin wave-induced perturbations in ozone, the change from a transport-dominated regime below 10 hPa to a photochemically controlled regime above 10 hPa is clearly apparent in the height dependence of the phase difference between temperature and ozone. The ratios of the ozone perturbation amplitude to the temperature perturbation amplitude for the various observed Kelvin wave modes are in agreement with model estimates and LIMS (Limb Infrared Monitor of the Stratosphere) observations in the lower half of the region sampled but appear to be too large in the upper stratosphere and lower mesosphere.

Canziani, Pablo O.↗

An investigation of the processes controlling ozone in the upper stratosphere

Photolysis of vibrationally excited oxygen produced by ultraviolet photolysis of ozone in the upper stratosphere is incorporated into the Lawrence Livermore National Laboratory 2-D zonally averaged chemical-radiative-transport model of the troposphere and stratosphere. The importance of this potential contributor of odd oxygen to the concentration of ozone is evaluated based upon recent information on vibrational distributions of excited oxygen and upon preliminary studies of energy transfer from the excited oxygen. When the energy transfer rate constants of previous work are assumed, increases in model ozone concentrations of up to 40 percent in the upper stratosphere are found, and the ozone concentrations of the model agree with measurements, including data from the Upper Atmosphere Research Satellite. However, the increase is about 0.4 percent when the larger energy transfer rate constants suggested by more recent experimental work are applied in the model. This indicates the importance of obtaining detailed information on vibrationally excited oxygen properties to evaluation of this process for stratospheric modelling.

Patten, Kenneth O., Jr.↗

Use of Fourier transforms for asynoptic mapping: Applications to the Upper Atmosphere Research Satellite microwave limb sounder

Fourier analysis has been applied to data obtained from limb viewing instruments on the Upper Atmosphere Research Satellite. A coordinate system rotation facilitates the efficient computation of Fourier transforms in the temporal and longitudinal domains. Fields such as ozone (O3), chlorine monoxide (ClO), temperature, and water vapor have been transformed by this process. The transforms have been inverted to provide maps of these quantities at selected times, providing a method of accurate time interpolation. Maps obtained by this process show evidence of both horizontal and vertical transport of important trace species such as O3 and ClO. An examination of the polar regions indicates that large-scale planetary variations are likely to play a significant role in transporting midstratospheric O3 into the polar regions. There is also evidence that downward transport occurs, providing a means of moving O3 into the polar vortex at lower altitudes. The transforms themselves show the structure and propagation characteristics of wave variations.

Elson, Lee S.↗

Abstract of Lectures

Three lectures will be given. The first one will draw from the general literature on microwave sounding from space. The next two will focus on a description of the Microwave Limb Sounder (MLS) and results obtained from its measurements relating to atmospheric chemistry and dynamics; this will draw from material recently published (or soon-to-be published) by the MLS team.

Froidevaux, Lucien↗

Upper Atmosphere Research Satellite (UARS) Microwave Limb Sounder (MLS) mapping - Validation, early results and applications

The results of limitation studies performed with the UARS MLS are presented. A consistent set of algorithms allows the extraction of the spectral coefficients in time and longitude from asynoptically sampled satellite data and the subsequent reconstruction of synoptic maps from that spectral information. In addition to providing synoptic maps, the asynoptic technique allows the use of standard spectral analysis tools such as autocorrelation and cross correlation.

Elson, Lee S.↗

The mean ozone profile and its temperature sensitivity in the upper stratosphere and lower mesosphere - An analysis of LIMS observations

Multiple simultaneous LIMS (Limb Infrared Monitor of the Stratosphere) observations of both O3 and temperature T in the upper stratosphere and lower mesosphere are analyzed to derive O3-T correlations for comparisons with model calculations. The zonally averaged O3 profile is compared with results from a simplified photochemical model that assumes O3 to be in a photochemical steady state. The model profile is systematically lower than the observed profile. Key parameters are identified in which changes can systematically increase the O3 profile in both the stratosphere and the mesosphere. The LIMS-derived values for the sensitivity of O3 to changes in T are compared with equilibrium model calculations which include the T-driven opacity feedback effect on photodissociation rate constants. The theoretical O3 response to temperature perturbations is investigated. It is shown how the O3-T sensitivity coefficient is affected by zonal and vertical advection terms as well as by the photochemical coupling between O3 and T.

Froidevaux, Lucien↗