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Clough, Shepard A.

Publications and source records attributed to Clough, Shepard A..

First Satellite Observations of Lower Tropospheric Ammonia and Methanol

The Tropospheric Emission Spectrometer (TES) on the EOS Aura satellite makes global measurements of infrared radiances which are used to derive profiles of species such as O3, CO, H2O, HDO and CH4 as routine standard products. In addition, TES has a variety of special modes that provide denser spatial mapping over a limited geographical area. A continuous-coverage mode (called ''transect'', about 460 km long) has now been used to detect additional molecules indicative of regional air pollution. On 10 July 2007 at about 05:37 UTC (13:24 LMST) TES conducted such a transect observation over the Beijing area in northeast China. Examination of the residual spectral radiances following the retrieval of the TES standard products revealed surprisingly strong features attributable to enhanced concentrations of ammonia (NH3) and methanol (CH3OH), well above the normal background levels. This is the first time that these molecules have been detected in space-based nadir viewing measurements that penetrate into the lower atmosphere.

methanol↗

Implementation of Cloud Retrievals for Tropospheric Emission Spectrometer (TES) Atmospheric Retrievals: Part 1. Description and Characterization of Errors on Trace Gas Retrievals

We develop an approach to estimate and characterize trace gas retrievals in the presence of clouds in high spectral measurements of upwelling radiance in the infrared spectral region (650-2260/cm). The radiance contribution of clouds is parameterized in terms of a set of frequency-dependent nonscattering optical depths and a cloud height. These cloud parameters are retrieved jointly with surface temperature, emissivity, atmospheric temperature, and trace gases such as ozone from spectral data. We demonstrate the application of this approach using data from the Tropospheric Emission Spectrometer (TES) and test data simulated with a scattering radiative transfer model. We show the value of this approach in that it results in accurate estimates of errors for trace gas retrievals, and the retrieved values improve over the initial guess for a wide range of cloud conditions. Comparisons are made between TES retrievals of ozone, temperature, and water to model fields from the Global Modeling and Assimilation Office (GMAO), temperature retrievals from the Atmospheric Infrared Sounder (AIRS), tropospheric ozone columns from the Goddard Earth Observing System (GEOS) GEOS-Chem, and ozone retrievals from the Total Ozone Mapping Spectrometer (TOMS). In each of these cases, this cloud retrieval approach does not introduce observable biases into TES retrievals.

aerosols↗

Nadir Measurements of Carbon Monoxide Distributions by the Tropospheric Emission Spectrometer Instrument Onboard the Aura Spacecraft: Overview of Analysis Approach and Examples of Initial Results

We provide an overview of the nadir measurements of carbon monoxide (CO) obtained thus far by the Tropospheric Emission Spectrometer (TES). The instrument is a high resolution array Fourier transform spectrometer designed to measure infrared spectral radiances from low Earth orbit. It is one of four instruments successfully launched onboard the Aura platform into a sun synchronous orbit at an altitude of 705 km on July 15, 2004 from Vandenberg Air Force Base, California. Nadir spectra are recorded at 0.06/cm spectral resolution with a nadir footprint of 5 x 8 km. We describe the TES retrieval approach for the analysis of the nadir measurements, report averaging kernels for typical tropical and polar ocean locations, characterize random and systematic errors for those locations, and describe instrument performance changes in the CO spectral region as a function of time. Sample maps of retrieved CO for the middle and upper troposphere from global surveys during December 2005 and April 2006 highlight the potential of the results for measurement and tracking of global pollution and determining air quality from space.

carbon monoxide↗

A Radiative Transfer Model for Climate Calculations

This paper describes a radiative transfer model developed to accurately predict the atmospheric radiant flux in both the infrared and the solar spectrum with a minimum of computational effort. We use a newly developed k-distribution model for both the thermal and solar parts of the spectrum. We employ a generalized two-stream approximation for the scattering by aerosol and clouds. To assess the accuracy of the model, the results are compared to other more detailed models for several standard cases in the solar and thermal spectrum. We perform several calculations focussing primarily on the question of absorption of solar radiation by gases and aerosols. We estimate the accuracy of the k-distribution to be approx. 1 W/sq m for the gaseous absorption in the solar spectrum. We estimate the accuracy of the two-stream method to be 3-12 W/sq m for the downward solar flux and 1-5 W/sq m for the upward solar flux at the top of atmosphere depending on the optical depth of the aerosol layer. We also show that the effect of ignoring aerosol absorption on the downward solar flux at the surface is 50 W/sq m for the TARFOX aerosol for an optical depth of 0.5 and 150 W/sq m for a highly absorbing mineral aerosol. Thus, we conclude that the uncertainty introduced by the aerosol solar radiative properties (and merely assuming some "representative" model) can be considerably larger than the error introduced by the use of a two-stream method.

Bergstrom, Robert W.↗

Improvement and Application of Atmospheric Radiative Transfer Models for Prediction of the Climatic Effects of Aerosol

This paper presents a radiative transfer model that has been developed to accurately predict the atmospheric radiant flux in both the infrared and the solar spectrum with a minimum of computational effort. The model is designed to be included in numerical climate models. To assess the accuracy of the model, the results are compared to other more detailed models for several standard cases in the solar and thermal spectrum. As the thermal spectrum has been treated in other publications, we focus here on the solar part of the spectrum. We perform several example calculations focussing on the question of absorption of solar radiation by gases and aerosols.

Bergstrom, Robert W.↗

An Improved Radiative Transfer Model for Climate Calculations

This paper presents a radiative transfer model that has been developed to accurately predict the atmospheric radiant flux in both the infrared and the solar spectrum with a minimum of computational effort. The model is designed to be included in numerical climate models To assess the accuracy of the model, the results are compared to other more detailed models for several standard cases in the solar and thermal spectrum. As the thermal spectrum has been treated in other publications, we focus here on the solar part of the spectrum. We perform several example calculations focussing on the question of absorption of solar radiation by gases and aerosols.

Bergstrom, Robert W.↗