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Bhartia, P. K.

Publications and source records attributed to Bhartia, P. K..

At least 91 records · Page 5

Comparisons of Satellite Retrieval of Aerosol Properties from SeaWiFS and TOMS to the AERONET Measurements during ACE-Asia

The primary goal of the ACE (Aerosol Characterization Experiment)-Asia mission is to increase our understanding of how atmospheric aerosol particles over the Asian-Pacific region affect the Earth climate system. In support of the day-to-day flight planning of ACE-Asia, we built a near real-time system to provide satellite data from the polar-orbiting instruments Earth Probe TOMS (Total Ozone Mapping Spectrometer) (in the form of absorbing aerosol index) and SeaWiFS (Sea-Viewing Wide Field-of-View Sensor) (in the form of aerosol optical thickness and Angstrom exponent). The results were available via web access. These satellite data provide a 'big picture' of aerosol distribution in the region, which is complementary to the ground based measurements. In this paper, we will briefly discuss the algorithms used to generate these data. The retrieved aerosol optical thickness and Angstrom exponent from SeaWiFS will be compared with those obtained from various AERONET (Aerosol Robotic Network) sites over the Asian-Pacific region. The TOMS aerosol index will also be compared with AERONET aerosol optical thickness over different aerosol conditions. Finally, we will discuss the climate implication of our studies using the combined satellite and AERONET observations.

Hsu, Christina N.↗

Calibration of the Shuttle Ozone Limb Sounding Experiment (SOLSE) and the Limb Ozone Retrieval Experiment (LORE)

The calibration and characterization of two new instruments designed to retrieve ozone profiles into the lower stratosphere will be presented. These instruments will fly as a single payload on the Space Shuttle Columbia currently scheduled to lift off July 11, 2002. The purpose of SOLSE (Shuttle Ozone Limb Sounding Experiment) and LORE (Limb Ozone Retrieval Experiment) is to provide a thorough test of the limb ozone retrieval technique, which is being employed on several satellite instruments currently deployed or planned for deployment in the near future. OSIRIS (Optical Spectrograph and Infrared Imager System) and SCIAMACHY (Scanning Imaging Absorption Spectrometer for Atmospheric Chartography) are already in orbit, while OMPS (the Ozone Mapping and Profiler Suite) is planned as the primary US ozone monitoring instrument in the next decade.. SOLSE is a Czerny-Turner spectrograph utilizing a 1k x 1k cooled CCD at the focal plane and covering the spectral range of 310-380 nm in the ultraviolet and 535-865 nm in the visible to near infrared. LORE is a 5 channel filter radiometer with center band wavelengths of 322, 350, 603, 675, and 1000 nm. The focus of this paper will be on measurements of the SOLSE spectrograph performance in the limb-viewing configuration including stray light rejection, spatial and spectral resolution and absolute radiometric response.

Janz, S. J.↗

Determining the Location and Radiative Impact of Thin Cirrus Clouds using Terra data

Thin cirrus clouds (with optical depth tau much less than 1) play a potentially important role in the Earth atmosphere. The Moderate Resolution Imaging Spectroradiometer (MODIS) onboard the Terra satellite has a channel at 1.375 microns that is specifically designed to detect these clouds. During two three-day periods from December 2000 and June 2001, I show that thin cirrus clouds are ubiquitous throughout the tropics. These thin cirrus generally have optical depths below 0.05 and appear with greater frequency and optical depth near deep convection. Regressing top-of-atmosphere outgoing longwave flux data from the Clouds and the Earth's Radiant Energy System (CERES) against optical depth, we calculate that these thin clouds decrease outgoing longwave flux by approx. 1 W/sq m/(0.01 tau). This translates into longwave forcing of several W/sq m near convection and zero away from convection. Averaging over the whole tropics, these thin cirrus decrease average longwave forcing is approx. 1.4 W/sq m.

Dessler, A. E.↗

The 1998-2000 SHADOZ (Southern Hemisphere ADditional OZonesondes) Tropical Ozone Climatology: Stratospheric and Tropospheric Ozone Variability and the Zonal Wave-One - 2

This is the second 'reference' or 'archival' paper for the SHADOZ (Southern Hemisphere Additional Ozonesondes) network and is a follow-on to the recently accepted paper with similar first part of title. The latter paper compared SHADOZ total ozone with satellite and ground-based instruments and showed that the equatorial wave-one in total ozone is in the troposphere. The current paper presents details of the wave-one structure and the first overview of tropospheric ozone variability over the southern Atlantic, Pacific and Indian Ocean basins. The principal new result is that signals of climate effects, convection and offsets between biomass burning seasonality and tropospheric ozone maxima suggest that dynamical factors are perhaps more important than pollution in determining the tropical distribution of tropospheric ozone. The SHADOZ data at ( ) are setting records in website visits and are the first time that the zonal view of tropical ozone structure has been recorded - thanks to the distribution of the 10 sites that make up this validation network.

Thompson, Anne M.↗

Changes in Earth 360 380 nm Reflectivity: 1980-2000

The TOMS (Total Ozone Mapping Spectrometer) reflectively time series 1980 to 1992 and 1997 to 2000 have been combined to estimate change that have occurred over a 21 year period. The relative calibration of the two TOMS (Nimbus-7, N7 and Earth-Probe, EP) has been validated using the measured reflectivity R over Hudson Bay, Canada and found to be within 1 RU (R=0.01). Some of the local trend features seen in the N7 time series (1980 to 1992) have been continued in the combined time series, but the overall zonal average and global trends have changed. The UV (ultraviolet) reflectivity data are compared with changes in the AVHRR outgoing long-wavelength radiation (OLR) and show an expected anti-correlation with cloud-cover changes over the same period for many, but not all, features. The key results include a continuing decrease in cloud cover over Europe and North America and an increase in reflectivity near Antarctica.

Herman, J. R.↗

Interseasonal Variations in the Middle Atmosphere Forced by Gravity Waves

In our Numerical Spectral Model (NSM), which incorporates Hines' Doppler Spread Parameterization, gravity waves (GW) propagating in the east/west direction can generate the essential features of the observed equatorial oscillations of the zonal circulation and in particular the QBO (quasi-biennial oscillation) extending from the stratosphere into the upper mesosphere. We report here that the NSM also produces inter-seasonal variations in the zonally symmetric meridional circulation. A distinct meridional oscillation (MO) is generated, which appears to be the counterpart to the QBO. With a vertical grid-point resolution of about 0.5 km, the NSM produces the MO through momentum deposition of GW's propagating in the north/south direction. This process is inherently non-linear, of third (odd) order, which enables the oscillation. Since the meridional winds are relatively small compared to the zonal winds, the vertical wavelength required to maintain the MO is also smaller, i.e., only about 10 km instead of the 30 km for the QBO. The corresponding viscous stress is then larger, and the period of the MO is thus short compared with that of the QBO, i.e., only about 3 to 4 months. Depending on the strength of the GW forcing, the computed amplitudes of the meridional wind oscillation are typically 5 m/s in the upper stratosphere and mesosphere, and the associated temperature amplitudes are between about 2 and 3 K. These amplitudes may be observable with the instruments on the TIMED spacecraft. Extended computer simulations with the NSM in 2D and 3D reveal that the MO at low latitudes is modulated by the QBO and in turn can influence it to produce a hemispherically asymmetric component. The annual circulation from the summer to the winter hemisphere is likely to play an important role.

Mayr, H. G.↗

Tropospheric Ozone during the TRACE-P Mission: Comparison between TOMS Satellite Retrievals and Aircraft Lidar Data, March 2001

Over the past several years, we have developed two new tropospheric ozone retrievals from the TOMS (Total Ozone Mapping Spectrometer) satellite instrument that are of sufficient resolution to follow pollution episodes. The modified-residual technique uses v. 7 TOMS total ozone and is applicable to tropical regimes in which the wave-one pattern in total ozone is observed. The TOMS-direct method ('TDOT' = TOMS Direct Ozone in the Troposphere) represents a new algorithm that uses TOMS radiances directly to extract tropospheric ozone in regions of constant stratospheric ozone. It is not geographically restricted, using meteorological regimes as the basis for classifying TOMS radiances and for selecting appropriate comparison data. TDOT is useful where tropospheric ozone displays high mixing ratios and variability characteristic of pollution. Some of these episodes were observed downwind of Asian biomass burning during the TRACE-P (Transport and Atmospheric Chemical Evolution-Pacific) field experiment in March 2001. This paper features comparisons among TDOT tropospheric ozone column depth, integrated uv-DIAL measurements made from NASA's DC-8, and ozonesonde data.

Frolov, A. D.↗

Are Solar Activity Variations Amplified by the QBO: A Modeling Study

Solar cycle activity effects (SCAE) in the lower and middle atmosphere, reported in several studies, are difficult to explain on the basis of the small changes in solar radiation that accompany the 11-year cycle. It is therefore natural to speculate that dynamical processes may come into play to produce a leverage. Such a leverage may be provided by the Quasi-Biennial Oscillation (QBO) in the zonal circulation of the stratosphere, which has been linked to solar activity variations. Driven primarily by wave mean flow interaction, the QBO period and its amplitude are variable but are also strongly influenced by the seasonal cycle in the solar radiation. This influence extends to low altitudes and is referred to as 'downward control'. Small changes in the solar radiative forcing may produce small changes in the period and phase of the QBO, but these in turn may produce measurable differences in the wind field. Thus, the QBO may be an amplifier of solar activity variations and a natural conduit of these variations to lower altitudes. To test this hypothesis, we conducted experiments with a 2D version of our Numerical Spectral Model that incorporates Hines' Doppler Spread Parameterization for small-scale gravity waves (GW). Solar cycle radiance variations (SCRV) are accounted for by changing the radiative heating rate on a logarithmic scale from 0.1% at the surface to 1% at 50 km to 10% at 100 km. With and without SCRV, but with the same GW flux, we then conduct numerical experiments to evaluate the magnitude of the SCAE in the zonal circulation. The numerical results indicate that, under certain conditions, the SCAE is significant and can extend to lower altitudes where the SCRV is small. For a modeled QBO period of 30 months, we find that the seasonal cycle in the solar forcing acts as a strong pacemaker to lock up the phase and period of the QBO. The SCAE then shows up primarily as a distinct but relatively weak amplitude modulation. But with a different QBO period between 30 and 34 (or less than 30, presumably) months, the seasonal phase lock is weak. Solar flux variations in the seasonal cycle then cause variations in the QBO period and phase. These amplify the SCAE to produce relatively large variations in the wind field. The SCAE in this case extends to mid-latitudes.

Mengel, J. G.↗

Tropospheric Ozone from the TOMS TDOT (TOMS-Direct-Ozone-in-Troposphere) Technique During SAFARI-2000

There are a number of published residual-type methods for deriving tropospheric ozone from TOMS (Total Ozone Mapping Spectrometer). The basic concept of these methods is that within a zone of constant stratospheric ozone, the tropospheric ozone column can be computed by subtracting stratospheric ozone from the TOMS Level 2 total ozone column, We used the modified-residual method for retrieving tropospheric ozone during SAFARI-2000 and found disagreements with in-situ ozone data over Africa in September 2000. Using the newly developed TDOT (TOMS-Direct-Ozone-in-Troposphere) method that uses TOMS radiances and a modified lookup table based on actual profiles during high ozone pollution periods, new maps were prepared and found to compare better to soundings over Lusaka, Zambia (15.5 S, 28 E), Nairobi and several African cities where MOZAIC aircraft operated in September 2000. The TDOT technique and comparisons are described in detail.

Stone, J. B.↗

Combined use of Satellite and Surface Observations to Infer the Imaginary Part of Refractive Index of Saharan Dust

We present a method for retrieval of imaginary part of refractive index of desert dust aerosol in UV part of spectrum along with aerosol layer height above the ground. The method uses Total Ozone Mapping Spectrometer' (TOMS) measurements of the top of atmosphere radiances (331 nm, 360 nm) and aerosol optical depth provided by Aerosol Robotic Network (AERONET) (440 nm). Obtained values of imaginary part of refractive index retrieved for Saharan dust aerosol at 360 nm are significantly lower than previously reported values. The average retrieved values vary between 0.0054 and 0.0066 for different geographical locations. Our findings are in good agreement with the results of several recent investigations. The time variability of retrieved values for aerosol layer height is consistent with the predictions of dust transport model.

Sinyuk, Alexander↗

Insights into Tropical Tropospheric Ozone from the 1998-2000 SHADOZ (Southern Hemisphere Additional Ozonesondes) Data Record

We describe the first overview of total, stratospheric and tropospheric ozone in the southern hemisphere tropics based on a three year, ten site record of ozone soundings from the Southern Hemisphere Additional Ozonesondes (SHADOZ) network. Observations covering 1998-2000 were made over Ascension Island; Nairobi, Kenya; Irene, South Africa; Reunion Island; Watukosek, Java; Fiji; Tahiti; American Samoa; San Cristobal, Galapagos; Natal, Brazil. The ozone data, with simultaneous temperature profiles to approximately 7 hPa and relative humidity to approximately 200 hPa, are at an archive: http://code9l6. gsfc.nasa.gov/Data_services/shadoz. Prominent features are highly variable tropospheric ozone, a zonal wave-one pattern in total (and tropospheric) column ozone, and signatures of the Quasi-Biennial Oscillation (QBO) in stratospheric ozone. Total, stratospheric and tropospheric column ozone amounts usually peak between August and November and are lowest in the first half of the year. Tropospheric ozone variability over the Indian and Pacific Ocean displays influences of the waning 1997-1998 Indian Ocean Dipole and ENSO (El Nino / Southern Oscillation), seasonal convection and pollution transport from Africa. Tropospheric ozone over the Atlantic Basin reflects regional subsidence and recirculation as well as pollution ozone from biomass burning.

Thompson, Anne M.↗

Atmospheric Chemistry Insights from the SHADOZ Data: An IGAC Paradigm

The first climatological overview of total, stratospheric and tropospheric ozone in the southern hemisphere tropical and subtropics is based on ozone sounding data from ten sites comprising the Southern Hemisphere Additional Ozonesondes (SHADOZ) network. The period covered is 1998-2000. Observations were made over: Ascension Island; Nairobi, Kenya; Irene, South Africa; Reunion Island; Watukosek, Java; Fiji; Tahiti; American Samoa; San Cristobal, Galapagos; Natal, Brazil. Campaign data were collected on a Trans-Atlantic oceanographic cruise and during SAFARI-2000 in Zambia. The ozone data, with simultaneous temperature profiles to approx. 7 hPa and relative humidity to approx. 200 hPa, reside at: http://code9l6.gsfc.nasa.gov/ Data-services/shadoz. SHADOZ ozone time-series and profiles give a perspective on tropical total, stratospheric and tropospheric ozone in 1998-2000. Prominent features are highly variable tropospheric ozone, a zonal wave-one pattern in total (and tropospheric) column ozone, and signatures of the Quasi-Biennial Oscillation (QBO) in stratospheric ozone. Total, stratospheric and tropospheric column ozone amounts peak between August and November and are lowest between March and May. Tropospheric ozone variability over the Indian and Pacific Ocean displays influences of the Indian Ocean Dipole, and convective mixing. Pollution transport from Africa, South American and the Maritime Continent is a seasonal feature. Tropospheric ozone seasonality over the Atlantic Basin shows effects of regional subsidence and recirculation as well as biomass burning. Dynamical and chemical influences appear to be of comparable magnitude though model studies are needed to quantify this.

Thompson, Anne M.↗

Fabry-Perot Interferometer for Column CO2

Global atmospheric CO2 measurements are essential to resolving significant discrepancies in our understanding of the global carbon budget and, hence, humankind's role in global climate change. The science measurement requirements for CO2 are extremely demanding (precision approx. 0.3%). No atmospheric chemical species has ever been measured from space with this precision. We are developing a novel application of a Fabry-Perot interferometer to detect spectral absorption of reflected sunlight by CO2 and O2 in the atmosphere. Preliminary design studies indicate that the method will be able to achieve the sensitivity and signal-to-noise detection required to measure column CO2 at the target specification. The objective of this program is to construct a prototype instrument for deployment on an aircraft to test the instrument performance and our ability to retrieve the data in the real atmosphere. To date we have assembled a laboratory bench system to begin testing the optical and electronic components. We are also measuring signal and noise levels in actual sunlight to evaluate component performance.

Heaps, William S.↗

An Intercomparison of 2-D Models Within a Common Framework

A model intercomparison among the Atmospheric and Environmental Research (AER) 2-D model, the Goddard Space Flight Center (GSFC) 2-D model, and the Lawrence Livermore National Laboratory 2-D model allows us to separate differences due to model transport from those due to the model's chemical formulation. This is accomplished by constructing two hybrid models incorporating the transport parameters of the GSFC and LLNL models within the AER model framework. By comparing the results from the native models (AER and e.g. GSFC) with those from the hybrid model (e.g. AER chemistry with GSFC transport), differences due to chemistry and transport can be identified. For the analysis, we examined an inert tracer whose emission pattern is based on emission from a High Speed Civil Transport (HSCT) fleet; distributions of trace species in the 2015 atmosphere; and the response of stratospheric ozone to an HSCT fleet. Differences in NO(y) in the upper stratosphere are found between models with identical transport, implying different model representations of atmospheric chemical processes. The response of O3 concentration to HSCT aircraft emissions differs in the models from both transport-dominated differences in the HSCT-induced perturbations of H2O and NO(y) as well as from differences in the model represent at ions of O3 chemical processes. The model formulations of cold polar processes are found to be the most significant factor in creating large differences in the calculated ozone perturbations

Weisenstein, Debra K.↗

Evaluation of Transport in the Lower Tropical Stratosphere in a Global Chemistry and Transport Model

Off-line models of the evolution of stratospheric constituents use meteorological information from a general circulation model (GCM) or from a data assimilation system (DAS). Here we focus on transport in the tropics and between the tropics and middle latitudes. Constituent fields from two simulations are compared with each other and with observations. One simulation uses winds from a GCM and the second uses winds from a DAS that has the same GCM at its core. Comparisons of results from the two simulations with observations from satellite, aircraft, and sondes are used to judge the realism of the tropical transport. Faithful comparisons between simulated fields and observations for O3, CH4, and the age-of-air are found for the simulation using the GCM fields. The same comparisons for the simulation using DAS fields show rapid upward tropical transport and excessive mixing between the tropics and middle latitudes. The unrealistic transport found in the DAS fields may be due to the failure of the GCM used in the assimilation system to represent the quasi-biennial oscillation. The assimilation system accounts for differences between the observations and the GCM by requiring implicit forcing to produce consistency between the GCM and observations. These comparisons suggest that the physical consistency of the GCM fields is more important to transport characteristics in the lower tropical stratosphere than the elimination bias with respect to meteorological observations that is accomplished by the DAS. The comparisons presented here show that GCM fields are more appropriate for long-term calculations to assess the impact of changes in stratospheric composition because the balance between photochemical and transport terms is likely to be represented correctly.

Douglass, Anne R.↗

Combined Use of Satellite and Surface Observations to Infer the Imaginary Part of Refractive Index of Saharan Dust

We present a method for retrieval of the imaginary part of refractive index of desert dust aerosol in the near UV part of spectrum. The method uses Total Ozone Mapping Spectrometer (TOMS) measurements of the top of the atmosphere radiances at 331 and 360 run and aerosol optical depth provided by the Aerosol Robotic Network (AERONET). Obtained values of imaginary part of refractive index retrieved for Saharan dust aerosol at 360 nm are significantly lower than previously reported values. The average retrieved values vary between 0.0054 and 0.0066 for different geographical locations. Our findings are in good agreement with the results of several recent investigations.

Sinyuk, Alexander↗

Correlations among the Optical Properties of Cirrus-Cloud Particles: Microphysical Interpretation

Cirrus measurements obtained with a ground-based polarization Raman lidar at 67.9 deg N in January 1997 reveal a strong positive correlation between the particle optical properties, specifically depolarization ratio delta(sub par) and extinction- to-backscatter (lidar) ratio S, for delta(sub par) less than approximately 40%, and an anti-correlation for delta(sub par) greater than approximately 40%. Over the length of the measurements the particle properties vary systematically. Initially, delta (sub par) approximately equals 60% and S approximately equals 10sr are observed. Then, with decreasing delta(sub par), S first increases to approximately 27sr (delta(sub par) approximately equals 40%) before decreasing to values around 10sr again (delta(sub par) approximately equals 20%). The analysis of lidar humidity and radiosonde temperature data shows that the measured optical properties stem from scattering by dry solid ice particles, while scattering by supercooled droplets, or by wetted or subliming ice particles can be excluded. For the microphysical interpretation of the lidar measurements, ray-tracing computations of particle scattering properties have been used. The comparison with the theoretical data suggests that the observed cirrus data can be interpreted in terms of size, shape, and, under the assumption that the lidar measurements of consecutive cloud segments can be mapped on the temporal development of a single cloud parcel moving along its trajectory, growth of the cirrus particles: Near the cloud top in the early stage of cirrus development, light scattering by nearly isometric particles that have the optical characteristics of hexagonal columns (short, column-like particles) is dominant. Over time the ice particles grow, and as the cloud base height extends to lower altitudes characterized by warmer temperatures they become morphologically diverse. For large S and depolarization values of approximately 40%, the scattering contributions of column- and plate-like particles are roughly the same. In the lower ranges of the cirrus clouds, light scattering is predominantly by plate-like ice particles. This interpretation assumes random orientation of the cirrus particles. Simulations with a simple model suggest, however, that the positive correlation between S and delta(sub par) which is observed for depolarization ratios less than 40% mainly at low cloud altitudes, can be alternatively explained by horizontal alignment of a fraction of the cirrus particle population.

Reichardt, J.↗

The Southern African Regional Science Initiative (SAFARI 2000). Dry-Season Campaign: An Overview

The Southern African Regional Science Initiative (SAFARI 2000) is an international science project investigating the southern African earth-atmosphere-human system. The experiment was conducted over a two-year period March 1999 - March 2001. The dry season field campaign (August-Steptember 2000) was the most intensive activity and involving over 200 scientists from 18 different nations. The main objectives of this campaign were to characterize and quantify the biogenic, pyrogenic and anthropogenic aerosol and trace gas emissions and their transport and transformations in the atmosphere and to validate the NASA Earth Observing System (EOS) satellite Terra within a scientific context. Five aircraft, namely two South African Weather Service aircraft, University of Washington CV-580, the UK Meteorological Office C-130 and the NASA ER-2, with different altitude capabilities, participated in the campaign. Additional airborne sampling of southern African air masses that had moved downwind of the subcontinent was conducted by the CSIRO over Australia. Multiple observations were taken in various sectors for a variety of synoptic conditions. Flight missions were designed to maximize synchronous over-flights of the NASA TERRA satellite platform, above regional ground validation and science targets. Numerous smaller-scale ground validation activities took place throughout the region during the campaign period.

Swap, R. J.↗