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Chadha, M. S.

Publications and source records attributed to Chadha, M. S..

Aminonitriles - Possible role in chemical evolution

The formation of HCN, ammonium cyanide, alkylnitriles, aminoacetonitrile and its C- and N-methyl homologs was demonstrated earlier in a simulated Jovian atmosphere. The polymeric material resulting in these experiments was shown to give glycine, alanine, sarcosine, aspartic acid and some imino dibasic acids on acid hydrolysis, suggesting thereby the participation of the monomeric nitriles in the formation of the polymeric product(s). Further examination of products resulting from semicorona and arc discharge through a mixture of methane and ammonia has provided evidence for the formation of alkylaminopropionitriles as a complex mixture and also some pyridyl and pyrimidyl type heterocyclic compounds. A gas chromatograph/mass spectrometer examination of the heterocyclics showed resemblance with those found in some carbonaceous chondrites. The significance of these findings in relation to chemical evolution is discussed.

Chadha, M. S.↗

Mass spectral analysis of C3 and C4 aliphatic amino acid derivatives.

Diagnostic criteria are obtained for the distinction of alpha, beta, gamma, and N-methyl isomers of the C3 and C4 aliphatic amino acids, using mass spectral analysis of the derivatives of these acids. The use of deuterium labeling has helped in the understanding of certain fragmentation pathways.

Lawless, J. G.↗

Experiments in Jovian atmosphere.

A 1000 ml reaction vessel, fitted with a stopcock, two joints for the electrodes, and a connecting joint, was used in the investigation. The flask, which has a cold finger at the bottom, was filled with an equimolar mixture of anhydrous methane and ammonia. The electrodes were adjusted to provide a gap of about 0.8 cm between them so that the current flowing through the electrodes was about 0.5 mA and a continuous spark could be observed. The operation was continued for 20 hr. The analysis of the reaction products showed the formation of amino nitriles under the conditions of the investigation.

Chadha, M. S.↗